Verzweigungsverhältnisse und Konversionskoeffizienten von angeregten Zuständen des208Tl

The branching ratios of theγ rays of the second and fourth excited states of²⁰⁸Tl have been investigated by coincidence measurements between the α rays of²¹²Bi and subsequent 40keVγ ray. The detectors employed were a silicon surface barrier counter for α particles, and a 1.5 in ×2 mm NaJ (Tl) crystal forγ rays. It has been found that (75.6±3.7)% of all transitions of the 328 keV state and (94±7)% of all transitions of the (492 keV+473 keV) states populate the first excited state of²⁰⁸Tl. The 40 keV state is excited to (3.4±0.3)% by transitions of higher excited states relative to the direct excitation by α particles. The number of α particles with energyE _α = 6.047 MeV and the number of subsequent 40keVγ rays resulted in a conversion coefficient α(40keV)=22.55± 0.46. Similarly coincidence measurements between Tl-x rays and α particles have been used to determine theK- conversion coefficients α_K(328 keV)=0.31±0.03 and α_K(492 keV+ 473keV)=0.100±0.015. The experimental results are in good agreement with the theoretical values ofSliv.     

Electron capture intensities in the decay of133Ba

The ground state decay of¹³³Ba was investigated using NaI(Tl) scintillation crystals.P _L/P_K electron capture ratios were measured for the transitions to the 437 keV and to the 384 keV level of¹³³Cs. The results are: (P _L/P_K)₄₃₇=0.371±0.007 and (PP _L/P_K)₃₈₄=0.221±0.005. From these data a mass difference between the ground states of the¹³³Ba- and the¹³³Cs-atom of (515±3) keV was derived. Besides, these capture ratios yield an exchange correction of 1.03±0.03. Furthermore, the intensity of the transition to the 161 keV level was determined to be smaller than 0.5% of all decays.     

The electron capture decay of125I and145Pm

The productP _K ω _K of theK-capture probability and theK-fluorescence yieldω _K was measured in the EC decay of 17.7 y¹⁴⁵Pm and 60.14d¹²⁵I by means ofK x-ray-γ-ray coincidences with semiconductor detectors. Accepting a best value ofω _K =0.920 forZ=60 from the literature, values ofP _K =0.606±0.025 and 0.554±0.025 for decay of¹⁴⁵Pm to the 67.2 and 72.4 keV levels in¹⁴⁵Nd, respectively, were determined, from which the application of EC theory givesQ _EC=153±4 keV to the ground state. TheP _K ω _K ratio to the 67.2 and 72.4 keV levels also was determined independently to be 1.11±0.01, which serves as a good check on theγ-ray-gatedP _K values. Theγ-ray energies were determined more accurately to be 72.4±0.1 and 67.2±0.1 keV, together with a ratio of their relative intensities,I _72.4/I _67.2=3.35±0.09. In the decay of¹²⁵I, a value ofP _K ω _K =0.699±0.030 was measured, and by using an independent determination ofQ _EC=178±2 keV to the ground-state from the literature, a value ofP _K=0.801 is calculated from allowed EC theory, from whichω _K =0.873±0.017 atZ=52 is obtained. This value is in good agreement with theoretical values and with a value of 0.875±0.028 predicted by the best fit curve of Bambyneket al.     

TheK-conversion coefficient near threshold of the 30 keV isomeric transition in108mAg decay

With calibrated Ge(Li) x-ray detectorsK x rays in the conversion of the 30 keV isomeric transition in the decay of^108mAg were observed in coincidence with 79 keV γ-rays. Thus, the fraction of 30 keV transitions which take place byK conversion was measured to be (2.44±0.23) × 10^?2. Making use of a theoretical total conversion coefficient (K conversion contributes only a minor part of the total conversion coefficient), an experimental value of theK-conversion coefficient was obtained, α_K=(1.07 ± 0.10) × 10⁴ (where the error represents twice the standard deviation to which the error in the detector efficiency has been added linearly). This value agrees with the theory of Hager and Seltzer forM4 conversion. The energy of the cascading γ-ray was remeasured to be 79.20 ± 0.05 keV.     

Messung von HalbwertszeitenK-verbotener Übergänge ingg-Kernen der Seltenen Erden

The half-life of the 1,490 keV level in¹⁶²Dy has been measured in the decay of¹⁶²Ho^m (68 min) by delayed coincidences ofKX rays and (900-1,300) keV gamma radiation to be (1.94 ± 0.19) nsec. A half-life in¹⁷⁶Hf has been remeasured in the decay of¹⁷⁶Ta (8.1h) by delayed coincidences of KX rays and (1,100–1,200) keV gamma radiation to be (4.75 ± 0.25) nsec. In order to fix the level with this half-life in the level scheme of¹⁷⁶Hf, the gamma spectrum delayed to KX rays was measured. It is suggested that probably the 1,227.4 keV-level of¹⁷⁶Hf is delayed and has the spin 2^? or 3⁺.     

Decay of194Os andL 1 subshell yields atZ=77

The relative intensities of x rays and gammas emitted in the beta decay of¹⁹⁴Os are measured. No evidence for the feeding of a level at 83 keV in¹⁹⁴Ir is found. An upper limit of 1.7×10^?4 was set for theK shell internal ionization probability in the beta decay to the ground state of¹⁹⁴Ir. TheL-conversion coefficient of 43 keV transition is found to be 12.1 and the transition is mainly ofM1 type with an admixture of 1.3%E2 type. TheL ₁ subshell yields atZ=77 are determined to beω ₁=0.16±0.04,f ₁₂=0.11±0.04 andf ₁₃=0.37±0.03.     

Mössbauer effect and nuclear moments of the 75 keV state of Dy161 and the 81 keV state of Dy162

The Mössbauer effect of theγ rays from the 74.5 keV state of Dy¹⁶¹ and the 80.7 keV state of Dy¹⁶² has been investigated. From hyperfine splitting patterns the magnetic moments μ(75 keV)=?(0.39±0.04) nm, μ(81 keV)=+(0.74±0.08) nm and the quadrupole momentQ(75 keV)=+(1.4±0.2)b have been determined. For the odd neutron nucleus Dy¹⁶¹ an effective spin g factorg _{s, eff}=0.76 g_{s, free} is deduced for the 75 keV level.     

Der Zerfall des125m Xe,des127m Xe und des127g Xe

The decay of^125m Xe produced by the reaction¹²²Te(α, n)^125m Xe using a target enriched in¹²²Te (95.4%) and the decay of^127m Xe produced by the reaction¹²⁷J(d, 2n)^127m Xe have been investigated: ^125m Xe decays with a half-life ofT _1/2=(56±3) sec by ayy- cascade withE _γ1=(140.4 ±0.5) keV andE _γ2=(110.5 ±0.5) keV. The experimental conversion coefficients yield multipolarities ofE3 for the 140.4 keV isomeric transition and predominantlyM1 for the 110.5 keV-transition. ^127m Xe decays with a half-life ofT _1/2=(71±2) sec. The decay also proceeds by aγγ-cascade with an isomeric E3 transition ofE _γ1=(172.5±0.3) keV and a predominantlyM1 transition ofE _γ2=(124.6±0.3) keV. In the decay of^127g Xe an additional branching of the electron capture to a level at (618.1±0.3) keV was observed. The relative probability forK-captureP _K618/P_K375=0.40 ±0.07 yields a total transition energyQ _EC=(664 ±4)keV. A spin of 1/2⁺ was assigned to the ground state.     

Multipole mixing ratios of transitions in168Er

Time-integral and time-differentialγ-γ directional correlation measurements were performed for cascades in¹⁶⁸Er populated from the electron-capture decay of¹⁶⁸Tm(87d). The¹⁶⁸Tm source was dissolved in HF acid to minimize extranuclear perturbations. The results of the time-differential experiment for the 448-99.3 keV and 448-198 keV cascades showed agreement with time dependent interaction and gaveλ ₂(1094)=(0.79±0.09) ×10⁷ sec^?1. The attenuation factors for the 80 keV level were determined asG ₂₂ (80)=0.90±0.01 and G₄₄(80)=0.94±0.01. OnlyI=4 spin value for the 1094 keV level is consistent with our measurements. The 632, 731, 741, and 816 keV transitions connecting theK=2⁺ andK = 0⁺ rotational bands were found to be of almost pureE2 character. The 99.3, 198, 547, 720, 830, and 1277 keV transitions are of practically pureE1 multipolarity. The 448 keVMl transition has (0.8 _?0.4 ^+2.0 )%E2 admixture. The results for the 1014?80keV cascade give (23±4)%E3 component in the 1014 keV transition.     

Measurements of someK-internal conversion coefficients near threshold

TheK-internal conversion coefficients have been measured by the XPG technique for a number of low energyγ-ray transitions whose energies do not exceed theK-binding energies by more than 4 keV. Using Si(Li) detectors in singles and coincidence arrangements, the following results were obtained: 63.1 keV El in¹⁶⁹Tm(α_K=1.02±0.15), 72.0 keV E1 in¹⁸⁷Re (0.75±0.05), 57.8 keV M1 in¹⁶²Ho (11.42±0.67), 56.6 keV M1 in¹⁶⁴Ho (12.04±0.70), and 67.1 keV M1 in¹⁷⁴Lu(10.25±0.58). The experimental results are compared with the theoretical calculations which include transition energies down to 1 keV above threshold.     

Der Zerfall des 1,5 min-Isomers Co54m

Co^54m (T _1/2=1.43 min) was produced in iron-foils by irradiation with_dE=19 MeV deuterons. The gamma ray spectrum was investigated using a NaJ(Tl) scintillation spectrometer, a coincidence circuit and a Ge(Li)-counter. There were observed three gamma rays having the following energies and intensities per Co_54m decay: 411 keV (0.97±0.07), 1130keV (0.98±0.05), 1407 keV (1.00±0.05). The directional correlation between the pairs of gamma rays were determined. These results correspond to spin and parityJ _π=2⁺ for the 1407 keV,J _π=4⁺ for the 2537 keV, andJ _π=6⁺ for the 2948 keV energy level of Fe⁵⁴. The last-mentioned level was not excited in previous scattering experiments. Our results are compatible withE=210keV andJ _π=6⁺ or 7⁺ of the isomeric state of Co^54m .     

Measurement ofK-electron capture probability (P k ) in the decay of197Hg (64.1 h)

TheK-electron capture probability (P _K ) for the 268.7 and 77.3 keV states of¹⁹⁷Au in the decay of¹⁹⁷Hg (64.1h) have been determined from theKX-ray gamma ray summing in a HPGe X-ray detector. The measured values,P _k (268.7)=0.746±0.033 andP _k (77.3)=0.774±0.036 are found to be in good agreement with the theoretical results.     

Innere Konversion der 161 keV- und 223 keV-Übergänge in133Cs

Using a Ge(Li)-Si (Li)-spectrometer the 161 keV and 223 keV transitions of¹³³Cs were investigated. TheK-conversion coefficients were deduced to beα _K =0.205±0.007 andK-conversion coefficients were deduced to beα _K =0.0743±0.0043, respectively. TheK/L ratio for the 161 keV transition is 4.72±0.37. From theK-conversion coefficients were deduced to beα _K -values,M1 penetration factors ofλ=8.6±3.4 andλ=7.8 _?2.8 ^3.0 were deduced which are inconsistent with known data from angular correlation experiments (λ=40±10 andλ=90±13). The penetration factor fromK/L-measurement for the 161 keV-transition isλ=52±19. A theoretical reinvestigation of the formulas used in the literature appears recommendable. Furthermore, theK/L ratio of the 1770 keV transition of²⁰⁷Pb was determined experimentally to be 5.52±0.54.     

Experimentelle Untersuchungen am Elektroneneinfang des85Strontium und88Yttrium

The electron capture decay of⁸⁵Sr and⁵⁵Y has been investigated using NaI(Tl)-detectors. Spectroscopic-coincidence techniques have been employed to examine theK-electron capture rates. The experimental results areP _K ω _K (Sr)=.5959 ± 0.0035 andP _K ω _K (Y)=0.6340± 0.0032. Using theK-capture probabilities, derived from the capture ratios ofBrysk andRose with the exchange correction ofBahcall:P _K (Sr)=0.880± 0.008 andP _K (Y)=0.883 ± 0.008, one can derive from these results the fluorescence yieldsω _K (Rb)=0.677± 0.009 andω _K (Sr)=0.712± 0.010. Functions ofω _K (Z) were fitted to recent experimental data and tabulated forZ=5–90. In addition to these results the half life of the 514 keV state of⁸⁵Rb and the branching ratios and the positron rate of the⁸⁸Y-decay have been measured with the same techniques. The data obtained partly disagree from measurements of other authors.     

Decay of the first excited state at 13.3 keV in73Ge

Singles and coincidence measurements of the 13.3 keV transition of⁷³Ge are reported. The total andK conversion coefficients of this gamma-ray and the half-life of this level have been determined. The results are: α _T =1095±55; α _K =312±30;T _1/2=2.98±0.05 μs.     

Isomeric states in180Os

Two new isomers have been observed in¹⁸⁰Os. A high-K isomer withI, K ≧20 and a half-life ofT _1/2=12+4 ns have been established. It deexcites via two transitions into the 18⁺ level of the yrare band indicating an unusually smallK-hindrance factor. Evidence for an isomer withI, K>16 and a half-life ofT _1/2=41±10 ns was found. A half-life of 17±3 ns was measured for the previously known 7^? state at 1862 keV. The decay scheme of the previously known 7^? isomer at 1928 keV has been extended and a revised version is presented.     

Conversion-electron-gamma and gamma-gamma directional angular correlations in 160Dy

Gamma-gamma and conversion-electron-gamma angular correlations in ¹⁶⁰Dy have been measured for the 298 keV–966 keV and 298 keV–879 keV cascades. Particle parameters of the 966 keV E2 transition were determined to be b₂(E2; e_K) = +1.23±0.08 and b₂(E2; e_{ΣL + ΣM) = +1.27±0.23}. The multipole mixing ratio for the 298 keV radiation was determined to be δ(M2/E1) = +0.04±0.01 and we have confirmed the value δ(E2/M1) = ?13±2 for the 879 keV. The E0–E2 mixture parameter for the 879 keV transition was determined as q_K = ?0.03±0.09 assuming penetration effects to be negligible.     

207Bi L-subshell orbital electron capture probabilities and decay energy

The L₁ subshell orbital electron capture probability P_L1 in the decay of 33.4 y ²⁰⁷Bi to the 2339.89 keV level in ²⁰⁷Pb is measured to be 0.518 ± 0.081 (95% confidence) by a new method in which L₁ subshell characteristic X-rays in the L_γ X-ray peak are observed in an Xγt coincidence mode with 1770.23 keV γ-rays. The value of P_L2is 0.047 ± 0.015 (95% confidence). From these results a value of Q_EC = 39_-8⁺²¹ keV is obtained for capture transitions to the 2339.89 keV level. The absence of K-capture to this level also is established by absence of K X-rays in coincidence with 1770.23 keV γ-rays.     

Q 1 production by hypercharge exchange in π- p interactions at 3.95 GeV/c

Q-meson production is studied in the hypercharge exchange reaction π^- p → (Kππ)Λ at 3.95 GeV/c by selecting events witht(π^- →Kππ)>1.2GeV². An enhancement with a mass of 1294±10 MeV and a width of 66±15 MeV is observed in the (Kππ) mass distribution. A spin-parity analysis of the (Kππ) decay Dalitz plot shows the enhancement to be in theJ ^P=1⁺ S(K?) wave and is therefore attributed toQ ₁-meson production. No evidence is found for the decayQ ₁→K ⁰ω but limited statistics allow only placing an upper limit of 30% for the decay ratioKω/K?⁰. TheQ ₁ production cross section fort(π^- →Kππ)>1.2GeV² is 8±1.3 μb. No evidence is found for the process π^- p→Q ₂Λ withQ ₂→K ^*π for which the partial wave analysis gives an upper cross section limit of 2.5 μb at the 95% confidence level.     

Erzeugung neuer isomerer Kernzustände durch Kernphotoreaktionen am Antimon und Thallium

The systematic search for new short-lived isomeric states has been continued by irradiation of an additional 32 selected elements with 26 MeV bremsstrahlung. Isomeric transitions were detected using a conventional scintillation spectrometer. Irradiation of antimony led to the production of a new (530±50) μsec isomeric state which decays through emission of partially converted (62±2) keV and (76±3) keV gamma rays. The 530 μsec half-life is tentatively associated with the 136 keV level in Sb¹²². An apparent inconsistency in the previously proposed level scheme of Sb¹²² can be removed if the 3.5 min Sb¹²²-activity is assigned to an isomeric level in Sb¹²² lying less than 15 keV above the 136 keV isomeric state. A new measurement of the half-life of this level yielded a value of (4.1₅±0.2) min. Another new isomeric state with a (2.l±0.2) msec half-life was produced by irradiating thallium. The isomeric state decays by emission of two gamma rays of (335±8) keV and (597±12) keV which were found to be in coincidence. Irradiation of erbium led to the production of a short-lived isomeric transition which may be identical with a previously reported Ho-isomer. Results are discussed in the appendix.