Halbwertszeit,Elektroneneinfangverhältnis und β-Spektrum des Tl204

Half-life,P _L /P _K -capture ratio andβ-spectrum of Tl²⁰⁴ were studied with a scintillation spectrometer. To avoid source absorption and scattering troubles, the Tl²⁰⁴ source was built in in the lattice of NaJ(Tl)-crystals. The half-life measurements were performed over a period of 2,2 years, and we obtained a half-life of 3.81±0.04 years. TheP _L /P _K -capture ratio was determined at 0.41±0.03. This ratio gives a desintegration energy of 442 _?24 ⁺³⁰ keV for the unique first forbidden electron capture decay of Tl²⁰⁴. For the branching ratio of electron capture toβ ^?-decay we found a value of (2.15±0.06)% and for the ratio ofK-capture toβ ^?-decay a value of (1.53±0.05)%. Theβ ^?-spectrum of Tl²⁰⁴ was measured from 200 down to 6 keV and yields an experimental shape factor which deviates below an energy of ～90 keV from the theoretical shape factorq ² L ₀+9L ₁. Reasons for this deviation which is opposite to the one obtained with magnetic spectrometers are discussed.     

DasL/K-Einfangverhältnis von51Chrom

We have investigated theL/K-capture ratio of⁵¹Cr. The values obtained for the transitions to the first excited state of⁵¹V and for both transitions to the first excited state and the ground state of⁵¹V are(N _L /N _K )_A=0.1044±2% and (N _L/N_K)_G=0.1033±3% respectively. They are in fairly good agreement with theoretical results which take exchange corrections into account. But there still remains a dependence of the results on the method used to obtain the capture numbers from the measured spectrum.     

Verzweigungsverhältnisse und Konversionskoeffizienten von angeregten Zuständen des208Tl

The branching ratios of theγ rays of the second and fourth excited states of²⁰⁸Tl have been investigated by coincidence measurements between the α rays of²¹²Bi and subsequent 40keVγ ray. The detectors employed were a silicon surface barrier counter for α particles, and a 1.5 in ×2 mm NaJ (Tl) crystal forγ rays. It has been found that (75.6±3.7)% of all transitions of the 328 keV state and (94±7)% of all transitions of the (492 keV+473 keV) states populate the first excited state of²⁰⁸Tl. The 40 keV state is excited to (3.4±0.3)% by transitions of higher excited states relative to the direct excitation by α particles. The number of α particles with energyE _α = 6.047 MeV and the number of subsequent 40keVγ rays resulted in a conversion coefficient α(40keV)=22.55± 0.46. Similarly coincidence measurements between Tl-x rays and α particles have been used to determine theK- conversion coefficients α_K(328 keV)=0.31±0.03 and α_K(492 keV+ 473keV)=0.100±0.015. The experimental results are in good agreement with the theoretical values ofSliv.     

The determination by an independent method ofP k electron capture probabilities in133Ba and139Ce decays gamma decay of133Ba

The electron capture decays of¹³³Ba (10.4 y) and¹³⁹Ce (140 d) were investigated with high resolution Ge(Li) detectors. By x-ray — γ-ray coincidences values of the quantityP _k ω _k ? _k for various transitions in the decay of¹³³Ba and¹³⁹Ce are obtained. The factor ω _k ? _k was measured independently by means ofK-conversion electron-K x-ray coincidences and was then used to determineP _k , theK-capture probability. The independent measurement of the product ω _k ? _k , together with recent accurate values of ω _k , provides a new method for the accurate calibration of semiconductor x-ray detectors. In the decay of¹³⁹Ce, a value ofP _k =0.78±0.03 is found (where the error represents twice the standard deviation) from whichQ _ec =326 _?30 ⁺⁷⁰ keV to the¹³⁹La ground-state is found by use of theory. In¹³³Ba decay, values are found ofP _k 1=0.72±0.04 for theEC transition to the 437 keV level in¹³³Cs,P _k 2=0.80±0.07 to the 384 keV level, and from an independent measurement, the ratioP _k 1/P _k 2=0.87±0.07. From these results the ground-state value ofQ _ec =522 _?10 ⁺²⁰ keV is derived from theory for¹³³Ba decay. The gamma spectrum of¹³³Ba also was remeasured. From the present gamma intensities and previous conversion electron intensities, new values forK-shell conversion coefficients are obtained. Previously reported γ-rays at 35 and 391 keV are not confirmed.     

Winkelkorrelationsmessungen an >30y Holmium 166 und Bestimmung desg R -Faktors des 4+-Rotationsniveaus von Erbium 166

The spins of several excited states of Er¹⁶⁶ have been investigated byγγ-angular correlation measurements. The spin sequence 0+, 2+, 4+, 6+ for the ground state rotational band was presumed to be correct. Unique assignments were derived for the states of 1076 keV, 1377 keV and 1785 keV asI=5, 7 and 6 respectively. These results are in agreement with the spins proposed byGallagher jr. andSoloviev. The multipolarities of theγ-transitions of 408 keV, 709 keV, 811 keV and 831 keV were derived as 95%E1+(5±1)%M2, 99·6%E1+(0·4±0·5)%M2, 99·1%E2+(0·9±0·3)%M1, and 96·1%E2+(3·9±1)%M1 respectively. The unusual mixing ratios of the transitions of 811 keV and 831 keV can be understood as a consequence of theK-selection rule. Eachγ-transition from the 1785 keV state should be stronglyK-forbidden and one expects a half-life ofT _1/2≈3·10^?9s. A measurement of the time spectrum of the coincidences between theβ-radiation and the high energyγ-lines gave however:T _1/2(1785 keV state)≦3·10^?10s. The rotation of the angular correlation between the 184 keV line and theγ-group at 820 keV has been measured in an external magnetic field of 53000 gauss as:ω·τ(4+)=0·083±0·006. This value contains small corrections for an additional rotation of the angular correlation of the 831 keV–184 keV triple cascade in the 6+state and for a small attenuation by internal fields. WithT _1/2(4+state)=1·23·10^?10s, andβ=7·08 one gets for theg-factorg _R=+0·266±0·024 in good agreement with recent results for the 2+ state.     

Die Lebensdauer des 23/2-Dreiteilchenniveaus des Hafnium 177 und sein Zerfall durchK-verbotene Gamma-Übergänge

An isomeric state of Hf¹⁷⁷ withT _1/2=(1,12±0,10)s was found by a fast chemical separation of the hafnium daughter from the 155d Lu^177m activity. We measured the same half-life by observing the delayedβ-γ-coincidences. A systematic investigation of the whole region 5s≧T _1/2≧10^?7s by the technique of delayed coincidences gave no further isomerism. We assign the observed half-life to the 23/2 three particle state of Hf¹⁷⁷ at 1315 keV and assume that the second hypothetical three particle state at 1337 keV does not exist. The 21/2 rotational state of theK=9/2 band is populated by a strongly converted 14,16 keVγ-transition from the isomeric state at 1315 keV. The 14,16 keVM _I andN _I conversion lines were observed by use of a double focusing magneticβ-spectrometer. The isomerism is caused by theK-selection rule. The retardation of the following threeγ-transitions by different degrees ofK-forbiddeness is discussed. The pulse height spectrum, measured by means of a Li-drifted Ge-detector, does not show the 36,52 keV-γ-transition which was previously assumed to populate the 1301keV-state. In addition to the knownγ-transitions we found a 40,9 keV-line. This is probably the transition between the 1301,1 keV and the 1260,3 keV-states.     

Kern-Isomerie bei In116

The short lived indium isomer produced by thermal neutron capture is confirmed to be In¹¹⁶. A new determination of half-live andγ energy yieldsT _1/2=(2.17α0.07) sec andE _γ=(164±1) keV. From measurement of theK shell conversion coefficient follows that the multipolarity of the transition isE 3, leading to a spin and parity assignment of 8^? for the isomeric level.     

Der Zerfall Co58m →Co58g

Co^58m , Co^58g and Co⁵⁵ were obtained by radiating nickel-foiles with deuterons of energies 11,5 MeV and 2,07 MeV. The γ-radiation was measured with NaJ scintillation spectrometers. For the isomeric transition of Co^58m was determinedT _1/2=(9.15±0.1)h,T _γ=(25±1)keV,α _K=2200±300 and α_L+M=1100±300. From these values it follows, that the radiation is ofM3-type. Twoγ-energies of 95 keV and 1322 keV were found belonging to Co⁵⁵.     

Determination of absoluteK-internal conversion coefficients of some transitions in Ce140 by the internal-external conversion method

The internalK-conversion coefficients of the 331, 431, 815 and 933 keV transitions following the decay of La¹⁴⁰ have been determined absolutely by the method of comparing internal and external conversion lines measured in a double — focusing beta — ray spectrometers. TheK-internal conversion coefficients of the 4+→2+ 487 keV transition in Ce¹⁴⁰ was used to normalize relativeK-electron and gamma-ray intensities for these transitions. The results obtained are:α _K (331)=0.04432±0.00471,α _K (431)=0.28110±0.02913,α _K (815)=0.00396±0.00043,α _K (933)=0.00282±0.00031. Multipolarity assignments based on these values are suggested. The 815 keV transition is found to be pure magnetic dipole character in good agreement with the theoretical values calculated bySliv andBand. The 331 and 933 keV transitions are proved to have magnetic dipole character withE2/M1 equal 0.2852±0.0143 and 0.1750±0.0088 respectively. The 431 keV transition was found to have magnetic octupole character. The results obtained are most consistent with the assignment 2+, 4+, 2+, 3+ and 1+ for the 1597, 2084, 2184, 2410 and 2515 keV levels respectively.     

Untersuchung des Zerfalls von Ag110m durch γ-γ-Richtungskorrelationsmessungen

Directional correlation measurements have been made of six different gamma-gamma-cascades in Cd¹¹⁰, following theβ-decay of Ag^110m. The observed correlation functions are:

764 keV?1505 keV-cascade:	W(?)=1?(0,1578±0,0075)P 2?(0,0075±0,0065)P 4
1505 keV?658 keV-cascade:	W(?)=1?(0,395±0,013)P 2?(0,032±0,012)P 4
1384 keV?884 keV-cascade:	W(?)=1?(0,2840±0,0110)P 2?(0,0137±0,0090)P 4
1384 keV?658 keV-cascade:	W(?)=1?(0,3013±0,0065)P 2?(0,0130±0,0055)P 4
937 keV?884 keV-cascade:	W(?)=1+(0,098±0,012)P 2+(0,0148±0,0058)P 4
884 keV?658 keV-cascade:	W(?)=1+(0,1004±0,0087)P 2+(0,0086±0,0046)P 4

     

Zerfallsschemata, β-Matrixelemente und γ-Multipolordnungen für die Übergänge Co56→Fe56 und J131→Xe131

In the decay of Co⁵⁶ the following quantities have been measured:γ-ray intensities,β-γ directional correlation, andβ-(circularly polarizedγ) correlation. The directional correlation anisotropy was found to be, forβ energies above 300 keV,A ₂=0.5±0.4 per cent, corresponding to small or vanishing twice forbidden contributions to the allowed decay. The asymmetry parameterA of theβ-(circularly polarizedγ) correlation was measured to beA=?0.01±0.05 which implies a ratiox between Fermi and Gamow-Teller contributions to the decay ofx=?0.10±0.07, in agreement with the isospin selection rule. In the decay of J¹³¹ the following quantities have been measured: shape of the 606 keVβ-ray group,γ-ray intensities, conversion coefficients, andβ-(circularly polarizedγ) correlations. The measuredK/L ratio of the 364 keVγ-transition,K/L=6.0±0.2, is compatible with the conversion tables of Sliv and Band only. The multipolarities of theγ rays of 364, 637, and 723 keV were deduced. The 606 keVβ-364 keVγ cascade was used as a new calibration standard for analysers of circularly polarizedγ-rays.     

Messungen derK-Konversionskoeffizienten und der Aktivierungsquerschnitte der isomeren Atomkerne Se77m,Se79m,Ge75m und Ge77m

TheK-conversion coefficients α _K of the nuclear isomers Se^77m , Se^79m , Ge^75m and Ge^77m have been measured by detecting theK-röntgen- andγ-radiation from neutron-irradiated Se- and GeO₂-samples with the aid of scintillation counters to be α _K =0.79±0.06, 7.4±0.6, 1.44±0.13, and 1.2±0.6, respectively. In all cases, the values obtained, are in agreement with those taken from the tables ofRose under the assumption of anE3-transition, thus confirming this assignment which was proposed earlier by other authors. In addition, the cross sectionsσ for inducing the activities by slowed down neutrons have been measured to beσ=22±2, 0.40±0.04, 0.20±0.02, and 0.12±0.03 barns, respectively, and are compared with earlier data of several authors.     

Das K-Auger-Spektrum von Neon

TheKLL-Auger spectrum of neon was investigated with an electrostatic spectrometer with an energy resolution of 0.12%. The ionization in theK-shell was caused by electron impact. The use of a gaseous target made it possible to measure the Auger electrons without any energy loss. The relative intensities of the KLL-lines were determined to be:KL ₁ L ₁(¹ S ₀)=1.0;KL ₁ L _2,3(¹ P ₁)=3.06±0.07;KL ₁ L _2,3(³ P _0,1,2)=0.98±0.05;KL _2,3 L _2,3(¹ S ₀)=1.67±0.08;KL _2,3 L _2,3(¹ D ₂)=13.1±0.6;KL _2,3 L _2,3(² P _0,2)=0. This is in agreement with an earlier measurement byKörber andMehlhorn but disagrees with all theoretical values calculated nonrelativistically for low Z. It is shown that agreement may be achieved by applying quantitatively the configuration interaction, introduced very recently byAsaad, and using improved wave functions for the calculation of the transition amplitudes. As a consequence of the ionization by electron impact also theKL-LLL Auger spectrum was caused. 10 lines of this spectrum were measured and identified. Moreover, from the Auger energies measured, the binding energyE(K) of neon was calculated to be E(K)=(870.0±0.4) eV.     

Zur Isomerie des Tl197

Tl^197m was produced by the (α, 4n) reaction on Au¹⁹⁷ using 49 MeVα particles. The following results were obtained: Half-lifeT _1/2=(0.55±0.02) sec; energy of the isomeric level (607±4) keV, determined directly by summing up the cascade transitions in a well-type scintillator; energy of the isomeric transition (222±2) keV; conversion coefficients of this transitionα _K222=0.41±0.05 andα _tot222=2.1±0.2, indicating anE3 multipolarity; energy of the second transition (385±3)keV; conversion coefficientsα _K385=0.09±0.03 andα _tot385<0.1. This transition was identified asE2 with aM1 admixture of 20 to 30%. Spins and parities are 1/2⁺, 3/2⁺ and 9/2^? for the ground state, the 385 keV state and the 607 keV isomeric state, respectively, in disagreement with the extreme single-particle model. If this model were correct, anotherM1 transition should appear. No furtherM1 transition having an energy greater than theL-shell binding energy of T1 was observed.     

Niederenergetische Gammalinien vom Neutroneneinfang in Lu 175 und Lu 176

The low energy gamma-rays from neutron-capture in Lu 175 and Lu 176 have been investigated by means of the bent crystal-spectrometer at the DR-3-reactor at Risø. From the transitions in Lu 177 3 rotational bands have been determined. The levels of the (404)K=7/2⁺ groundstate rotational band are: 121,62 keV (I=9/2), 268,79keV (I=11/2), 440,66 keV (I=13/2), 636,22 keV (I=15/2), 854,34 keV (I=17/2). The level-sequence of the (514)K=9/2^?-band is: 150,39 keV (I=9/2), 288,99 keV (I=11/2), 451,49 keV (I=13/2), 637,05 keV (I=15/2) and 844,88 keV (I=17/2). At 457,92 keV is the basis for the (402)K=5/2⁺-band the higher levels of which are 552,05 keV (I=7/2), 671,89 keV (I=9/2), 816,63 keV (I=11/2), 985,23 keV (I=13/2), 1176,73keV (I=15/2) and probably 1389,5 keV (I=17/2). The energies of the levels apart from the 1389 keV-level have an accuracy of 7×10^?5. The energy differences between the 3 bands agree very well with the values expected from the Bohr-Mottelson-formulaE=A·I(I+1)+B·I ²(I+1)². The calculated branching-ratios within the 3 bands are in fairly good agreement with the experimental values. Theg _K -factors have been determined for 2 bands: It was found that for the (514)-bandg _K =1,16±0,04 and for the (402)-bandg _K =1,33±0,07.     

Der Zerfall des Tb158m

Tb^158m was produced from Tb¹⁵⁹ by (n, 2n) reaction and investigated using scintillation spectrometers. The following results were obtained: half-life\(T_{\tfrac{1}{2}} = (10.5 \pm 0.2)\) sec; energy of the isomeric transitionE _γ =(109.9±1.4) keV; conversion coefficients α _K =56±3; α _L +α _M +?=50±8; α_total=106±10;K/L-ratioK/L=1.3±0.3, yielding the multipole order of the isomeric transition to beM3. Upper limits for the direct beta transitions from the isomeric state to the ground states of the neighbouring even-even nuclei Gd¹⁵⁸ and Dy¹⁵⁸ are 10^?4 and 6·10^?3, respectively.     

Das Auger-Spektrum derL III- Schale von Wismut

A thin Bi layer is irradiated by X-rays so thatL-Auger electrons are emitted. A magnetic lens spectrometer is used to measure the electron spectrum. Energy, transition, and relativ intensity are given for 14 lines. Under the most favourable conditions the number ofL _III ionisations is about ten times that ofL _II ionisations. In this case only a small intensity ofL _II-Auger electrons is superposed on theL _III-Auger spectrum. The ratiod of intensities of line groupL _III M N to line groupL _III M M is found by extrapolation to bed=0·46±0·02. This combined with earlier results gives anL _III-Auger yielda ₃= 0·64±0·04. TheL _III fluorescenc yield isω ₃=0·36±0·04, correspondingly. A further application of the experimental method is described.     

DasK/β+-Verhältnis beim Zerfall J128→T128

In the decay of J¹²⁸ the intensity of a weak positron activity was measured to be (3.1±0.7)·10^?5 per disintegration. The remeasurement of the totalK capture was found to be 0.059±0.007 in agreement with the results of other authors. From this theK/β ⁺-ratio of the decay to the ground state of Te¹²⁸ is 1800±400. Theoretical calculations ofK/β ⁺ for allowed transitions show that the maximum energy of the positrons is 245±12 keV. In the decay of Rh¹⁰⁴ and Lu^176m no positrons more than 5·10^?6 could be detected.     

Suche nach Zweiquantenprozessen beim Zerfall von Xe131m

The decay of Xe^131m was investigated in order to detect nuclear double decay processes, in which the transition energy is distributed either between twoγ-quanta or between oneγ-quantum and oneK-conversion electron or between twoK-conversion electrons. By analyzing the emittedγ-radiation in a two-dimensional way an upper limit of 2.2 · 10^?5 was derived for the ratio of theγγ- toγ-transition probability. An investigation of theγ-spectrum in coincidence withK-quanta yielded an upper limit of 3 · 10^?2 for the rate ofe _Kγ-transitions relative toγ-transitions. The simultaneous emission of twoK-quanta was actually observed. These doubleK-quanta result either from the doubleK-conversion that was sought or from the internal conversion of the internal Compton-effect. For the doubleK-electron emission toγ-emission probability a value of (3.6±0.7) · 10^?3 was obtained. TheK-conversion coefficient and the half-life of Xe^131m were measured to be 32.1±0.4 and 11.94±0.04 d, respectively.     

Die absolute Intensität der durch Elektronenstoß in einer dicken Wolfram-Antikathode erzeugtenL α -Strahlung

The number\(N_{L_\alpha }^{dir} \) (produced) ofL _α -photons produced by electron-bombardment in a thick target of tungsten per incident electron has been measured absolutely with the Ross-filter method and relatively with the crystal-spectrometer method in the energyregion up to the 3.6 times theL _III-ionization energy\(E_{L_{III} } \). The result can be presented in the following empirical form:\(N_{L_\alpha }^{dir} \) (produced)=4π·?·(U ₀?1) ⁿ with ?=0.52·10^?4±5% andn=1.44±0.02\((U_0 = E_0 /E_{L_{III} }< 3.6)\). Out of this the number\(n_{L_{III} } \) ofL _III-ionizations per electron which is slowed down to the energy\(E_{L_{III} } \) within the target, has been evaluated. The computation of\(n_{L_{III} } \) out of the elementary process by usingBethe's non-relativistic formulae for totalL _III-ionization cross sectionQ _L and energy loss-dE/ds is in full agreement with experiment in the region 2<U ₀<3.6, if the constants in\(Q_{L_{III} } \) are chosen as follows:\(B = 4E_{L_{III} } , b_{L_{III} } = 0.25 \cdot 5.89\). By comparison of this result for\(b_{L_{III} } \) with the corresponding value ofb _K in the totalK-ionization cross-sectionQ _K for copper (b _K=0.35·2.26) it is concluded that\(Q_{L_{III} } \) is considerably higher than predicted by theory. The necessary correction factors as e.g. loss ofL _III-ionizations by rediffusion of electrons and portion of indirectly producedL _α -radiation-radiation are determined for tungsten quantitatively.