Nuclear structure of 18F: (IV). Negative-parity states

Studies via the ¹⁶O(³He, pγ)¹⁸F, ¹⁴N(α,γ)¹⁸F and ¹⁷O(p, γ)¹⁸F reactions have resulted in new J^π assignments for 11 states or negative parity: E_x(keV) (J^π) = 3791(3^?), 4226(2^(?)), 4398(4^?), 4860(1^(?)), 5502(3^(?)), 5785(2^?), 6097(4^?), 6108(1^(?), 2^(?), 3^(?)), 6241(3^?, T = 1), 6643(2^?, T = 1) and 6878(3^(t-), 4^?). The 6241 keV state is probably isospin mixed. New information for 5 states of positive parity has also been obtained: E_x(keV) (J^π) = 3838(2⁺), 4115(3⁺), 4652(4⁺, T = 1), 4753((0⁺), T = 1) and 4964(2⁺, T = 1). Mean lives, branching and mixing ratios are reported for all states. The results for the negative-parity states are discussed in the framework of the various models available. The states at E_x = 1080(0^?), 2100(2^?) and 4398(4^?) keV are interpreted as the first three members of a K^π = 0^? rotational band.     

EPR study of Fe3+ and Mn2+ in CeO2 and ThO2

Attempts were made to grow CeO₂ and ThO₂ single crystals doped with transition metal ions. Only Fe³⁺ and Mn²⁺ could be detected by the EPR technique. The EPR spectrum of Fe³⁺ in CeO₂ exhibits the well-known fine structure in cubic fields. The parameters areg=2.0044(1) anda=15.6(1)·10^?4 cm^?1. The hyperfine constantA for⁵⁷Fe in hexahedral coordination was found to be 8.9(1)·10^?4 cm^?1. The EPR spectrum of Mn²⁺ in CeO₂ reveals two cubic Mn²⁺ centers. The parameters for center 1 areg=1.9999(1) andA=86.9(1)·10^?4 cm^?1 and for center 2g=1.9984(1) andA=87.0(1)·10^?4 cm^?1. Heating the Mn doped CeO₂ samples in hydrogen, the Mn²⁺ centers transform from cubic into trigonal centers with approximate values ofg=1.9988(2),A=84.5(6)·10^?4 cm^?1 andD=203(1)·10^?4 cm^?1. The two observed Mn²⁺ centers in ThO₂ exhibita priori axial symmetry with approximate values ofg=2.0006(2),A=88.9(4)·10^?4 cm^?1 andD=33(3)·10^?4 cm^?1.     

Isotope shifts of neutron-deficient gold isotopes with 193≧A≧190

The isotope shift between¹⁹⁷Au (stable) and the radioactive Au isotopes¹⁹⁰Au,¹⁹¹Au,¹⁹²Au and¹⁹³Au were determined by resonance fluorescence spectroscopy in the 6s ² S _1/2–6p ² P _1/2.λ=267.6nm line. The unstable Au isotopes were produced at the ISOLDE mass separator at CERN. The nuclei were investigated semi on-line in a resonance vessel, heated to 1,400°C. The results areδν ^190,197=?11.12(39) GHz,δν ^191,197=?9.67(12) GHz,δν ^192,197=?8.32(15) GHz,δν ^193,197=?6.29(11) GHz, corresponding to a change of the mean-square charge radius byδ〈r ²〉^190,197 =0.261(12) fm²,δ〈r ²〉^191,197=0.227(5) fm²,δ〈r ²〉^192,197=0.195(5) fm²,δ〈r ²〉^193,197 =0.148(4) fm².     

First measurement of the exclusive (p,e+e−) reaction

We present the first data on the exclusive (p,e⁺e⁻) reaction in a nucleus. Cross sections for populating the ground state and first excited state in the residual nucleus are presented for the reaction ¹¹B(p, e⁺e⁻)¹²C at 98 MeV. The e⁺e⁻ momentum vectors were measured with a high-resolution magnetic pair spectrometer. The distributions of the virtual photon invariant mass and of the direction of the electron in the virtual photon rest system are compared with a simple single-nucleon model. The (p,e⁺e⁻) cross sections are compared with corresponding data for the (p, γ) reaction obtained with the same apparatus. The (p,e⁺e⁻) cross sections show substantial enhancement over what is expected from the simple model.     

InclusiveΔ ++ (1232) and∑ ± (1385) production inK − p interactions at 32 GeV/c

We have studied inclusiveΔ ⁺⁺ (1232),∑ ⁺ (1385), and∑ ^? (1385) baryon resonance production inK ^? p interactions at 32 GeV/c. The inclusive and topological cross sections are estimated and compared with published results at lower energies. No energy variation of the cross section is observed forΔ ⁺⁺ (1232) and only a slight decrease is seen in case of∑ ^± (1385). The production properties are investigated through longitudinal and transverse momentum distributions. TheΔ ⁺⁺ (1232) is dominantly produced in the target fragmentation region. The∑ ⁺ (1385) is produced both in the target fragmentation region and in the central region, while the∑ ^? (1385) is predominantly produced in the central region. About 20% of the final state protons are produced via aΔ ⁺⁺ (1232) decay and about 25% of the Λ produced come from the decay of∑ ⁺ (1385) and∑ ^? (1385).     

Measurement of 232Th(n, γ) and 232Th({n}, {2n}) cross-sections at neutron energies of 13.5, 15.5 and 17.28?MeV using neutron activation techniques

The ²³²Th(n, ??) reaction cross-section at average neutron energies of 13.5, 15.5 and 17.28?MeV from the ⁷Li(p, n) reaction has been determined for the first time using activation and off-line ??-ray spectrometric technique. The ²³²Th(n, 2n) cross-section at 17.28?MeV neutron energy has also been determined using the same technique. The experimentally determined ²³²Th(n, ??) and ²³²Th(n, 2n) reaction cross-sections from the present work were compared with the evaluated data of ENDF/BVII and JENDL-4.0 and were found to be in good agreement. The present data, along with literature data in a wide range of neutron energies, were interpreted in terms of competition between ²³²Th(n, ??), (n, f), (n, nf) and (n, xn) reaction channels. The ²³²Th(n, ??) and ²³²Th(n, 2n) reaction cross-sections were also calculated theoretically using the TALYS 1.2 computer code and were found to be in good agreement with the experimental data from the present work but were slightly higher than the literature data at lower neutron energies.     

Hyperspherical Three-Body Calculation for Exotic Atoms

Ground state energies of atomic three-body systems like negatively charged hydrogen, normal helium, positively charged-lithium, beryllium, carbon, oxygen, neon and negatively charged exotic- muonium and positronium atoms have been calculated adopting hyperspherical harmonics expansion method. Calculation of matrix elements of two body interactions needed in the hyperspherical harmonics expansion method for a three body system is greatly simplified by expanding the bra- and ket-vector states in the hyperspherical harmonics (HH) basis states appropriate for the partition corresponding to the interacting pair. This involves the Raynal–Revai coefficients (RRC), which are the transformation coefficients between the HH bases corresponding to the two partitions. Use of RRC become particularly essential for the numerical solution of three-body Schr?dinger equation where the two-body potentials are other than Coulomb or harmonic. However in the present work the technique is used for two electron atoms ¹H^?(p ⁺ e ^? e ^?), D^?(d ⁺ e ^? e ^?), Mu^?(μ ⁺ e ^? e ^?),⁴He(⁴ He ²⁺ e ^? e ^?),⁶Li(⁶ Li ³⁺ e ^? e ^?),¹⁰Be(¹⁰ Be ⁴⁺ e ^? e ^?),¹²C(¹² C ⁶⁺ e ^? e ^?),¹⁶O(¹⁶ O ⁸⁺ e ^? e ^?) etc. and the exotic positronium negative ion Ps ^?(e ⁺ e ^? e ^?) where the interactions are purely Coulomb. The relative convergence in ground state binding energy with increasing K _max for ²⁰Ne has been demonstrated as a representative case. The calculated energies at K _max ?=?28 using RRC’s have been compared with those obtained by a straight forward manner in some representative cases to demonstrate the appropriateness of the use of RRC. The extrapolated energies have also been compared with those found in the literature. The calculated binding energies agree within the computational error.     

Backward production of the B meson in K−p interactions at 4.2 GeVc

The backward production of the B(1235) meson is studied in the reaction K^?p→Σ^?π⁺ω. This reaction is observed in the final state Σ^?π⁺π⁺π^?π⁰. A π⁺ω mass enhancement is visible in the region of the B meson for events with small |u|K^? →Σ^?) squared four-momentum transfer. The properties of the enhancement agree with those of the B meson. The cross section for K^?p→Σ^?B⁺ at $\text{4.15}\text{GeV}\text{c}$ incident K^? momentum is (3.2 ± 0.5) μb. The backward production of the B meson is compared with similar baryon exchange productions of the A₁ and C(Q₁) axial vector mesons observed in the same experiment.     

Jet-cooled laser-induced fluorescence spectroscopy of B2Σ+–X2Σ+ system of scandium monoxide: Improved molecular constants at equilibrium

The investigation on B²Σ⁺–X²Σ⁺ system of ScO was extended to higher vibrational levels by laser-induced fluorescence (LIF) spectroscopy in a free-jet. We have observed rotationally resolved excitation spectra for (4,0), (3,0), (2,0), and (1,2) bands in addition to the previously observed (0,0) and (1,0) bands. The wavenumbers of these bands were fitted to a Hamiltonian matrix to determine the molecular constants for the vibrational levels up to ν′=4 of the B²Σ⁺ state and ν″=2 of the X²Σ⁺ state. In addition, the vibration constants of the ground states were determined from the dispersed fluorescence wavenumbers between B²Σ⁺ (ν′=0–4) and X²Σ⁺ (ν″=0–8) transitions. The equilibrium molecular constants, derived from the extensive set of molecular constants for individual vibrational levels, were used to construct RKR potential energy curves for both the electronic states. The Franck–Condon factors were also calculated for the B²Σ⁺–X²Σ⁺ transition.     

Rovibronic structure in the electron energy spectrum for associative ionization: Ne(3 P 2), Ar(3 P 2)+H

Associative ionization in thermal energy (300 K) collisions between Ne(2p ⁵ 3s ³P₂), Ar(3p ⁵ 4s ³ P ₂) metastable atoms and hydrogen atomsH(1s ² S _1/2) has been studied by high resolution (20 meV) electron spectrometry. The spectra exhibit structure due to the formation of different vibrational states in the molecular ion and show superimposed rotational structure. Direct information is obtained on the relative population of the rovibronic states and on their energy positions. The well depth of the ionic potential curves has been determined as:D _e (NeH ⁺ X ¹ Σ ⁺)=2.27 (3) eV,D _e (ArH ⁺ X ¹ Σ ⁺)=4.02(3) eV.     

Collisional relaxation of ionic2 P 3/2 excited states in rare gases

Optical pumping with theD ₂ line is used to study the depolarization of the first excited² P _3/2 states of alkaline earth ions and Yb⁺ ions in collisions with rare gas atoms. The deorientation cross sections for the even isotopes of Ba⁺ and Yb⁺ ions are obtained (in units of 10^?16 cm²): rare gas He Ne Ar Kr Xeσ ₁ (Ba⁺ 6p ² P _3/2) 79(11) 89(13) 123(18) 152(22) 204(30)σ ₁ (Yb⁺ 6p ² P _3/2) 60(10) 62(9) 107(18) 133(17) 167(37) The cross sections are discussed in comparison with theoretical calculations and those of isoelectronic atoms. The comparison of the² P _3/2 relaxation of even and odd (I=3/2) isotopes of Ba⁺ allows to draw conclusions on the nature of the depolarization interaction.     

Experimental investigation of highly excited states of the 5,6He and 5,6Li nuclei in the (6Li, 7Be) and (6Li, 7Li) one-nucleon pickup reactions

The (⁶Li, ⁷Be) and (⁶Li, ⁷Li) reactions on ⁶Li and ⁷Li nuclei were investigated in the angular interval 0°–20° in the laboratory system at a ⁶Li energy of 93 MeV. In addition to low-lying states of the ^5,6He and ^5,6Li nuclei, broad structures were observed near the t(³He)+d and t(³He)+t thresholds at the excitation energies of 16.75 (3/2⁺) and ～20 MeV (for ⁵He), 16.66 (3/2⁺) and ～20 MeV (⁵Li), 14.0 and 25 MeV (⁶He), and ～20 MeV (⁶Li). The angular distributions measured in the ⁷Li(⁶Li, ⁷Be)⁶He reaction for transitions to the ground state (0⁺) and excited states at E _x=1.8 MeV (2⁺) and 14.0 MeV of the ⁶He nucleus were analyzed by the finite-range distorted-wave method assuming the 1p-and 1s-proton pickup mechanism. The (⁶Li, ⁷Be) and (⁶Li, ⁷Li) reactions were shown to proceed predominantly through the one-step pickup mechanism, and the broad structures observed at high excitation energies are considered as quasimolecular states of the t(³He)+d and t(³He)+t types.     

Electric quadrupole moments of the K π = 8− and 23/2− isomeric states in 170, 171, 172Hf

The spectroscopic quadrupole moments of the K ^π = 8^? isomers in ¹⁷⁰Hf and ¹⁷²Hf, Q _s ?=?4.91(17) b and 5.40(19) b, respectively and Q _s ?=?4.92(17) b for K ^π ?=?23/2^? in ¹⁷¹Hf have been measured using the time differential perturbed angular distribution technique. The nuclear reaction ¹⁶⁰Gd(¹⁶O, xnγ) was used to excite the respective isomeric states and for the recoil implantation of Hf nuclei into the Hf foil. The quadrupole deformation for the 8^? isomer and the ground state has the same value. The deformation corresponding to 23/2^? isomeric state is observed to be reduced with respect to the ground state due to the i _13/2 neutron alignment. The results are in good agreement with the multi-quasiparticle calculations.     

Investigation of theβ +-decay of105,106,109In and of100,102Ag

Isomers in the nuclei¹⁰⁰Ag (I=5⁺),¹⁰²Ag (I=5⁺),¹⁰⁵In (I=9/2⁺),¹⁰⁶In (I=6⁺),¹⁰⁸In (I=6⁺) were selectively populated by the reactions⁹⁰Zr(¹⁹F,xnγ),⁹²Mo(¹⁹F, 2pnγ),⁹²Mo(¹²C,pxnγ),⁹⁰Zr(¹⁹F,α3nγ) atE _lab=72 and 66MeV, and their (β ⁺+EC)-decay was studied with an Anticomptonγ-spectrometer. Spins of the beta-decaying isomers are determined. The results obtained for the beta strength functions are discussed as well as new information on the structure of the neutron-deficient even-even daughter nuclei nearZ=50.     

Atomic beam magnetic resonance investigations in the3 F 2 Ground State of177Hf,179Hf and180Hf

The 5d ²6s ^{2 3} F ₂ ground state of¹⁷⁷Hf,¹⁷⁹Hf and¹⁸⁰Hf has been studied using the atomic beam magnetic resonance method. The atomic beam was produced by an universal evaporation technique described in a previous paper. The results are¹⁸⁰Hfg _j (³ F ₂)=0.695812 (10)¹⁷⁷Hf Δv(³ F ₂;F=11/2?F=9/2)=991.7917 (10) MHz Δv(³ F ₂;F=9/2?F=7/2)=477.0081 (10) MHz Δv(³ F ₂;F=7/2?F=5/2)=162.8890 (10) MHz¹⁷⁹HfΔv(³ F ₂;F=13/2?F=11/2)=82.1320 (10) MHz Δv(³ F ₂;F=11/2?F=9/2)=392.8498 (10) MHz. The magnetic dipole and electric quadrupole moments of the¹⁷⁷Hf and¹⁷⁹Hf nuclear ground states as calculated from these hyperfine structure measurements are the following: μ(177)=0.75(8)μ _k , Q(177)=4.34 (65) barns μ(179)=?0.61 (6)μ _k , Q(179)=4.90 (75) barns.     

Die elektrischen Kernquadrupolmomente von Cäsium 131 und Cäsium 132 aus Doppelresonanzmessungen am 72 P 3/2-Term

The hyperfine splitting of the 7² P _3/2-state of the radioactive isotopes¹³¹Cs and¹³²Cs has been investigated by optical double resonance. The hyperfine interaction constants deduced from the measured hfs transition frequencies are¹³¹Cs¹³²CsA(7² P _3/2)+31.73(6) MHz +25.03(12) MHzB(7² P _3/2)?28.63(35) MHz + 23.60(60) MHz These values yield spectroscopic nuclear quadrupole momentsQ _s (corrected for the Sternheimer effect) ofQ _s (¹³¹Cs)=?0.57(1) barnQ _s (¹³²Cs)=+0.47(1) barn. The magnetic interaction constantA of¹³²Cs results in a slightly improved precision of the nuclear magnetic dipole momentμ ₁ (¹³²Cs)=+2.22(1)μ _K . The Cesium isotopes have been produced by (d, xn)-reactions on natural Xenon. Total cross sections of the reactions¹³²Xe(d, 2n)¹³²Cs;¹³⁴Xe(d, 4n)¹³²Cs;¹³⁴Xe(d, 2n)¹³⁴Cs;¹³⁶Xe(d, 4n)¹³⁴Cs;¹³⁶Xe(d, 2n)¹³⁶Cs have been measured between 10 and 29 MeV.     

Investigation of the electromagnetic structure of the η meson in the decay η → μ+μ−γ

600 events of the rare electromagnetic decay η → μ⁺μ^?γ have been detected. The branching ratio has been measured as BR(η → μ⁺μ^?γ) = (3.1 ± 0.4) × 10^?4. The electromagnetic form factor of the η meson, F(m_μμ²;0) = (1 ? m_μμ²/Λ²)^?1, has been determined. Λ = (0.72 ± 0.09) GeV/c² is in good agreement with the vector meson dominance model.     

Excitation of isomeric states in the (γ,n), (n, 2n), and (γ, 2n) reactions on the 113In nucleus

The induced-activity method was used to measure the isomeric ratio of the yields of the (γ, n), (n, 2n), and (γ, 2n) reactions on the ¹¹³In nucleus. The energy dependence of the isomeric ratios of the yields of the photonuclear reactions ¹¹³In(γ, n)^112m,g In and ¹¹³In(γ, 2n)^111m,g In is studied in the energy range of 12–35 MeV.     

Atomic beam magnetic resonance investigations in the 2p 2 3 P ground multiplet of the stable carbon isotopes12C and13C

The hyperfine structure seperations Δv andg _J -factors have been measured in the 2p ^{2 3} P states of¹³C(I=1/2) and¹²C(I=0), respectively, using the atomic beam magnetic resonance method. The results are Δv(³ P ₁,¹³C)=4.200 (25) MHz, Δv(³ P ₂,¹³C)=372.593 (25) MHz,g _J (³ P ₁,¹²C)=1.501052 (13), andg _J (³ P ₂,¹²C)=1.501039 (15). After applying corrections due to perturbations by neighbouring fine structure levels one deduces the constants of the magnetic dipole interactionA(³ P ₁,¹³C)=+2.838 (17) MHz, A(³ P ₂,¹³C)=+149.055 (10) MHz. No signs of theA-factors were determined by the experiment; they follow from the known positive sign of the nuclear magnetic moment μ _I of¹³C. CombiningA(³ P ₂,¹³C) with the results of other measurements on¹¹C, yields μ _I (¹¹C)=?0.964 (1) nm.     

Spectroscopy of 7Li in stopped pion absorption reactions

The structure of excited levels in the ⁷Li isotope is studied via inclusive and correlation measurements in the stopped π^? meson absorption reactions ¹⁰B(π^?, t)X and ¹²C(π^?, dt)X, respectively. The experiment is conducted using a low-energy pion beam at the LAMPF meson factory. Analysis of the missing mass spectra reveals ⁷Li states with the resonance parameters (E _x , Γ) (4.7, 0.1), (6.6, 0.9), (7.3, 0.1), (9.1, 2.8), and (9.6, 0.4) MeV. A highly excited state with E _x ≈ 11.2 MeV (i.e., an isobar analog of ⁷He) is observed in the ¹⁰B(π^?,t)X reaction. An excited state with E _x = 10.3 ± 0.1 MeV and γ = 1.8 ± 0.4 Mev is observed for the first time in the ¹²C(π^?,dt)X reaction.