Magnetic phases in Mn<Subscript>1</Subscript>_<Subscript>x</Subscript>Fe<Subscript>x</Subscript>WO<Subscript>4</Subscript> studied by neutron powder diffraction

The magnetic structures of Mn_1-xFe_xWO₄ with x = 0.0, 0.16, 0.21, 0.225, 0.232, 0.24, 0.27, 0.29, and 1.0 were refined from neutron powder diffraction data. The magnetic phase diagram could be completed in the coexistence range of different magnetic structures up to x = 0.29. For the magnetic state at 1.5 K a commensurate antiferromagnetic structure with a propagation vector = (±1/4, 1/2, 1/2) was found for x ⩽ 0.22 while the magnetic spins order with = (1/2, 0, 0) for x ≥ 0.22. In the latter phase, additionally, weak magnetic reflections indexed to an incommensurate ordering with = (- 0.214, 1/2, 0.457) occur in the diffraction pattern up to x = 0.29 indicating the occurence of a reentrant phase. For 0.12 ⩽ x ⩽ 0.29 the low temperature phases are separated from a magnetic high temperature phase showing only magnetic reflections indexed to a spin arrangement with = (1/2, 0, 0). The magnetic phase diagram is discussed qualitatively considering random superexchange between the statistically distributed Mn²⁺- and Fe²⁺-ions in the coexistence range 0.12 ⩽ x ⩽ 0.29 of different magnetic structures related to those of pure MnWO₄ and FeWO₄. Received 9 October 2002 Published online 14 March 2003     

Magnetic properties of LaNi <Emphasis Type="Bold">1-</Emphasis><Emphasis Type="Bold">x</Emphasis>Mn <Emphasis Type="Bold">x</Emphasis>O <Emphasis Type="Bold">3+δ</Emphasis> perovskites

Magnetic measurements have been carried out in different LaNi_1-xMn_xO _{3 + δ} samples with 0.1 ⩽ x ⩽ 0.9. All these samples show two magnetic anomalies, one at relatively high temperature characteristic of a ferromagnetic ordering and the other at low temperature, typical of magnetic relaxation phenomena. Neutron diffraction patterns indicate that long-range ferromagnetic ordering is only achieved for x ≥ 0.5. Neutron patterns of LaNi_0.5Mn_0.5O _{3 + δ} samples show an ordered arrangement of Ni and Mn atoms in the perovskite lattice. LaNi_0.5Mn_0.5O _{3 + δ} is then, a double perovskite A₂BB'O₆ whereas Ni and Mn atoms are randomly distributed for the rest of the samples. X-ray magnetic circular dichroism experiments confirm the presence of collinear ferromagnetism in LaNi_0.5Mn_0.5O _{3 + δ} . The role of competitive magnetic interactions, structural disorder, magnetic anisotropy and magnetic disaccommodation is also discussed Received 19 July 2002 / Received in final form 23 October 2002 Published online 31 December 2002     

A new quasi-Ising magnet

We have performed measurements of the magnetization and differential magnetic susceptibility of Dy_0.62Y_2.38Fe₅O₁₂ single crystals in pulsed magnetic fields up to 45 T at liquid-helium temperature for three orientations of the external field: H‖[100], H‖[110], and H‖[111]. It was found that the magnetization reversal in the rare-earth magnetic subsystem occurs via several phase transitions, whose number depends on the direction of the external field, as is characteristic for Ising magnets. The anomalies in the field dependences of the magnetization are interpreted on the assumption of quasi-Ising ordering of the rare-earth ions. Pis’ma Zh. éksp. Teor. Fiz. 67, No. 8, 552–556 (25 April 1998)     

Preparation, magnetoresistance and magnetocaloric effect of two-layered perovskite La 2.5- x K 0.5+ x Mn 2 O 7+δ

Polycrystalline two-layered perovskite La_2.5-xK_0.5+xMn₂O _{7 + δ} (0 < x < 0.5) samples have been prepared by a modified sol-gel method and their magnetoresistance and magnetocaloric effects have been studied. A large deviation between the metal-insulator (MI) transition temperature (T _ρ ) and the magnetic transition temperature (T_C) is observed. Large magnetoresistance (MR) effects with Δρ/ρ of ∼40% at 12 kOe are obtained in wide temperature ranges. The maximum of the magnetic entropy change peaks at its Curie temperature (T_C), far above its MI transition temperature (T _ρ ). The large magnetic entropy change (∼1.4 J/kg.K) is obtained in the sample La_2.5-xK_0.5+xMn₂O _{7 + δ} (x = 0.35) upon 10 kOe applied magnetic field. Received 2 May 2002 / Received in final form 1st October 2002 Published online 19 December 2002 RID="a" ID="a"e-mail: wzhong@ufp.nju.edu.cn     

More about neutron–mirror neutron oscillation

It was pointed out recently that oscillation of the neutron n into a mirror neutron n′, a sterile twin of the neutron with exactly the same mass, could be a very fast process with baryon number violation, even faster than the neutron decay itself. This process is sensitive to magnetic fields and it could be observed by comparing the neutron loss rates in the UCN storage chambers for different magnetic backgrounds. We calculate the probability of the n−n′ oscillation in the case when a mirror magnetic field B′ is non-zero and show that in this case it can be suppressed or resonantly enhanced by applying the ordinary magnetic field B, depending on its strength and on its orientation with respect to B′. The recent experimental data, under this hypothesis, still allow for an n−n′ oscillation time of order 1 s or even smaller. Moreover, they indicate that the neutron losses are sensitive to the orientation of the magnetic field. If these hints will be confirmed in future experiments, this would point to the presence of a mirror magnetic field on the Earth of the order of 0.1 G, or some equivalent spin-dependent force of other origin that makes a difference between the neutron and mirror neutron states.     

Magnetic susceptibility of multilayered carbon nanotubes

A theoretical study of the magnetic susceptibility of multilayered carbon nanotubes in fields both parallel, H _∥, and perpendicular, H _⊥, to the tube axis has been carried out disregarding electron-electron interaction. The temperature dependences of the magnetic susceptibility obtained exhibit a nontrivial form for H _∥, which is related to the quasi-one-dimensionality of such a system as the nanotube. The dependences of the magnetic susceptibility on chemical potential χ(μ) have also been derived. At low temperatures, χ(μ) has sharp peaks in fields H _∥, which is connected with the presence of singularities in the density of states of nanotubes. The effect of interlayer coupling on magnetic susceptibility of small-radius tubes has been investigated numerically. Fiz. Tverd. Tela (St. Petersburg) 40, 1950–1954 (October 1998)     

Magnetic structure of Ce<Subscript>2</Subscript>Fe<Subscript>17 − <Emphasis Type="Italic">x</Emphasis></Subscript>Mn<Subscript><Emphasis Type="Italic">x</Emphasis></Subscript> intermetallic compounds

The magnetic structure of intermetallic compounds Ce₂Fe_{17 − x} Mn _x (0 ≤ x ≤ 3) was studied using neutron diffraction. The neutron diffraction patterns measured at 4.2 K contain satellites indicating a modulated structure with the wave vector k = [0, 0, τ]. As the concentration x increases, the value of τ increases, while the average magnetic moment of Fe/Mn atoms decreases. A change in the magnitudes of the average magnetic moment and wave vector k is explained by competition between exchange interactions at distances of nearest neighbor transition element atoms.     

Magnetic susceptibility in quasi one-dimensional Ba<Subscript>a2</Subscript>V<Subscript>3</Subscript>O<Subscript>9</Subscript>: chain segmentation versus the staggered field effect

A pronounced Curie-like upturn of the magnetic susceptibility χ( T ) of the quasi one-dimensional spin chain compound Ba₂V₃O₉ has been found recently [#!kaul:02!#]. Frequently this is taken as a signature for a staggered field mechanism due to the presence of g-factor anisotropy and Dzyaloshinskii-Moriya interaction. We calculate this contribution within a realistic structure of vanadium 3 d- and oxygen 2 p-orbitals and conclude that this mechanism is far too small to explain experimental results. We propose that the Curie term is rather due to a segmentation of spin chains caused by broken magnetic bonds which leads to uncompensated S = ? spins of segments with odd numbers of spins. Using the finite-temperature Lanczos method we calculate their effective moment and show that ∼ 1% of broken magnetic bonds is sufficient to reproduce the anomalous low-T behavior of χ( T ) in Ba₂V₃O₉. Received 19 December 2002 / Received in final form 29 January 2003 Published online 14 March 2003     

Manifestation of ferromagnetism in lightly oxygen-doped La2CuO4 single crystals in magnetic fields H<50 Oe

The temperature and field dependences χ(T,H) in La₂CuO_4+δ single crystals with δ<0.015 have been investigated in magnetic fields 0.1<H<450 Oe by the differential magnetic susceptibility method. It was found that under oxygen doping conditions ferromagnetic regions are formed. These regions produce a characteristic curve of the magnetic susceptibility χ(T,H), which is observed only in magnetic fields of less than 50 Oe. This can be explained by the formation of ferrons [A. Aharony et al. Phys. Rev. Lett. 60, 1330 (1988); L. I. Glazman and A. S. Ioselevich, Z. Phys. B 80, 268 (1990)] in an antiferromagnetic matrix. Pis’ma Zh. éksp. Teor. Fiz. 64, No. 3, 152–155 (10 August 1996)     

Insulator-metal transition shift related to magnetic polarons in La<Subscript>0.67-x</Subscript>Y<Subscript>x</Subscript>Ca<Subscript>0.33</Subscript>MnO<Subscript>3</Subscript>

The magnetic transport properties have been measured for La_0.67-xY_xCa_0.33MnO₃ ( 0 ⩽ x ⩽ 0.14) system. It was found that the transition temperature T _p almost linearly moves to higher temperature as H increases. Electron spin resonance confirms that above T _p , there exist ferromagnetic clusters. From the magnetic polaron point of view, the shift of T _p vs. H was understood, and it was estimated that the size of the magnetic polaron is of 9.7 ∼ 15.4 ? which is consistent with the magnetic correlation length revealed by the small-angle neutron-scattering technique. The transport properties at temperatures higher than T _p conform to the variable-range hopping mechanism. Received 27 August 2002 / Received in final form 2 December 2002 Published online 14 March 2003     

An analytical solution of the Klein–Fock–Gordon equation for a 2D pion atom moving in a constant uniform magnetic field

The Klein–Fock–Gordon equation is solved for a 2D pion moving in a constant uniform magnetic field. A relativistic energy spectrum is calculated for fixed values of the angular momentum and magnetic field Н. An analysis of the results of these calculations allows us to conclude that the Klein–Fock–Gordon equation, unlike the Schr?dinger equation, cannot describe the energy of the particle s-state in the magnetic field. It is elucidated that a correction for the relativistic energy level caused by the constant magnetic field is noticeable for the magnetic field H > 100. Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 3, pp. 91–96, March, 2009.     

Magnetic-field-induced coherence in hyper-Rayleigh scattering

Second harmonic generation by a disordered array of superparamagnetic nanoparticles in a static magnetic field H is studied experimentally. For H = 0, only hyper-Rayleigh scattering takes place; i.e., the second-harmonic radiation is diffuse and unpolarized. For H ≠ 0, a coherent (specular and linearly polarized) component appears against the hyper-Rayleigh scattering background. The phase of the coherent component changes by π when the direction of the magnetic field is reversed. It is shown that the effect can be explained by correlations in the spatial fluctuations of the nonlinear-optical and magnetic polarizabilities of the particles, taking into account the nonuniformity of the effective (local) static magnetic field.     

Characteristics of the statistical distribution of the current transmitted by a cathode spot of a vacuum arc in variously oriented magnetic fields

The influence of variously oriented uniform magnetic fields on the cathodic attachment of a low-current vacuum arc with electrodes made of oxygen-free copper and CuCr30 composition is studied. It is found that, if the current is fixed, cathode spots in the arc attachment are distributed by the normal law in the entire range of variation of the amplitude of magnetic induction vector B and angle α between this vector and the normal to the cathode surface. The parameters of the distribution depend on the magnetic field and cathode material. The magnetic field dependence is appreciable only when angle α exceeds some critical value α* (α* ≈ 30° and ≈45° for cathodes made of copper and CuCr30, respectively). At α > α*, the parameters of the distribution become strongly dependent on α, while the B dependence remains weak. Only when α → π/2 does the field amplitude have a pronounced effect on the parameters of the distribution. From the obtained results, we determine the statistical characteristics of the distribution of the mean current transmitted by a cathode spot in variously oriented magnetic fields. The found relationships make it possible to explain the peculiarities of the structure of the cathodic attachment of the high-current vacuum arc stabilized by an external axial magnetic field.     

Dynamic self-organization of magnetic domains in amorphous films with perpendicular anisotropy

Dynamic self-organization of magnetic domains is observed in amorphous gadolinium-cobalt films in narrow temperature intervals on both sides of the magnetic compensation point. Spiral dynamic domains form in a limited range of ac magnetic field amplitudes and frequencies. Pis’ma Zh. éksp. Teor. Fiz. 66, No. 11, 688–692 (10 December 1997)     

Photoinduced changes in the space-modulated magnetic order of a FeBO<Subscript>3</Subscript>:Mg single crystal

An effect of nonpolarized white light on the modulated magnetic structure of a FeBO₃:Mg single crystal, which arises in this light-plane weak ferromagnet in the low temperature range during technical magnetization, has been revealed. It has been found that the degree of the light action on the magnetic state of FeBO₃:Mg depends both on its duration and on the orientation of the spontaneous magnetization vector M of the crystal during illumination. Interpretation of the results obtained has been performed in the context of the “magnetic ripple” theory on the assumption that the absorbed light induces additional uniaxial magnetic anisotropy in the easy plane of the crystal and that the anisotropy axis is collinear to the vector M during illumination.     

Magnetization and neutron scattering studies of the pressure effect on the magnetic transition in Er Y Co

Neutron powder diffraction was employed to study the pressure effect on the magnetic transition in the pseudobinary Laves-phase compound Er_0.57Y_0.43Co₂ and to determine the magnetic moments of the Er- and Co-subsystems. Our studies reveal that the onset of long-range magnetic order for both the localized 4 f (Er) and itinerant 3 d (Co) electron moments appears at about the same temperature at ambient pressure. The pressure effect on T_c is found to be negative and equal for both sublattices, namely T _c / p ∼ - 0.4 K/kbar. The values of the magnetic moments of the Er and the Co ions are found = 5.40±0.15μ _B /atom, = 0.50±0.07μ _B /atom and 5.35±0.15μ _B /atom, 0.37±0.09μ _B /atom, for p = 0 and 6 kbar, respectively. Our experimental results give evidence for short-range magnetic order formation at temperatures already above T_c and for a coexistence short- and long-range order below T_c down to 4 K. Received 20 December 2001 / Received in final form 12 June 2002 Published online 31 October 2002 RID="a" ID="a"e-mail: andrew.podlesnyak@psi.ch     

Ohm’s law in a chiral plasma

The motion of plasma electrons in a stochastic electromagnetic field is studied in the low-conductivity limit. It is shown that under very general conditions, in the presence of a nonzero average chirality of the small-scale electromagnetic field, the effective current depends on the curl of the applied electric field, j=§ E+§_κcurl E, just as for similar dependences for the electric displacement and magnetic induction vectors in optically active and artificial chiral media. Under certain conditions such an Ohm’s law leads to growth of the magnetic field, the structure of the growth being dependent on the conductivity of the medium. Pis’ma Zh. éksp. Teor. Fiz. 70, No. 4, 268–273 (25 August 1999)     

Dynamic magnetic susceptibility of a superconductor with a relaxing magnetic moment

Within the framework of the diffusion approximation for the dynamic magnetic flux, a model is constructed for the dynamic magnetic susceptibility of a superconductor with a nonuniform and time-dependent magnetic field distribution in the sample. The possibility of appearance of peaks in the temperature (or frequency) dependence of χ″ in a structurally homogeneous superconducting sample in the presence of a magnetic-field-induced nonuniformity of the diffusion parameter is demonstrated. The character of the temporal evolution of the magnetic susceptibility during relaxation of the magnetic moment of the sample is predicted and its properties are investigated. Fiz. Tverd. Tela (St. Petersburg) 39, 811–815 (May 1997)     

Nuclear magnetic resonance of 55Mn in the antiferromagnet CsMnBr3 in a variable longitudinal magnetic field

The spectrum and intensities of NMR lines are investigated experimentally and theoretically for excitation by an alternating magnetic field h‖ parallel to a static field H in the quasi-one-dimensional, six-sublattice antiferromagnet CsMnBr₃. According to theory, two new NMR lines, which are not excited by a transverse magnetic field h _⊥, are observed near the phase transition from triangular to collinear structure (H=H _c ) [JETP 86, 197 (1998)]. Zh. éksp. Teor. Fiz. 115, 2228–2241 (June 1999)