共查询到19条相似文献,搜索用时 62 毫秒
1.
基于描述低能离子与原子碰撞的分子库仑过垒模型,详细阐述了与入射离子速度相关的反应窗理论,并对影响势垒变化的平均径向速度做了修正.根据该理论,计算了C5 -He和He2 -He碰撞体系单电子俘获过程的态选择微分截面,并分别与Kamber等人和Mergel等人的实验结果进行了比较. 相似文献
2.
离子与原子碰撞中多电子转移的经典描述 总被引:1,自引:1,他引:0
马新文 《原子与分子物理学报》1998,15(1):91-100
讨论了几各地独立电子模型(IEM)描述离子与原子碰撞中电子转移的经典模型,即Bohr-Lindhardt模型,过垒模型OBM和分子库仑垒模型MCBM。较详细阐述了描述碰撞过程的经典物理图象,着重讨论了MCBM描述的多电子转移过程,分析了几各模型的特点和适用性,最后在考虑了入射离子量子数亏损和出射过程电子束缚能移动的修正后,给出了修正后的MCBM的计算结果,并与Niehaus的计算结果玫实验结果进行 相似文献
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利用冷靶反冲离子动量谱仪装置系统研究了20-40 keV He2+-He碰撞体系的态选择单电子俘获过程,实验获得了单电子俘获过程的态选择截面以及角微分截面.在所研究的能区范围,电子俘获到L壳层的截面最大,为主要的反应道,这与分子库仑过垒模型的反应窗理论的预测一致.实验测量的态选择截面与原子轨道紧耦合的计算结果很好地符合,与光谱方法的测量结果存在一定的差别,主要原因是光谱方法不能测量完整的反应通道信息.实验结果表明,总角微分截面在小角度范围主要来源于电子俘获到基态的贡献,在大角度范围主要来自电子俘获到激发态的贡献;电子俘获到基态的和激发态的角微分截面均出现振荡结构,这种振荡来源于电子俘获反应中分子轨道之间的相干效应.实验测量的角微分截面与其他实验和紧耦合方法的计算结果进行了比较和分析. 相似文献
5.
利用冷靶反冲离子动量谱仪装置系统研究了20—40 keV He2+-He碰撞体系的态选择单电子俘获过程,实验获得了单电子俘获过程的态选择截面以及角微分截面.在所研究的能区范围,电子俘获到L壳层的截面最大,为主要的反应道,这与分子库仑过垒模型的反应窗理论的预测一致.实验测量的态选择截面与原子轨道紧耦合的计算结果很好地符合,与光谱方法的测量结果存在一定的差别,主要原因是光谱方法不能测量完整的反应通道信息.实验结果表明,总角微分截面在小角度范围主要来源于电子俘获到基态的贡献,在大角度范围主要来自电子俘获到激发态的贡献;电子俘获到基态的和激发态的角微分截面均出现振荡结构,这种振荡来源于电子俘获反应中分子轨道之间的相干效应.实验测量的角微分截面与其他实验和紧耦合方法的计算结果进行了比较和分析.
关键词:
冷靶反冲离子动量谱仪
态选择电子俘获
态选择截面
角微分截面 相似文献
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利用四体模型计算了100 和 2 MeV/amu裸碳单电离氦原子的全微分截面,其结果与实验数据和其它理论进行了比较。对于高能入射情况,在散射平面小动量转移和中间动量转移时现在的理论结果和实验符合的很好,然而在大动量转移时和在垂直平面有明显差异。对于低能入射情况,四体结果定性与实验结果一致,而且优于三体扭曲波(3DW-EIS)结果,表明四体效应在低能入射比在高能入射时明显。 相似文献
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利用四体模型计算了100和2MeV/amu裸碳单电离氦原子的全微分截面,其结果与实验数据和其它理论进行了比较.对于高能入射情况,在散射平面小动量转移和中间动量转移时现在的理论结果和实验符合的很好,然而在大动量转移时和在垂直平面有明显差异.对于低能入射情况,四体结果定性与实验结果一致,而且优于三体扭曲波(3DW-EIS)结果,表明四体效应在低能入射比在高能入射时明显. 相似文献
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用模型势方法对正电子与氪,氙原子散躯有分布进行了系统计算,通过对算得的微分截面的数据分析,结合作者以前对正电子与氦,氖,氩原子散射角分布的研究结论总结出了代能正电子与稀有气体原子散射角分布规律。 相似文献
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本文利用交叉分子束方法和离子速度成像技术,对H+HD→H2+D反应在1.17 eV碰撞能下的态-态反应动力学开展了高分辨实验研究. 实验采用1+1''(真空紫外+紫外)近阈值激光电离方式对反应中的D原子产物进行探测,获得了高角度分辨和高能量分辨的产物离子速度影像,进而精确获得了反应的态-态微分截面. 实验观测到了H2(v''=0,j''=1)和H2(v''=0,j''=3)振转产物角分布中与散射过程的干涉效应相联系的前向散射振荡. 这一研究进一步表明了化学反应微分截面的精确测量在气相态-态反应动力学研究中的重要性. 相似文献
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介绍了对于Na+ 离子和Rb(5s ,5p)原子碰撞中态选择单电子俘获微分截面的理论计算,并与实验数据进行比较,实验结果是离子与在磁光学阱中用激光冷却的碱金属靶原子碰撞而测量到的;还对高能量质子引起的He原子的转移电离进行了理论研究,在Shakeoff模型的基础上 ,分析解释了转移电离截面与单电子俘获截面的比值 ,并与最新实验结果作了比较. We report a theoretical study of state-selective differential single-electron capture cross sections between Na + and Rb(5s, 5p) atoms. The experimental data have been obtained with laser cooled target in a magnetic optical trap. We also report a theoretical study of transfer ionization of He by protons at high collision energies and analyze the transfer ionization cross section with respect to single electron capture cross section in terms of a shakeoff model. 相似文献
11.
ECPSSR理论是解释离子-原子碰撞内壳层电离最成功的理论之一.我们用VISUAL FORTRAN编写了ECPSSR理论计算程序,修正了ISICS程序中的错误,本程序可以对各种入射离子与靶原子的组合进行计算,给出K,L,M的壳层及次壳层电离截面以及相应的X射线产生截面,并根据需要选择是否对入射离子运动进行相对论修正.采用所编写的程序计算了一些碰撞体系的电离截面和X射线产生截面,并与其他程序的计算结果和实验数据分别进行了比较. 相似文献
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Jun Wang XiMeng Chen BaoWei Ding HongBin Fu Ying Cui JianXiong Shao YanXia Lu ZhiMin Gao YuWen Liu Juan Du GuangZhi Sun Lin Chen 《中国科学G辑(英文版)》2008,51(7):750-754
The ratios of the cross section of the transfer-ionization to the single-electron-capture of Argon induced by C
q+ (q = 1, 2, 3) ions are measured by means of position sensitive and time-of-flight techniques. Our experimental results are compared
with the data of Heq+ (q = 1, 2) − Ar of DuBois. A qualitative interpretation is presented based on the Classical-Over-Barrier Model of Bohr. 相似文献
13.
FAN Guang-Wei XU Wang M.Fukuda PAN Qiang-Yan CAI Xiao-Lu FAN Gong-Tao LI Yong-Jiang LUO Wen XU Ben-Ji YAN Zhe YANG Li-Feng 《中国物理C(英文版)》2010,34(10)
We study the reaction cross sections(σR) and root-mean-square(RMS) radii of 8Li and 8B,the halo-like nuclei,with stable target 12C,27Al and 9Be within the standard optical-limit Glauber model,using densities obtained from relativistic mean-field(RMF) formalisms and other types of distributions.It is found that the experimental σR can be reproduced well at high energy.The RMS radius and △r extracted by RMFtheory and harmonic oscillator distribution are compared.We find that the RMS radius and △r of 8B are larger than those of 8Li.In addition,we analyze in detail the relationship between σR and density distribution. 相似文献
14.
We study the reaction cross sections (σR) and root-mean-square (RMS) radii of ^8Li and ^8B, the halo-like nuclei, with stable target ^12C, ^27Al and ^9Be within the standard optical-limit Glauber model, using densities obtained from relativistic mean-field (RMF) formalisms and other types of distributions. It is found that the experimental σR can be reproduced well at high energy. The RMS radius and Ar extracted by RMF- theory and harmonic oscillator distribution are compared. larger than those of SLi. In addition, we analyze in detail the We find that the RMS radius and Ar of SB are relationship between σR and density distribution. 相似文献
15.
Calculations of state-selective differential cross sections for charge transfer in collisions between O3+ and H2
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The non-dissociative charge-transfer processes in collisions between O^3+ and H2 are investigated by using the quantum-mechanical molecular-orbital coupled-channel (QMOCC) method. The adiabatic potentials and radial coupling matrix elements utilized in the QMOCC calculations are obtained with the spin-coupled valence-bond approach. Electronic and vibrational state-selective differential cross sections are presented for projectile energies of 0.1, 1.0 and 10.0eV/u in the H2 orientation angles of 45° and 89°. The electronic and the vibrational state-selective differential cross sections show similar behaviours: they decrease as the scattering angle increases, and beyond a specific angle the oscillating structures appear. Moreover, it is also found that the vibrational state-selective differential cross sections are strongly orientation-dependent, which provides a possibility to determine the orientations of molecule H2 by identifying the vibrational state-selective differential scattering processes. 相似文献
16.
G. Kessedjian B. Jurado M. Aiche G. Barreau A. Bidaud S. Czajkowski D. Dassié B. Haas L. Mathieu L. Audouin N. Capellan L. Tassan-Got J.N. Wilson E. Berthoumieux F. Gunsing Ch. Theisen O. Serot E. Bauge I. Ahmad J.P. Greene R.V.F. Janssens 《Physics letters. [Part B]》2010
Neutron-induced fission cross sections for 242,243Cm and 241Am have been obtained with the surrogate reaction method. Recent results for the neutron-induced cross section of 243Cm are questioned by the present data. For the first time, the 242Cm cross section has been determined up to the onset of second-chance fission. The good agreement at the lowest excitation energies between the present results and the existing neutron-induced data indicates that the distributions in spin and parity of states populated with both techniques are similar. 相似文献
17.
The product angular momentum polarization of the reaction of H+NH is calculated via the quasiclassical trajectory method (QCT)
based on the extended London-Eyring-Polanyi-Sato (LEPS) potential energy surface (PES) at a collision energy of 5.1 kcal/mol.
The calculated results of the vector correlations are denoted by using the angular distribution functions. The polarization-dependent
differential cross sections (PDDCSs) demonstrate that the rotational angular momentum of the product H2 is aligned and oriented
along the direction perpendicular to the scattering plane. Vector correlation shows that the angular momentum of the product
H2 is aligned in the plane perpendicular to the velocity vector. It suggests that the reaction proceeds preferentially when
the reactant velocity vector lies in a plane containing all three atoms. The orientation and alignment of the product angular
momentum affects the scattering direction of the product molecules. The polarization-dependent differential cross sections
(PDDCSs) reveal that scattering is predominantly in the backward hemisphere.
相似文献
18.
Elastic scattering angular distributions and total reaction cross-sections of ~(7,10,11,12)Be projectiles are predicted by the systematic ~9 Be global phenomenological optical model potential for target mass numbers ranging from24 to 209. These predictions provide a detailed analysis by their comparison with the available experimental data.Furthermore, these elastic scattering observables are also predicted for some targets out of the mass number range.The results are in reasonable agreement with the existing experimental data, and they are presented in this study. 相似文献
19.
Bo Mei Dimiter L. Balabanski Wei Hua Yu-Hu Zhang Xiao-Hong Zhou Cen-Xi Yuan Jun Su 《中国物理C(英文版)》2021,45(5):054001-054001-5
Fusion-evaporation cross sections of ~(238)U (~9Be,5n)~(242)Cm are measured over a wide energy range around the Coulomb barrier.These measured cross sections are compared with model calculations using two codes,namely HIVAP2 and KEWPIE2.HIVAP2 calculations overestimate the measured fusion-evaporation cross sections by a factor of approximately 3.In KEWPIE2 calculations,two approaches,namely the Wentzel-Kramers-Brillouin(WKB) approximation and the empirical barrier-distribution (EBD) method,are used for the capture probability;both of them properly describe the measured cross sections.Additionally,fusion cross sections of ~(7,9)Be+~(238)U measured in two experiments are applied to constrain model calculations further through three codes,i.e.,HIVAP2,KEWPIE2,and CCFULL.Parameters in these codes are also examined by comparison with measured fusion cross sections.All the comparisons indicate that the KEWPIE2 calculations using the WKB approximation agree well with the measured cross sections of both fusion reactions ~(7,9)Be+~(238)U and the fusion-evaporation reaction ~(238)U (~9Be,5n)~(242)Cm.Calculations using the fusion code CCFULL are also in good agreement with the measured fusion cross sections of ~(7,9)Be+~(238)U. 相似文献