Detailed Ge(Li)-Ge(Li) coincidence studies of levels in152Sm and152Gd

The decay of 12.4 y¹⁵²Eu to¹⁵²Sm and¹⁵²Gd was studied in a high resolution singles measurement and two 4096×2048 Ge(Li)-Ge(Li) coincidence studies. Forty-five gates were analyzed in order to confirm or establish the placement of the γ rays as well as to accurately determine the intensities of the 12 doublets, which included several not previously reported. A new γ-β interband transition, 4 _γ ⁺ →2 _β ⁺ (561.4 keV), a possible 3 _γ ⁺ →2 _β ⁺ (423.7 keV) transition, and a new 330.9 keV transition between the 4 _γ ⁺ level and theI ^π K=3^?0 octupole level were established from coincidence data. Levels at 1757.0 keV in¹⁵²Sm and 1282.5, 1318.7, and 1692.2 keV in¹⁵²Gd are now established on the basis of coincidence data. These data also establish for the first time the population in the¹⁵²Eu decay levels at 1680.0 and 1047.9 keV in¹⁵²Sm and¹⁵²Gd, respectively, as well as a new level at 1700.8 keV in¹⁵²Sm.     

E2 andE3 transition strengths in some rare-earth nuclei

Coulomb excitation byα-particles of vibrational-like states in even-mass rare-earth nuclei is used to determine the reduced transition probabilitiesB(E2; 0 _gs ⁺ →2 _γ ⁺ ),B(E2; 0 _gs ⁺ →2 _β ⁺ ),B(E2; 2 _gs ⁺ →0 _β ⁺ ) andB(E2; 0 _gs ⁺ →3 _oct ^? ) in¹⁵⁰Nd,^{152, 154}Sm,^{154, 158}Gd,¹⁶⁴Dy and¹⁶⁶Er. TheB(Eλ; 0 _gs ⁺ →I=λ)-values range from 2.4 to 6.5 single-particle units for transitions to the 2 _γ ⁺ -states, 0.8 single-particle units for the 2 _β ⁺ -states and from 14.1 to 21.7 single-particle units for the 3^?-states.     

g-Factor of the first 2+ state in theN=82 nucleus138Ba

The 2 ₁ ⁺ level of¹³⁸Ba has been Coulomb excited with a 105 MeV³²S beam. The precession of the gamma ray angular distribution induced by the transient magnetic field when traversing a 2.14 mg/cm² iron foil, has been measured to be 15.6(1.7) mr. A value of g(¹³⁸Ba 2 ₁ ⁺ )=0.72(11) was obtained assuming for the transient field strength the Chalk River calibration. The field parametrization has been checked using the first 2⁺ state in¹⁵⁰Sm as probe. Theg value obtained is sensibly lower than predicted by large scale shell model calculations in a proton subspace. Theg-factor of the first 2⁺ state in¹⁴⁸Sm has been remeasured yieldingg(¹⁴⁸Sm 2 ₁ ⁺ )=0.246(22).     

Pion photoproduction on197Au to ground and isomeric states in197Hg

The lifetime of the 331.3 keV 0 ₂ ⁺ state in¹⁰⁰Zr has been measured at the gas-filled recoil separator for fission products JOSEF. By observing the delayed coincidences between theβ-particles populating the level and theE0 conversion electrons from its decay into the ground state, a half-life of 3.37±0.30 ns has been obtained. From the measured lifetime and the relative intensities of the 0 ₂ ⁺ →0 ₁ ⁺ and 0 ₂ ⁺ →2 ₁ ⁺ transitions, values of 0.493±0.015 for theE0 strength parameterρ, and of 16 single particle units forB(E2,2 ₁ ⁺ → 0 ₂ ⁺ ) have been deduced. The enhanced nature of theE0 transitions suggests mixing of the 0 ₁ ⁺ and 0 ₂ ⁺ states which may be estimated by comparing the experimentalB(E2) values for the 2 ₁ ⁺ →0 ₁ ⁺ and 2 ₁ ⁺ →0 ₂ ⁺ transitions with the predictions of the asymmetric VMI model.     

Evidence for a 3.6 minute isomeric 12− state of the πh 11 2/−1 vi 13 2/−1 configuration in206Tl and effective two-particle interactions

Using the²⁰⁴Hg(α, pn)-reaction andα-particles of energies 39–55 MeV, we have found an isomeric 3.6 min 12^? state in²⁰⁶Tl at 2,642.9 keV which has the two-hole configurationπh ₁₁ ^2/?1 vi ₁₃ ^2/?1 The 12^? state decays mainly by anE5 transition of energy 1,021.4 keV to a 7⁺ state at 1,621.5 keV whose main configuration isπs ₁ ^2/?1 vi ₁₃ ^2/?1 There is, in addition, evidence for a weak 565 keVM 4 branch to an 8⁺ state at 2,078 keV whose main configuration should beπh ₁₁ ^2/?1 vf ₅ ^2/?1 . The 7⁺ state decays by a stretched cascade ofγ-rays to states of the following values ofJ ^π and excitation energy: 5 _? ⁺ , 1,405.4 keV; 4^?, 952.1 keV; 2^?, 265.8 keV and 0^?, 0 keV. The main configurations of these states areπh ₁₁ ^2/?1 vp ₁ ^2/?1 ,πd ₃ ^2/?1 vf ₅ ^2/?1 ,πd ₃ ^2/?1 vp ₁ ^2/?1 andπs ₁ ^2/?1 vp ₁ ^2/?1 respectively. From the nuclear masses of²⁰⁸Pb,²⁰⁷Pb,²⁰⁷Tl, and²⁰⁶Tl and the experimental excitation energies it is possible to obtain the proton hole-neutron hole interaction in²⁰⁶Tl. This interaction is compared with the calculations of Kuo and Herling and the discrepancies are discussed. The 12^?→8⁺ M4 transition rate is reduced because of destructive interference between the protonh _11/2→d _3/2 and the neutroni _13/2→f _5/2 contributions. The magnitude of the reduction is accurately reproduced by the wave functions of Kuo and Herling. The 12^?→7⁺ E5 transition rate is about twice as large as the single-holeπh ₁₁ ^2/?1 πs ₁ ^2/?1 transition rate. This deviation is fully explained by the configuration admixtures in the 7⁺ state, given by Kuo and Herling.     

High-spin levels in138Ce and140Nd Observed in the (α, 4n γ) reactions

Levels of¹³⁸Ce and¹⁴⁰Nd have been studied using the¹³⁸Ba(α,4nγ)¹³⁸Ce and¹⁴⁰Ce(α, 4nγ)¹⁴⁰Nd reactions. Singleγ-ray spectra,γ-γ coincidence spectra, angular and time distributions with respect to the beam bursts have been measured. A number of higher excited states with excitation energies up to about 5 MeV and with spin value up to 12 are populated in both nuclei. The lower states with spins and parities 7^?, 5^?, 6^? and 10⁺ can be explained by two-quasiparticle neutron configurations of the types (h _11/2 ^?1 ,d _3/2 ^?1 ) 7^? , (h _11/2 ^?1 ,S _1/2 ^?1 ) 5^?, 6^? and (h _11/2 ^?2 ) 10⁺. Several high-spin states observed in¹³⁸Ce and¹⁴⁰Nd can be explained qualitatively as four-quasiparticle states with two-proton-two-neutron configurations. The 3^? state at an energy of 2,137.4 keV is observed in¹³⁸Ce. The evidence for the existence of the low-lying 3^? states in¹⁴⁰Nd at 2,124.0 keV is discussed. Beside the known 9.6 ms (7^?) isomeric state in¹³⁸Ce another state at 3,538.5keV (10⁺) with a half life of about 200 ns has been observed. The observed levels in the¹³⁸Ce and¹⁴⁰Nd nuclei are compared with theoretical predictions using delta force interaction.     

An interpretation of the energy-momentum tensor of the dirac field with anomalous magnetic moment

The ground state radiative widths of the 1.56 MeV (3/2⁺) and the 1.35 MeV (5/2^?) levels in¹⁹F were determined by inelastic electron scattering. The measured cross sections have been analysed using DWBA calculations. The resultsΓ _y ⁰ (5/2^?→1/2^?,E3)=(8.1±1.7)·10^?10eV andΓ _y ⁰ (3/2⁺→1/2⁺,E2=(1.76±0.15)·10^?4eV are in agreement with, but more accurate than, former measurements.     

Multiplicities of charged particles prior to fission

Electric monopole transitions between the 0 ₂ ⁺ , 0 ₁ ⁺ and 2 ₂ ⁺ , 2 ₁ ⁺ levels in⁷⁶Se, populated in the decay of⁷⁶Br, were investigated by means of conversion electrons and gammaray spectroscopy. TheK-electron intensity ratios ofE0 andE2 transitions connecting the 0 ₂ ⁺ level to the 0 ₁ ⁺ and 2 ₁ ⁺ levels and of theE0 andE2 components in the 2 ₂ ⁺ →2 ₁ ⁺ transition were determined. The ratioX(E0/E2) of theE0 toE2 reduced transition probabilities and, from the available lifetimes, theE0 strength parameters ρ(E0) were deduced for the two transitions. The results are compared with the predictions of current models.     

g-factors of the lowest 2+ and 4+ states in198, 200, 202Hg

Theg-factors of the 2 ₁ ⁺ and 4 ₁ ⁺ states in^198,200,202Hg were simultaneously measured by means of the transient-field perturbed angular correlation method in Coulomb excitation using multi-isotopic targets and thin polarized Gd foils as ferromagnetic host. Theg(2 ₁ ⁺ ) andg(4 ₁ ⁺ ) were found identical within errors in^{198, 200}Hg, while in²⁰⁰Hg lowerg-factor values have been determined. The experimentalg-factors were compared with the predictions of the pairing-plus-quadrupole, dynamical deformation and interacting boson models.     

Identification of180Pb

Theα decay of the new isotope¹⁸⁰Pb was observed in⁴⁰Ca bombardments of¹⁴⁴Sm:E _α = 7.23(4)MeV, and,T _1/2=(4 _?2 ⁺⁴ )ms. With this decay energy and the known mass of¹⁷⁶Hg, the mass excess of¹⁸⁰Pb was calculated to be ?1.98(5)MeV.     

Resonance strengths,branching ratios and mean lifetimes of nuclear energy levels in23Na

The gamma decay of the²²Ne(p, y)²³Na resonances in the proton energy rangeE _p=1.0→2.0 MeV has been investigated with a 20cm³ Ge(Li) detector. Implanted targets were used. The absolute strengths of the strongest resonances were determined and the branching ratios of twenty resonance levels and several bound states are reported. Mean lifetimes of the levels atE _x=2.078 MeV (18.7±3.5 fs), 2.393 MeV (580 _?190 ⁺³⁷⁰ fs), 2.641 MeV (88 _?14 ⁺²⁰ fs), 2.985 MeV (4.0 _?1.0 ^+1.3 fs), 3.679 MeV (24 _?4 ⁺⁵ fs), 3.915 MeV (7.4 _?2.0 ^+2.5 fs) and 4.775 MeV (<2.0 fs) were obtained from measurements of the gamma ray Doppler shifts.     

The 235 ns 9+ isomer in 63 148 Eu85

From (p, xn) in-beamγ-ray and electron measurements aT _1/2=235(14) ns isomer at 720 keV was identified in ₆₃ ¹⁴⁸ Eu₈₅ and the levels populated in its decay have been characterized. The results determineI ^π=9⁺ for the isomeric state, and we assign it as the (πh _11/2 j ₀ ^?2 ν f ₇ ^2/3 )9⁺ shell model state, analogous to the configuration of the 235 μs isomer in ₆₃ ¹⁴⁶ Eu₈₃.     

The 0 1 + →0+ electric monopole transition in112Cd

The low-lying levels of¹¹²Cd have been populated in the decay of¹¹²In (T _1/2=14 ^m ) produced through the¹¹²Cd (p, n)¹¹²In reaction atE _p=6.5–7 MeV. The intensity ratio of theE0 toE2K-conversion electrons from the 0 ₁ ⁺ level to the ground (0⁺) and to the first (2⁺) excited state in¹¹²Cd has been measured and the ratioX(E0/E2) =B(E0;0 ₁ ⁺ →0⁺)/B(E2;0 ₁ ⁺ →2⁺) has been determined. The result is compared with the predictions of current macroscopic models.     

Nuclear structure of the heavyN=82 isotones:144Sm and146Gd

For single-closed shell nuclei with a large number of extra-protons, outside theZ=50,N=82 double-closed shell nucleus, a standard shell-model calculation yields dimensions of the Hamiltonian matrices beyond the scope of present computer technology. A quasi-particle (QP) calculation however, is able to describe the most important proton-excitations in a much restricted configuration space. Extended BCS+TDA calculations are performed on the single-closed shell¹⁴⁴Sm and¹⁴⁶Gd nuclei with a Gaussian force as effective two-body interaction. The influence of the nonconservation of the exact number of extra-protons in the BCS-approach is studied by performing a projection onto the states with an exact number of extra-protons (BCS+P). The first excited 2⁺, 4⁺ and 6⁺ states in¹⁴⁶Gd are described mainly by the (1g7/2) ₀ ⁸ (2d5/2) ₀ ⁴ \((1h11/2)_{J^\pi }^2 \) configuration.     

Conserved-vector-current hypothesis and the\bar v_e e^ - \to \pi ^ - \pi ^0 process

Based on the conserved-vector-current (CVC) hypothesis and a four-ρ-resonance unitary and analytic VMD model of the pion electromagnetic form factor, theσ _tot(E _v ^lab ) and dσdE _π ^lab of the weak \(\bar v_e e^ - \to \pi ^ - \pi ^0\) process are predicted theoretically for the first time. Their experimental approval could verify the CVC hypothesis for all energies above the two-pion threshold. Since, unlike the electromagnetic e⁺e^?→π⁺π^? process, there is no isoscalar vector-meson contribution to the weak \(\bar v_e e^ - \to \pi ^ - \pi ^0\) reaction, accurate measurements of theσ _tot(E _v ^lab ) that moreover is strengthened with energyE _v ^lab linearly could solve now a widely discussed problem of the mass specification of the first excited state of theρ(770) meson. As a by-product, an equality \(\sigma _{tot} (\bar v_e e^ - \to \pi ^ - \pi ^0 ) = \sigma _{tot} (e^ + e^ - \to \pi ^ - \pi ^0 )\) is predicted for \(\sqrt s \approx 70 GeV\) .     

Experimental study of the energy dependence of the reaction rate coefficients of the reaction CH 3 + with N2O and NH3

The kinetics of the reaction of CH ₃ ⁺ ions with N₂O and NH₃ has been investigated in He and Ar buffers using Selected Ion Flow Drift Tube technique (SIFDT). Both studied reactions proceed with nearly collisional rate at near thermal energies. The rate coefficient of the reaction of CH ₃ ⁺ with N₂O is decreasing more than one order of magnitude (from 1.2×10^?9cm³s^?1 up to 8×10^?11cm³s^?1) with reactant ion/reactant neutral average centre-of-mass kinetic energy (E _r) increasing from near thermal up to 2 eV. The dominant product of this reaction is the isomer HCO⁺ (≥94%) and the minor product is CH₃O⁺. The reaction of CH ₃ ⁺ with NH₃ has two binary channels with the dominant product ion CH₂NH ₂ ⁺ (>70%) and the minor product ion NH ₄ ⁺ (≈10%) and three body association channel with product CH₃NH ₃ ⁺ (≈20% at 0.32 Torr). The rate coefficient of this reaction is decreasing nearly by one order of magnitude with increasingE _r from near thermal up to 0.8eV, forE _r>0.8 eV the rate coefficient increases with increasingE _r. The experimental results are interpreted in terms of a simple model assuming the reactions to proceed via the formation of long-lived collision complexes.     

Messung der zirkularen polarisation von γ-strahlung nach einfang polarisierter thermischer neutronen in kernen

A 70% polarized thermal neutron flux of 6 · 10⁶ s^? was obtained by total reflexion of a 1 m long Co-Fe mirror. Naturel targets of Al, Co, Mo and Sm where exposed to this beam. The measurement of the circular polarization of high energy captureγ-rays yielded some information about nuclear properties: For the transition from the compound state to the ground state in²⁸Al we derived theE2/M1 mixing ratioδ=?2.0 _+1.0 ^?0.5 . In⁹⁶Mo we obtained for the spin of the 2.25 MeV levelJ ^π=2^? or 3^?. If in agreement with theory the spin for this level isJ ^π=3^? the compound state for this decay hasJ ^π=2⁺ for over 50% of the transitions. In accordence with a previous measurement we found for the spins of the doublet in⁶⁰Co at 0.278 and 0.288 MeVJ ^π=3⁺ or 4⁺. For¹⁵⁰Sm we determined the overall circularγ-polarization. The measurement is in agreement with the statistical nuclear model yielding for the compound stateJ ^π=4^?. We confirmed the earlier spin assignementJ ^π=4⁺ for the 0.777 MeV level of¹⁵⁰Sm.     

The magnetic moment of the 10+ isomer in140Ce andE1 transitions inN=82 isotones caused by outer subshell configurations

Using the reaction¹³⁸Ba(α,2n)¹⁴⁰Ce the magnetic moment of the 10 ₁ ⁺ isomer atE _x =3714.7 keV in theN=82 nucleus¹⁴⁰Ce has been determined by means of the TDPAD method toμ=+10.3(4)μ _N . Measuredg-factors in¹⁴⁰Ce are compared to calculations within the shell model with configuration mixing. For the 10 ₁ ⁺ isomer in¹⁴⁰Ce the four proton configuration π(1g ₇ ^2/2 ,2d ₅ ^2/2 ) has been found to be dominant. From theg-factor measurement strong contributions of multiparticle excitations to thegp2d _3/2,π3s ₁ ² or π1h ₁₁ ² shells and admixtures of neutron excitations to the wave function of the 10 ₁ ⁺ state could be excluded. The strongE1γ-branch of the deexcitation of the 10 ₁ ⁺ isomer in¹⁴⁰Ce can be explained by means of small admixtures of configurations which contain the outer subshell excitationsπ2f _7/2 andπ1h _9/2. On this basisE1 transitions experimentally observed in theN=82 nuclei¹⁴⁰Ce,¹⁴¹Pr and¹⁴⁵Eu may be understood.     

B(E2)-values of even-a nuclei with 82 neutrons

Coulomb excitation of the first excited 2⁺-state was measured usingα-particles to determine reduced transition probabilities,B(E2; 0 _gs ⁺ →2 ₁ ⁺ ), in nuclei with a closed shell of 82 neutrons. TheB(E2; 0 _gs ⁺ →2 ₁ ⁺ -values are 10.2 single-particle units (spu) for¹³⁸Ba, 13.5 spu for¹⁴⁰Ce, 11.9 spu for¹⁴²Nd and 11.6 spu for¹⁴⁴Sm. The uncertainty ranges from 1.3 % to 2.3 %.