高温稠密金等离子体辐射不透明度的多极效应

使用平均原子模型研究了电四极及更高阶跃迁对高温稠密金等离子体辐射不透明度的贡献.计算并讨论了在不同温度密度条件下,电四极,电八极,电十六极跃迁对束缚-束缚跃迁的影响.计算了密度为96.405 g/cm3时,不同温度条件下,电四极,电八极跃迁对Rosseland平均不透明度的贡献.考虑了电四极、电八极跃迁后金等离子体不透明度的相对改变最大分别为4.67%和1.5%,并和其它文献的理论结果进行了比较.     

核运动中的某些集体观察量

在低能核结构研究中,电四极跃迁的B(E2,)值和基态带的态与态能量比值R常被用来衡量核的集体运动属性.本文通过标准的位能面计算,系统地探讨了这些量与核形变参数间的关系.指出B(E2,)值主要取决于核的平衡(静态)形变,目前的Nilsson-Strutinsky-BCS方法可以良好地求得从Z=30到锕系区偶-偶核的合理的形变值,而能量比值R则反映的是位能面的整体结构,例如硬度及非谐和性等.     

偶偶 Ra 同位素的八极形变研究

用反射不对称的相对论平均场理论(RAS-RMF)对偶偶Ra同位素的八极形变进行了系统研究,并与实验数据和有限力程小液滴模型(FRDM)结果进行了比较.结果表明：RAS-RMF理论很好地描述了Ra同位素的基态性质,计算的结合能、双中子分离能和形变与实验数据和FRDM一致.RAS-RMF理论获得的中子、质子密度分布清晰地展现出偶偶Ra同位素由球形逐渐转变为八极形变,到四极形变的过程,与实验观察的八极形变不稳定现象一致. 关键词： 反射不对称平均场(RAS-RMF) 八极形变 偶偶核     

Os-Pt区核的基态三轴形状

在偶-偶核基态中寻找稳定的三轴形状,其中最大三轴形变为|γ|≈30°,仍然是核结构的一个主要主题。在本工作中,使用推转Woods-Saxon(WS)壳模型来研究Os-Pt区基态和集体转动态中可能的三轴形状。为寻找核态可能存在的三轴形变,具体用对力-形变-转动频率自洽推转壳模型对偶-偶^176-202Os和^182-204Pt同位素进行了总Routhian面计算。计算是在四极形变(β₂,γ)网格中进行的,而十六极形变β₄可变。事实上,在四极形变(β₂,γ)的每个网格点上,计算的能量相对于十六极形变β₄最小化。发现某些核的基态譬如¹⁹⁶Os和^188-194Pt既非扁椭球亦非长椭球,而是在这些核中基态极小值是形状非轴对称的,即三轴形变。同时,我们把从实验数据提取出的转动惯量与我们的计算结果作比较,显示实验数据不能很好地与转动假定相一致,说明有振动行为。此外,我们使用一种辅助的方法提取了平衡γ₀值,该值...     

相对论平均场理论对Se，Kr，Sr和Zr同位素链形状共存的系统研究

在约束形变的相对论平均场理论下,用NL3参数组系统地研究了Se,Kr,Sr和Zr四个同位素链中的偶-偶核,理论计算的基态束缚能和实验值符合得非常好.通过对这些核的位能曲面的分析,发现在此区域内有着丰富的形状共存现象,系统地指出可能存在形状共存现象的原子核,并且进一步指出在这些核的位能曲面上两个能量极小点的能量差.另外通过对位能曲面以及单中子能级的研究,提出在此区域内N＝70可能是一个中子幻数. 关键词： 形状共存 相对论平均场 位能曲面 幻数     

通过超宽139La固体核磁共振波谱研究层状La(OH)2NO3

层状稀土氢氧化物是一类新型的稀土功能材料，本文采用固体核磁共振（SSNMR）方法研究了同时具备离子交换能力和非线性光学特性的层状La（OH）₂NO₃化合物，探讨了通过四极核CPMG（QCPMG）脉冲序列和变频谱图采集获取超宽¹³⁹La SSNMR谱图的方法，并描述了适用于此类实验的滤波方程和谱图重建方法.重建谱图同时包含四极核中心跃迁和卫星跃迁信息，本文使用QUEST软件对超宽¹³⁹La NMR谱图进行了模拟，获取的四极耦合常数C_Q和非对称因子η_Q均与CASTEP密度泛函理论计算值高度吻合.SSNMR实验结果证实层状La（OH）₂NO₃化合物属于非中心对称结构（P2₁），解决了对其结构长期以来存在的争论.     

双Λ超核同位旋标量巨共振性质的相对论研究

基于相对论平均场理论(RMF),采用TM1以及有效超子-核子和超子-超子相互作用,首先研究了¹⁶O和_ΛΛ¹⁸O的单粒子能级受超子的影响情况,发现超子的加入使得核子能级能量降低.其次基于相对论无规位相近似方法 (RRPA),自洽地计算了¹⁶O和_ΛΛ¹⁸O同位旋标量巨单极和四极共振态.发现相比于¹⁶O各巨共振的响应函数,超核的响应函数会发生改变.研究表明:这种改变主要来自于超子的加入导致的核子单粒子能级的改变,以及超子粒子-空穴组态跃迁的贡献,而超子-超子剩余相互作用对单极和四极共振在低能区的响应函数的影响比较小,特别对高能区的响应函数基本没有影响.     

电多极矩跃迁选择定则的对称分析

只有由群的对称性才可能导出每个不可约表示的对称性波函数, 即对称化基函数.也只有由群的对称性才可能导出电子状态跃迁的最一般选择定则 , 即电偶极跃迁E1, 电四极跃迁E2 和 电八极跃迁E3跃迁的选择原则. 本文以 和 为例, 导出电多积跃迁的选择原则. 角动量的选择定则只是特例. 并用方法SAC-CI/6-31G 计算了 H2O和 CC的基态以及其激发态的激发能和振子强度.本文只适合单光子过程. 计算都与理论相合.     

电多极矩跃迁选择定则的对称分析

只有由群的对称性才可能导出每个不可约表示的对称性波函数, 即对称化基函数.也只有由群的对称性才可能导出电子状态跃迁的最一般选择定则 , 即电偶极跃迁E1, 电四极跃迁E2 和 电八极跃迁E3跃迁的选择原则. 本文以 和 为例, 导出电多积跃迁的选择原则. 角动量的选择定则只是特例. 并用方法SAC-CI/6-31G 计算了 H2O和 CC的基态以及其激发态的激发能和振子强度.本文只适合单光子过程. 计算都与理论相合.     

铅(208)集体3~-态电四极矩、电八极跃迁和跃迁密度的研究——生成坐标方法的应用

用生成坐标方法(GCM)~([1]_α)考虑集体3~-态与非集体粒子空穴对(ph)_(l~ )耦合模型计算了铅(208)3~-集体态的电四极矩Q_([3~-])、电八极约化跃迁几率B(E3)和跃迁密度ρ_(3~-)~(tr)随核的径向距离r的变化曲线。结果是:Q_([3~-])=-0.098eb,B(E3)=38w.u.。计算中没有像通常那样假设一个有效核子电荷而是在GCM框架下考虑核心激发进行微观计算,其结果与实验符合,说明GCM能够对核元激发的耦合作微观研究。     

Microscopic analysis of octupole shape transitions in neutron-rich actinides with relativistic energy density functional

Quadrupole and octupole deformation energy surfaces, low-energy excitation spectra, and electric transition rates in eight neutron-rich isotopic chains – Ra, Th, U, Pu, Cm, Cf, Fm, and No – are systematically analyzed using a quadrupole-octupole collective Hamiltonian model, with parameters determined by constrained reflectionasymmetric and axially-symmetric relativistic mean-field calculations based on the PC-PK1 energy density functional.The theoretical results of low-lying negative-parity bands, odd-even staggering, average octupole deformations β_3,and B(E3;3_1~- →0_1~+) show evidence of a shape transition from nearly spherical to stable octupole-deformed, and finally octupole-soft equilibrium shapes in the neutron-rich actinides. A microscopic mechanism for the onset of stable octupole deformation is also discussed in terms of the evolution of single-nucleon orbitals with deformation.     

E2 transitions between positive- and negative-parity states of the ground-state alternating-parity bands

Experimental transition probabilities between states of the ground-state alternating-parity bands of ¹⁴⁴Ba and their theoretical analysis are presented. Lifetimes of states in ¹⁴⁴Ba have been measured using the recoil distance method following spontaneous fission of ²⁵²Cf. The experiment was performed at the Lawrence Berkeley National Laboratory employing the Gammasphere array and the New Yale Plunger Device. The experimental data show a significantly larger value of the E2 transition probability between the negative-parity states compared to the positive-parity ones. It is shown that this effect can be explained by a higher weight of the deformed component in the wave functions of the odd-I states. In the framework of the cluster approach it is explained by a higher weight of the alpha-cluster component in the wave function of the negative-parity states compared to the positive-parity ones. In the framework of the traditional collective model with the quadrupole and octupole degrees of freedom the same effect is explained by a higher value of the quadrupole deformation at the minima of the potential energy as a function of β₂₀ and β₃₀ compared to its value at the top of the barrier separating two physically equivalent minima, having opposite signs of the octupole deformation. Additionally, the dependence on parity of the E2 transition probability is analyzed qualitatively in nuclei with a minimum at β₃₀ = 0 in the collective potential energy and compared to experimental data for ¹⁴⁸Nd.     

实验探索原子核中手征与空间反射对称性的联立自发破缺

原子核的手征对称性和空间反射对称性研究是近来原子核结构研究的前沿热点问题,吸引了大量的实验和理论研究。通过在束伽玛谱学的实验方法,在原子核78Br中发现了两对宇称相反的手征双重带,以及它们之间表征八极关联的电偶极跃迁。这是首次在原子核中发现了八极关联的多重手征带,给出了原子核存在手征对称性和空间反射对称性联立自发破缺的实验证据。Spontaneous symmetry breaking is a fundamental concept in nature. Chiral Symmetry Breaking and reflection-asymmetry in nuclei has been a subject of intensive experimental and theoretical investigation. Two pairs of positive-and negative-parity doublet bands together with eight strong electric dipole transitions linking their yrast positive-and negative-parity bands have been identified in 78Br by means of in-beam gamma-ray spectroscopy techniques. These four rotational bands are suggested as multiple chiral doublet bands with octupole correlations. This observation indicates that nuclear chirality can be robust against the octupole correlations. It is of highly scientific interest to search for the chirality-parity quartet bands in nucleus with both stable triaxial and octupole deformations.     

Band structures of Se and Se

Band structures of ⁷⁶Se and ⁷⁸Se have been studied with the ^74,76Ge(, 2nγ)^76,78Se reactions by using a variety of in-beam γ-techniques : γ-ray singles spectra, γ-ray excitation functions, γ-γ-t coincidences, γ-ray angular distributions and γ-ray linear polarizations.

Spins and parities have been assigned uniquely for many new levels in ⁷⁶Se and ⁷⁸Se and four bands have been identified in both nuclei: (i) the ground-state band, (ii) a positive-parity ΔJ = 1 band built on the second 2⁺ state (γ-vibrational band), (iii) a negative-parity Δ J = 2 band built on the 3⁻ state (octupole band) and (iv) a ΔJ = 2 band built on the high-lying J = 4 state. In addition, the second 8 ⁺ and 10⁺ states, which are possibly the lowest members of a band, have been found in both nuclei.

Systematics of the band structures obtained are discussed. Level energies of the band members and B(E2) ratios for some of the inter-band transitions between γ- and ground-state bands have been calculated with the proton-neutron interacting boson model IBM-2 and a reasonable agreement with the present data has been obtained.     

微波场对(Ba,Sr)3MgSi2O8：Eu2+,Mn2+荧光粉中Mn2+ 660 nm红光能量传递的影响

研究了2.45 GHz微波灼烧(Ba,Sr)₃MgSi₂O₈：Eu²⁺,Mn²⁺荧光粉的非热效应对Mn²⁺离子660 nm红光发射强度的影响。在相同的加热温度条件下,增加微波场的输出功率,微波非热效应导致Eu²⁺离子蓝光的跃迁概率增加,Eu²⁺通过(Ba,Sr)₃MgSi₂O₈基质晶格把能量传递给Mn²⁺,进而使Mn²⁺的跃迁概率增加,导致红光发射增强。提出了一种微波场非热效应对能量传递影响的新观点,认为在微波加热过程中强微波磁场可能会对像Mn²⁺这样具有顺磁性的激活剂离子的能级结构和能量传递性质产生干扰作用。     

Microscopic Description of g Factors and M1 Properties in Platinum Isotopes

Starting from the shell model configurations, valence nucleon effective interactions and fermion M1 transition current density operator, the counterparts in the proton-neutron interacting boson model (sdIBM-2) of the fermion Hamiltonian and M1 transition current density operator are derived microscopically with the help of Dyson expansion technique. The boson g factors are abstracted from the boson M1 transition current density operator. Spectra, g factors of 2₁⁺, 2₂⁺, 4₁⁺ states and M1 matrix elements between 2₂⁺ and 2₁⁺ are calculated for the even ^192-198Pt isotopes in the sdIBM-2. The theoretical results fit experimental data quite well.     

Octupole deformation for Ba isotopes in a reflection-asymmetric relativistic mean-field approach

The potential energy surfaces of even-even 142-156Ba are investigated in the constrained reflectionasymmetric relativistic mean-field approach with parameter set PK1. It is shown that for the ground states, 142Ba is near spherical,156Ba well quadrupole-deformed, and in between 144-154Ba octupole deformed. In particular, the nuclei 148,150Ba with N=92, 94 have the largest octupole deformations. By including the octupole degree of freedom, energy gaps N = 88, N = 94 and Z = 56 near Fermi surfaces for the singleparticle levels in 148Ba with β2 ～ 0.26 and β3 ～ 0.17 are found. Furthermore, the performance of the octupole deformation driving pairs (ν2f7/2, ν1i13/2) and (π2d5/2, π1h11/2) is demonstrated by analyzing the singleparticle levels near Fermi surfaces in 148Ba.     

Yb (Ba, Sr)2Cu4O8: a “124” phase superconductor with a reduced unit cell volume

Yb(Ba_1−xSr_x)₂Cu₄O₈ (0.1x0.3) superconductors of the YBa₂Cu₄O₈(“124”) structure were successfully synthesized using an O₂-hot-isostaticc-pressing (HIP) technique. The samples were characterized with respect to the crystal structure and superconducting properties. The lattice parameters of the samples decreased as the substitution of Sr for Ba proceeded. The superconducting transition temperatures of all the Yb-“124” samples were more or less the same, being around 80 K.     

Octupole instability induced by rotation in the nuclei Nd

Levels in ^146,148Nd have been populated in the ¹⁵⁰Nd(, ′ xn) reactions. Cascades of enhanced E1 transitions have been observed. B(E1)/B(E2) branching ratios, of the order of 10⁻⁶ fm⁻² as well as the presence of low energy negative-parity bands indicate strong octupole effects. Shell correction type calculations suggest an explanation in terms of octupole correlations at medium spins.