Connection between charge fluctuations and the coherent temperature in the heavy-fermion system SmOs4Sb12: a {121, 123}Sb NQR study

We report {121, 123}Sb nuclear quadrupole resonance measurements under pressure in a novel heavy fermion (HF) system SmOs4Sb12. The nuclear spin-spin relaxation rate 1/T{2} exhibits a distinct peak near the coherent temperature of the Kondo effect. The isotope effect of 121Sb and 123Sb indicates that the peak in 1/T{2} is electrical in origin. The connection between the peak in 1/T{2} and the development of coherency of the Kondo effect is robust even under pressure. It is conjectured that charge fluctuation plays an important role in forming the HF state in SmOs4Sb12.     

Fermi liquid theory of the impurity-lattice relaxation for a simple mixed-valence impurity model

Ward identities are used to relate the charge relaxation of a simple spinless mixed-valence impurity with its charge susceptibility at low temperatures. The result is compared with the Korringa relation for the Anderson model and the Kondo problem.     

Phonon-assisted thermoelectric effects in strongly interacting quantum dot

The joint effects of the electron-phonon interaction and Kondo effect on the charge and heat transport through a single molecule transistor are investigated by applying the improved canonical transformation and noncrossing approximation technique. We find that the electron-phonon interaction decreases the conductance, thermopower and the Wiedemann-Franz law in the Kondo regime due to the splitting and the decreasing of the main Kondo peak. However, the thermoelectric figure of merit achieves enhancement with the electron-phonon coupling strength increasing. In addition, the dip value of the thermopower at the Kondo temperature for the different electron-phonon coupling strength can give a straightforward reliable estimate of the electron-phonon coupling strength.     

Bethe ansatz approach to the Kondo effect within density-functional theory

Transport through an Anderson junction (two macroscopic electrodes coupled to an Anderson impurity) is dominated by a Kondo peak in the spectral function at zero temperature. We show that the single-particle Kohn-Sham potential of density-functional theory reproduces the linear transport, despite the lack of a Kondo peak in its spectral function. Using Bethe ansatz techniques, we calculate this potential for all coupling strengths, including the crossover from mean-field behavior to charge quantization caused by the derivative discontinuity. A simple and accurate interpolation formula is also given.     

Kosterlitz–Thouless transition,spectral property and magnetic moment for a two-dot structure with level difference

By means of the numerical renormalization group method, we study the phase transition, the spectral property, and the temperature-dependent magnetic moment for a parallel double dot system with level difference, where the dot energies are kept symmetric to the half-filled level. A Kosterlitz–Thouless(KT) transition between local spin triplet and singlet is found. In the triplet regime, the local spin is partially screened by the conduction leads and spin-1 Kondo effect is realized.While for the singlet, the Kondo peak is strongly suppressed and the magnetic moment decreases to 0 at a definite low temperature. We attribute this KT transition to the breaking of the reflection symmetry, resulting from the difference of the charge occupations of the two dots. To understand this KT transition and related critical phenomena, detailed scenarios are given in the transmission coefficient and the magnetic moment, and an effective Kondo model refers to the RayleighSchrdinger perturbation theory is used.     

Mesoscopic charge relaxation

We consider charge relaxation in the mesoscopic equivalent of an RC circuit. For a single-channel, spin-polarized contact, self-consistent scattering theory predicts a universal charge relaxation resistance equal to half a resistance quantum independent of the transmission properties of the contact. This prediction is in good agreement with recent experimental results. We use a tunneling Hamiltonian formalism and show in Hartree-Fock approximation that at zero temperature the charge relaxation resistance is universal even in the presence of Coulomb blockade effects. We explore departures from universality as a function of temperature and magnetic field.     

Spin-flip Fano–Kondo resonant tunneling through a quantum dot interferometer responded by a rotating magnetic field

The Fano and Kondo cooperated resonant tunneling through a quantum dot interferometer under the perturbation of a rotating magnetic field is investigated theoretically. The spin-polarized current components have been derived generally by employing the Keldysh nonequilibrium Green?s function method, through which the charge and spin currents are determined directly. The numerical calculations on spin and charge currents are performed to show the compound features of mesoscopic transport associated with the Kondo, Fano, and Zeeman effects intimately. The induced spin current in the Kondo regime is much different from the one in the non-interacting regime. The spin current is tuned from resonant peak to valley by varying external parameters.     

Charge distribution in a Kondo-correlated quantum dot

We report on direct measurement of charge and its distribution in a Kondo correlated quantum dot (QD). A noninvasive potential-sensitive detector, in proximity with a QD, reveals that, although the conductance of the QD is significantly enhanced as it enters the Kondo regime, the average charge remains unaffected. This demonstrates the separation between spin and charge degrees of freedom. We find, however, under certain conditions, an abrupt redistribution of charge in the QD, taking place with an onset of Kondo correlation. This suggests a correlation between the spin and charge degrees of freedom.     

Kondo resonance assisted thermoelectric transport through strongly correlated quantum dots

We theoretically studied the thermoelectric transport properties of a strongly correlated quantum dot system in the presence of the Kondo effect based on accurate numerical evaluations using the hierarchical equations of motion approach. The thermocurrent versus gate voltage shows a distinct sawtooth line-shape at high temperatures. In particular, the current changes from positive(hole charge) to negative(particle charge) in the electron number N = 1 region due to the Coulomb blockade effect. However,at low temperatures, where the Kondo effect occurs, the thermocurrent's charge polarity reverses, along with a significantly enhanced magnitude. As anticipated, the current sign can be analyzed by the occupation difference between particle and hole.Moreover, the characteristic turnover temperature can be further defined at which the influences of the Coulomb blockade and Kondo resonance are in an effective balance. Remarkably, the identified characteristic turnover temperature, as a function of the Coulomb interaction and dot-lead coupling, possessed a much higher value than the Kondo temperature. When a magnetic field is applied, a spin-polarized thermocurrent can be obtained, which could be tested in future experiments.     

Nonequilibrium noise as a probe of the Kondo effect in mesoscopic wires

We study the nonequilibrium noise in mesoscopic diffusive wires hosting magnetic impurities. We find that the shot-noise to current ratio develops a peak at intermediate source-drain biases of the order of the Kondo temperature. The enhanced impurity contribution at intermediate biases is also manifested in the effective distribution. The predicted peak represents an increased inelastic scattering rate at the nonequilibrium Kondo crossover.     

Double-dot charge qubit and transport via dissipative cotunneling

We investigate transport through an exotic charge qubit composed of two strongly capacitively coupled quantum dots, each being independently connected to a side gate which in general exhibits a fluctuating electrostatic field (i.e., Johnson-Nyquist noise). Two quantum phases are found: the "Kondo" phase where an orbital-Kondo entanglement emerges and a "local moment" phase in which the noise destroys the Kondo effect leaving the orbital spin unscreened and resulting in a clear suppression of the conductance. In the Kondo realm, the transfer of charge across the setting is accompanied by zero-point charge fluctuations in the two dissipative environments and then the I-V characteristics are governed by what we call "dissipative cotunneling."     

Nonequilibrium dynamics of anisotropic large spins in the kondo regime: time-dependent numerical renormalization group analysis

We investigate the time-dependent Kondo effect in a single-molecule magnet (SMM) strongly coupled to metallic electrodes. Describing the SMM by a Kondo model with large spin S>1/2, we analyze the underscreening of the local moment and the effect of anisotropy terms on the relaxation dynamics of the magnetization. Underscreening by single-channel Kondo processes leads to a logarithmically slow relaxation, while finite uniaxial anisotropy causes a saturation of the SMM's magnetization. Additional transverse anisotropy terms induce quantum spin tunneling and a pseudospin-1/2 Kondo effect sensitive to the spin parity.     

Even-odd effect in Andreev transport through a carbon nanotube quantum dot

We have measured the current (I)-voltage (V) characteristics of a single-wall carbon nanotube quantum dot coupled to superconducting source and drain contacts in the intermediate coupling regime. Whereas the enhanced differential conductance dI/dV due to the Kondo resonance is observed in the normal state, this feature around zero-bias voltage is absent in the superconducting state. Nonetheless, a pronounced even-odd effect appears at finite bias in the dI/dV subgap structure caused by Andreev reflection. The first-order Andreev peak appearing around V=Delta/e is markedly enhanced in gate-voltage regions, in which the charge state of the quantum dot is odd. This enhancement is explained by a "hidden" Kondo resonance, pinned to one contact only. A comparison with a single-impurity Anderson model, which is solved numerically in a slave-boson mean-field approach, yields good agreement with the experiment.     

Kondo effect in a quantum dot coupled to ferromagnetic leads: a numerical renormalization group analysis

We investigate the effects of spin-polarized leads on the Kondo physics of a quantum dot using the numerical renormalization group method. Our study demonstrates in an unambiguous way that the Kondo effect is not necessarily suppressed by the lead polarization: While the Kondo effect is quenched for the asymmetric Anderson model, it survives even for finite polarizations in the regime where charge fluctuations are negligible. We propose the linear tunneling magnetoresistance as an experimental signature of these behaviors. We also report on the influence of spin-flip processes.     

Hanbury Brown-Twiss correlations and noise in the charge transfer statistics through a multiterminal Kondo dot

We analyze the charge transfer statistics through a quantum dot in the Kondo regime, when coupled to an arbitrary number of terminals N. Special attention is paid to current cross correlations between concurring transport channels, which show distinct Hanbury Brown-Twiss antibunching for N>2 reflecting the fermionic nature of charge carriers. While this effect weakens as one moves away from the Kondo fixed point, a new type of correlations between nonconcurring channels emerges which are due entirely to the virtual polarization of the Kondo singlet. As these are not obscured by the background from fixed-point correlations they provide a promising means for extracting information on the parameters of the underlying Fermi-liquid model from the experimental data.     

Why could electron spin resonance be observed in a heavy fermion Kondo lattice?

We develop a theoretical basis for understanding the spin relaxation processes in Kondo lattice systems with heavy fermions as experimentally observed by electron spin resonance (ESR). The Kondo effect leads to a common energy scale that regulates a logarithmic divergence of different spin kinetic coefficients and supports a collective spin motion of the Kondo ions with conduction electrons. We find that the relaxation rate of a collective spin mode is greatly reduced due to a mutual cancellation of all the divergent contributions even in the case of the strongly anisotropic Kondo interaction. The contribution to the ESR linewidth caused by the local magnetic field distribution is subject to motional narrowing supported by ferromagnetic correlations. The developed theoretical model successfully explains the ESR data of YbRh₂Si₂ in terms of their dependence on temperature and magnetic field.     

Kondo effect in the presence of magnetic impurities

We measure transport through gold grain quantum dots fabricated using electromigration, with magnetic impurities in the leads. A Kondo interaction is observed between dot and leads, but the presence of magnetic impurities results in a gate-dependent zero-bias conductance peak that is split due to a RKKY interaction between the spin of the dot and the static spins of the impurities. A magnetic field restores the single Kondo peak in the case of an antiferromagnetic RKKY interaction. This system provides a new platform to study Kondo and RKKY interactions in metals at the level of a single spin.     

Splitting and Restoration of Kondo Peak in a Deformed Molecule Quantum Dot Coupled to Ferromagnetic Electrodes

We adopt the nonequilibrium Green＇s function method to theoretically study the Kondo effect in a deformed molecule, which is treated as an electron-phonon interaction （EPI） system. The self-energy for phonon part is calculated in the standard many-body diagrammatic expansion up to the second order in EPI strength. We find that the multiple phonon-assisted Kondo satellites arise besides the usual Kondo resonance. In the antiparallel magnetic configuration the splitting of main Kondo peak and phonon-assisted satellites only happen for asymmetrical dot-lead couplings, but it is free from the symmetry for the parallel magnetic configuration. The EPI strength and vibrational frequency can enhance the spin splitting of both main Kondo and satellites. It is shown that the suppressed zero-bias Kondo resonance can be restored by applying an external magnetic field, whose magnitude is dependent on the phononic effect remarkably. Although the asymmetry in tunnel coupling has no contribution to the restoration of spin splitting of Kondo peak, it can shrink the external field needed to switch tunneling magnetoresistance ratio between large negative dip and large positive peak.     

Spin fractionalization of an even number of electrons in a quantum Dot

We find that Kondo resonant conductance can occur in a quantum dot in the Coulomb blockade regime with an even number of electrons N. The contacts are attached to the dot in a pillar configuration, and a magnetic field B( perpendicular) along the axis is applied. B( perpendicular) lifts the spin degeneracy of the dot energies. Usually, this prevents the system from developing the Kondo effect. Tuning B( perpendicular) to the value B(*) where levels with different total spin cross restores both the degeneracy and the Kondo effect. We analyze a dot charged with N = 2 electrons. Coupling to the contacts is antiferromagnetic due to a spin selection rule and, in the Kondo state, the charge is unchanged while the total spin on the dot is S = 1/2.     

SU(4) Fermi liquid state and spin filtering in a double quantum dot system

We study a symmetrical double quantum dot (DD) system with strong capacitive interdot coupling using renormalization group methods. The dots are attached to separate leads, and there can be a weak tunneling between them. In the regime where there is a single electron on the DD the low-energy behavior is characterized by an SU(4)-symmetric Fermi liquid theory with entangled spin and charge Kondo correlations and a phase shift pi/4. Application of an external magnetic field gives rise to a large magnetoconductance and a crossover to a purely charge Kondo state in the charge sector with SU(2) symmetry. In a four-lead setup we find perfectly spin-polarized transmission.