驻波声场中单分散细颗粒的相互作用特性

利用外加声场促进悬浮在气相中的细颗粒发生相互作用,进而引起颗粒的碰撞和凝并,使得颗粒平均粒径增大、数目浓度降低,是控制细颗粒排放的重要技术途径.为探究驻波声场中单分散细颗粒的相互作用,建立包含曳力、重力、声尾流效应的颗粒相互作用模型,采用四阶经典龙格-库塔算法和二阶隐式亚当斯插值算法对模型进行求解.将数值模拟得到的颗粒声波夹带速度和相互作用过程与相应的解析解和实验结果进行对比,验证模型的准确性.进而研究颗粒初始条件和直径对相互作用特性的影响.结果表明,初始时刻颗粒中心连线越接近声波波动方向、颗粒位置越接近波腹点,颗粒间的声尾流效应就越强,颗粒发生碰撞所需要的时间就越短.研究还发现,颗粒直径对颗粒相互作用的影响取决于初始时刻颗粒中心连线偏离声波波动方向的程度.当偏离较小时,颗粒直径越大,颗粒发生碰撞所需要的时间越短;当偏离很大时,直径较小的颗粒能够发生碰撞,而直径较大的颗粒则无法发生碰撞.     

Describing Hydrodynamic Particle Removal from Surfaces Using the Particle Reynolds Number

The fundamental processes related to the removal of fine particles from surfaces in a hydrodynamic flow field are not adequately understood. A critical particle Reynolds number approach is proposed to assess these mechanisms for fine particles when surface roughness is small compared to particle diameter. At and above the critical particle Reynolds number, particle removal occurs, while below the critical value, particles remain attached to a surface. The system under consideration consists of glass particles adhering to a glass surface in laminar channel flow. Our results indicate rolling is the removal mechanism, which is in agreement with the literature. Theoretical results of the critical particle Reynolds number model for rolling removal are in general agreement with experimental data when particle size distribution, particle and surface roughness, and system Hamaker constant are taken into account.     

Multiple size group analysis for transient radiative heating of particle polydispersions

The transient radiative heating of particle polydispersions initially at uniform temperature is numerically analyzed. Due to the different radiative heating characteristics between particles, the temperature evolution of particle changes with particle diameter. To take local thermal nonequilibrium between particles into consideration, the particles are discretized into several size groups. The radiative transfer equation in particle polydispersions and the transient energy equation for each particle group are solved by the discrete ordinates method and an implicit finite difference method, respectively. The effects of the standard deviation of particle diameter and the emissivity of particle surface on the thermal evolution of particle polydispersions are analyzed. The results show that, omitting thermal nonequilibrium of particles will result in significant errors in the calculation of radiative heat transfer, especially when the nonuniformity of particle diameter is large.     

Aerosol light absorption and its measurement: A review

Light absorption by aerosols contributes to solar radiative forcing through absorption of solar radiation and heating of the absorbing aerosol layer. Besides the direct radiative effect, the heating can evaporate clouds and change the atmospheric dynamics. Aerosol light absorption in the atmosphere is dominated by black carbon (BC) with additional, significant contributions from the still poorly understood brown carbon and from mineral dust. Sources of these absorbing aerosols include biomass burning and other combustion processes and dust entrainment.For particles much smaller than the wavelength of incident light, absorption is proportional to the particle volume and mass. Absorption can be calculated with Mie theory for spherical particles and with more complicated numerical methods for other particle shapes.The quantitative measurement of aerosol light absorption is still a challenge. Simple, commonly used filter measurements are prone to measurement artifacts due to particle concentration and modification of particle and filter morphology upon particle deposition, optical interaction of deposited particles and filter medium, and poor angular integration of light scattered by deposited particles. In situ methods measure particle absorption with the particles in their natural suspended state and therefore are not prone to effects related to particle deposition and concentration on filters. Photoacoustic and refractive index-based measurements rely on the heating of particles during light absorption, which, for power-modulated light sources, causes an acoustic signal and modulation of the refractive index in the air surrounding the particles that can be quantified with a microphone and an interferometer, respectively. These methods may suffer from some interference due to light-induced particle evaporation. Laser-induced incandescence also monitors particle heating upon absorption, but heats absorbing particles to much higher temperatures to quantify BC mass from the thermal radiation emitted by the heated particles. Extinction-minus-scattering techniques have limited sensitivity for measuring aerosol light absorption unless the very long absorption paths of cavity ring-down techniques are used. Systematic errors can be dominated by truncation errors in the scattering measurement for large particles or by subtraction errors for high single scattering albedo particles. Remote sensing techniques are essential for global monitoring of aerosol light absorption. While local column-integrated measurements of aerosol light absorption with sun and sky radiometers are routinely done, global satellite measurements are so far largely limited to determining a semi-quantitative UV absorption index.     

部分状粒子处理方法及其对云微物理参数测量的影响

作为云微物理过程测量的重要利器,机载云降水粒子成像仪在云降水物理与人工影响天气研究中具有重要的作用.从采样结果来看,机载云降水粒子成像仪所测粒子图像中含有大量的粒子图像仅是粒子的一部分而已,即部分状粒子.因其数量较多,对该类粒子所选处理方法不同,会引起测量结果的很大差异.本文介绍并分析了现有部分状粒子处理方法的优劣,通过对部分状粒子的再定义与粒子形状分类,提出了一个融合粒子形状识别技术、"粒径重构"和"中心在内"方法的新的部分状粒子处理方法;利用实测数据,对所提方法与现有方法进行了云微物理参量处理结果的对比,发现本文所提方法与"粒径重构"方法处理结果比较一致,能较好地克服"整体在内"与"中心在内"两种方法存在的缺陷;同时,在针柱状粒子占比较多情形下,本文所提方法要比"粒径重构"方法处理后的结果相对合理.因此本文所提方法对仪器所测粒子数据处理具有更好的适应性.     

基于拟颗粒的气固两相曳力模型研究

为了研究气固两相流动大涡模拟中合适的曳力计算模型,本文引入拟颗粒和拟颗粒表面能的概念,通过拟颗粒表面能与外界输入能量之间的平衡关系来确定拟颗粒的粒径。根据拟颗粒粒径,得到运算量较小且考虑颗粒团聚效应的曳力计算模型。应用本文的曳力计算模型对二维竖直槽道内稠密气固两相流动进行了大涡模拟,结果表明颗粒的浓度分布具有上稀下浓,壁面附近浓中心稀及颗粒聚集等特点。这与实验结果在定性上是一致的。对气相和颗粒相的瞬时速度场进行了分析,发现气相和颗粒相速度场分布的非对称性是形成颗粒浓度分布壁面附近浓中心稀的重要原因之一。     

圆截面直流道中微粒黏弹性聚焦机理研究

微粒黏弹性聚焦技术近年来受到了广泛的研究重视, 但影响粒子聚焦特性的关键参数调控机理仍不清楚. 基于此目的, 本文量化研究了圆截面直流道中非牛顿流体诱导微粒黏弹性聚焦的行为, 给出了流速和流道长度对粒子聚焦特性的调控机理. 具体而言: 首先, 对比分析不同黏度牛顿流体(水和22 wt%甘油水溶液)和非牛顿流体(8 wt%聚乙烯吡咯烷酮水溶液)中粒子横向迁移行为, 发现非牛顿流体中粒子将在弹性力主导下聚焦至流道中心区域, 而牛顿流体中粒子则在惯性升力主导下迁移形成Segré-Silberberg圆环. 其次, 量化分析粒子尺寸和驱动流速对黏弹性聚焦效果的影响, 发现随着流速的增加, 粒子聚焦效果逐渐变好并最终趋于稳定, 且大粒子较小粒子具有更好的聚焦效果. 最后, 研究粒子沿流道长度的动态聚焦过程, 推导并验证了粒子聚焦所需安全流道长度的数学模型, 发现大粒子聚焦所需安全流道长度显著短于小粒子. 上述研究结果对于提升粒子黏弹性聚焦机理和过程的理解, 实现微粒聚焦特性的灵活控制具有非常重要的意义.     

透过率起伏光谱分析法测粒技术

提出的透过率起伏光谱分析法是一种新的颗粒测量方法。采用一细小光束照射匀速流动的颗粒系统,通过采集透射光起伏信号,经统计处理得到透过率的平均值与起伏谱。通过求解逆问题,从透过率的起伏谱中得到颗粒粒径分布信息,再结合透过率的平均值得到颗粒的体积分数信息。给出了关于单层颗粒透过率的平均值与起伏谱的理论表达式,并推广到三维单分散和多分散的颗粒系统。对粒径在32~425μm内的稀薄颗粒系进行了部分实验测试和模拟计算,结果表明该方法可同时对颗粒粒径分布和体积分数进行有效测量。     

Accumulating particles at the boundaries of a laminar flow

The accumulation of small particles is analyzed in stationary flows through channels of variable width at small Reynolds number. The combined influence of pressure, viscous drag and thermal fluctuations is described by means of a Fokker-Planck equation for the particle density. It is shown that for extended spherical particles the shape of the fluid domain gives rise to inhomogeneous particle densities, thereby leading to particle accumulation and corresponding depletion. For extended spherical particles, conditions are specified that lead to inhomogeneous densities and consequently to regions with particle accumulation and depletion.     

Microwave scattering properties of sand particles: Application to the simulation of microwave radiances over sandstorms

The single-scattering properties of sand/dust particles assumed to be ellipsoids are computed from the discrete dipole approximation (DDA) method at microwave frequencies 6.9-89.0 GHz in comparison with the corresponding Lorenz-Mie solutions. It is found that the single-scattering properties of sand particles are strongly sensitive to the shapes of the particles. The bulk scattering properties of sandstorms composed of spherical or nonspherical particles are investigated by averaging the single-scattering properties of these particles over log-normal particle size distributions. Furthermore, a vector radiative transfer model is used to simulate microwave radiances. The microwave brightness temperatures in the vertical polarization model are essentially not sensitive to sand particle habit, whereas microwave brightness temperature polarization differences are influenced by particle habit. It is shown that microwave brightness temperatures and brightness temperature polarization differences may be useful for estimating the effective particle sizes and mass loading of sandstorms.     

Flame structure and burning velocity of flames propagating in binary iron aerosols

A numerical study was performed for binary dispersed iron aerosols in air using different particle sizes with constant average particle size. The effects of particle size and density of the two aerosols on flame structure and speed are systematically investigated. Varying the amount of small and big particles results in separated and overlapped flame fronts. For higher values of particle size ratio (ratio between the size of big and small particles) and density of small particles, flame fronts are observed to overlap. The flame speed of the binary mixture is compared with the mono-dispersed case and the difference is analyzed for different particle size ratios. The addition of a small fraction of small particles in the binary mixture is found to result in a substantial increase in the flame speed if the particle size ratio is large. Detailed analyses on the variation of the total amount of fuel shows the particle size ratio determines the equivalence ratio at which the maximum flame speed occurs. The maximum flame speed as a function of equivalence ratio was observed to move from the lean to the rich side for particle size ratio sufficiently large enough.     

Characterization of Agglomerated and Aggregated Aerosol Particles Using Image Analysis

Accurate particle size characterization of aggregated and agglomerated particles is only possible by analysis of photographs. Both the primary particle size and the morphology of the aggregate are important experimental results. Since standard image analysis techniques for particle size analysis usually recognize only single particles, a new programme, called here Sparse Hough Transformation, was developed for the automated recognition of spherical particles within an aggregate. The method is shown to perform well, even for images with many overlapping particles. The structure of the aggregate is analysed using the fractal dimension, determined from the density-density correlation function. Finite size effects, important when dealing with aggregates containing few primary particles, are taken into account by including a cut-off function.     

Light scattering by coated Gaussian and aggregate particles

Light scattering by nonspherical and inhomogeneous small particles is studied by varying particle shapes, sizes, and compositions. We introduce an efficient tool for deforming particle shape and composition by adding a coating on an initial particle. This concave-hull transformation is applied to wavelength-scale Gaussian and aggregate particles, and the differences in the optical properties of the coated particles are compared to those of the uncoated geometries. The light-scattering computations are performed using the discrete-dipole approximation method which allows for internal inhomogeneity and irregular particle shapes. The results are analyzed concentrating on the intensity of the scattered light, the degree of linear polarization for unpolarized incident light, and the depolarization ratio. Polarization results yield the most significant differences and, moreover, coated aggregates are observed to produce net positive polarization, whereas it is negative for the Gaussian particles, also resembling the polarization of a spherical particle. As for the depolarization ratio, an intriguing double-lobe feature is observed near the backscattering direction for both particle geometries regardless of size, shape, and composition. The double-lobe maxima and minima generally coincide with those of the intensity and polarization.     

Interactions of charged dust particles in clouds of charges

Two charged dust particles inside a cloud of charges are considered as Debye atoms forming a Debye molecule. Cassini coordinates are used for the numerical solution of the Poisson-Boltzmann equation for the charged cloud. The electric force acting on a dust particle by the other dust particle was determined by integrating the electrostatic pressure on the surface of the dust particle. It is shown that attractive forces appear when the following two conditions are satisfied. First, the average distance between dust particles should be approximately equal to two Debye radii. Second, attraction takes place when similar charges are concentrated predominantly on the dust particles. If the particles carry a small fraction of total charge of the same polarity, repulsion between the particles takes place at all distances. We apply our results to the experiments with thermoemission plasma and to the experiments with nuclear-pumped plasma.     

Traffic of indistinguishable particles in complex networks

In this paper, we apply a simple walk mechanism to the study of the traffic of many indistinguishable particles in complex networks. The network with particles stands for a particle system, and every vertex in the network stands for a quantum state with the corresponding energy determined by the vertex degree. Although the particles are indistinguishable, the quantum states can be distinguished. When the many indistinguishable particles walk randomly in the system for a long enough time and the system reaches dynamic equilibrium, we find that under different restrictive conditions the particle distributions satisfy different forms, including the Bose--Einstein distribution, the Fermi--Dirac distribution and the non-Fermi distribution (as we temporarily call it). As for the Bose--Einstein distribution, we find that only if the particle density is larger than zero, with increasing particle density, do more and more particles condense in the lowest energy level. While the particle density is very low, the particle distribution transforms from the quantum statistical form to the classically statistical form, i.e., transforms from the Bose distribution or the Fermi distribution to the Boltzmann distribution. The numerical results fit well with the analytical predictions.     

On aggregate structures in a rod-like haematite particle suspension by means of Brownian dynamics simulations

We have investigated aggregation phenomena in a suspension composed of rod-like haematite particles by means of Brownian dynamics simulations. The magnetic moment of the haematite particles lies normal to the particle axis direction and therefore the present Brownian dynamics method takes into account the spin rotational Brownian motion about the particle axis. We have investigated the influence of the magnetic particle–field and particle–particle interactions, the shear rate and the volumetric fraction of particles on the particle aggregation phenomena. Snapshots of aggregate structures are used for a qualitative discussion and the cluster size distribution, radial distribution function and the orientational correlation functions of the direction of particle axis and magnetic moment are the focus for a quantitative discussion. The significant formation of raft-like clusters is found to occur at a magnetic particle–particle interaction strength much larger than that required for a magnetic spherical particle suspension. This is because the rotational Brownian motion has a significant influence on the formation of clusters in a suspension of rod-like particles with a large aspect ratio. An applied magnetic field enhances the formation of raft-like clusters. A shear flow does not have a significant influence on the internal structure of the clusters, but influences the cluster size distribution of the raft-like clusters.     

Combustion of micron-sized particles of titanium and zirconium

Particles of titanium and zirconium in the size range of 2–25 μm are ignited while passing through a CO₂ laser beam and their combustion is monitored optically. Prior to ignition, particles pass through a low-power auxiliary laser beam so that the diameter of each ignited particle is measured in situ based on the amplitude of the scattered light pulse. The particles of both Ti and Zr are observed to exhibit micro explosions, similar to those observed for larger size particles of these metals. Particle emission traces are recorded, and a data processing routine is established for discounting emission signals produced by unignited particles and particles partially combusted within the CO₂ laser beam. Burn times and combustion temperatures are measured and compared to earlier measurements for coarser particles of the same metals. For both metals, average combustion temperatures implied by the emission spectra are very close to their respective adiabatic flame temperatures. For both metals, for the particle size range considered, particle combustion temperatures do not depend on the particle size. The particle burn times were found to be only weak functions of the particle size; burn times for Zr are shorter and temperatures are higher compared to the similarly sized Ti particles.     

Colloidal Analysis of Particles Extracted from Microalloyed Steels

Different colloidal particle characterization methods are examined for their suitability to determine the particle size distribution of particles extracted from steels. Microalloyed steels are dissolved to extract niobium and titanium carbonitride particles that are important for the mechanical properties of these steels. Such particles have sizes ranging from several nanometers to hundreds of nanometers depending on the precipitation stage during the thermomechanically controlled rolling process. The size distribution of the particles is analyzed by dynamic light scattering (DLS), analytical ultracentrifugation (AUC), and hollow fiber flow field-flow fractionation (HF5) and compared to data obtained for reference particles as well as data from electron microscopy, the standard sizing technique used in metallurgy today. AUC and HF5 provide high-quality size distributions, average over large particle numbers that enables statistical analysis, and yield useful insights for alloy design; however, DLS fails due to a lack of resolution. Important aspects in the conversion and comparison of size distributions obtained for broadly distributed particle systems with different measurement principles and the role of surfactants used in sample preparation are discussed.     

Algorithm for particle packing based on Aristotelian mechanics

A dynamic algorithm is proposed for three-dimensional packing of spherical solid particles. The particles are deposited within a specified region with a fixed rigid boundary. The velocity of each particle is proportional to its weight and forces due to contact of the particle with the boundary and neighbor particles. Dimensional analysis of the equations of particle motion is performed. The average density and coordination number distribution for an equilibrium packing are calculated. The dependence of these characteristics on viscosity, granulometric composition, and representation of initial conditions (numerical analogue of material pouring into a specified volume) is studied.