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1.
The Pr(Fe1 ? x Al x )2 alloys with concentrations x = 0–1 have been synthesized under a high pressure. The phase composition and lattice parameters (a and c) have been determined as a function of x. The magnetic and Mössbauer measurements have been performed at T = 90–400 K. It has been established that the Curie temperatures of alloys linearly depend on their composition.  相似文献   

2.
The thermodynamic and magnetic properties of the La1 − x Pb x MnO3 (0.24 ≤ x ≤ 0.40) solid solution system were investigated in the temperature range of 4.2–340 K. All objects were ferromagnetics with Curie temperature T C ≈ 320–340 K, which slowly increased with x. The M(T) behavior in the magnetic ordering region indicated a nonuniform ground state, due possibly to the competition of ferromagnetic and antiferromagnetic interactions. The increase in the saturation magnetic moment with x can be described by a simple model of the binary bonds in La1 − x Pb x MnO3.  相似文献   

3.
Co x Pt1−x (x≥0.7) alloy nanowires are grown into self-synthesized anodic alumina templates by electrodeposition. Magnetic and magnetization properties of Co x Pt1−x alloy nanowires are measured as functions of wire length, temperature, and field orientation. X-ray diffraction shows that as-prepared CoPt nanowires are of fcc polycrystalline structure. A crossover of easy axis of magnetization is observed from parallel to perpendicular of the nanowire axis as a function of length. The coercivity (H c) and remanent squareness (SQ) of Co x Pt1−x nanowire arrays are derived from hysteresis loops measured at various angles (θ) between the field and wire axis. H c(θ) and SQ(θ) curves show bell-shaped or otherwise bell-shaped behavior corresponding to the easy axis of their magnetization.  相似文献   

4.
The electronic structure and ground state parameters of B2 RuAl-based refractory alloys have been investigated in the framework of the density functional theory using the exact muffin-tin orbital method in combination with the coherent potential approximation. It has been demonstrated that the number of states at the Fermi level for the Ru1 − x Me x Al alloys as a function of the alloying metal content has a minimum, which indicates a change in the Fermi surface topology and the presence of specific features in the behavior of elastic constants. It has been concluded that the electronic structure of the alloys can be described in terms of the rigid band model. The nonlinear variations of the lattice parameters of the alloys has been explained.  相似文献   

5.
Magnetic properties of Ge1 ? x Mn x (x = 0.02, 0.04, 0.08) thin films obtained by ion-implanting Mn+ ions into single-crystal Ge plates are investigated. The contributions of the subsystem of dispersed Mn2+ ions, Ge3Mn5 ferromagnetic clusters, and Mn-enriched ferromagnetic domains of Ge to the magnetic moment of Ge1 ? x Mn x films are distinguished. In the subsystem of dispersed Mn2+ ions in Ge1 ? x Mn x films at temperatures below 10 K, a spin-wave resonance is observed in the magnetically ordered state due to percolation ferromagnetism. It is established that, in the films with percolation ferromagnetism, the exchange integrals determined from static measurements correspond to those determined by dynamic measurements.  相似文献   

6.
The capacitance and dielectric loss tangent of GdxMn1–xS (x ≤ 0.2) solid solutions have been measured at a frequency of 10 kHz without magnetic field and in a magnetic field of 8 kOe in the temperature range of 90–450 K. An increase in the permittivity and a dielectric loss maximum have been detected in the low-temperature region. It has been found that the temperature of the maximum of the imaginary part of the permittivity shifts to higher temperatures with increasing concentration. The magnetocapacitance effect has been revealed for two compositions. The dielectric loss has been described in the Debye model with “freezing” dipole moments and in the orbital-charge ordering model.  相似文献   

7.
To clarify the origin of the giant magnetoresistance (GMR) observed in La1?x A x MnO3 (A2+=Sr2+, Pb2+, Ba2+ and Ca2+), we have investigated theoretically the electrical resistivity ρ of carriers in the background of Mn spins which interact with each other through the double exchange interaction. It has been found that extraordinarily large pin fluctuations caused by the instability of the ferromagnetic state are responsible for the transport anomalies including the GMR.  相似文献   

8.
A generalized expression relating the magnetoresistance of manganites La1 − x Ag x MnO3 with the change in the magnetic entropy has been proposed. The correct inclusion of the acting mechanisms of appearance of the magnetoresistance is shown to lead to adequate agreement between the experimental and calculated values of ΔS M .  相似文献   

9.
In this article, we assume that there exist hidden charmed tetraquark states with spin–parity J P=1, and we calculate their masses with the QCD sum rules. The numerical result indicates that the masses of the vector hidden charmed tetraquark states are about M Z =(5.12±0.15) GeV or M Z =(5.16±0.16) GeV, which are inconsistent with the experimental data on the π + χ c1 invariant-mass distribution. The hidden charmed mesons Z 1, Z 2 or Z may be scalar hidden charmed tetraquark states, hadro-charmonium resonances or molecular states.  相似文献   

10.
The structure of high-temperature SrFe1 − x Mo x O3 − z (0 ≤ x ≤ 0.5) phases was studied. Such studies are necessary to understand the mechanism of oxygen transport in membrane materials used for high-temperature oxygen separation.  相似文献   

11.
The effect of charge disorder on the formation of an inhomogeneous state of the electron system in the conduction band in BaPb1 − x Sb x O3 superconducting oxides is investigated experimentally by NMR methods. The NMR spectra of 17O are measured systematically, and the contributions from 17O atoms with different cation nearest surroundings are identified. It is found that microscopic regions with an elevated spin density of charge carriers are formed within two coordination spheres near antimony ions. Nuclei of the superconducting phase of the oxide (regions with an elevated antimony concentration) microscopically distributed over the sample are detected in compounds with x = 0.25 and 0.33. Experiments in which a double resonance signal of the spin echo of 17O-207Pb and 17O-121Sb are measured in the metal phase of BaPb1 − x Sb x O3 oxides are carried out for the first time. The constants of indirect heteronuclear spin-spin 17O-207Pb interaction are determined as functions of the local Knight shift 207 Ks. The estimates of the constants of the indirect interaction between the nuclei of the nearest neighbors (O-Pb and Pb-Pb atoms) and analysis of evolution of the NMR spectra of 17O upon a change in the antimony concentration are convincing evidence in favor of the development of a microscopically inhomogeneous state of the electron system in the metal phase of BaPb1 − x Sb x O3 oxides.  相似文献   

12.
Results of an experimental study of MnS, FeS, and Fe x Mn1?x S single crystals are presented. The phase composition, the lattice parameters, and the state of paramagnetic ions in Fe x Mn1?x S have been determined by x-ray diffraction analysis and Mössbauer spectroscopy. A sequence of transitions have been found in iron manganese sulfide with x = 0.29 at temperatures T 1 ≈ 25–50 K, T 2 ≈ 125 K, and T 3 ≈ 190 K with a change in kinetic properties and the formation of a metallic state at low temperatures T ≈ 2 K. The possibility of a Mott-Hubbard transition in Fe x Mn1?x S sulfides with variation of the composition and the temperature is discussed.  相似文献   

13.
The magnetostriction of Fe x Mn1 − x S (x = 0.27) single crystals in strong magnetic fields up to 120 kOe has been investigated. It has been found that the magnetostriction reaches colossal values (±3 × 10−4) atypical of compounds of 3d elements. It has been found that the magnetostriction changes sign when varying temperature and magnetic field; this behavior indicates an important role of the spin-phonon interactions in the formation of the magnetic order in solid solutions of iron-manganese sulfides.  相似文献   

14.
15.
The crystal structure of samples in the (CuInSe2)1 ? x (2MnSe) x system at room temperature and their magnetic susceptibility in the temperature range 77–1000 K are investigated. It is established that compositions with concentrations 0≤ x ≤ 0.2 form solid solutions with a tetragonal structure, space group I \(\bar 4\)2d (122). The specific magnetic susceptibility χ of samples with 0.1 ≤ x ≤ 0.4 at 77 K lies in the range 9 × 10?4?1.6 × 10t-3cm3/g. The temperature dependence of the inverse magnetic susceptibility of the sample with x = 0.4 suggests the presence of a component with antiferromagnetic ordering and a reliably measured Néel temperature that is characteristic of MnSe. The dependences χ = f(T) of the compositions with x = 0.1, 0.2, 0.3, and 0.4 indicate the occurrence of magnetic phase transitions with a change in the spin state.  相似文献   

16.
We report Eu-local-spin magnetism and Ni-doping-induced superconductivity (SC) in a 112-type ferroarsenide system Eu(Fe1?xNix)As2. The non-doped EuFeAs2 exhibits two primary magnetic transitions at ~100 and ~40 K, probably associated with a spin-density-wave (SDW) transition and an antiferromagnetic ordering in the Fe and Eu sublattices, respectively. Two additional successive transitions possibly related to Eu-spin modulations appear at 15.5 and 6.5 K. For the Ni-doped sample with x = 0.04, the SDW transition disappears, and SC emerges at Tc = 17.5 K. The Eu-spin ordering remains at around 40 K, followed by the possible reentrant magnetic modulations with enhanced spin canting. Consequently, SC coexists with a weak spontaneous magnetization below 6.2 K in Eu(Fe0.96Ni0.04)As2, which provides a complementary playground for the study of the interplay between SC and magnetism.  相似文献   

17.
Previously, iron—silicon alloys were investigated using X-ray diffraction and Mössbauer spectroscopy. It was demonstrated that, at low silicon concentrations, the alloys undergo a local separation into regions of the α iron phase depleted in silicon and silicon-rich clusters with a B2 ordering. The structure of locally ordered regions of the B2 phase is characterized by a pair ordering of silicon atoms: the Si—Si pairs are formed by next-nearest neighbors, and the axes of pairs are oriented along the 〈100〉 directions, which are the easy-magnetization axes. The thermomagnetic treatment in a constant magnetic field applied along the 〈100〉 axis induces an axial magnetic anisotropy, results in the formation of an anisotropic distribution of the B2 phase, and leads to a slight decrease in the volume fraction of the coordination 6: 2 with two silicon atoms in the first coordination shell of the iron atom. Therefore, the formation of an anisotropic local order of pairs of silicon atoms occurs as a result of their reorientation.  相似文献   

18.
We investigate the inclusive photoproduction of J/ψ mesons at HERA within the framework of the k T -factorization QCD approach. Our study is based on the color singlet model supplemented with the relevant off-shell matrix elements and the CCFM and KMR unintegrated gluon densities in a proton and in a photon. Both the direct and resolved photon contributions are taken into account. Our predictions are compared with the recent experimental data taken by the H1 and ZEUS collaborations. Special attention is put on the J/ψ polarization parameters λ and ν, which are sensitive to the production dynamics.  相似文献   

19.
Intracenter luminescence (IL) of Mn2+ in Zn1?xMnxSe (x=0.07, 0.02) was studied under pulsed excitation by the neodymium laser second harmonic. At 4 K, the IL saturation originates from the nonlinearity of the system only at the instant of excitation, the IL decay kinetics after the exciting pulse termination depending only weakly on the pumping level. At 77 K, the decay kinetics in Zn0.93Mn0.07Se depends substantially on the pumping level, because the migration of intracenter excitation over the manganese ions initiates up-conversion, which is a slow nonlinear process. As shown by IL decay measurements in Zn0.98Mn0.02Se (x=0.02), excitation migration over the Mn2+ ions is insignificant even at a high temperature and under strong optical pumping.  相似文献   

20.
Magnetic properties of La1−x Ca x MnO3 (0.5 ≤ x ≤ 0.8) samples with an equivalent average particle size ~50 nm prepared by a sol–gel method were investigated. The charge ordering (CO) transition that is observed in the bulks disappears and the ferromagnetic (FM) transition occurs in all the prepared samples. For all the samples, the spontaneous magnetization (M S) value is much lower than the corresponding theoretic value, which shows that the majority of the sample is antiferromagnetic (AFM). However, the M S value is much larger than the corresponding value reported by some other groups. The invisible of CO transition and the large M S value can be attributed to the good connection among the adjacent particles. Moreover, the exchange bias (EB) phenomenon is observed except the x = 0.5 sample. With x increasing, the M S value decreases and the EB field increases, which can be understood by considering the coexistence of FM phase with Mn3+–Mn4+ spin clusters in the shell and the AFM phase in the core of the nanoparticles.  相似文献   

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