The structure of28Si above 10 MeV excitation energy III: Level scheme and shell model interpretation

²⁸Si level scheme up to 14.5 MeV excitation energy is reevaluated using information from two preceding papers. It consists of approximately 250 levels which are almost completely characterized according to the quantum numbersI, π, T of the levels. The properties of positive-parity states are compared to the predictions of shell model calculations within the completes-d basis space using the unifieds-d shell Hamiltonian. A spectrum of 48 experimentalT=1 states between 9.3 and 16 MeV is reproduced with a rms deviation of only 150 keV. A calculation of radiative widths and γ-decay modes which uses free-nucleong-factors yields excellent agreement with experiment and confirms that quenching of M1 transitions is only marginal in²⁸Si. The detailed shell model analysis of theT=0 spectrum is extended to the limiting energy whereT=1 wave function admixtures, not contained in the theory, become important experimentally. This happens at 6–8 MeV above the yrast state, depending on the spin value. Altogether it appears that a spectrum of 171 levels below 14.5 MeV, which have positive or unassigned parity, is almost completely accounted for by the model. Apparent intruder states from outside thes-d shell space are observed atE _x =10 945 keV (I ^π=4⁺) and 12 860 keV (I ^π=6⁺) and are interpreted as members of aK ^π=0⁺ rotational band.     

The structure of25Mg

Gamma-decay modes and spin(-parity) assignments of levels in²⁵Mg have been systematically investigated up to 10 MeV excitation energy by particle-γ-ray angularcorrelation measurements with the²⁴Mg(d, pγ) reaction at 6.5 MeV bombarding energy and with the²²Ne(α,nγ) reaction at 11.8, 12.5, 14.4 and 15.5 MeV bombarding energy. A level scheme has been established which is comprehensive up to 8.3 MeV excitation energy forI≦9/2 and up to 10 MeV for 9/2O d _5/2 — 1s _1/2-O d _3/2 shell and the unifieds-d shell Hamiltonian. The agreement is good to excellent. The first intruder states are located near 6.8 MeV excitation energy. The collective properties of²⁵Mg beyond the well established rotational bands are investigated using both the new experimental information and theB(E2)'s obtained from the shell model. The spectrum of²⁵Mg is completely rotational for the first five to six MeV above the yrast line. Shell modelB (M 1)'s reflect the Nilsson model structure of²⁵Mg in great detail. The prospectiveI ^π=9/2^?, 13/2^?, and 15/2^? members of the established negative-parity,K=1/2 band are found in levels atE _x=7801, 9410, and 8896 keV.     

High-spin states in26Mg

Theγ-decays of levels in²⁶Mg have been investigated up to 12.5 MeV excitation energy by proton-γ-ray coincidence measurements in the²³Na(α, pγ) reaction at 14.2 and 16 MeV bombarding energy. Lifetime-measurements, made with the Doppler-shift attenuation method, and proton-γ-ray angular-correlation measurements were performed at E_α=14.2 MeV. Many high-spin states were observed, among them levels at 6,978 (5⁺), 7,283(4^?), 7,395(5⁺), 7,953(5^?), 8,202(6⁺), 8,472(6⁺), 9,065(5), 9,112(6⁺), 9,169(6^?), 9,383 (6⁺), 9,542(5), 9,829(7⁺), 9,989(6⁺) and 12,479(8⁺, 7^?) keV excitation energy. The spectrum of positive-parity states and their electromagnetic properties are reproduced with good accuracy by shell-model calculations which employ a unifieds-d shell Hamiltonian and the unrestricted configuration space of the 0d _5/2 1s _1/2 0d _3/2 shell. Members of five inferred rotational bands, withK ^π=0⁺, 2⁺, 3⁺, 0⁺ and 3^? have been observed up to at leastI=6. TheK ^π=2⁺ band shows strong anomalies of excitation energies andE2 transition rates near theI=6 state. The static intrinsic quadrupole moments calculated from the shell model wave functions indicate transitions from prolate to oblate deformation within theK ^π=2⁺ band and also the ground state band. The lowest lyingI ^π=4⁺ state appears to be “spherical” and cannot be associated with a rotational band.     

Spectroscopy of highly excited states in29Si

Particleγ-ray coincidences have been measured in the²⁸Si (d,pγ) reaction at 6.5 and 7 MeV bombarding energy, in the²⁶Mg (α,nγ) reaction at 12, 14 and 15 MeV, and in the²⁷A1 (τ,pγ) reaction at 9 MeV. Theγ-decay has been observed for all bound states of²⁹Si and for 56 unbound states up to 12,960 KeV excitation energy. Particleγ-ray angular correlations were measured in the²⁸Si (d,pγ) reaction at 6.5 MeV and in the²⁶Mg (α,nγ) reaction at 12 MeV. Spin (-parity) assignments or restrictions were obtained for nearly all bound states and some high-spin states above the binding energy. The assignment of mirror levels in²⁹Si and²⁹P has been extended to 8.2 MeV excitation energy. The excitation energies of 41 positive-parity states are reproduced by shell model calculations. The possible existence of aK ^π=5/2⁺ band with prolate deformation is discussed.     

The structure of 26Mg investigated with the (d,p) reaction

Angular distributions have been measured for the ²⁵Mg(d, p)²⁶Mg reaction at 13 MeV leading to excited states between E_x = 0 and 8 MeV. Experimental cross sections are compared with DWBA calculations and extended shell-model calculations in the full sd shell. Spin and parity restrictions are obtained for several levels in the region E_x = 6?;8 MeV. Spectroseopic factors for transitions to the lowest four positive-parity states of each spin are well reproduced by the shell-model calculations; however, in mixed configurations the largest component is systematically underestimated by the shell model. Only 60% of the strength for $\text{s}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$ transfer is observed.     

Three-nucleon yrast states in145Sm

In-beamγ-ray and conversion electron measurements with (α, xn) reactions have established the¹⁴⁵Sm highspin states up toI ^π=25/2⁺ at 3.5 MeV excitation. A shell model analysis using empirical two- and one-body energies from neighbouring nuclei classifies the low-lying odd-parity levels as 3-quasiparticle states formed by the¹⁴⁴Sm two-proton-hole excitations and thef _7/2 valence neutron. The higher-lying positive-parity states involve particle-hole core excitations with one proton inh _11/2.     

Low-lying states of 6He studied via the 6Li(t,3He)6He reaction

We present the recent experimental results on the ⁶He structure studied by the ⁶Li(t, ³He)⁶He reaction at 336 MeV. Above the conspicuous peaks for ground and first excited states for ⁶He, we have observed a broad structures at E _x∼ 5 MeV, and E _x∼ 15 MeV. The angular distribution of this structure exhibits the dominance of a ΔL = 1 transition, indicating the existence of intruder dipole states at low excitation energies in ⁶He. A slight admixture of positive-parity states in this structure has been indicated as well. Received: 1 May 2001 / Accepted: 4 December 2001     

Low-lying levels, γ-ray transitions,and vibrational structure in 198Pt from (n,n'γ) reaction spectroscopy

Low-lying states in ¹⁹⁸Pt have been studied by (n, n'γ) reaction spectroscopy at incident neutron energies below 2.5 MeV. Using detailed γ-ray excitation functions and angular distribution measurements, we have established a level scheme which includes 16 excited levels and is believed to include all levels below an excitation energy of 1.5 MeV. The positive-parity structure is similar to that expected for an anharmonic vibrator; however, difficulties in asserting that the first 0⁺ excited level is a collective excitation are encountered. Only two negative-parity states are observed, and they are adequately described in the semi-decoupled model.     

Four-nucleon transfer with the 32S(16O, 12C)36Ar reaction

Angular distributions have been measured for the ³²S(¹⁶O,¹²C)³⁶Ar reaction at 45.5 MeV leading to excited states between E_x, = 0 and 8 MeV. Experimental cross sections are compared with exact finite-range DWBA calculations in combination with extensive shell-model calculations, which include sd- and fp-shell configurations. Transitions to low-energy positive-parity states and bound negative-parity states are well reproduced. The calculations, however, fail to describe some high-energy positive-parity states. Calculations with a complete cluster expansion for the four transferred nucleons give about 50% larger cross sections, but can not explain the observed discrepancies. Possible interference of reaction processes other than direct α-transfer and special structure effects are discussed.     

Microscopic and macroscopic aspects of 135 MeV proton scattering from 16O

Differential cross sections have been measured for the scattering of 135 MeV protons from ¹⁶O and data from the transitions to 13 states (up to 19.5 MeV excitation) have been analysed using microscopic and macroscopic nuclear reaction models. Extensive collective model calculations have been made of the transitions to all natural-parity states. The deformation parameters for the 4p4h rotational band are in good agreement with theoretical models. The inelastic scattering data from the excitation of the negative-parity states have also been analysed in the distorted-wave approximation using microscopic (shell and RPA) models of nuclear structure and with density-dependent two-nucleon t-matrices. For positive-parity states, we report the first shell-model calculation using the complete 2?ω basis space and find that the triplet of 2p2h states (4⁺, 2⁺, 0⁺) around 11 MeV excitation is quite well described by this model, as may be a 1⁺ state which is observed for the first time by proton scattering from ¹⁶O.     

Spectrum of the high spin neutron hole states of205Pb

The high resolution (³He,α) reaction on²⁰⁶Pb shows the distribution of the 2f _7/2, 1h _9/2 and 1i _{1 3/2} neutron states of²⁰⁵Pb within the 6 MeV excitation energy of²⁰⁵Pb. The spectrum of these three-hole states is obtained within the hole-core vibrational coupling scheme. The shell model energies of the neutron hole states arising from the core-polarization effect are compared with the Bansal-French energy weighted sum rule. The possible implication of the present neutron hole energies has been discussed in the light of the deduced shell model wave functions of the collective states of²⁰⁶Pb.     

Influence of shell effects on the angular distributions of fission fragments

A dynamical-statistical model is used to analyze the experimental angular distributions of fission fragments in the reactions α + ²³⁸U, ²³⁷Np at E _α = 20–100 MeV, as well as to determine the Am isotope fission probabilities and the shape isomer yields in the reactions d + ^242,240Pu at E _d = 20–30 MeV. Manifestations of shell effects are found in the fission barrier structure up to the excitation energies of 50–60 MeV.     

The structure of27Al

Gamma decay modes and spin assignments of levels in²⁷Al have been investigated by proton-γ-ray angular correlation measurements in the²⁴Mg(α, pγ) reaction at 14.2, 15 and 15.6 MeV bombarding energy and byγ-ray angular distribution measurements on the E_p=1820, 2114, 2293 and 2574 keV resonances of the²⁶Mg(p, γ) reaction. Unique spin assignments were obtained as follows: I=3/2 for the 5827 keV state, I=5/2 for the 6115, 6465, 6765, 7577, 7721, 8097, 8136, 8324 keV states, I=7/2 for the 5433, 6533, 7413, 8037, 8442, 8586 keV states, I=9/2 for the 5418, 6512, 6713, 7997 keV states, I=11/2 for the 5500, 6948, 7400, 8396 keV states. The level scheme and electromagnetic properties of levels are compared with the results of shell model calculations which use the complete configuration space of the 0d_5/2-1s_1/2-0d_3/2 shell and the unifieds-d shell Hamiltonian. The agreement is good to excellent and extends into the region of high level density above 7 MeV excitation energy. The total B(M1↑) below 8.5 MeV excitation energy is evaluated, using published resonance fluorescence and (e, e′) data, and quenching relative to the free-nucleon predictions is reexamined. Evidence in favour of a prolate ground state deformation of²⁷Al and implications of this work for the astrophysically interesting²⁶Al(p, γ) reaction are discussed.     

Shell-model calculations inA=28–32 nuclei

Shell-model calculations for positive-parity levels of A=28–32 nuclei have been performed in a 1d_5/2 2s_1/2 1d_3/2 configuration space. Configuration mixing of at most 250 lowest-lying pure configurations for each (A, J, T) set was taken into account. By a variation of the four effective interaction (MSDI) parameters and three single-particle energies a search was made for the best fit of the calculated energies to the experimental values. The average deviation between theory and experiment for the energies of the 110 fitted levels is 0.44 MeV. By adjusting all the 63 two-body matrix elements (ASDI) and the three single-particle energies, the average deviation of the binding energies was reduced to 0.16 MeV. For the lowest 10–15 levels in all A=28–32 nuclei a one to one correspondence exists between theory and experiment. Electromagnetic transition strengths were calculated both with MSDI and with ASDI wave functions. The ASDI wave functions reproduce the experimental E2 data much better than the MSDI wave functions. For the M1 transition strengths only a minor improvement has been achieved.     

The collective bands of positive parity states in odd-A (fp) shell nuclei

The low-lying collective bands of positive parity states in (fp) shell nuclei are described in the deformed Hartree-Fock method by projecting states of definite angular momenta from ‘the lowest energy intrinsic states in (sd)⁻¹ (fp) ⁿ⁺¹ configurations. The modified Kuo-Brown effective interaction for (fp) shell and modified surface delta interaction (MSDI) for a hole in (sd) shell with a particle in (fp) shell have been used. The collective bands of states are in general well reproduced by the effective interactions. The excitation energies of the band head states are however off by about one MeV. The calculated magnetic moments of the band headj=3/2⁺ states are in reasonable agreement with experiment. Using effective chargese _p=1.33e ande _n=0.64e we get fairly good agreement forE(2) transitions. The hinderedM(1) transition strengths are reproduced to the correct order however they are slightly higher compared to experiment.     

Polarization and phase shifts in Be(p, p)Be from 0.8 TO 2.7 MeV and the structure of B

Angular distributions of the analyzing power in Be have been measured to an accuracy of about ±0.03 at 21 energies from 0.9 to 2.7 MeV with a target thickness of 20 keV at 1 MeV. These data and the cross section measurements of others are reproduced well in the region from 0.8 to 1.6 MeV by a set of phase shifts that vary reasonably with energy. The ³S₁, ⁵S₂, ⁵P₁, and ⁵P₂ phases suffice to describe the data, although channel spin and s-d mixing are required. Three levels satisfy the data: at 0.980±0.010 MeV are two levels, a 1⁺ of width 0.10 MeV and a 2⁻ of width 0.11 MeV; at 1.37±0.02 MeV is a 1⁻ level of width 0.30 MeV. The 1⁺ and 1⁻ states do not agree with earlier assignments. Outside of the energy region from 0.8 to 1.6 MeV a satisfactory set of phases could not be obtained, owing to inadequate data. These regions were studied in the analysis, however, and the results are discussed.     

Beta decays of 44V and 52Co

We have studied the prevously unknown β⁺ decay branches from ^44,44mV and ⁵²Co to particle-bound states in ⁴⁴Ti and ⁵²Fe, respectively. These intense branches populate a few states in the daughters from an excitation energy of about 1 MeV up to the isobaric analogue states at about 6 MeV. We have measured the first precise energy values for the latter states as well as the β-branching ratios to all states in this excitation energy region. We have calculated the β⁺ decay of ^44,44mV in the full fp shell model space as well as in a truncated space. Renormalized transition operators are constructed for the truncated space and tested against experimental data in ⁴⁴V and ⁵²Co. In general there is good agreement between theory and experiment for the half-lives, level energies and beta branches, but not all the states found are reproduced by the calculations.     

Identification and structure of high spin particle-hole states in89Mo

Particle-γ andγ-coincidences of the reaction⁵⁸Ni(³⁶Ar, 4pn)⁸⁹Mo have been used to gain more information about high spin states in⁸⁹Mo and to establish the yrast sequence up to 7.6 MeV excitation energy and probable spin 37/2 ?. Spins and parities were assigned on the basis of DCO-ratios measured with the OSIRIS spectrometer and a large volume Ge detector placed at 162° to the beam. Furthermore, aγ-ray angular distribution experiment was carried out using the reaction⁵⁸Ni(³⁵Cl, 3pn)⁸⁹Mo. As in the neighboring isotopes⁸⁸Mo and⁹⁰Mo, the positive-parity high-spin states can be grouped into shell model multiplets characterized by increasing seniorities of proton particles and neutron holes in the 1g_9/2 shell. The negative-parity states can be explained with one nucleon moving in thep _1/2 orbit. The energies and wave functions of these states have been deduced by means of the shell model code RITSSCHIL. The 2584 keV (21/2⁺) is an isomeric state the mean life of which has been estimated from delayedγγ-coincidences.