二维GaAs 基光子晶体微腔的制作与光谱特性分析

研究了以InAs量子点为有源区的二维GaAs基光子晶体微腔的设计与制作,测试并分析了室温下微腔的光谱特性.观察到了波长约为1137 nm,谱线半高宽度约为1 nm的尖锐低阶谐振模式发光峰.我们比较了不同刻蚀条件下光子晶体微腔的发光谱线,结果表明空气孔洞截面的垂直度是影响光子晶体微腔发光特性的重要因素之一.通过调节干法刻蚀工艺,改变空气孔半径与晶格常数的比率,可以在较大范围内调节谐振模式发光峰位置,达到谐振模式与量子点发光峰调谐的目的.     

All-optical switch based on photonic crystal microcavity with multi-resonant modes

We present a design of all-optical switches based on one-dimensional photonic crystals (1D PhC) doped with nonlinear optical materials. The 1D PhC switch structure is composed of a PhC cavity sandwiched by two accessional PhC microcavities. The center PhC cavity has two resonant frequencies with nearly the same quality factors (Q), while the accessional PhC cavities have the same resonant frequency, which is equal to one of the resonant frequencies of the center cavity. The two accessional PhC cavities cause reduction of Q value in this resonant frequency and result in different Q values of two modes. We realize all-optical switch effect by selecting pump light wavelength at the low Q mode and probe light wavelength at the other mode. The theoretical simulations by using the finite difference time domain method show that the pump light intensity required to realize optical switch effect in the designed switch is 50 times smaller than that in one-dimensional photonic crystals cavity with only one resonant mode.     

Controlling the spontaneous emission rate of single quantum dots in a two-dimensional photonic crystal

We observe large spontaneous emission rate modification of individual InAs quantum dots (QDs) in a 2D photonic crystal with a modified, high-Q single-defect cavity. Compared to QDs in a bulk semiconductor, QDs that are resonant with the cavity show an emission rate increase of up to a factor of 8. In contrast, off-resonant QDs indicate up to fivefold rate quenching as the local density of optical states is diminished in the photonic crystal. In both cases, we demonstrate photon antibunching, showing that the structure represents an on-demand single photon source with a pulse duration from 210 ps to 8 ns. We explain the suppression of QD emission rate using finite difference time domain simulations and find good agreement with experiment.     

Investigation of cavity modes and direct observation of Purcell enhancement in 2D photonic crystal defect microcavities

We demonstrate our ability to control and manipulate the optical modes in 2D Photonic Crystal Defect cavities and investigate their coupling to InGaAs self-assembled quantum dots. Our results enable us to probe the nature of individual cavity modes and directly investigate cavity QED phenomena. For the lowest mode volume cavities investigated, consisting of a single missing air hole within a hexagonal lattice, we have measured a clear Purcell enhancement of the light-matter interaction in the weak coupling regime. For QDs on-resonance with localized cavity modes this translates to a shortening of the quantum dot spontaneous emission lifetime by a factor 2 when compared to off-resonance dots.     

立体耦合光子晶体薄板微腔的高Q值特性研究

利用微腔之间的立体耦合,提出了基于无源材料硅的双层光子晶体薄板H1(DLPCS-H1)腔,薄板之间为空气层.使用三维时域有限差分方法和Padé近似方法分析了DLPCS-H1腔的偶极模的场分布和品质因子.通过对中间空气层高度的优化使DLPCS-H1腔的偶极模的品质因子得到了显著的提高,大约为单层光子晶体薄板H1腔的偶极模的品质因子的4倍.此外,还研究了三层光子晶体薄板H1腔,它的偶极模的品质因子约为单层光子晶体薄板H1腔的偶极模的品质因子的7倍.     

光子晶体微腔中高偏振单偶极模的研究

三角晶格排列的光子晶体微腔中的偶极模式是简并的,通过改变其晶格的对称性可以消除模式简并.晶格的整体形变破坏了晶格对称性从而影响光场的分布,同时还改变了电磁场的偏振分布.晶格整体形变使得简并的偶极模式分离成x极和y极偶极模式.通过计算分析发现分离后的模式具有良好的偏振特性,从而为实现单偏振光子晶体激光器提供了一种很好的途径.文中针对光子晶体薄板结构的微腔,主要计算了偶极模中x极偶极模式在不同拉伸时以及不同填充因子情况下的Q值,并分别计算了x关键词： 光子晶体 偶极模 品质因子 偏振度     

Design of high-Q cavities in 2D photonic crystals air holes filled with polymer

We design novel photonic crystal heterostructure, substituting the air in the holes with materials of refractive index higher than n = 1. This can be achieved by infiltrating the photonic crystal (PC) with polymer. We theoretically investigate the L₂ cavity with two missing holes in the center, where the six holes surrounding the cavity are locally filled with polymer. We show that cavity modes can be differently tuned depending on the size and the position of the first hole adjacent to the cavity. A photonic microcavity with a high Q factor of 5.5 × 10⁶ and a modal volume V of 0.1919 is demonstrated. We demonstrate that the calculated Q factor for the designed cavity increases by a factor of 22 relative to that for a cavity without displaced and reduced air holes, while the modal volume remains almost constant.     

Single photon sources with single semiconductor quantum dots

In t.his contribution, we briefly recall the basic concepts of quantum optics and properties of semicon- ductor quantum clot. （QD） which a.re necessary to the nnderstanding of the physics of single-photon generation with single QDs. Firstly, we address the theory of quantmn emitter-cavity system, the fluorescence and optical properties of semiconductor QDs, and the photon statistics as well as opti- cal properties of the QDs. We then review the localizatioll of single semiconductor QDs in quantum confined optical microcavity systems to achieve their overall optical properties and perfornances in terms of strong coupling regime, elfieiency, directionality, and polarization control. Furthermore, we will discuss the recenl, progress on the fabrication of single photon sources, and various a.pproaehes for embedding single QDs into mieroca,vities or photonic crystal nanoeavities and show how to ex- tend the wavelength range. We focus in part;icular on new generations of electrically driven QD single photon source leading to high repetition rates, efficiencies at elevated temperature operation. Besides strong eoupling regime, and high collection new development;s of room temperature sin- gle photon emission in the strong coupling regime are reviewed. The generation of indistinguishable photons and remaining challenges for pract ical single-photon sources are also discussed.     

Ensemble of asymmetric quantum dots in a cavity as a terahertz laser source

The possibility of establishing a terahertz laser generation at a transition between the dressed states formed by the interaction of an intense optical field with an ensemble of asymmetric quantum dots (QDs) in a high-Q terahertz cavity is discussed. It has been shown that the population inversion in the system of dressed states is achieved owing to spontaneous relaxation of the excited state of the QDs. The set of Maxwell–Bloch equations for the difference between dressed-state populations, polarization, and population of the cavity mode has been analyzed in the mean-field approximation. The lasing conditions have been clarified and the possibility of controlling the terahertz radiation intensity has been studied, including the case of an inhomogeneously broadened ensemble of QDs.     

Application of LDOS and multipole expansion technique in optimization of photonic crystal designs

We introduced a procedure of using local density of states for increasing the quality factor and Purcell factor of photonic crystal cavities. We used multipole expansion method for accurate calculation of local density of photonic states, stationary field profile, Q-factor, mode volume and Purcell factor of photonic crystal cavities. We found out that the quality factor exponentially increases with the number of additional photonic crystal layers around the cavity while the mode frequencies stay unchanged. We also demonstrated the method in studying the defect mode??s behavior in photonic crystal cavities and showed that high Q-factor, small mode volume and high Purcell factor could be obtained with optimization of geometrical parameters of first neighboring layer.     

Quantum computing by optical control of electron spins

We review the progress and main challenges in implementing large-scale quantum computing by optical control of electron spins in quantum dots (QDs). Relevant systems include self-assembled QDs of III–V or II–VI compound semiconductors (such as InGaAs and CdSe), monolayer fluctuation QDs in compound semiconductor quantum wells, and impurity centres in solids, such as P-donors in silicon and nitrogen-vacancy centres in diamond. The decoherence of the electron spin qubits is discussed and various schemes for countering the decoherence problem are reviewed. We put forward designs of local nodes consisting of a few qubits which can be individually addressed and controlled. Remotely separated local nodes are connected by photonic structures (microcavities and waveguides) to form a large-scale distributed quantum system or a quantum network. The operation of the quantum network consists of optical control of a single electron spin, coupling of two spins in a local nodes, optically controlled quantum interfacing between stationary spin qubits in QDs and flying photon qubits in waveguides, rapid initialization of spin qubits and qubit-specific single-shot non-demolition quantum measurement. The rapid qubit initialization may be realized by selectively enhancing certain entropy dumping channels via phonon or photon baths. The single-shot quantum measurement may be in situ implemented through the integrated photonic network. The relevance of quantum non-demolition measurement to large-scale quantum computation is discussed. To illustrate the feasibility and demand, the resources are estimated for the benchmark problem of factorizing 15 with Shor's algorithm.     

Cavity QED effects with single quantum dots

A single quantum dot embedded in a photonic crystal defect cavity allows for the investigation of cavity quantum electrodynamics effects in a solid-state environment. We present experiments demonstrating the quantum nature of this fundamental system in the strong coupling regime. Photon correlation measurements are used to characterize the fundamental properties of this unique system: through these experiments, we identify an unexpected, efficient sustaining mechanism that ensures strong cavity emission and is quantum correlated with the exciton resonance, even when all the quantum dot resonances are far detuned from the cavity mode. To cite this article: A. Badolato et al., C. R. Physique 9 (2008).     

A three‐level dark state and double‐control single‐photon logic gates via quantum coherent control

Multilevel quantum coherence and its quantum‐vacuum counterpart, where a three‐level dark state is involved, are suggested in order to achieve new photonic and quantum optical applications. It is shown that such a three‐level dark state in a four‐level tripod‐configuration atomic system consists of three lower levels, where constructive and destructive quantum interference between two control transitions (driven by two control fields) arises. We point out that the controllable optical response due to the double‐control tunable quantum interference can be utilized to design some fascinating new photonic devices such as logic gates, photonic transistors and switches at quantum level. A single‐photon two‐input XOR logic gate (in which the incident “gate” photons are the individual light quanta of the two control fields) based on such an effect of optical switching control with an EIT (electromagnetically induced transparency) microcavity is suggested as an illustrative example of the application of the dark‐state manipulation via the double‐control quantum interference. The present work would open up possibility of new applications in both fundamental physics (e.g., field quantization and relevant quantum optical effects in artificial systems that can mimic atomic energy levels) and applied physics (e.g., photonic devices such as integrated optical circuits at quantum level).     

偶极子位置及偏振对激发光子晶体H1微腔的影响

光子晶体微腔和量子点的集成是实现量子信息处理非常具有潜力的平台之一,利用微腔和量子点的耦合可以制备纠缠光子对,实现对量子态的操控.因为光子晶体微腔具有品质因子高、模场体积小等优点,可以极大地增强光与物质之间的相互作用,从而易于实现量子态在不同物理体系之间的转换.通过单量子点和光子晶体H1微腔的耦合可以产生纠缠光子对,因为H1微腔具有简并的、模式偏振正交的基态模式.通常微腔模式的激发随着量子点在微腔中的位置变化而改变,本文用时域有限差分方法研究了偶极子光源的位置及偏振对激发光子晶体H1微腔模式的影响.结果表明:通过改变偶极子光源位置可以选择性地激发H1微腔简并模式中的一个;具有某一偏振的偶极子光源只能激发相应偏振的微腔模式;模式激发强度的大小也是由偶极子光源在微腔中的位置决定的.鉴于目前量子点在微腔中的位置尚不能精确控制,所以微腔模式受激发光源位置的影响的研究具有重要意义.     

Phase Sensitive Photonic Flash

We theoretically propose a photonic flash based on a linearly coupled cavity system. Via driving the two side cavities by external fields, it forms a cyclic energy-level diagram and therefore the phase difference between the driving fields acts as a controller of the steady state due to the quantum interference effect. In the optical trimer structure, we show that the perfect photonic flash can be realized in the situation of resonant driving. The perfect photonic flash scheme is furthermore generalized to multiple coupled cavity system, where the cavities with odd and even number turn bright and dark alternatively. Our proposal may be applied for designing the quantum neon and realizing a controllable photonic localization.     

Charge controlled self-assembled quantum dots coupled to photonic crystal nanocavities

The system of charge controlled self-assembled quantum dots coupled to high-Q photonic crystal cavity modes is studied. The quantum dots are embedded in a p-i-n diode structure. Different designs of photonic crystal cavities are used, namely H1 and L3 and the Purcell effect is demonstrated. Furthermore, the fine tuning of the H1 cavity design is studied in order to achieve far field emission profiles that result in higher collection efficiency. An increase in the overall signal from the quantum dot when it is coupled to a cavity is observed, due to the Purcell effect and the improved collection efficiency. This together with the deterministic charging of the quantum dot that is demonstrated, can be used for a single electron spin measurement.     

Phase Sensitive Photonic Flash

We theoretically propose a photonic flash based on a linearly coupled cavity system. Via driving the two side cavities by external fields, it forms a cyclic energy-level diagram and therefore the phase difference between the driving fields acts as a controller of the steady state due to the quantum interference effect. In the optical trimer structure,we show that the perfect photonic flash can be realized in the situation of resonant driving. The perfect photonic flash scheme is furthermore generalized to multiple coupled cavity system, where the cavities with odd and even number turn bright and dark alternatively. Our proposal may be applied for designing the quantum neon and realizing a controllable photonic localization.     

On‐chip single photon sources using planar photonic crystals and single quantum dots

We review the basic light‐matter interactions and optical properties of chip‐based single photon sources, that are enabled by integrating single quantum dots with planar photonic crystals. A theoretical framework is presented that allows one to connect to a wide range of quantum light propagation effects in a physically intuitive and straightforward way. We focus on the important mechanisms of enhanced spontaneous emission, and efficient photon extraction, using all‐integrated photonic crystal components including waveguides, cavities, quantum dots and output couplers. The limitations, challenges, and exciting prospects of developing on‐chip quantum light sources using integrated photonic crystal structures are discussed.     

Coupling effects in a photonic crystal microcavity with embedded semiconductor quantum dot

The present work investigates the effects of relevant parameters of InAs/GaAs quantum dot and photonic crystal slab-based microcavity on the QD–cavity coupling characteristics, in detail. We employ variational approach to find exciton state in QD and to find cavity modes we use the open source GME code. Calculations have performed in linear regime where excitons behave as bosons which correspond to the limit of low excitation. The dynamics of the system are studied using the first order correlation function (G⁽¹⁾(t,τ)). We will show how G⁽¹⁾ varies with time in both strong and weak coupling regimes. Our results indicate that the achieving of strong coupling regime is affected by the size of the quantum dot and how to engineer the photonic crystal microcavity to maximize the ratio of quality factor and mode volume.     

微腔增强发射的半导体量子点单光子源

单光子源是实现量子密匙分配、线性光学量子计算的基本单元。作者回顾了单光子源在量子信息科学发展中的作用,讨论了光子的统计特性,分析了具有类似原子二能级结构的半导体量子点作为单光子发射源的特点,介绍了微腔与二能级系统的耦合以及微腔量子电动力学基本原理。在弱耦合区,Purcell效应导致微腔中量子点激子复合寿命降低,因此可用微腔来改善量子点单光子发射效率。文章总结了近年来在半导体微腔增强量子点单光子发射领域的进展,探讨了分布式布拉格反射微腔、柱状微腔和光子晶体微腔等结构对改善半导体量子点单光子发射和收集效率、光子极化以及光子全同性等方面的作用,并对未来半导体量子点单光子源的发展进行了展望。