强外加电场与大调制度下光折变动力学光栅形成研究

强外加电场与大调制度在光折变效应的研究中已经得到了广泛应用。采用PDECOL算法,严格求解光折变带输运方程,得到外加电场时不同调制度下光折变晶体中随时间变化的空间电荷场、载流子浓度,并讨论了外加电场对它们的影响。通过将物质方程与耦合波方程联立数值求解,可得到光折变光栅形成过程中两波耦合增益系数以及光束条纹相位的变化。模拟结果表明,在强外加电场作用下,两束记录光之间的光强与相位耦合都得到了增强,而原有的解析式忽视了强外加电场与大调制度对空间电荷场相位耦合的影响,此时不再适用。同时发现折射率光栅与记录光束条纹均发生弯曲,并不再保持平行。     

GaN晶体在飞秒紫外波段激发下的可变非线性吸收效应和光动力学过程研究

采用Z扫描和泵浦-探测技术研究了GaN薄膜在370 nm时的非线性光学效应和非线性光动力学过程。首先,基于GaN薄膜的透射光谱,结合线性光学理论分析得到了其在370 nm的线性折射率n₀、线性吸收系数α₀、光学带隙E_g等线性光学性质。采用飞秒激光Z扫描技术,得到了不同光强激发下的Z扫描实验响应结果,结合非线性光学理论提取出GaN薄膜可变的光学非线性吸收效应。在激发光子能量接近GaN带隙情况下,低光强时材料表现为饱和吸收而高光强时为反饱和吸收,这是因为低光强下单光子吸收占主导而高光强下以单光子感应自由载流子吸收为主。闭孔Z扫描测量得到了GaN薄膜的三阶非线性折射系数为n₂=-(1.0±0.1)×10-3 cm2·GW-1,它几乎比传统非线性介质的高出一个数量级。为了探究上述非线性过程的动力学弛豫时间以及进一步探究GaN薄膜非线性光动力学过程的深层物理机制,采用了交叉偏振飞秒退相泵浦探测技术观察GaN薄膜的光激发载流子动力学弛豫过程。实验结果表明,在低光强下,饱和吸收效应来源于瞬态单光子吸收,高光强下单光子感应自由载流子吸收为非瞬态光动力学过程,其自由载流子弛豫时间约为17 ps。该工作将为GaN薄膜在紫外非线性纳米器件应用以及GaN薄膜非线性过程的机制分析理解提供新的思路。     

GaAs(111)衬底上生长的GaN的极性与生长方法和生长条件的关系

研究了在GaAs(111)衬底上生长的六角相GaN的极性的相关关系.在高Ⅴ/Ⅲ比的条件下用MOVPE和MOMBE方法生长的GaN的极性和GaAs衬底的极性一致;在(111)A-Ga表面上的生长层呈现Ga的极性,而在(111)B-As表面上的生长层呈现N的极性.然而,在低的Ⅴ/Ⅲ比,或采用一个AIN中间层的条件下,用HVPE和MOMBE方法在GaAs(111)B表面上生长的GaN呈现出Ga的极性.目前,其原因尚不清楚,但是这些结果表明采用HVPE生长方法或用一高温AlN阻挡层可以得到高质量的GaN.     

用MOVPE和RF-MBE方法极性控制生长GaN

本文报道了用低压MOVPE和RF-分子束外延法在蓝宝石衬底上作极性控制的GaN生长.以“双Al单层”模型讨论了用MOVPE和MBE法在蓝宝石衬底上生长GaN的极性选择的机理,并对AlN在极性转换过程中的作用给出了适当的解释.通过极性控制的生长,使MBE法生长的GaN的表面形貌和电学特性都得到了改善;并对LP-MOVPE生长开发出了一种“三步生长法”,这样就可以用更多的外延方式在蓝宝石衬底上生长出高质量的GaN膜.     

半导体光放大光纤环形激光器的偏振混沌与相干性

研究了基于半导体光放大器(SOA)的光纤环形激光器的偏振混沌光的特性及其相干性。实验采集激光器的输出功率和偏振度,得到了基于半导体光放大器的光纤环形激光器的输出从自发辐射到受激辐射、再到偏振态混沌激光辐射的演化过程。利用马赫-曾德尔(M-Z)干涉仪验证了混沌激光的相干性,并发现混沌干涉只有零级。测量不同光程差时干涉仪的输出功率,计算相应的干涉条纹可见度,进一步算得混沌激光的相干时间约为40 ps。这一结果与根据光谱计算的该混沌激光的相干时间43 ps基本一致。实验还测得该混沌激光的相干性与半导体光放大器的电流无关。并指出了混沌激光相干应用于低相干光源探测领域的灵敏度和分辨力优势。     

多偏振组合同时测量的高灵敏飞秒时间分辨和频光谱系统

Characterization of real-time and ultrafast motions of the complex molecules at surface and interface is critical to understand how interfacial molecules function. It requires to develop surface-sensitive, fast-identification, and time-resolved techniques. In this study, we employ several key technical procedures and successfully develop a highly sensitive femtosecond time-resolved sum frequency generation vibrational spectroscopy (SFG-VS) system. This system is able to measure the spectra with two polarization combinations (ssp and ppp, or psp and ssp) simultaneously. It takes less than several seconds to collect one spectrum. To the best of our knowledge, it is the fastest speed of collecting SFG spectra reported by now. Using the time-resolved measurement, ultrafast vibrational dynamics of the N-H mode of α-helical peptide at water interface is determined. It is found that the membrane environment does not affect the N-H vibrational relaxation dynamics. It is expected that the time-resolved SFG system will play a vital role in the deep understanding of the dynamics and interaction of the complex molecules at surface and interface. Our method may also provide an important technical proposal for the people who plan to develop time-resolved SFG systems with simultaneous measurement of multiple polarization combinations.     

基于格子Boltzmann大密度比模型的多孔介质内气泡动力学行为数值模拟

基于格子Boltzmann两相流大密度模型,研究气泡穿过多孔介质的动力学行为.研究发现:当孔隙率较大时,气泡只变形不破裂,能完整地通过多孔介质;而孔隙率较小时,气泡变形更加剧烈且发生破裂,穿过多孔介质所需的时间更长.另外,当障碍物表面接触角(θ)较小时,气泡均能完整地通过多孔介质,随着接触角的增大,气泡开始发生破裂,且...     

Visualization of Intracellular CA2+ Dynamics with Simultaneous 2-Photon Excited Fluorescence and Third Harmonic Generation Microscope

We show that the simultaneous coupling of two laser scanning non-linear microscopies (2-photon excited fluorescence and third harmonic generation microscopy) give functional and morphological information for improving our understanding on intracellular calcium flows.     

Dissipative Particle Dynamics Simulations of Domain Growth and Phase Separation in Binary Immiscible Fluids

用并行耗散粒子动力学方法研究了二维和三维体系中不同淬火深度下二元不相容流体旋节线分离的相区增长过程. 在二维体系中,在浅度淬火条件下得到了动力学标度指数为1/2的融合机制和2/3的惯性流体动力学机制,在深度淬火情况下发现了有限尺寸效应. 在三维体系中,浅度淬火条件下n=1/3的扩散机制和两种不同淬火深度下n=2/3的惯性流体动力学机制. 由于耗散粒子动力学软相互作用势的本质,所以粘性效应无法被清晰地反映,在该时间区间里,不论是浅度还是深度淬火都表现出n=1/2的指数关系.     

Dynamics of Optical Switching and Stability Analysis of a Polarization Bistable Laser Diode with Detuned External Light Injection

Dynamic behaviors of a polarization-bistable laser diode with detuned light injection are studied, including slow, fast and overshoot switching processes. Dependences of switching time of optical outputs between locked and free oscillating modes on the detuning and power of optical input, carrier injection rate and cross-gain saturation coefficients are investigated. Based on linear stability analysis the system stability is analyzed and analytical expressions are developed to predict the switching time. Our analytical results, in which the switching of optical output from locked to unlocked modes is shown to be composed of two relaxation processes with short and long time constants, are in agreement with the numerical results showing fast and slow switching behaviors dependent on the initial locked state, in contrast to the dynamic behavior of the carrier density dominated by a single relaxation process.