强扰动区C~(q+)离子与He原子碰撞中有效电荷研究

本文利用经典过垒电离模型(Class Over Barrier Ionization)处理100-400ke V/amu强扰动区(q/v1)的不同价态非全裸离子Cq+(q=1-4)与全裸离子H1+,He2+,Li3+与He原子碰撞过程.发现相同价态下,全裸离子的双单电离截面比R21明显低于非全裸离子,原因在于两者的电子结构明显不同.非全裸离子的外壳层电子在碰撞过程中会有一定几率过垒,这在以往的研究中并未考虑.利用模型计算结果与实验数据的比对,估计入射离子第二有效电荷,最终确定入射离子在电离过程中的第一和第二有效电荷.     

中低能非全裸C离子与He原子的碰撞研究

采用反冲离子飞行时间-散射离子位置灵敏符合测量技术，测量了能量范围在0.7v₀—4.4v₀(v₀为玻尔速度)的碳离子C^q+(q=1—4)与He原子碰撞过程不同出射道靶原子的双电离与单电离截面比R，包括入射离子不损失电子(直接电离)的出射道(R_q,q),入射离子俘获一个电子的出射道(R_q,q-1)和入射离子损失一个电子的出射道(R_q,q+1)，并研究了R随入射C离子的能量及电荷态的变化关系.实验表明，对给定电荷态的入射离子，靶原子的双电离与单电离截面比R与出射道有很强的依赖关系，即R_q,q<R_q,q+1<R_q,q-1.直接电离出射道截面比R_q,q与入射离子电荷态几乎无关，而入射离子俘获一个电子的出射道和损失一个电子的出射道靶原子双电离与单电离截面比R_q,q-1和R_q,q+1却与入射离子电荷态有很强的关系.采用原子极化理论和电子屏蔽与反屏蔽作用对实验结果进行了解释. 关键词： 离子-原子碰撞 电离 截面比     

Investigation of transfer ionization in collisions of partially stripped carbon ions with helium at low to intermediate velocities

The ratios of transfer ionization (TI) to single-electron capture (SC) cross sections have been measured for the collisions of partially stripped C^q+ ions (q=1--4) with He. The collision velocity ranges from 0.7 to 4.4v₀ (v₀ is the Bohr velocity). The projectile-ion and recoil-ion coincidence technique is used to separate the processes of TI and SC. The ratios reach the maximum when the velocity is about 3.7v₀ This can be explained qualitatively based on the two-step mechanism. The experimental results are also compared with the results calculated using the classical trajectory Monte Carlo (CTMC) method. The CTMC results are in agreement with the experimental data basically. The discrepancies in higher velocity region are interpreted by the effective charge effect.     

Simple model for the ionization of helium atoms by fully and partially stripped ions in the strong interaction region

Theoretical calculations employing the modified over-barrier model to investigate single and double ionization cross sections of helium in collisions with highly charged ions are presented in the strong perturbation region. It shows the velocity and charge state dependences of cross sections, which coincides with the available experimental data. In order to determine the reliability of this model for partially stripped projectiles, the cross-section ratios have been measured for CZp+, OZp+-He (Zp=1-4) by the coincidence technique in the velocity range of 1-4.5 a.u. The calculated results are approximately in agreement with the experimental data.     

Investigation of the transfer ionization process in collisions of partially stripped ions on He

In this paper a projectile ion-recoil ion coincidence technique is used to investigate the transfer ionization processes in collisions of 0.22--6.30~MeV C^{q + } ions and 0.25--6.35~MeV O^{q + } ions (q=1, 2, 3, 4) with the He atom separately. The cross section ratio f of transfer ionization to single electron transfer is measured, and the dependence of f on both charge state q and energy E of the projectiles is investigated. The electron-structure and the mechanisms leading to transfer ionization affect the dependence of f on q and E. Our measurements, along with other data published previously, suggest a similar dependence of f on charge state and energy of projectile for partially stripped ions over a large energy range. The maximum value of f is approximately 0.17q^{0.60}; the energy corresponding to maximum f is about 160q^{0.60}~keV/u.     

Investigation of transfer ionization processes in the collision of partially stripped carbon ions on Argon

The ratios of the cross section of the transfer-ionization to the single-electron-capture of Argon induced by C ^q+ (q = 1, 2, 3) ions are measured by means of position sensitive and time-of-flight techniques. Our experimental results are compared with the data of He^q+ (q = 1, 2) − Ar of DuBois. A qualitative interpretation is presented based on the Classical-Over-Barrier Model of Bohr.     

Single-and-double electron loss of O2+ in collisions with argon and helium

This paper reports that the ratios of double to single electron loss cross-section （R） of O^2＋ in collision with Ar and He at the velocity of 1 -4 vo（vo is the Bohr velocity） have been obtained by the coincidence technique. The trend of R - V in the experiment indicates that the effective charge varies with injected velocity. The effective charge can be obtained by the n-body classical trajectory Monte Carlo method, which is interpreted by the molecular Coulomb over barrier model.     

Transfer ionization cross-sections measured in collisions of highly charged argon ions with neon target

: Multiple electron transfer processes are studied for Arq+n- Ne (q= 8, 9, 11, 12) collisions by using multi-parameter coincidence techniques. Various electron transfer processes are identified experimentally and the related cross-sections are measured. The dependence of transfer ionization cross-sections on the recoil charge states is compared with the results from the modified molecular classical overbarrier model. It is found that the modified model described the experimental results reasonably.     

氧离子与氦、氖原子碰撞中转移电离过程的研究

采用位置灵敏探测和散射离子-反冲离子飞行时间测量技术,测量了氧离子与氖和氦原子碰撞过程中转移电离截面与单电子俘获截面之比.通过比较发现测量结果与文献结果的趋势一致,并对测量结果进行了讨论.     

Application of multiquantum ionization to measuring the ionization potentials of atoms and molecules of substances in the gas phase

A technique for measuring the ionization potentials of atoms and molecules is suggested which is distinguished by its accuracy and simplicity. N. E. Zhukovskii Air Force Engineering Academy, 40, Leningradskii Ave., Moscow, 125167, Russia. Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 64, No. 6, pp. 842–844, November–December, 1997.     

Multiple ionization of atoms and the energy of recoil ions in collisions with fast,multiply charged ions

On the basis of the sudden perturbation approximation and the model of independent electrons, simple analytical expressions are obtained for the cross sections of multiple ionization of atoms and the average energies of recoil ions in collisions between atoms and fast, multiply charged ions in the range of parameters in which the Born approximation is inapplicable. An expression for the energy distribution function of recoil ions is also obtained.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 4, pp. 111–116, April, 1996.     

中高能入射条件下裸碳离子碰撞氦原子单电离的全微分截面(英文)

利用四体模型计算了100和2MeV/amu裸碳单电离氦原子的全微分截面,其结果与实验数据和其它理论进行了比较.对于高能入射情况,在散射平面小动量转移和中间动量转移时现在的理论结果和实验符合的很好,然而在大动量转移时和在垂直平面有明显差异.对于低能入射情况,四体结果定性与实验结果一致,而且优于三体扭曲波(3DW-EIS)结果,表明四体效应在低能入射比在高能入射时明显.     

中高能入射条件下裸碳离子碰撞氦原子单电离的全微分截面

利用四体模型计算了100 和 2 MeV/amu裸碳单电离氦原子的全微分截面,其结果与实验数据和其它理论进行了比较。对于高能入射情况,在散射平面小动量转移和中间动量转移时现在的理论结果和实验符合的很好,然而在大动量转移时和在垂直平面有明显差异。对于低能入射情况,四体结果定性与实验结果一致,而且优于三体扭曲波(3DW-EIS)结果,表明四体效应在低能入射比在高能入射时明显。     

Fragmentation of fast positive and negative C ions in collisions with rare gas atoms

The fragmentation of anions and cations resulting from 50 keV collisions with rare gas targets is studied. Positive ion fragment patterns are recorded, and dramatic changes in these patterns are observed as a function of target atom number. The fragment pattern dependence on the target atom size is investigated within a simple model, normally used for stopping power calculations. Fair agreement is obtained between calculated and experimental spectra. From these comparisons we conclude that the range of the screened atomic potentials, as e.g., the Thomas-Fermi potential, is an essential parameter in the collisional induced fragmentation process. Received: 13 February 1998 / Revised: 27 October 1998 / Accepted: 29 October 1998     

Measurement of the spin-exchange and chemical ionization rate constants in collisions of polarized metastable 23 S 1 helium atoms with 32 S 1/2 sodium atoms

Experimental data on the spin-exchange rate constants for the He(2³ S ₁)-Na(3² S _1/2) system are reported for the first time. Measurements show that the spin-exchange rate constant is C _se = (23 ± 11) × 10⁻¹⁰ cm³ s⁻¹ and the chemical ionization rate constant is C _si = (29 ± 14) × 10⁻¹⁰ cm³ s⁻¹ at a temperature of 420 K. The results are compared with the data calculated from the rate constants.     

Tracks of He and S ions with different energies in the PM-355 SSNTDs. Scanning electron microscopy investigations

The Solid State Nuclear Track Detectors PM-355 type were irradiated with helium and sulphur ions with different energies. To develop ion tracks the PM-355 detectors have been chemically etched under the standard conditions. Scanning electron microscopy (SEM) technique was used for observation of surfaces and fractures for determination of diameter and depth of the developed tracks. Shapes of the tracks induced by the projectiles are also presented.     

The effect of negative ions on the dust acoustic wave in dusty electronegative plasma with positively charged dust grains

The effect of negative ions on the modulational instability properties of nonlinear dust acoustic (DA) waves in the electronegative dusty plasmas was investigated by considering Boltzmann-distributed electrons, negative ions, positive ions as well as positively charged dust grain under the ultraviolet irradiation. It is shown that the modulational instability properties of the DA waves were strongly affected by the temperature and proportion of negative ions. The modulational instability can occur only if the proportion of negative ions was smaller than critical value. The instability growth rate has a maximum value when the proportion of negative ions was a critical one in the unstable region. The effect of photoelectron generated by ultraviolet irradiation on the modulational instability of dust acoustic waves was also discussed by numerical method.     

强激光场中长程势与短程势原子产生高次谐波与电离特性研究

用数值方法求解含时薛定谔方程，研究了具有长程势和短程势的一维原子在强激光场中的高次谐波和电离特性. 在强激光场中，长程势和短程势原子产生的高次谐波具有相似的特性，对应的平台和截止位置相同，但是短程势原子没有低阶的高次谐波，而长程势和短程势原子在激光场中的电离概率明显不同. 研究结果表明，原子的激发态结构对低阶的高次谐波和原子的电离概率有重要影响. 关键词： 强激光场 高次谐波 电离概率     

The multiphoton ionization rate and the energy shift of atoms interacting with weak dichromatic fields with commensurate frequencies are simple functions of the phase difference

By implementing a time-independent, nonperturbative many-electron, many-photon theory (MEMPT), cycle-averaged complex eigenvalues were obtained for the He atom, whose real part gives the field-induced energy shift, Δ(ω ₁, F ₁;ω ₂, F ₂,ϕ), and the imaginary part is the multiphoton ionization rate, Γ(ω ₁, F ₁;ω ₂, F ₂,ϕ), where ω is the frequency, F is the field strength and ϕ is the phase difference. Through analysis and computation we show that, provided the intensities are weak, the dependence of Γ(ω ₁, F ₁;ω ₂, F ₂,ϕ) on ϕ is simple. Specifically, for odd harmonics, Γ varies linearly with cos(ϕ) whilst for even harmonics it varies linearly with cos(2ϕ). In addition, this dependence on ϕ holds for Δ(ω ₁, F ₁;ω ₂, F ₂,ϕ) as well. These relations may turn out to be applicable to other atomic systems as well, and to provide a definition of the weak field regime in the dichromatic case. When the combination of (ω ₁, F ₁) and (ω ₂, F ₂) is such that higher powers of cos(ϕ) and cos(2ϕ) become important, these rules break down and we reach the strong field regime. The herein reported results refer to Γ(ω ₁, F ₁;ω ₂, F ₂,ϕ) and Δ(ω ₁, F ₁;ω ₂, F ₂,ϕ) for He irradiated by a dichromatic ac-field consisting of the fundamental wavelength λ = 248 nm and its 2nd, 3rd and 4th higher harmonics. The intensities are in the range 1.0×10¹²-3.5×10¹⁴ W/cm², with the intensity of the harmonics being 1-2 orders of magnitude smaller. The calculations incorporated systematically electronic structure and electron correlation effects in the discrete and in the continuous spectrum, for ¹S, ¹P, ¹D, ¹F, ¹G, and ¹H two-electron states of even and odd parity. Received 9 July 2000 and Received in final form 2 November 2000     

电子回旋共振放电的电离特性PIC/MCC模拟(Ⅰ)——物理模型与理论方法

采用粒子模拟与蒙特卡罗相结合(PIC/MCC)的方法对电子回旋共振(ECR)放电中的电离过程进行了模拟，其中带电粒子与微波的相互作用由PIC方法的电磁模型描述，粒子间的碰撞过程由MCC方法描述.考虑的碰撞类型有电子与中性粒子的弹性、激发、电离碰撞，离子与中性粒子的弹性、电荷交换碰撞，碰撞截面均依赖于能量而变化.阐述了理论分析的过程，为数值模拟ECR放电奠定了基础. 关键词： 电子回旋共振放电 粒子模拟 蒙特卡罗 电离