基于旋转相干光谱的整形飞秒激光转动动力学调控

我们实验上发展了基于飞秒激光旋转相干光谱的整形飞秒激光转动动力学调控方法,通过脉冲整形技术调控激发脉冲的光谱相位,从而实现对飞秒激光作用下转动态相干激发过程中复原信号及转动布居数的调控. 研究了飞秒激光旋转相干光谱对激光频谱相位的响应机制,突出了飞秒激光频谱相位在气相分子转动态相干激发中的重要作用. 为飞秒激光作用下生物大分子和团簇鉴别及结构探测研究提供了新的参考.     

用SPIDER法测量飞秒激光脉冲的光谱相位

介绍了用SPIDER测量光谱相位的实验装置和模拟计算飞秒激光特性参数的原理；提出了Ω 和τ等重要参数的确定方法.实验上用自建的SPIDER进行了掺钛蓝宝石飞秒振荡器输出脉 冲的相位测量，并以此为基础还原出了原输入脉冲的时域形式，模合计算所得的脉宽为107 fs，与利用二次相关法直接测量的结果十分一致. 关键词： 飞秒激光 SPIDER 光谱相位 光谱相干     

飞秒激光与超快现象(Ⅰ)

文章第Ⅰ部分介绍飞秒激光的发展过程和应用概况，讨论了飞秒脉冲产生和测量的基本原理，以及近年来在物理和技术上的新进展．特别介绍了在飞秒激光器全固体化、小型化、高效化方面的进步．有关飞秒激光技术在超快现象研究中的应用将在第Ⅱ部分介绍．     

用SPIDER法重构飞秒脉冲位相中参数的选择

为了更精确地测量飞秒脉冲特性以满足其不断拓宽的应用，基于光谱相位相干直接电场重构法（SPIDER）测量飞秒激光脉冲的基本原理和重构相位的反演算法，数值模拟了SPIDER重构飞秒脉冲相位的过程，分析了时间延迟τ、光谱剪切量Ω及滤波窗口宽度的选取原则。以宽度约为20fs的高斯型线性啁啾脉冲为例，通过选取不同的时间延迟τ和光谱剪切量Ω重构脉冲的相位，发现重构位相曲线与原输入脉冲位相曲线最接近时，时间延迟τ约为1210fs,相对光谱剪切量Ω/Δω约为9%，滤波窗口宽度约为τ/3。     

飞秒光谱技术的现状与展望

自１９８１年Ｒ．Ｌ．Ｆｏｒｋ等人利用环型腔可饱和吸收体的对撞锁模技术首次产生了飞秒（１０－１５ｓ）激光脉冲后，多频段飞秒光脉冲的产生、放大、频率扩展及光脉冲压缩等技术的发展十分迅速．目前在物理学、生物学和化学等各领域中，利用飞秒光谱技术观测各种原初过程以及超快速现象，巳经成为一种崭新而有效的研究手段，越来越受到各国科学家的高度重视．本文介绍了飞秒光源的现状、飞秒光谱的主要测量方法以及飞秒光脉冲放大、压缩等技术的基本原理，并对飞秒光谱技术的未来发展及应用前景进行了讨论．     

采用光谱展宽技术的钛宝石飞秒激光放大器

报道了飞秒激光啁啾脉冲放大器中的激光脉冲光谱展宽技术，实验中使用了几种光谱展宽元件，结果表明使用激光光谱展宽元件能有效地将飞秒激光脉冲 光谱展宽，抑制了飞秒激光放大器中常见的激光脉冲光谱增益窄化现象，从飞秒放大系统的振荡级输出28fs种子脉冲，放大后得到了重复频率为10Hz、峰值功率为1．6TW、脉冲宽度37．5fs的超短强飞秒激光脉冲 。     

自锁模钛宝石激光实现全固化运转

自锁模钛宝石激光实现全固化运转＊魏志义陈毓川李健何京良侯炜房哓军许祖彦（中国科学院物理研究所光物理实验室，北京１０００８０）邓佩珍徐军周永宗乔景文（中国科学院上海光学精密机械研究所，上海２０１８００）超短脉冲激光的实用化研究是近年飞秒技术发展的重要方...     

单次飞秒激光脉冲在玻璃内部产生多次微爆的研究

在入射能量不同的情况下，用近红外飞秒激光脉冲在重钡火石玻璃（ZBaF15）内部产生了色心和微爆，在熔融石英的内部产生了多次微爆现象.实验表明：入射能量较高时，色心的中间会产生微爆；在松聚焦条件下，一个飞秒激光脉冲在透明介质内会激发多次微爆.基于飞秒激光脉冲在透明介质内的自聚焦效应和自由电子等离子体的自散焦效应，理论分析了多次微爆产生的原因；也讨论了飞秒激光脉冲诱导玻璃折射率改变的机理.     

化学反应飞秒相干动力学与激光相干控制——1999年诺贝尔化学奖介绍

文章主要介绍了１９９９ 年诺贝尔化学奖得主艾哈默德·泽维尔（Ａｈｍｅｄ．Ｈ．Ｚｅｗａｉｌ） 教授的获奖工作———用飞秒技术和飞秒光谱的方法研究化学反应飞秒相干动力学,叙述了它们的原理、方法和应用,并简要介绍了其获奖背景、重要意义、相关研究及应用展望．     

不同波长飞秒脉冲的相位测量

飞秒脉冲技术的不断发展能够较方便地产生不同波段和结构特性的飞秒脉冲. 对已有的改进型零附加相位光谱相位相干电场重构系统进行优化整合,使之胜任不同特性飞秒脉冲的测量. 利用该系统测量了两台飞秒激光系统输出不同波长的脉冲及其通过厚度为80 mm的BK7玻璃块而得到的啁啾脉冲. 实验结果表明,该系统的适用范围较宽. 关键词： 光谱相位相干直接电场重构法 飞秒脉冲测量 波长     

Pulse‐shape instabilities and their measurement

Multi‐shot pulse‐shape measurements of trains of ultrashort pulses with unstable pulse shapes are studied. Measurement techniques considered include spectral‐phase interferometry for direct electric‐field reconstruction (SPIDER), second harmonic generation frequency‐resolved optical gating (FROG), polarization gate FROG, and cross‐correlation FROG. An analytical calculation and simulations show that SPIDER cannot see unstable pulse‐shape components and only measures the coherent artifact. Further, the presence of this instability cannot be distinguished from benign misalignment effects in SPIDER. FROG methods yield a better, although necessarily rough, estimate of the pulse shape and also indicate instability by exhibiting disagreement between measured and retrieved traces. Only good agreement between measured and retrieved FROG traces or 100% SPIDER fringe visibility guarantees a stable pulse train.     

Coherent artifact in modern pulse measurements

We simulate multishot intensity-and-phase measurements of unstable trains of complex ultrashort pulses using second-harmonic-generation (SHG) frequency-resolved optical gating (FROG) and spectral-phase interferometry for direct electric-field reconstruction (SPIDER). Both techniques fail to see the pulse structure. But FROG yields the correct average pulse duration and suggests the instability by exhibiting significant disagreement between measured and retrieved traces. SPIDER retrieves the correct average spectral phase but significantly underestimates the average pulse duration. In short, SPIDER measures only the coherent artifact. An analytical calculation confirms this last fact.     

Generation of double pulses in-line by using reflective Dammann gratings

Doubled femtosecond laser pulses in-line are needed in the collinear pump-probe technique, collinear second harmonic generation frequency-resolved optical gating (SHG FROG) and the spectral phase interferometry for direct electric-field reconstruction (SPIDER), etc. Normally, it is generated by using a Michelson's structure. In this paper, we proposed a novel structure with two-layered reflective Dammann gratings and the reflective mirrors to generate doubled femtosecond laser pulses in line without transmission optical elements. Angular dispersion and spectral spatial walk-off are both compensated. In addition, this structure can also compress the positive chirped pulse, which cannot be realized with a Michelson's structure. By adopting triangular grating and blazed gratings, the efficiency of the system would in principle be increased as the Michelson's scheme. Experiments demonstrated that this method should be an alternative approach for generation of the double compressed pulses of femtosecond laser for practical applications.     

飞秒激光脉冲宽度和脉冲波形测试技术

飞秒激光在激光核聚变、卫星精密测距、激光微加工等领域具有重要的应用前景,同时也是产生太赫兹波的主要泵浦源。介绍了国内外飞秒激光脉冲宽度和脉冲波形的测试方法,比较了自相关法、频率分辨光学快门法、光谱相位相干直接电场重构法的优缺点。自相关法具有脉宽测量范围广、结构简单等特点,但不具备脉冲波形测试能力。光谱相位相干直接电场重构法对待测激光光束质量要求较高, 不适合大量程范围激光脉宽快速测量。为满足10 fs~5 ps大量程范围超短激光脉冲宽度和脉冲波形的测试需求,采用自相关法及二次谐波频率分辨光学开关法研制飞秒激光脉冲宽度和脉冲波形测试仪,时间分辨率优于2 fs。     

Characterization of a broadband pulse for phase controlled multiphoton microscopy by single beam SPIDER

We present what we believe to be a new version of spectral phase interferometry for direct electric field reconstruction (SPIDER) using only a single-phase and polarization controlled laser beam. Two narrow pulses and one broadband pulse are selected out of an ultrafast laser pulse by a polarization and phase control technique to generate second harmonic generation (SHG) signals, which are equivalent to a spectral shear interferogram in the conventional SPIDER method. The spectral phase of the broadband laser pulse is extracted analytically with double quadrature spectral interferometry (DQSI). An arbitrary spectral phase can be retrieved with great precision and compensated in situ at the sample position of a microscope. This new method requires no separate reference beam and is suitable for nonlinear optical microscopy with a phase controlled laser pulse.     

The criterion of pulse reconstruction quality based on Wigner representation

We propose a new criterion for the assessment of ultrashort pulse reconstruction quality. Our idea is based on the use of a two-dimensional Wigner representation of the electric field. This allows introducing a single measure to represent the quality of both phase and amplitude retrieval. The new criterion is employed to examine two contemporary pulse characterization techniques: FROG (Frequency Resolved Optical Gating) and SPIDER (Spectral Interferometry for Direct Electric-field Reconstruction). For SPIDER, the influence of reference pulse stretching on the quality of phase extraction is investigated. Next, we ascertain the limitations in the use of a Fabri-Perrot etalon in the SPIDER apparatus for producing delayed pulse replicas. For the FROG technique we examine the impact of the doubling crystal orientation on the quality of the amplitude-phase retrieval of sub-5-fs pulses. The introduced criterion is also applied to study the respective sensitivity of FROG and SPIDERto the limited phase-matching bandwidth of the non-linear medium and detector noise.     

Shaping, propagation and characterization of ultrafast pulses in optical fibers

The characterization of medium- to low-energy shaped pulses at 1.55 7m through frequency-resolved optical gating (FROG) is illustrated. This capability enables the study of ultrafast pulse propagation through optical fibers. The phase dynamics detected furnishes insight on pulse evolution, specifically on soliton formation - a subject of great importance for telecommunication applications. The combination of shaping and propagation of ultrafast pulses in fibers is examined theoretically using an adaptive pulse-shaping model, based on genetic algorithms, that furnishes optimized pulse shapes for fiber propagation.     

The Measurement of Ultrashort Light Pulses—Simple Devices,Complex Pulses

We review the state of the art of ultrashort-light-pulse measurement using frequency-resolved-optical-gating (FROG). Recent developments have extended the state of the art considerably. FROG devices for measuring the intensity and phase of ultrashort laser pulses have become so simple that almost no alignment is required. In addition, such devices not only operate single shot, but they also yield the two most important spatio-temporal distortions, spatial chirp and pulse-front tilt. With other FROG variations, it is now possible to measure more general ultrashort light pulses (i.e., pulses much more complex than common laser pulses), with time-bandwidth products as large as several thousand and as weak as a few hundred photons, and despite other difficulties such as random absolute phase and poor spatial coherence.     

Spectral phase and amplitude interferometry for direct electric-field reconstruction

An extension of the well-known technique for spectral phase interferometry for direct electric-field reconstruction (SPIDER) has been developed that permits the reconstruction of the spectral amplitude and the spectral phase of ultrashort laser pulses from the acquisition of only one spectrum. Temporal intensity and temporal phase can therefore easily be retrieved. The characterization of pulses from a Ti:sapphire oscillator by use of an extended SPIDER is discussed. Advantages and drawbacks of the modified technique are also discussed.     

Temporal characterization of mid-IR free-electron-laser pulses by frequency-resolved optical gating

We performed what we believe are the first practical full-temporal-characterization measurements of ultrashort pulses from a free-electron laser (FEL). Second-harmonic-generation frequency-resolved optical gating (FROG) was used to measure a train of mid-IR pulses distorted by a saturated water-vapor absorption line and showing free-induction decay. The measured direction of time was unambiguous because of prior knowledge regarding free-induction decay. These measurements require only 10% of the power of the laser beam and demonstrate that FROG can be implemented as a pulse diagnostic simultaneously with other experiments on a FEL.