Natural radiative lifetimes in the1 P 1 and1 F 3 sequences of Sr I

We have measured radiative lifetimes in the 5s n p ¹ P ₁ (n=5–29) and 5s n f ¹ F ₃ (n=4–11) Rydberg series in neutral strontium. The measurements were performed with single-step laser excitation starting from the ground state or from a metastable state populated by collisions. The decay photons were detected using delayed coincidence technique or a transient recorder. The presence of configuration interaction in the 5s n p ¹ P ₁ series can be observed aroundn=8. The perturbation in the 5s n f ¹ F ₃ series is not reflected in the behaviour of the lifetime values.     

Soft X-ray appearance potential spectroscopy (SXAPS) study of TiO2(1 1 0)-1 × 2 and (0 0 1)-1 × 1 surfaces

A soft X-ray appearance potential spectroscopy (SXAPS) apparatus with high sensitivity was built to measure non-derivative spectra. SXAPS spectra (non-derivative) of Ti 2p and O 1s for TiO₂(1 1 0)-1 × 2 and (0 0 1)-1 × 1 surfaces have been measured using low incident currents (about 10 μA/cm²) and a photon counting mode. Density of empty states on Ti and O sites are deduced by self-deconvoluting the spectra. The self-deconvoluted SXAPS spectra are qualitatively similar to those measured by X-ray absorption spectroscopy (XAS). The Ti 2p_3/2 spectrum shows two strong peaks which correspond to t_2g and e_g states. For the O 1s spectrum two strong peaks near the threshold are also found which can be ascribed to O 2pπ and O 2pσ states. These results suggest that the spectra almost obey the dipole selection rule, so-called the “approximate dipole selection rule”. The SXAPS spectra of Ti 2p and O 1s for the (1 1 0) and (0 0 1) surfaces resemble qualitatively, which is consistent with the XAS results. The spectra measured on the (1 1 0)-1 × 2 surface at an incident angle of 45° off normal to the surface and on the (1 1 0) surface sputtered by Ar ions indicate that SXAPS is very sensitive to the surface electronic states.     

Levelcrossing experiments in the first excited1 P 1 states of the alkaline earths

The hyperfine structure of the lowest¹P₁ state of²⁵Mg,⁴³Ca,⁸⁷Sr,¹³⁵Ba and¹³⁷Ba have been measured by the level-crossing and anticrossing technique. The magnetic dipole and electric quadrupole coupling constants determined by these measurements are²⁵Mg(3s3p¹P₁):A=? 7.7(5) MHz; 16 MHz>B>0 MHz,⁴³Ca(4s4p¹P₁):A=? 15.3(4) MHz; ¦B¦<12 MHz,⁸⁷Sr (5s5p¹P₁:A=? 3.4(4) MHz;B=39(4) MHz,¹³⁵Ba(6s6p¹P₁):A=? 97.5(1.0) MHz;B=31(9)MHz,¹³⁷Ba(6s6p¹P₁):A=?109.2(1.2) MHz;B=51(12)MHz. The results have been compared with the predictions of the Breit-Wills theory of the two-electron hyperfine structure using the experimental data on the³P states. Large discrepancies have been observed which are due to different radial wave functions of thes andp electron in the triplet and singlet system. This effect has been taken into account by fitting the data with the aid of two additional parameters. That this procedure is justified is shown by an analysis of the fine structure splitting, the life times, and the isotopic shifts in thesp configurations of group II elements.     

Facteur de landé du niveau (6s26p 7s) 3P1 du plomb et constante de structure hyperfine de l'isotope 207Pb dans ce niveau

The Landé factor g_J of the (6s² 6p 7s)( ³P₁ level of the even isotopes of lead has been measured by Fabry-Pérot interferometry. The result is: g_J=1.3500(4). The agreement with the previously measured hyperfine splitting of this level for the isotope ²⁰⁷Pb and with the level crossing results is good when small corrections (nuclear Zeeman interaction, second-order hyperfine and Zeeman corrections) are taken into account. The corrected hyperfine dipole coupling constant for this level of ²⁰⁷Pb is: A=293.60(13) mK.     

Hyperfine structure of the 4s4p1P1-state of67Zn by level crossing spectroscopy

The magnetic dipole coupling constantA of the 4s 4p¹P₁ state of⁶⁷Zn was measured in a level crossing experiment. The result is A(4s4p¹P₁ ⁶⁷Zn)= 17.7(5) MHz. In a modified Breit-Wills theory thisA factor leads to a parameter λ_P= 0.71(3), which describes the difference in the radial wave functions of thep-electron in 4s4p¹P₁ and³P₁ states respectively. The lifetime of the 4s4p¹P₁ state was remeasured by Hanle-effect experiments. The result τ=1.41± 0.04 nsec is in good agreement with other measurements.     

Measurements of the probability for 1 sσ excitation in very heavy ion-atom-collisions and determination of the binding energy of the 1 σ molecular orbital

Using particle x-ray coincidence techniques, the probability to produceK-shell vacancies in 4.7 MeV/u Pb+Z₂ (42≦Z ₂≦92) collisions for impact parametersb<100 fm was measured. For these impact parameters, the 1sσ excitation probability is greater than 1 σ 10^?2 and the 2p _1/2 σ excitation probability is greater than 1 σ 10^?1. Binding energies of the 1sσ state derived from the measured probabilities agree well with theoretical calculations.     

Half-life and magnetic moment of the 1+ first excited state in116Sb

The life-time and the magnetic dipole moment of the 1⁺ isomeric state in¹¹⁶Sb have been measured by the TDPAD method. The state was populated in the reaction¹¹⁶Sn(p, n)¹¹⁶Sb atE _p =15 MeV. The obtained results,μ(1⁺,¹¹⁶Sb)=+2.47(9) n.m. andT _1/2= 194(4) ns, support the pure single particle [πd _5/2*vd _3/2] configuration for the 1⁺ isomeric state.     

Effect of melanin on phosphorus T1s in human melanoma xenografts studied by 31P MRS

³¹P MRS resonance ratios of tumors depend on the T₁s of the phosphorus compounds. The objective of the ³¹P MRS study reported here was to investigate whether the phosphorus T₁s of melanomas are influenced by the presence of melanin. One amelanotic (COX-t) and one melanotic (ROX-t) human melanoma xenograft line were studied at two different tumor volumes: 200 and 1000 mm³. ³¹P MRS was performed in nonanaesthetized mice at 4.7 T. The T₁s were measured by using the superfast inversion recovery technique. Fraction of necrotic tissue in the tumors was determined by histological examination. The ROX-t tumors showed shorter T₁s than the COX-t tumors at a volume of 200 mm³, where the fraction of necrotic tissue in the tumors was insignificant. The difference was similar in magnitude for all resonances. The T₁s were not significantly different for COX-t and ROX-t at a volume of 1000 mm³, where the tumors of both lines had developed significant necrosis. The phosphorus T₁s of melanomas without necrosis can be shortened significantly by the presence of melanin. The magnitude of the T₁ shortening is similar for all major compounds. ³¹P MRS resonance ratios of melanomas are not altered significantly by correcting for effects of partial saturation.     

Forward K1+ (892) production in K+p → π+Ks0p at 12.7 GeV/c

We have measured 618 K⁺p → π⁺K_S⁰p events at 12.7 GeV/c incident lab momentum, mass range 790 ? m_π⁺Ks⁰ ? 990 MeV and t range 0.01 ? ?t ? 0.60 (GeV/c)². The π⁺K_S⁰ mass spectrum is dominated by the K¹⁺ (892) resonance and a Breit-Wigner fit yields a mass m = 893.5 ± 1.1 MeV and a width Γ = 33.2 ± 4.1 MeV which is much narrower than measured hitherto. The t distribution of K¹⁺ (892) events shows a dip in the forward direction and an exponential fall off thereafter, consistent with dominance of helicity flip amplitudes. The spin density matrix is almost saturated by ρ₁₁ and ρ_1?1 which are very close to their maximum allowed value of $\text{1}\text{2}$ throughout the measured t range except in the very forward direction where ρ₀₀ and Re ρ₁₀ deviate from zero. Natural parity exchanges, therefore, dominate with unnatural parity exchanges being restricted to a small region in the forward direction. A Regge pole analysis of the differential cross sections of the present measurement in conjunction with previously measured total cross sections supports the f-coupled-pomeron hypothesis.     

Measurements of the polarization of the 2p and 1s states in muonic atoms and the helicity of the muon in pion decay

We have measured the polarization of the 2p and 1s states in muonic selenium (amorphous and metallic modifications), cadmium, palladium and iodine, in order to study the depolarization of muons in the cascading process and to measure the helicity of the μ^?. In the cases of cadmium, palladium and amorphous selenium good agreement between the measurements and cascade calculations is found. There is an unexpected depolarization of the 2p_{$\text{1}\text{2}$} state in metallic selenium. The helicity of the muon after the pion decay was measured to h_μ^? = + 0.99 ± 0.16.     

Half-life and configuration of the 1/2+ intruder state in203Bi

The decay properties of theJ ^π=1/2⁺,E _exc=1,098 keV state in²⁰³Bi were studied. The state was populated via the²⁰⁴Pb(p, 2n) reaction and the activity was studied with the ion guide isotope separator on-line system IGISOL. The half-life of the 1/2⁺ state was measured to beT _1/2=303 ±5 ms. From this value the partial half-lives of the three depopulating branches 1/2⁺ →7/2^? (E3), 1/2⁺→5/2^? (E3 +M2) and 1/2⁺→9/2 _g.s. ^? (M4) were deduced. Since all the transitions are configuration forbidden in first order, a detailed study of second-order shell-model configuration mixing could be performed.     

Level-Crossing-Untersuching der Stark-Aufspaltung der tiefsten1 P 1-Terme von Ca,Sr und Ba

Using the level-crossing technique, magnitude and sign of the tensor polarizability α_ten of the lowest¹ P ₁-levels of Ca, Sr, and Ba have been measured by investigating the splitting into Zeeman-sublevels in superimposed homogeneous electric and magnetic fields. The experimental results are: α_ten/g _J =?13.6(3) kHz/(kV/cm)² for Ca α_ten/g _J =?14.32(15) kHz/(kV/cm)² for Sr α_ten/g _J =?10.72(10) kHz/(kV/cm)² for Ba, where theg _J -values are approximatelyg _J≈1. With greater accuracy the ratios of these constants have been determined by eliminating the electric-field strength measurement: (α_ten(Sr)/g _J (Sr))/(α_ten(Ca)/g _J (Ca))=1.050(8) (α_ten(Sr)/g _J (Sr))/(α_ten(Ba)/g _J (Ba))=1.336(2). The polarizability constants are discussed with regard to the state vectors of the lowestsp ¹ P ₁- and³ P ₁-levels. The tensor polarizability of the 6s 6p¹ P ₁-level of Ba I is considered in relation to oscillator strengths of electric dipole transitions to neighbouring levels.     

Stark interaction in then s n p z 3 P 1 levels of zinc and cadmium

The tensor polarizabilities of then s n p z ³ P ₁ levels of Zn and Cd were measured using optical double resonance. From the rf-resonance signals in parallel electric and magnetic fields, the following tensor polarizabilities were deduced: Zn,α _ten(4s4pz ³ P ₁)=1.83(8) kHz/(kV/cm)²; Cd,α _ten(5s5pz ³ P ₁)=1.77(8) kHz/(kV/cm)². Theoretical values were calculated using Coulomb approximation. The results were then compared with previous theoretical and experimental values and, in addition, with values for Hg. Theoretical results obtained by a modified Sternheimer method (E.J. Robinson: J. Opt. Soc. Am.59, 782 (1969)) are in better agreement with the experimental values than the results of the Coulomb approximation calculations.     

Measurement of the f1(1285) → π+π−π0 decay

The isospin symmetry-breaking (ISB) decay f ₁(1285) → π⁺π^?π⁰ has been studied at the VES facility. The branching ratio is measured: $\frac{{BR\left( {f_1 \to \pi ^ + \pi ^ - \pi ^0 } \right)}} {{BR\left( {f_1 \to \eta \pi ^ + \pi ^ - } \right)}} = 0.86 \pm 0.16_{ - 0.20}^{ + 0.70} \%Low-energy resonances in ³¹P(p, α ²⁸Si and ³⁵Cl(p, α)³²S were studied directly in order to gain a better understanding of reaction cycling in the Si-Ar region in novae. New resonance strengths at E _c.m. = 600 and 622 keV in ³¹P(p, α)²⁸Si were measured (ωγ _{p, α} = (2.2#x00B1;0.7) × 10^?2 eV and ωγ _{p, α} = (0.99±0.08) eV, respectively) as well as the E _c.m. = 610 keV resonance in ³⁵Cl(p, α)³²S [ωγ _{p, α} = (1.2±0.2) × 10^?2 eV], the lowest energy that any resonance in this reaction has been observed, directly or indirectly. The strengths of these resonances were found to be lower than previously determined, resulting in even weaker cycling in the Si-Ar region.     

Study of some two-nucleon pick-up reactions in the 1p shell with 39.8 MeV protons

Differential cross sections at a proton energy of 39.8 MeV (lab) have been measured for the following reactions (energies in MeV): ¹²C(p,τ)¹⁰B(g.s., 0.72, 1.74, 2.15, 3.59), ¹⁴C(p, t)¹²C(g.s., 4.43), ¹⁴N(p, τ)¹²C(g.s., 4.43), and ¹⁶O(p,τ)¹⁴N(g.s., 2.31, 3.95). A zero-range DWBA analysis of the data has been performed using the 1p shell wave functions of Cohen and Kurath. The fits we find are overall somewhat worse in shape than those found in the (p, t) survey of the 1p shell performed by Kahana and Kurath, the principal reason being that of the (p, τ) transitions which proceed with both L = 0 and L = 2 components we find several which occur with a much weaker L = 0 strength than the calculations predict. When ratios of experimental integrated cross sections to DWBA integrated cross sections are compared for all transitions, an rms deviation about the mean of 39% of the mean is found, whereas if only ratios for transitions from a given target nucleus are compared, then the rms deviations are considerably smaller.     

The 56Fe(α, γ)60Ni reaction at excitation energies in the region of the giant dipole resonance

Excitation functions for the ⁵⁶Fe(α, γ₀)⁶⁰Ni and ⁵⁶Fe(α, γ₁)⁶⁰Ni reactions have been measured at 90° to the beam direction over the bombarding energy range 8.0–17.6 MeV. Gamma-ray angular distributions were measured at ten bombarding energies. Excitation functions for the ⁵⁹Co(p, γ₀)⁶⁰Ni and ⁵⁹Co(p, γ₁)⁶⁰Ni reactions were measured over the range E_x = 16.58–16.92 MeV and compared with the (α, γ) data. The angular distribution data indicate that the (α, γ₀) and (α,γ₁) reactions proceed through 1^?, and 1^? and 3^? states, respectively. The (α, γ) excitation functions are discussed with respect to isospin splitting of the ⁶⁰Ni giant dipole resonance. The fine structure observed in the excitation functions is shown to be most probably due to Ericson fluctuations. The gross (α, γ) cross sections are shown to be in reasonable agreement with the results of calculations made using the theory of Hauser and Feshbach assuming excitation of the giant dipole resonance.     

Energies and chemical shifts of the sulphur 1s level and the KL2L3(1D2) Auger line in H2S,SO2 and SF6

The sulphur 1s binding energies and KL₂L₃(¹D₂) Auger energies have been measured in gaseous H₂S, SO₂ and SF₆. The experimental data, including the chemical shifts, are compared with various theoretical ab initio results. Theoretical and experimental values agree within 1-2 eV for the chemical shift and the binding energy of the 1s level, provided in the latter case relaxation, relativistic and correlation corrections are applied. Likewise, Shirley's method²⁰, which uses empirical energies, predicts the Auger energies satisfactorily. The measured S 1s binding energies are 2478.5(1) eV, 2483.7(1) eV and 2490.1(1) eV, and KL₂L₃(¹D₂) Auger energies are 2098.7(1) eV, 2095.5(2) eV, 2092.6(1) eV for H₂S, SO₂ and SF₆, respectively. The chemical shift for the 1s electron is found to be greater than for the 2s or 2p electron and in better accord with the prediction of the potential model. Data suggest the molecular relaxation energy to be small compared with the atomic relaxation energy.     

Doppelresonanzexperimente zur Untersuchung der Hyperfeinstruktur des 6s6p 3 P 1-Zustandes von171Yb und173Yb

For the odd Yb isotopes¹⁷¹Yb and¹⁷³Yb the hyperfine splitting of the 6s6p ³ P ₁ state has been measured by optical double resonance in zero magnetic field. Taking into account second order corrections due to the influence of the 6¹ P ₁ and 6³ P _0,2 states, the following results for the magnetic splitting constantA and the electric quadrupole interaction constantB have been derived: A(¹⁷¹Yb)=3958.228 (60) Mc/s, A(¹⁷³Yb)=?1094.318 (35) Mc/s, S(¹⁷³Yb)=?825.904 (85) Mc/s. The hyperfine structure anomaly of the isotopes¹⁷¹Yb and^{171 173}Yb was determined to be Δ=?0.352 (10)%.     

Origin of threshold electrons produced in decay of the Xe 4d−1 np resonance

Coincidence spectra of energetic electrons with threshold electrons were measured following photo-excitation of the Xe 4d_3/2, 5/2 → np resonances, in order to investigate the origin of threshold electrons, and the mechanism leading to formation of the Xe²⁺ 5p⁻² and 5s⁻¹5p⁻¹ final states. A two-step decay process was observed in the production of Xe²⁺ 5p⁻²(¹D) following decay of the 7p resonance, where the intermediate state is Xe^+* 5p⁻²(¹S)8p that autoionizes emitting a pseudo-threshold electron. This process was confirmed in a time-of-flight analysis of the coincidence spectra of the energetic electrons with the threshold photoelectrons. It is suggested that a similar two-step process also contributes to the population of excited Xe²⁺ states and is the main origin for the production of threshold electrons in decay of the 4d⁻¹ np resonances.     

Formation of 24Mg* in the spallation of 28Si nuclei by 1-GeV protons

The ²⁸Si(p, p′γ₀ X)²⁴Mg reaction has been studied at the ITEP accelerator by the hadron-gamma coincidence method for a proton energy of 1 GeV. Two reaction products are detected: a 1368.6-keV γ-ray photon accompanying the transition of the ²⁴Mg* nucleus from the first excited state to the ground state and a proton p′ whose momentum is measured in a magnetic spectrometer. The measured distribution in the energy lost by the proton in interaction is attributed to five processes: the direct knockout of a nuclear α cluster, the knockout of four nucleons with a total charge number of 2, the formation of the _ΔSi isobaric nucleus, the formation of the Δ isobar in the interaction of the incident proton with a nuclear nucleon, and the production of a π meson, which is at rest in the nuclear reference frame. The last process likely corresponds to the reaction of the formation of a deeply bound pion state in the ²⁸P nucleus. Such states were previously observed only on heavy nuclei. The cross sections for the listed processes have been estimated.