Cyclotron resonance in the organic conductor (BEDO-TTF)2ReO4(H2O) in the millimeter wavelength band

Resonant microwave absorption in a (BEDO-TTF)₂ReO₄(H₂O) organic conductor single crystal at a temperature of 1.9 K, a magnetic field of up to 70 kOe, and in the frequency band between 30 and 120 GHz has been studied. A spectral component due to the cyclotron resonance (CR) of two-dimensional charge carriers has been identified for ν⩾80 GHz and H⩾10 kOe. The effective mass m(ω) increases with the frequency from m≈0.8m ₀ at ν=80 GHz to m≈0.95m ₀ at ν=120 GHz. Measurements of the CR line position and FWHM as functions of frequency yield an independently determined imaginary part of the memory function M(ω), which controls the dynamic magnetoconductivity, and the relaxation time τ(ν=100 GHz)≈2.9×10⁻¹¹ s, which is more than thirty times the value of this parameter in the low-frequency limit τ(ν→0). The anomalous behavior of the CR line position and FWHM is caused by the dispersion of both real and imaginary parts of M(ω), which are probably due to strong Fermi-liquid effects. Zh. éksp. Teor. Fiz. 111, 979–987 (March 1997)     

Anisotropic impurity scattering in palladium silver alloys

Measurements have been made of the Hall coefficientR of some alloys of silver in palladium over the temperature range 1°K to 120°K. The alloys contain between ∼1 and ∼10 at.-% silver. Values ofR were also obtained at room temperature and these were in good agreement with earlier published work. The values ofR are negative in all the alloys, and |R| increases both on reducing the temperature and increasing the silver concentration,c. Below ∼10°K, |R| becomes independent of temperature but shows a linear dependence onc, increasing by a factor of 2.5 over the concentration range measured. This increase is too great to be accounted for in terms of band structure changes alone, so we have examined the effects of anisotropic impurity scattering. To a first approximation it can be shown thatR is proportional to an anisotropy parameterA, defined asA=〈τ ²(k)〉/〈τ(k)〉², whereτ(k) represents the relaxation time of an electron in a statek, and 〈〉 is an average over the Fermi surface. In palladium we assume that the majority of the current is carried by the s-electrons. In the presence of silver impurities these electrons can be scattered into s-states or d-states with relaxation times given byτ _ss α1/c(1−c) andτ _sd α1/c ²(1−c) respectively. FollowingPlate we have assumed thatτ _ss is isotropic and thatτ _sd is anisotropic, leading to an overall anisotropic relaxation time for impurity scattering. We then find the parameterA increases approximately linearly with silver content, in accordance with our experimental results.     

On the phase boundaries of the integer quantum Hall effect. Part II

It has been shown that the observation of the transitions between the dielectric phase and the integer-quantum-Hall-effect phases with the quantized Hall conductivity σ _xy ^q ≥ 3e ²/h announced in a number of works is unjustified. In these works, the crossing points of the magnetic-field dependence of the diagonal resistivity ρ _xx at different temperatures T and ω_cτ = 1 have been misidentified as the critical points of the phase transitions. In fact, these crossing points are due to the sign change of the derivative dρ _xx /dT owing to the quantum corrections to the conductivity. Here, ω_c = eB/m is the cyclotron frequency, τ is the transport relaxation time, and m is the effective electron mass.     

Proton NMR relaxation in albumin solutions doped with Mn(II)

The aim of this study is to obtain further information about the source of proton relaxation in the Mn(II)-human serum albumin complex. For this purpose, proton relaxation rates in albumin solutions 1/T ₁ and 1/T ₂ were measured versus increasing amounts of manganese [Mn_t]. The fractions of manganese bound to albumin [Mn_b] and free manganese [Mn_f] were then determined from proton relaxation rate enhancement data. Paramagnetic contributions of bound manganese to the observed relaxation rates (1/T _1p^*)_b and (1/T _2p^*)_b were also determined. Finally, the (1/T _2p^*)_b/(1/T _1p^*)_b ratio was used in a derived equation to estimate an effective correlation time τ. Mean τ value of the complex was found to be in the order of 3 ns, while the hydration number of bound manganese q was estimated to be about 4. The 1/τ was found to be the sum of the inverse values of rotational correlation time 1/τ _r, mean residence time of water in hydration spheres of the complex 1/τ _m, and longitudinal electronic relaxation time of manganese 1/τ _s in the complex. In conclusion, the relaxation mechanism in albumin solutions containing Mn(II) can be interpreted through dipolar and scalar interactions modulated by τ _r, τ _m and τ _s. This analysis enables one to get reasonable figures for the τ _r and q of Mn(II) in albumin solution.     

Nuclear matter properties in relativistic mean-field model with σ- ω coupling

The σ-ω coupling is introduced phenomenologically in the linear σ-ω model to study the nuclear matter properties. It is shown that not only the effective nucleon mass M^* but also the effective σ meson mass m _σ ^* and the effective ω meson mass m _ω ^* are nucleon-density-dependent. When the model parameters are fitted to the nuclear saturation point, with the nuclear radius constant r ₀ = 1.14 fm and volume energy a ₁ = 16.0 MeV, as well as to the effective nucleon mass M ^* = 0.85M, the model yields m _σ ^* = 1.09m _σ and m _ω ^* = 0.90m _ω at the saturation point, and the nuclear incompressibility K ₀ = 501 MeV. The lowest value of K₀ given by this model by adjusting the model parameters is around 227 MeV. Received: 23 March 2001 / Accepted: 8 June 2001     

In-vivo study of the nuclear quadrupole interaction of99Mo (β- 99)Tc in nitrogenase of Klebsiella pneumoniaein nitrogenase of Klebsiella pneumoniae

We report on the first TDPAC-measurements of the nuclear quadrupole interaction (NQI) of (NQI) of⁹⁹Mo(β^-)⁹⁹Tc in the nitrogenase of the bacteria Klebsiella pneumoniae. Because nitrogenase is the only Mo-containing enzyme in Klebsiella pneumoniae under the chosen conditions, no further isolation of this enzyme was necessary. The majority of the incorporated⁹⁹Mo is subjected to a well defined NQI with ω=365(7) Mrad/s, η=1 and a reorientational correlation time of τ_coττ≈10nsec and is attributed to the active site of the FeMo cofactor. During sample preparation we noted a pronounced affinity of the bacteria to^99mTc.     

Mesonic decays of τ− lepton: Effects of neutrino mass and mass mixing

Experimentally established mesonic decays ofτ ⁻ lepton have been reexamined with the inclusion of the effects of finite neutrino mass and the associated mass mixing in the form of Kobayashi-Maskawa mixing matrix. A comparison with the experimentally predicted decay probabilities provides limits for thev _τ mass which are finite in all decays except for the lower limit in mass mixing case of the decayτ ⁻→K*⁻ (892)+v _τ for which MeV. The large error in this value is because of (i) large errors in the experimental values of life time and branching ratio for this decay and (ii) thekm mixing used in the calculations. The ratio of parity-violating to parity-conserving terms in the differential decay probabilities of various decays differs slightly from their values corresponding to those with varishingv _τ mass.     

On the investigation of magnetic critical phenomena in ferromagnets by μSR and PAC

On the basis of current theoretical views on the critical phenomena in isotropic Heisenberg ferromagnets the power temperature behavior Λ=c(τ)λ₀τ^-w has been derived for the muon spin relaxation rate Λ as π-T _c ⁻¹ (T-T _c ) → 0⁺. It is shown that the crossover from an exchange critical regime to a dipolar one is accompanied not only with the change in the critical exponentw in the above law, but also with the reduction of the coefficientc(π). A comparison with the temperature behaviour of the inverse nuclear relaxation timet _R ⁻¹ measured in the PAC experiment is carried out.     

In vivo oximetry by a pulsed longitudinally detected ESR spectrometer

By using a narrow single electron spin resonance (ESR) line agent, triarylmethyl, tris(8-carboxy-2,2,6,6-tetrahydroxyethylbenzo[1,2-d:4,5-d′] bis(1,3)dithiole-4-yl)methyl sodium salt (TAM OX063), pulsed longitudinally detected ESR (LODESR) measurements of a phantom or the chest of a living mouse at the operating frequency of ca. 300 MHz were taken and the effective longitudinal relaxation time (T ₁^*) was estimated for oximetry. Under irradiation of a pair of π-pulses with a variable interval between pulses (τ), in-phase LODESR signal intensities were obtained from the phantoms containing TAM dissolved in a physiological saline solution at a concentration of 1 mM and various concentrations of oxygen. TheT ₁^* of the phantom was calculated from the plotted curve of the LODESR signal intensity against τ. It was found that the reciprocal ofT ₁^*, i.e., the longitudinal relaxation rate, increased with the concentration of oxygen. In vivo pulsed LODESR measurements of the chest of living mice that had received a TAM injection via the intraperitoneal route were made. While the LODESR measurements were being made, the mice in one group breathed normal air and those in another group breathed 100% oxygen. It was found that the longitudinal relaxation rate of the mice breathing 100% oxygen was significantly greater than that of mice breathing normal air, indicating that breathing 100% oxygen elevates the thoracic longitudinal relaxation rate.     

Phonon scattering by paraelastic defects

The relaxation timeτ(ω) for the scattering of the lattice waves of frequencyω by the paraelastic defects has been calculated by using the Feynman graph method, applied to a previous theoretical model [8]. A simple expression for the resonance component ofτ(ω)⁻¹ has been derived.

---

Zusammenfassung Die Relaxationszeitτ(ω) für die Streuung der Gitterwellen der Frequenzω an den paraelastischen Defekten wurde nach der Methode der Feynmanschen Graphen berechnet, wobei ein früheres theoretisches Modell [8] angewendet wurde. Ein einfacher Ausdruck für den Resonanzteil vonτ(ω)⁻¹ wurde hergeleitet.

---

Résumé Nous avons calculé le temps de relaxationτ(ω) des ondes du réseau de fréquenceω, qui sont diffusées par des défauts para-élastiques, en appliquant la méthode des graphes de Feynman à un modèle théorique antérieur [8]. Une simple expression pour la partie résonante deτ(ω)⁻¹ a été dérivée.

     

Event horizons in static electrovac space-times

The following theorem is established. Among all static, asymptotically flat electrovac fields with closed, simply-connected equipotential surfacesg _{0 0}=const.. the only ones which have regular event horizonsg _{0 0}=0 are the Reissner-Nordström family of spherisymmetric solutions withmG ^1/2|e|/c. In the special case where the gravitational coupling of the electromagnetic energy density is neglected (G=0) all solutions are computed explicitly, thus extending an earlier result ofGinzburg for a magnetic dipole inSchwarzschild's space-time. Possible implications for gravitational collapse are briefly discussed.On leave of absence from the Mathematics Department, University of Alberta, Edmonton, Canada.     

Prospects for the measurement of the structure of the coupling of a Higgs boson to weak gauge bosons in weak boson fusion with the ATLAS detector

The prospects for the measurement of the tensor structure of the vertex between a standard model Higgs boson and two weak gauge bosons using the distribution of the azimuthal angles between the two tagging jets in the weak boson fusion channel are studied in a Monte Carlo analysis using the fast simulation of the ATLAS detector. The decay channels H→τ⁺τ^-→ll+4ν, H→τ⁺τ^-→lh+3ν at m_H=120 GeV and H→W⁺W^-→llνν at m_H=160 GeV are used in the analysis. For a standard model Higgs boson it is found that purely anomalous couplings are expected to be excluded at a confidence level corresponding to 2σ or more at m_H=120 GeV and more than 5σ at m_H=160 GeV from 30 fb^-1 of data. With a value of 1 roughly reproducing the standard model cross section for a purely anomalous coupling, the standard deviation in a measurement of a contribution of a CP even anomalous coupling in addition to the standard model coupling is estimated to be 0.20 at m_H=120 GeV and 0.09 at m_H=160 GeV.     

Crystal structure of N-m-tolyl phthalimide

N-m-tolyl phthalimide, C₁₅NO₂H₁₁ crystallizes in the space group Cc with unit cell dimensions,a=8·54(1),b=19·89(2),c = 7·59(1)A, β=114·53(1)° andZ=4.V=1173(2)A³,D _m =1·35(1),D _c = 1·344 mg.m⁻³,M _r =237 λCoK_a=1·7903A. The structure was solved byMULTAN and refined to an R-factor of 0·116 for 632 counter reflections. The molecules are held together by van der Waal’s forces. The angle between the tolyl plane and the plane through the phthalimide group is 53·4(4)°. Contribution No. 607.     

Fluctuation-induced pseudogap in high-temperature superconductors

We study the effect of fluctuations on the ac conductivity of a layered superconductor for c-axis electromagnetic wave polarization. The fluctuation contributions of different physical nature and sign (paraconductivity, Maki-Thompson anomalous contribution, one-electron density-of-states renormalization) are found to be suppressed by the external field at different characteristic frequencies (ω _AL∼T-T _c , ω _MT∼max{T-T _c ,τ _ϕ ⁻¹ }, ω _DOS∼min{T, τ ⁻¹}). As a result, the appearance of a nonmonotonic frequency dependence (pseudogap) in the infrared optical conductivity of high-temperature superconductor is predicted. Pis’ma Zh. éksp. Teor. Fiz. 64, No. 6, 397–401 (25 September 1996) Department of Theoretical Physics Moscow Institute of Steel and Alloys. Published in English in the original Russian journal. Edited by Steve Torstveit.     

Determination of very slow μ+ hop rates in Cu by LLF-μSRhop rates in Cu by LLF-μSR

Muon spin relaxation in low (weak) longitudinal magnetic field (LLF-μSR) provides a means of independently determining the static dipolar width Δ characterizing the μ⁺ lattice site and the correlation time τ_c for μ⁺ hopping, in a manner that is nearly model-independent for τ_c and especially accurate in the near-static limit (τ_c>τ_μ). The advantages of this method are illustrated by its application to muon hopping in Cu near the τ_c maximum around 50 K.     

Magnetic relaxation in a three-dimensional ferromagnet with weak quenched random-exchange disorder

Isothermal remanent magnetization decay,M _r(t), and ‘in-field’ growth of zero-field-cooled magnetization,M _ZFC(t), with time have been measured over four decades in time at temperatures ranging from 0.25T _c to 1.25T _c (whereT _c is the Curie temperature, determined previously for the same sample from static critical phenomena measurements) for a nearly ordered intermetallic compound Ni₃Al, which is an experimental realization of a three-dimensional (d = 3) ferromagnet with weak quenched random-exchange disorder. None of the functional forms ofM _r(t) predicted by the existing phenomenological models of relaxation dynamics in spin systems with quenched randomness, but only the expressions and closely reproduce such data in the present case. The most striking features of magnetic relaxation in the system in question are as follows: Aging effects are absent in bothM _r t andM _ZFC(t) at all temperatures in the temperature range covered in the present experiments. A cross-over in equilibrium dynamics from the one, characteristic of a pured = 3 ferromagnet with complete atomic ordering and prevalent at temperatures away from T_c, to that, typical of ad = 3 random-exchange ferromagnet, occurs asT → T_c. The relaxation times τ₁(T)(τ₁ ^′(T)) and τ₂(T)(τ₂ ^′(T)) exhibit logarithmic divergence at critical temperatures and ; and both increase with the external magnetic field strength,H, such that at any given field value, . The exponent characterizing the logarithmic divergence in τ ₁ ^′ (T) and τ ₂ ^′ T possesses a field-independent value of ≃16 for both relaxation times. Of all the available theoretical models, the droplet fluctuation model alone provides a qualitative explanation for some aspects of the present magnetic relaxation data     

Microwave dielectric characterization of binary mixture of formamide with <Emphasis Type="Italic">N,N</Emphasis>-dimethylaminoethanol

Dielectric relaxation measurements of formamide (FMD)-N,N-dimethylaminoethanol (DMAE) solvent mixtures have been carried out over the entire concentration range using time domain reflectometry technique at 25, 35 and 45°C in the frequency range of 10 MHz to 20 GHz. The mixtures exhibit a principle dispersion of the Davidson-Cole relaxation type at microwave frequencies. Bilinear calibration method is used to obtain complex permittivity ɛ*(ω) from complex reflection coefficient ρ*(ω) over the frequency range of 10 MHz to 10 GHz. The excess permittivity (ɛ ^E), excess inverse relaxation time (1/τ)^E, Kirkwood correlation factor (g ^eff), activation energy and Bruggeman factor (f _B) are also calculated to study the solute-solvent interaction.      

Breakdown of the linear current regime in periodic structures

We study the effect of a weak nonlinearity in media on the linear regime of current flow in two-dimensional periodic structures with two equal component concentrations. We find that the asymptotic behavior of the electric field and current as functions of the distance between the angles in heterogeneous media is determined by the parameter h=σ ₂/σ ₁ (here σ ₁ and σ ₂ are the linear conductivities of the cells) and the external magnetic field B. This dependence leads to divergence of the higher-order moments of field and current at certain critical values h _c and B _c and to divergence of the response functions related to the higher-order moments. For square cells the effective nonlinear conductivity diverges at h⩽h _c, with . For structures of general shape we find the dependence of h _c on the angles and the external magnetic field. We show that for a given structure the linear regime of current flow in the system can be reversibly transformed into a nonlinear one by varying the magnetic field strength. The critical field B _c is approximately determined from the condition ω _c τ∼1, where ω _c and τ ⁻¹ are, respectively, the cyclotron frequency and the collision rate. Finally, we discuss the feasibility of detecting these effects experimentally. Zh. éksp. Teor. Fiz. 112, 643–660 (August 1997)     

A local moment approach to the gapped Anderson model

We develop a non-perturbative local moment approach (LMA) for the gapped Anderson impurity model (GAIM), in which a locally correlated orbital is coupled to a host with a gapped density of states. Two distinct phases arise, separated by a level-crossing quantum phase transition: a screened singlet phase, adiabatically connected to the non-interacting limit and as such a generalized Fermi liquid (GFL); and an incompletely screened, doubly degenerate local moment (LM) phase. On opening a gap (δ) in the host, the transition occurs at a critical gap δ_c, the GFL [LM] phase occurring for δ<δ_c [ δ>δ_c] . In agreement with numerical renormalization group (NRG) calculations, the critical δ_c = 0 at the particle-hole symmetric point of the model, where the LM phase arises immediately on opening the gap. In the generic case by contrast δ_c > 0, and the resultant LMA phase boundary is in good quantitative agreement with NRG results. Local single-particle dynamics are considered in some detail. The major difference between the two phases resides in bound states within the gap: the GFL phase is found to be characterised by one bound state only, while the LM phase contains two such states straddling the chemical potential. Particular emphasis is naturally given to the strongly correlated, Kondo regime of the model. Here, single-particle dynamics for both phases are found to exhibit universal scaling as a function of scaled frequency ω/ω_m ⁰ for fixed gaps δ/ω_m ⁰, where ω_m ⁰ is the characteristic Kondo scale for the gapless (metallic) AIM; at particle-hole symmetry in particular, the scaling spectra are obtained in closed form. For frequencies |ω|/ω_m ⁰ ≫δ/ω_m ⁰, the scaling spectra are found generally to reduce to those of the gapless, metallic Anderson model; such that for small gaps δ/ω_m ⁰≪ 1 in particular, the Kondo resonance that is the spectral hallmark of the usual metallic Anderson model persists more or less in its entirety in the GAIM.