The electric quadrupole moment of the first excited state of 204Hg

The static electric quadrupole moment Q₂₊ and the B(E2; 0⁺ → 2⁺) value of the 2⁺ first excited state of ²⁰⁴Hg have been determined using the reorientation effect in Coulomb excitation. An annular Si surface-barrier detector was used to detect back-scattered ⁴He, ¹²C and ¹⁶O projectiles. In a subsidiary experiment, spectra were obtained from ²⁰⁴Hg(p, p')²⁰⁴Hg using Si surface-barrier detectors, and the results were used in conjunction with previously existing data to provide information on higher states of ²⁰⁴Hg which might participate in the Coulomb excitation of the 2⁺ state. From a 3-level analysis, we find Q₂₊ = +0.40 ± 0.20 e · b and B(E2; 0⁺ → 2⁺) = 0.423 ± 0.005 e² · b². These results are in good agreement with the predictions of particle-vibrational coupling calculations. The value obtained for $\text{Q}{}_{\mathrm{2+}}\text{(}{}^{204}\text{Hg)}$ is substantially smaller in magnitude than values of Q₂₊ previously determined for ^{198, 200, 202}Hg.     

Determination of the spectroscopic quadrupole moments of 131Cs, 132Cs and 136Cs

Nuclear spectroscopic quadrupole moments of the radioactive isotopes ¹³¹Cs, ¹³²Cs, and ¹³⁶Cs have been determined from the hyperfine structure of the $\text{6}{}^2\text{P}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}$ state by the level crossing method. The results including a Sternheimer correction are: $\text{Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{131}\text{Cs}\text{) = ?0.625(6)}\text{b}$, $\text{Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{132}\text{Cs}\text{) = +0.508(7)}\text{b}$, $\text{Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{136}\text{Cs}\text{) = +0.225(10)}\text{b}$. The quadrupole moments of all the Cs isotopes from A = 131 to A = 137 are recalculated. It is shown, that nuclear quadrupole moments of a specific isotope obtained from different atomic P-states only agree within the limits of error after application of the Sternheimer correction. The increase of Q_s with decreasing neutron number conforms with other observations and theoretical calculations stating that for elements around Z = 55 nuclear deformation develops below N = 82. The staggering of the sign of Q_s may be interpreted as consequence of an oblate-prolate degeneracy of the nuclear energy surface. Some magnetic moments have been slightly improved: $\text{μ}{}_{\mathrm{<mtext>I</mtext>}}\text{(}{}^{132}\text{Cs}\text{) = 2.219(7) μ}{}_{\mathrm{<mtext>N</mtext>}}$, $\text{μ}{}_{\mathrm{<mtext>I</mtext>}}\text{(}{}^{136}\text{Cs}\text{) = 3.705(15)μ}{}_{\mathrm{<mtext>N</mtext>}}$ (corrected for diamagnetism).     

Study of low-lying states in 92Tc with the 92Mo(3He,t) reaction

States in ⁹²Tc have been studied by means of the ⁹²Mo(³He, t) reaction at 27.5 MeV. The Q-value for this reaction and the excitation energy of the isobaric ground state analogue of ⁹²Mo were determined to be ?7.882 ± 0.030 MeV and 3.813 ± 0.030 MeV respectively. Strongly populated levels in ⁹²Tc appear to belong to configurations arising from the $\text{(1g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}_{\mathrm{\pi }}\text{(1g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}_{\mathrm{\nu }}{}^{\mathrm{?1}}$ multiplet.     

Core polarization effects in the πh92 shell and g-factors of the 8+ states in 204Po and 206Po

The $\text{g-}\text{values of}\text{[(π}\text{h}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}^2\text{, 8}{}^{\mathrm{+}}\text{]}$ isomeric levels in ²⁰⁴Po and ²⁰⁶Po have been measured with the stroboscopic method. The results obtained are: $\text{g(}{}^{204}\text{Po}\text{) = 0.923±0.013}\text{and}\text{g(}{}^{206}\text{Po}\text{) = 0.919±0.013}$. These and other known $\text{g-}\text{factors of}\text{(π}\text{h}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}^{\mathrm{n}}$ states in the ²⁰⁸Pb region are compared with theoretical predictions in order to analyze the dependence of the $\text{h}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ proton g-value on the core constitution. The variation of the g-values is systematically smaller than expected from first-order configuration mixing theory, if pure shell-model wave functions are assumed.     

The quadrupole moments of the 5− states in 116Sn, 118Sn and 120Sn

The quadrupole interaction frequencies $\text{ω}{}_0\text{=}\text{3eQ}{}_1\text{V}{}_{\mathrm{zz}}\text{41(21-1)}\text{h}\text{?}$ in the 5^? state of ¹¹⁸Sn have been measured by time differential perturbed angular correlation technique in Sn, Sb and (95% Sn+5% Sb) environments. The ω₀ for ¹¹⁶Sn was determined in Sn environment only. With the help of the known electric field gradient ¹) of Sn in a Sn lattice the quadrupole moments have been deduced as $\text{Q(5}{}^{\mathrm{?}}\text{,}{}^{118}\text{Sn}\text{) = ±0.10(4) b}\text{and}\text{Q(5}{}^{\mathrm{?}}\text{,}{}^{116}\text{Sn}\text{) = ±0.165(60)}\text{b}$. These values together with the known²) quadrupole moment of the analogous 5^? state in ¹²⁰Sn are interpreted in terms of the pure single-particle model. The data exhibit the expected strong systematic variation of Q_I with the number of particles in the h_{$\text{11}\text{2}$}. subshell which is being filled with 1, 3 and 5 neutrons in ¹¹⁶Sn, ¹¹⁸Sn, and ¹²⁰Sn, respectively.     

The electric quadrupole moment of the 6+ state of 112Sn

The spectroscopic quadrupole moment of the isomeric 6⁺' (2552 keV) state of ¹¹⁷Sn has been derived from TDPAD measurements in a Cd metal host target at 500 K as $\text{Q}{}_{\mathrm{<mtext>I</mtext>}}\text{(6}{}^{\mathrm{+}}\text{,}{}^{112}\text{Sn}\text{) = ± 0.29(6)}\text{b}$. The calibration of the effective field gradient for Sn in Cd at 500 K, given by Herrlander et al. has been used. A comparison of the results with shell model estimates makes a mixed configuration of $\text{|(}\text{g}\text{7}\text{2}\text{)}{}^{\mathrm{?2}}\text{6}{}^{\mathrm{+}}\text{〉)}\text{and}\text{(}\text{g}\text{7}\text{2}{}^{\mathrm{?1}}\text{d}\text{5}\text{2}{}^{\mathrm{?1}}\text{)6}{}^{\mathrm{+}}\text{〉)}$ for the 6⁺ state most likely.     

Projectile Coulomb excitation of 24Mg

The static quadrupole moment of the first excited J^π = 2⁺ state in ²⁴Mg and the reduced electric quadrupole transition probability between this state and the ground state were measured via projectile Coulomb excitation. The quadrupole moment was deduced from the shapes of γ-ray angular distributions. The result is $\text{Q(}{}^{24}\text{Mg}\text{, 2}{}^{\mathrm{+}}\text{) = ?0.27±0.05}\text{b}$. The transition strength was deduced from yield measurements and by comparison with the yields of target γ-rays, The result is $\text{B(}\text{E}\text{2; 0}{}^{\mathrm{+}}\text{→ 2}{}^{\mathrm{+}}\text{,}{}^{24}\text{Mg}\text{) = 0.044±0.003 e}{}^2\text{·}\text{b}{}^2$. The experimental measurements are compared with theoretical predictions and previous measurements and a detailed discussion is given of corrections to this type of reorientation experiment.     

Neutron resonance parameters and radiative capture cross sections of 147Sm and 149Sm

Neutron capture and transmission measurements have been carried out on the separated isotopes of ¹⁴⁷Sm (98.34 %) and ¹⁴⁹Sm (97.72 %) at the 55 m time-of-flight station of the Japan Atomic Energy Research Institute electron linear accelerator. Resonance energies and neutron widths for a large number of resolved resonances were determined up to 2 keV for ¹⁴⁷Sm and 520 eV for ¹⁴⁹Sm. Radiation widths for 5 resonances in ¹⁴⁷Sm + n and 7 resonances in ¹⁴⁹Sm + n were derived. The s-wave strength functions, average level spacings and average radiation widths were obtained to be: $\text{10}{}^4\text{S}{}_0\text{= 4.8 ± 0.5,}\text{D}\text{= 5.7 ± 0.5}\text{eV}$ and $\text{Γ}{}_{\mathrm{\gamma }}\text{= 69 ± 2}\text{meV for}{}^{147}\text{Sm}$; a $\text{10}{}^4\text{S}{}_0\text{= 4.6 ± 0.6,}\text{D}\text{= 2.2 ± 0.2}\text{eV}$ and $\text{Γ}{}_{\mathrm{\gamma }}\text{= 62 ± 2}\text{meV for}{}^{149}\text{Sm}$. The average capture cr sections were deduced from 3.3 to 300 keV with an estimated accuracy of 5 to 15 %. The measured capture cross sections for ¹⁴⁹Sm are largely different from the evaluated data, which are obtained based on the statistical model calculation. Possible reasons for this disagreement are discussed.     

Magnetic moment of a core-excited isomeric state in 210Po

The g-factor of the core-excited isomeric 13^? state in ²¹⁰Po has been determined to be +0.546 ± 0.012 with the time-differential spin-rotation method in the ²⁰⁸Pb(α, 2n)²¹⁰Po reaction. This value supports the configuration of $\text{[(π}\text{h}{}^2{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)8}{}^{\mathrm{+}}\text{? 5}{}^{\mathrm{?}}\text{(}{}^{208}\text{Pb}\text{)] 13}{}^{\mathrm{?}}$.     

Lifetime and g-factor results for the 132− 1985 keV level in 91Nb and the 152− 2288 keV level in 91Zr

Lifetime and g-factor measurements have been made with pulsed beam-γ time-differential techniques using the ⁸⁹Y(α, 2n)⁹¹Nb and ⁸⁸Sr(α, n)⁹¹Zr reactions. A mean lifetime τ = 14.4 ± 0.5 nsec and a g-factor of 1.26 ± 0.04 were obtained for the $\text{13}\text{2}{}^{\mathrm{?}}$ 1985 keV level in ⁹¹Nb and τ = 41.9 ± 1.2 nsec and g = 0.70 ± 0.01 were obtained for the $\text{15}\text{2}{}^{\mathrm{?}}$ 2288 keV level in ⁹¹Zr. These results are compared to theoretical calculations for $\text{(π}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}^2\text{(π}\text{p}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{)}$ and $\text{(π}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)(π}\text{p}\text{1}\text{2}\text{)(v}\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}\text{)}$ configurations in ⁹¹Nb and ⁹¹Zr, respectively.     

The g-factor of the72+[404] ground state of 177Ta

With the technique of nuclear magnetic resonance on oriented nuclei the hyperfine splitting $\text{ν}{}_{\mathrm{<mtext>M</mtext>}}\text{= ¦gμ}{}_{\mathrm{<mtext>N</mtext>}}\text{B}{}_{\mathrm{<mtext>HF</mtext>}}\text{/h¦}\text{of}{}^{177}\text{Ta}\text{(j}{}^{\mathrm{\pi }}\text{7}\text{2}{}^{\mathrm{+}}\text{; T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 56.6h)}$ in Fe has been measured With the known hyperfine field $\text{B}{}_{\mathrm{<mtext>HF</mtext>}}\text{(}\text{Ta}\text{Fe}\text{) = ?648 (13)}\text{kG the}\text{g-}\text{factor of the}\text{7}\text{2}{}^{\mathrm{+}}\text{[404]}$ ground state of ¹⁷⁷Ta is deduced to be $\text{¦g¦ = 0.643 (13)}$.     

Strong sequential transfer processes in 0+ → 0+ (p,t) reactions on Pb isotopes

A marked difference of experimental analyzing powers $\text{A (θ)}\text{for}{}^{208}\text{Pb}\text{(}\text{p}\text{,}\text{t}\text{)}{}^{206}\text{Pb}\text{(0}{}_{\mathrm{<mtext>g</mtext>}}{}^{\mathrm{+}}\text{and}\text{0}{}_2{}^{\mathrm{+}}\text{)}$ reaction is explained by considering sequential transfer as wesses as well as the one-step process. The calculated A(0θ) for the 0₂⁺ state is very sensitive to the wave functions employed. An enhancement of the cross sections for the ground-state transitions of three Pb isotopes is found to be due to sequential transfer processes.     

Polarization of 12B in deep-inelastic heavy-ion reaction 100Mo(14N, 12B)

Spin polarization of ¹²B was measured for ¹⁰⁰Mo(¹⁴N, ¹²B) at $\text{E}{}_{\mathrm{<mtext>i</mtext>}}\text{(}{}^{14}\text{N}\text{) ? 200}\text{MeV}$ as a function of $\text{Q}$ value down to $\text{Q ? ?150}\text{MeV}$, and was found anti-parallel to $\text{k}{}_{\mathrm{f}}\text{×}\text{k}{}_{\mathrm{i}}$ in the deep-inelastic region. The data together with those at lower incident energies show a systematic trend in $\text{Q}$-value dependence of the polarization.     

Negative-parity states in Pb isotopes: g-factor of the 480 ns,if Jπ = 9− isomer in 200Pb

The g-factor of the 480 ns, 9^? isomer at 2.237 MeV in ²⁰⁰Pb was measured by the time-differential perturbed angular distribution method. The result, g = ?0.0285±0.0011 confirms the rather pure $\text{(}\text{f}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}{}^{\mathrm{?1}}\text{i}{}_{\mathrm{<mtext>13</mtext><mtext>2</mtext>}}{}^{\mathrm{?1}}\text{)}$ quasiparticle structure of this state. Half-lives of 480±20 ns, 43±3 ns and 42±4 ns have been measured for the 2237 keV 9^?, 2154 keV 7^? states in ²⁰⁰Pb and the 2208 keV state in ²⁰²Pb, respectively; E2 transitions and g-factors of negative-parity states in even, neutron-deficient Pb isotopes are discussed.     

The g-factor difference for the 61+ and 88+ states in 210Po

The difference in g-factors for the 6₁⁺ and 8₁⁺$\text{(πh}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}{}^2\text{)}$ states in ²¹⁰Po has been measured as $\text{(g}{}_6\text{? g}{}_8\text{)}\text{g}{}_8\text{= 2.0 ± 0.7\%}$. This result represents a small violation of additivity. A value of g₈ = 0.909 ± 0.011, independent of g₆, was also obtained.     

The electronic isotope shift in the A2Π-X2Σ+ bands of BeH,BeD and BeT

The 0-0, 1-1, 2-2, and 3-3 bands of the A²Π-X²Σ⁺ transition of the tritiated beryllium monohydride molecule have been observed at 5000 Å in emission using a beryllium hollow-cathode discharge in a He + T₂ mixture. The rotational analysis of these bands yields the following principal molecular constants.

$\text{A}{}^2\text{Π:}\text{B}{}_{\mathrm{e}}\text{= 4.192}\text{cm}{}^{\mathrm{?1}}\text{; r}{}_{\mathrm{e}}\text{= 1.333}\text{A}\text{?}$

$\text{X}{}^2\text{Σ:}\text{B}{}_{\mathrm{e}}\text{= 4.142}\text{cm}{}^{\mathrm{?1}}\text{; r}{}_{\mathrm{e}}\text{= 1.341}\text{A}\text{?}$

$\text{ω}{}_{\mathrm{e}}\text{′ ? ω}{}_{\mathrm{e}}\text{″ = 16.36}\text{cm}{}^{\mathrm{?1}}\text{; ω}{}_{\mathrm{e}}\text{′X}{}_{\mathrm{e}}\text{′ ? ω}{}_{\mathrm{e}}\text{″X}{}_{\mathrm{e}}\text{″ = 0.84}\text{cm}{}^{\mathrm{?1}}$

From the pure electronic energy difference (E_Π - E_Σ)_BeT = 20 037.91 ± 1.5 cm^?1 and the corresponding previously known values for BeH and BeD, the following electronic isotope shifts are derived

$\text{ΔE}{}_{\mathrm{e}}{}^{\mathrm{i}}\text{(}\text{BeH}\text{?}\text{BeT}\text{) = ?4.7 ≠ 1.5}\text{cm}{}^1\text{, ΔE}{}_{\mathrm{e}}{}^{\mathrm{i}}\text{(}\text{BeH}\text{?}\text{BeT}\text{) = ?1.8 ≠ 1.5}\text{cm}{}^1$

and related to the theoretical approach given by Bunker to the problem of the breakdown of the Born-Oppenheimer approximation.     

The ππ and KK amplitudes,the S1 and the quark structure of 0++ resonances

The nature of mesons in the 0⁺⁺ nonet is studied. In particular we discuss the parameterization of the I = 0 S wave in terms of the S¹ and possible ? mesons. The S¹ parameters are determined by fitting to π^?π⁺ and K^?K⁺ production data. In particular we find .     

Coulomb excitation of 85Rb and 87Rb

Energy levels of ⁸⁵Rb and ⁸⁷Rb have been studied via de-excitation γ-rays following Coulomb excitation with ³⁵Cl ions. In addition to the known negative-parity states at 151.2 keV and 868.2 keV in ⁸⁵Rb, two states at 281.0 keV and 731.8 keV have been found with fourγ-ray transitions of 129.8, 281.0, 450.8 and 731.8 keV. Only one Coulomb excited state at 402.6 keV in ⁸⁷Rb has been observed. The B(E2↑) values (in units e² · b²) have been determined as 0.0035±0.0004 (151.2 keV), 0.0016±0.0002 (281.0 keV), 0.0101 ±0.0010 (731.8 keV), and 0.036±0.004 (868.2 keV) for the states in ⁸⁵Rb, and as 0.0054±0.0006 (402.6 keV) for the state in ⁸⁷Rb. The mean lifetimes of the 731.8 keV and 868.2 keV states have been measured by the Doppler shift attenuation method as 6.4±0.7 psec and 4.2±0.5 psec respectively. Angular distribution measurements allow unique spin and parity assignments of $\text{1}\text{2}{}^{\mathrm{?}}$ and $\text{3}\text{2}{}^{\mathrm{?}}$ to the 281.0 keV and 731.8 keV levels respectively. The spin and parity of the 868.2 keV level has been restricted to $\text{5}\text{2}{}^{\mathrm{?}}$ or $\text{7}\text{2}{}^{\mathrm{?}}$.     

Measurement of the g-factor and mean lifetime of the 13C(52+1) state

The g-factor and mean life of the $\text{5}\text{2}{}^{\mathrm{+}}{}_1$ state at 3.85 MeV in ¹³C have been determined by a recoil-into-vacuum plunger measurement. The state was populated by the ²H(¹²C, p) reaction at E = 15.0 MeV. The analysis of the time-differential deorientation effect on the p-γ angular correlation leads to a g-factor of $\text{¦g¦ = 0.558 ± 0.015}$. For the mean lifetime a value of τ = 12.2 ± 0.4ps is obtained.     

Measurement of the electric quadrupole moment of the 482 keV state of 181Ta by the time differential perturbed angular correlation technique

The electric quadrupole interaction of the 482 keV state of ¹⁸¹Ta in an environment of metallic rhenium has been investigated by time differential angular correlation measurements. For the field gradient calibration a recent observation^{1, 2}) of the quadrupole splitting of the 6.3 keV line of ¹⁸¹Tain the same environment has been used. Adopting the quadrupole moment of the ground state which was derived from muonic X-ray data ³) we obtain $\text{Q}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}\text{(482}\text{keV}\text{) = 2.51 ± 0.15}\text{b}$. A comparison of the intrinsic quadrupole moment Q₀ with that of the ground state revealed that the excited state is slightly less deformed: $\text{Q}{}_0\text{(}\text{5}\text{2}{}^{\mathrm{+}}\text{)/Q}{}_0\text{(}\text{7}\text{2}{}^{\mathrm{+}}\text{) = 0.936 ± 0.014}$. A measurement of the temperature dependence between liquid nitrogen and room temperature showed that the electric quadrupole interaction remains essentially constant.