Control of the distribution of surface plasmon local field by altering the surrounding material

The field distribution of the surface plasmon (SP) around a silver nanowire greatly influences its applications for both spectrum enhancement and nano-waveguide. This paper demonstrates the change of the SP local field distribution of a silver nanowire on glass substrate with the refractive index of the covering medium by numerical simulation. The hot energy site is observed focusing on the interface between the nanowire and the surround material of larger refractive index. Moreover, we also find that the surface plasmon field becomes more confined as the refractive index between the substrate and medium has a larger gap, while a homogeneous distribution of the surrounding dielectric material around the nanowire shows a uniform local field distribution with a larger surface plasmon propagation length. The change of related parameters, such as effective index, mode area, and propagation length are also comprehensively investigated against the refractive index for nanowires with 100, 200, 300 nm diameter. Considering the wide use of polymethyl methacrylate (PMMA) material, the field distribution of silver nanowire partially imbedded in PMMA against the PMMA thickness is also studied.     

Numerical Analysis and Comparison of Three Metal-Oxide-Type Super-Resolution Near Field Structures

Based on the Fresnel-Kirchhoff diffraction theory, we build up a Gaussian diffraction model of metal-oxide-type super-resolution near field structure （super-liENS）, which can describe far field optical properties. The spectral contrast induced by refractive index and the structural changes in AgOg, PtOx and PdOz thin films, which are the key functional layers in super-RENS, are studied by using this model. Comparison results indicate that the spectral contrast depends intensively on the laser-induced distribution and change of the refractive index in the metal-oxide films. The readout mechanism of the metal-oxide-type super-RENS optical disc is further clarified. This Gaussian diffraction model can be used as a simple and effective method for choosing proper active materials in super-RENS.     

High-Sensitivity Sensor Based on Surface Plasmon Resonance Enhanced Lateral Optical Beam Displacements

We present a new optical sensor based on surface plasmon resonance （SPIt） enhanced lateral optical beam displacements. Compared with the traditional SPIt methods, the new method provides higher sensitivity to the sensor system. Theoretical simulations show that the refractive index （RI） detection sensitivity of the SPR sensor based on the displacement measurement has a strong dependence on the thickness of the metal film. When the optimal thickness of the metal film is selected, the RI resolutlon of the SPIt sensor is predicted to be 2.2 × 10^-7 refractive index units （RIU）. Furthermore, it is found that the incidence angle can be used as a parameter to adjust the operating range of the sensor to different refractive index ranges.     

Properties of the angular gap in a one-dimensional photonic band gap structure containing single negative materials

Properties of the angular gap in a one-dimensional photonic band gap structure containing single negative materials are investigated. This gap forms at oblique incidence due to the total internal reflection into air when the Snell's law breaks down. Its lower edge occurs at the frequency where the refractive index of one or both layers of the structure approaches zero. This gap is found to be highly sensitive to the incident angle and the polarization of the incident light, but is not affected by the thickness ratio of the layers. It is also shown that the electric field gets extremely enhanced at the lower edge of this gap for transverse magnetic polarization. This highly enhanced electric field can be utilized for certain applications.     

折射率对金属-电介质-金属光子晶体强透射特性的影响

通过改变一个薄电介质层的折射率来研究其对金属-电介质-金属光子晶体(M-D-MPhC)强透射特性的影响。采用与CMOS工艺兼容技术制作了由折射率分别为[nd(SU-8)=1.6,nd(SiO2.1N0.3)=1.6和nd(SiO0.6N1)=1.8]组成的三个正方形晶格圆孔阵列M-D-MPhC结构,利用傅里叶变换红外光谱仪测量其透射光谱。实验结果发现,金-SiO2.1N0.3-金结构能够获得较强的光透射增强效果和较窄的透射峰,证明了M-D-MPhC强透射特性既与中间电介质折射率大小有关,又与其材料制作工艺差异有关。采用时域有限差分(FDTD)法模拟了在相同条件下折射率分别为1.6和1.8组成的M-D-MPhC透射光谱和电场强度密度分布,模拟结果较好地符合了实验发现。     

Electromagnetic Parameters Model and Microwave Absorption for Composite Coatings Containing Magnetic Particles

Considering the eddy current effect of the magnetic metal particles in a high frequency electromagnetic field, we extend the Maxwell-Garnett law by introducing the eddy-effect parameter A which is as functions of the radius, permeability and electric conductivity of the metal particle medium. It is obvious that the computational result agrees with the experiment, which indicates that the extended Maxwell-Garnett law can be used to predict the effective electromagnetic parameters of a dilute metal-insulator composite medium in a high-frequency electromagnetic field.     

The preparation and refractive index of BST thin films

Radio-frequency magnetron sputtering technique is used to deposit Ba_0.65Sr_0.35TiO₃ (BST) thin films on fused quartz substrates. In order to prepare the high-quality BST thin films, the crystallization and microstructure of the films were characterized by X-ray diffraction (XRD), field emission scanning electron microscopy (FESEM) and atomic force microscopy (AFM). More intense characteristic diffraction peaks and better crystallization can be observed in BST thin films deposited at 600 °C and subsequently annealed at 700 °C. The refractive index of the films is determined from the measured transmission spectra. The dependences of the refractive index on the deposition parameters of BST thin films are different. The refractive index of the films increases with the substrate temperature. At lower sputtering pressure, the refractive index increases from 1.797 to 2.197 with pressure increase. However, when the pressure increases up to 3.9 Pa, the refractive index reduces to 1.86. The oxygen to argon ratio also plays an important effect on the refractive index of the films. It has been found that the refractive index increases with increase in the ratio of oxygen to argon. The refractive index of BST thin films is strongly dependent on the annealing temperature, which also increases as the annealing temperature ascends. In a word, the refractive index of BST thin films is finally affected by the films’ microstructure and texture.     

用于飞秒激光纳米加工的TiO_2粒子阵列诱导多种基底表面近场增强

利用纳米粒子辅助对飞秒激光能量进行空间局域化,使其在基底表面诱导产生纳米尺度的近场增强,这对超衍射极限微结构加工具有重要意义.目前对于粒子阵列诱导飞秒激光纳米孔加工的研究仅限于金属Au粒子及低折射率聚苯乙烯介电粒子等,本文提出并开展了应用高折射率TiO_2介电粒子阵列作为辅助诱导激光近场增强从而进行飞秒激光超衍射纳米孔加工的研究.对TiO_2介电粒子阵列在Si,Pt及SiO_2表面的近场强度分布进行了数值模拟,研究其基底表面近场增强的规律及物理过程.研究结果发现,使用硅基底时,阵列与单一TiO_2球形粒子相比其近场增强仅下降约30%;相对于入射激光强度而言,在直径约为100nm的空间范围内获得140倍的近场增强,这一现象可用于百纳米孔的激光加工.同时在其他典型基底的理论计算结果中也表明,几乎在所有金属及介电材料表面均可以实现良好的百纳米空间范围内的近场增强,并且具有近场随着基底折射率变大而增强的规律.这些现象的产生归因于TiO_2粒子中磁四极振荡产生的激光前向场增强及粒子与基底的耦合作用.进一步引入镜像电荷模型对基底光学参数对其表面近场增强的影响规律进行了分析和解释.本文的模拟结果对飞秒激光近场超衍射极限纳米加工的应用有着重要的意义.     

Electrically controlled optical bandgap in a structurally chiral material

The propagation of light along the axis of non-homogeneity of a structurally chiral medium (SCM) under the influence of a low-frequency (dc) electric field aligned along the same axis is investigated. The Pockels effect is assumed to occur, and the SCM is taken to possess locally a point group symmetry. The frequency-domain Maxwell curl equations are cast in a 4 × 4 matrix representation, and the Oseen transformation is invoked. The band structure is analyzed, as are also the eigenvectors as well as the transfer matrix. Finally, the reflection and transmission of a plane wave due to a SCM of finite thickness is considered. The low-frequency electric field is shown to control the bandgap.     

Dielectric supported ring-shaped metal disks on a metal film for ultrasensitive refractive index sensing

We experimentally report a magnetic plasmonic metamaterial, which is constructed with a metal ring-shaped disk array supported by a dielectric layer on a metal film for high sensitive refractive index sensing. An ultrasensitive refractive index sensitivity of about 1842?nm per refractive index unit is achieved through the reflection spectrum measurement. We attribute the high sensitivity to greatly enhanced electric field intensity and its large spatial overlapping with the surrounding medium to sense. The present plasmonic structure provides an effective way for high sensitive chip-based biochemical sensors and integrated devices.     

带有多孔二氧化硅间隔层的导模共振光栅实现染料激光器发射增强

导模共振光栅是一种典型的平面波导共振结构,可在光栅表面或波导层内形成较强的局域电场,能增强光与物质的相互作用.本文在导模共振结构的光栅层和基底层之间,引入低折射率的多孔二氧化硅间隔层,显著增强了局域电场与增益介质的接触度.结果表明,引入多孔二氧化硅后,共振产生的电场增强区域上移至激光染料层,增加了激光染料与电场的相互作用,实现了激光出射增强.本文基于时域有限差分法,对结构参数进行分析优化,研究了820 nm共振波长激发下的出射激光特性,得到了连续的激光出射,其能量阈值约为2.5 mJ/cm^2,线宽约为0.3 nm.本文提出的结构实现了对表面局域电场的有效调控,增强了激发光与增益介质的相互作用,不但可应用于激光器,还为其它发光器件的设计提供了参考.     

三角形银纳米柱阵列传感乙醇气体方法研究

提出了一种基于金属纳米结构局域表面等离子体共振光谱的有机气体的传感方法.通过时域有限差分法设计了一种具有较高折射率灵敏度的三角形纳米柱阵列,并利用纳米球光刻法进行了制作.对乙醇蒸汽的传感实验结果证明,所制作的三角形银纳米柱对乙醇分子浓度非常敏感,其探测灵敏度达到24ppm/nm.该金属纳米结构传感有机气体的方法有望应用于环境监测等方面.     

一种简单精准的渐变折射率分布光波导分析方法

渐变折射率分布的光波导分析对光波导器件的设计和研究至关重要, 近年来已提出了多种分析方法, 然而在简便性或准确性上都存在着不足. 为此, 提出了一种分析渐变折射率分布光波导的方法, 能够结合现有的Wentzel-Kramers-Brillouin近似法和离散化的波动方程, 构建模场分布, 再结合变分运算方程和修正的模式本征方程, 计算出较为精确的有效折射率. 与其他分析方法相比, 该方法较为简单, 而且有一定的精度.     

Generalized wave coupling theory of linear electro-optic effect in absorbent medium

Starting from Maxwell’s equations and considering the linear electro-optic effect as a perturbation, we present a generalized wave coupling theory of linear electro-optic effect in absorbent medium. We give the rigorous solution of the resultant equations for a light wave propagating along any direction with an external dc electric field along an arbitrary direction. As an application, we use the theory to discuss the influence of absorption on the light wave in a KTP crystal. The results demonstrate that the absorption coefficients influence not only the amplitude but also the phase of the light wave.     

利用Ag@SiO_2纳米粒子等离子体共振增强发光二极管辐射功率的数值研究

金属纳米粒子利用其局域表面等离子体共振效应(LSPR),可以增强附近荧光分子的自发辐射速率,因而在光学传感、光电器件等领域中具有潜在的应用价值.金属纳米粒子的LSPR与其自身的材料、形状、尺寸以及周围环境介质密切相关,这影响着纳米粒子在具体器件中的应用.本文利用三维时域有限差分法,研究了相同体积的球形、椭球形、立方形与三棱柱形银纳米粒子对薄膜发光二极管辐射功率的影响;计算了不同形状银纳米粒子对偶极子光源辐射功率和薄膜器件光出射强度的增强,并结合LSPR效应讨论了辐射功率变化的物理机理.研究结果表明:银纳米粒子自身形状尖锐程度的增加有利于提高LSPR的共振强度;同时纳米粒子的形状影响了LSPR共振电场与薄膜器件中偶极子辐射电场之间的耦合作用,其中立方形纳米粒子因为能实现最强的耦合作用而对器件的辐射功率增强最大.在此基础上进一步讨论了不同薄膜材料对LSPR共振及光源辐射功率的影响,发现较高的材料折射率有利于增强金属纳米粒子的LSPR与器件的耦合作用,从而改善发光二极管性能.     

偏振方向及结构间耦合作用对空心方形银纳米结构表面等离子体共振的影响

空心方形纳米结构能够激发更大面积的增强电场,故其可以作为衬底用于表面增强拉曼散射.应用离散偶极子近似算法研究了空心方形银纳米结构的消光光谱及其近场电场分布与入射光偏振方向之间的关系.研究表明,空心方形银纳米结构的表面等离子体共振峰不随入射光偏振方向的改变而移动,但是其表面增强电场分布却强烈地依赖于入射光的偏振方向.另外,还讨论了空心方形银纳米结构间的耦合作用对其表面等离子体共振模式的影响.结果发现,可以通过调节结构间的距离来改变结构间的耦合作用,同时改变了表面等离子体共振峰的位置.这些结果将为理解闭合纳米 关键词： 空心方形银纳米结构 表面等离子体 偏振 电场耦合     

Plasmonic refractive index sensor based on the combination of rectangular and circular resonators including baffles

We numerically designed a plasmonic refractive index sensor with high sensitivity and tunable optical feature based on two metal-insulator-metal bus waveguides connecting with the central-coupled rectangular and circular ring resonators, including silver (Ag) baffles. In the design process, Ag baffles' influence on transmittance spectrum, magnetic and electric field distributions, surface power flow intensity, energy streamlines, and sensor performance are investigated using the finite element method. The proposed structure can use as a high precision plasmonic refractive index sensor for refractive index in the increment range of 0.01. The maximum sensitivity can reach 3400 nm/RIU (RIU is a refractive index unit), which remarkably increases the sensitivity of 1.36 times compared to the case without Ag baffles. Besides, the figure of merit and quality factor can achieve 36.00 and 42.28, respectively. The sensitivity and figure of merit can be increased by adding the Ag baffles in the proposed plasmonic sensor system, generating an additional gap plasmon resonance mode that cannot find in a typical case.     

Optical and structural parameters of the ZnO thin film grown by pulsed filtered cathodic vacuum arc deposition

Transparent conductive ZnO film was deposited on glass substrate by pulsed filtered cathodic vacuum arc deposition (PFCVAD). Optical parameters such as absorption coefficient α, the refractive index n, energy band gap E_g and dielectric constants have been determined using different methods. Kramers-Kronig and dispersion relations were employed to determine the complex refractive index and dielectric constants using reflection data in the ultraviolet-visible-near infrared regions. The spectra of the dielectric coefficient were used to calculate the energy band gap and the value was 3.24 eV. The experimental energy band gap was found to be 3.22 eV for 357 nm thick ZnO thin film. The envelope method was also used to calculate the refractive index and the data were consistent with K-K relation results. The structure of the film was analyzed with an x-ray diffractometer and the film was polycrystalline in nature with preferred (002) orientation.     

Refractive index of aqueous solution of CdTe quantum dots

The refractive index of aqueous solution of CdTe quantum dots is measured by the retroreflection method on the fiber-optic end face. The dependence of the refractive index on the temperature and the concentration of the quantum dots aqueous solution are investigated. The data of refractive index we measured in this paper may be useful in photonics applications of aqueous solution of CdTe quantum dots.     

Nonlinear refraction of silver nanowires from nanosecond to femtosecond laser excitation

In order to investigate the effect of pulse width and solvent on the nonlinear properties of metal nanostructures, silver nanowires were fabricated in a direct current electric field (DCEF) using a solid-state ionic method and characterized by transmission electron microscopy (TEM) and X-ray diffraction (XRD). The nonlinear refractive index (γ) of silver nanowires suspended in ethanol was measured using the Z-scan technique and laser radiation of various (femto-, pico-, and nanosecond) pulse durations. Experimental results indicated that silver nanowires have obvious positive refractive nonlinearities and γ (the Kerr-induced self-focusing) increases as the pulse duration increases from 7.4×10⁻⁸ cm²/GW at 110 fs to 1.6×10⁻⁴ cm²/GW at 8 ns, due to the additional influence of the atomic reorientational Kerr effect in the case of longer pulses. Due to the solvent dependence of the nonlinear behavior of the silver nanowires, the nonlinear absorption and refraction of silver nanowires suspended in de-ionized water are smaller than those of silver samples suspended in ethanol. The thermal nonlinearities are insignificant in our experimental conditions.