Resonant Scattering of Picosecond Laser Pulses by Atoms in Alkali Metal Vapors

Resonant scattering of ultrashort laser pulses (ULPs) in the vicinity of spectral doublets in monatomic lithium and sodium vapors is studied theoretically. The scattering probability over the entire time of pulse action is calculated as a function of various parameters of the problem (carrier frequency and ULP duration, as well as vapor pressure and temperature). It is shown that the dependence of the total scattering probability on the pulse duration is generally nonlinear by nature.     

Dependence of the Two-Photon Absorption Coefficient of Steel on the Pulse Duration During Its Ablation by Femto- and Picosecond Laser Pulses

JETP Letters - The dependences of the depth of single-pulse ablation of the steel surface on the energy density of ultrashort laser pulses (0.3–12 ps) with a wavelength of 515 nm have the...     

Optical Switch Formation in Antimony Super-Resolution Mask Layers Induced by Picosecond Laser Pulses

Sb is a classic material of a super-resolution near field structure （super-RENS） mask layer in which the optical switch formation is often realized by nanosecond laser pulse stimulation. We achieve fast and repeatable optical switching driven by picosecond laser pulses in a proper fluence range on Sb thin films. The optical properties of Sb thin films before and after switching are studied by surface-sensitive micro-area ellipsometry. The change of optical constants after switching is less than 2% in the whole visible range. The Sb mask layer is shown to be very promising for ultrafast super-resolution optical storage applications.     

Direct Generation of Tunable UV Picosecond Laser Pulses Using Spectrotemporal Selection

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Spectrally Adjustable Picosecond Dye Laser Pulses Generated with Nanosecond Nitrogen Lasers

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A Hydrodynamic Model of the Interaction of Picosecond Laser Pulses with Condensed Targets

We consider a physical model of the interaction of highpower laser pulses with plasma created upon irradiation of condensed targets. The model is based on the equations of singlefluid, twotemperature hydrodynamics taking into account the ponderomotive force, and the Maxwell equations for laser radiation at oblique incidence in the cases of s and ppolarizations. The model takes into account the generation of fast electrons in the conditions of plasma resonance at the critical surface, and their transport with consideration for the friction force, caused by the ionization losses. Heating of ions in the plasma due to beats of the ponderomotive potential is considered. The results of numerical modeling of the interaction of a picosecond laser pulse, containing a prepulse, with a deuterium target at power densities of 10¹⁶–10¹⁷ W/cm² are presented. It is shown that the neutron yield of the DDreaction decreases with increase in prepulse energy, because the plasma created inhibits heating of the dense region of the target where a high rate of the reactions can be realized. It is also shown that the laser radiation losses caused by the stimulated scattering increase with increase in prepulse energy.     

Silicon Ablation by Single Ultrashort Laser Pulses of Variable Width in Air and Water

The ablation of silicon by single laser pulses of variable width (0.3–9.5 ps) with a wavelength of 515 nm has been comparatively studied in air and water. A nonmonotonic behavior of ablation thresholds with a minimum at 1.6 ps, which is due to achieving the thermalization time of the electron and ion subsystems in silicon, has been revealed. It has been shown that, with an increase in the pulse width in the considered width range, the efficiency of the ablation of silicon decreases by a factor of 2.5 in air and increases by a factor of 2 in water. This behavior of ablation in air is attributed to a partial transition from phase explosion to surface evaporation, which is suppressed in water.     

High Repetition Rate Fiber Laser Coupled to a Linear Cavity Generating Picosecond Pulses

An experimental investigation is presented for obtaining picosecond (ps) pulses at a repetition rate of 11 GHz using a fiber laser coupled to an external cavity. Without applying active mode locking and without a nonlinear element in the coupled cavity, pulses of about 15 ps with an average power of 20 mW have been generated using a (cw) diode pump laser. The pulse duration decreases with increasing repetition rate.     

皮秒激光烧蚀Al膜的理论分析与实验验证

为研究Al膜受短脉冲激光作用时的能量传输过程,建立了一维半经典双温热传导模型。根据材料加工过程的熔化现象,对模型的相变区域进行有效设置。通过有限元法求解,得到晶格温度随时间分布的规律。根据自由电子气理论优化了模型,得到Al膜表面反射率和热吸收系数随时间的分布图。得到了激光辐照所产生热电场的分布规律,并分析了电子温度梯度对其影响。描绘出电子漂移运动速度的分布规律,证实激光作用产生的热电场是电子漂移运动的主导因素,发现最大漂移速度位置随时间的延长而加深。对激光作用后的晶格温度进行了区域性分析,定义了过热加热区,并得到激光烧蚀深度随时间的变化关系。实验结果表明,不同功率皮秒激光烧蚀Al膜的深度接近于理论计算结果。     

不同烧蚀条件下飞秒激光脉冲诱导ZnO纳米结构研究

烧蚀条件对飞秒激光脉冲诱导氧化锌纳米结构有重要影响.研究了800 nm,150 fs,250 kHz的飞秒激光脉冲分别在空气中,去离子水中以及无水乙醇中垂直聚焦于氧化锌晶体表面,诱导形成不同形态的纳米结构.实验结果表明,在空气中利用飞秒激光脉冲辐照样品表面,形成了周期为180 nm的纳米线;在去离子水中辐照诱导形成了由氧化锌纳米线聚集而成的"纳米球";在无水乙醇中形成出现分叉结构的纳米线.拉曼光谱分析辐照前后晶体晶相结果表明,形成的纳米结构相对于辐照前特征峰437 cm-1强度有所下降,在570 cm-1处的峰值则显著增强.分析了在各种烧蚀条件下诱导形成纳米结构的演化过程以及物理机理.     

热物性参量对飞秒激光烧蚀金属影响的分子动力学模拟

利用结合双温模型的分子动力学模拟方法,研究了飞秒激光与金属相互作用的烧蚀机制.采用中心波长为800 nm,能量密度从0.043 J·cm~(-2)到0.40 J·cm~(-2)不等,脉宽分别为70 fs和200 fs的激光烧蚀金属镍和铝材料.靶材的温度、原子位型以及内部压力随时间的演化展示了材料热物性参量特性和激光参量对烧蚀结果的影响.结果显示材料电子热传导率对飞秒脉宽激光下的影响仍然较大;对比铝和镍的结果可知,铝的电子晶格耦合系数比镍的小,故电子晶格间的温度梯度持续时间较长;铝的电子热传导系数比镍的大,所以材料上下表面电子温度耦合的时间缩短.铝薄膜表面在能量密度为0.40 J·cm~(-2)激光烧蚀下呈现纳米尺寸的晶体结构.     

Nanoparticles by Laser Ablation

This review concerns nanoparticles collected in the form of nanopowder or a colloidal solution by laser ablating a solid target that lies in a gaseous or a liquid environment. The paper discusses the advantages of the method as compared with other methods for nanoparticle synthesis, outlines the factors on which the properties of the produced nanoparticles depend, explains the mechanisms and models involved in the generation of nanoparticles by laser ablation, clarifies the differences between nanoparticle generation in gaseous and liquid environments, presents some experimental desigins and equipment used by the several groups for nanoparticle generation by laser ablation, describes the techniques used for “tuning” the width of the nanoparticles size distribution, and finally presents a few interesting examples of nanoparticles generated by laser ablation.     

Focusing Waveguide Structure for High-Gradient Electron Acceleration by Picosecond Terahertz Pulses

Radiophysics and Quantum Electronics - We propose an ultra-wideband metal–dielectric structure for high-gradient acceleration of electrons by the field of an ultrashort terahertz pulse. The...     

时空分布的超短激光脉冲烧蚀电介质材料时等离子体的产生

若考虑聚焦平面内固定区域,脉冲空间分布可简化为一维问题.在此基础上,从脉冲的传输过程出发,本文分析了时空分布的超短激光脉冲与电介质材料相互作用时等离子体形成模式.在材料内部累积的能量与脉冲宽度、与空间相关的损伤区域、等离子体形成时间及其吸收系数有关.     

铒激光脉冲消融泌尿结石和胆结石比较研究

利用光学弱相干显微成像系统对脉冲激光消融硬生物组织后形成的凹坑二维和三维形貌进行了扫描,分析了Erbium∶YAG激光脉冲消融生物硬组织特性.结果表明:相同激光参量条件下,消融胆结石比消融泌尿结石具有更高的消融效率;消融胆结石或消融泌尿结石时,脉冲能量越大,消融效率越高;消融效率提高主要体现在凹坑表面直径更宽、高度更深...     

铒激光脉冲消融泌尿结石和胆结石比较研究

利用光学弱相干显微成像系统对脉冲激光消融硬生物组织后形成的凹坑二维和三维形貌进行了扫描,分析了Erbium∶YAG激光脉冲消融生物硬组织特性.结果表明：相同激光参量条件下,消融胆结石比消融泌尿结石具有更高的消融效率|消融胆结石或消融泌尿结石时,脉冲能量越大,消融效率越高|消融效率提高主要体现在凹坑表面直径更宽、高度更深、体积更大|光学弱相干显微成像技术比光学弱相干光层析成像技术测量准确度提高约一个量级,更适合于测量脉冲激光消融生物硬组织后形成的凹坑形貌.     

Obtaining Single Picosecond Pulses in a Short-Cavity Dye Laser with Switching of Lasing to the Saturable Absorber

A new method of lasing of single picosecond pulses in a short-cavity dye laser with spatial separation of the lasing medium and the saturable absorber in the case of pumping by nanosecond pulses with energies much higher than the oscillation threshold has been developed and experimentally realized. The method is based on the use of a high-Q, external cavity tuned to the amplification wavelength of the saturable absorber. The first picosecond pulse is lased at a lasing-medium wavelength and the subsequent pulses are lased at a saturable-absorber amplification wavelength.     

Phase Conjugation with Picosecond Pulses in BaTi03

The self-pumped phase conjugate signal of picosecond laser pulses is observed. The width of the incident laser pulses is about 1.5 ps and their repetition rate is 82 MHz. The wavelength of the pulses can be tuned in the range from 710 nm to 850 nm. The pulse character of the conjugate signal is determined by an autocorrelator. The quality of the conjugate pulses is found to be good by the well-known phase distorter method.