MEND——-—个计算250 MeV以下中重核数据的程序(英文)

基于球型光学模型、 预平衡发射和Hauser Feshbach统计等理论, 编制了MEND程序（Medium Energy Nuclear Data）, 该程序适用于中重原子核在入射粒子能量低于250 MeV的中低能区的全套核数据计算。对于中子和质子在250 MeV以下诱发的核反应, 其全截面、 反应截面、 弹性散射微分截面、 双微分截面和能谱等理论计算值与相应的实验值基本一致。MEND是计算中低能核反应的基础程序, 在我国已被广泛用于核数据计算及建立中能核数据库Based on the spherical optical model, pre equilibrium statistical theory, and Hauser Feshbach theory, etc., the code MEND (Medium Energy Nuclear Data) is written for calculating the complete set of nuclear data of medium heavy nuclei in medium low energy region (≤250 MeV). For the reactions induced by neutron and proton below 250 MeV, the total cross sections, reaction cross sections, elastic scattering differential cross sections, double differential cross sections and energy spectra, etc. calculated by the code MEND, generally agree with those corresponding experimental data. MEND is a foundational program for nuclear reaction in medium low energy region and is wildely used for nuclear data calculation and establishing ENDF/B6 format files of medium low energy region in China.     

Mass dependence of pion-induced fission cross sections on the level density parameter

Fission probabilities and fission cross sections strongly depend on the mass number of the target and energy of the projectile. In this research work, a cascade-exciton model (using CEM95 computer code) has been implemented to observe the dependence of pion-induced fission cross sections and fission probabilities on the target mass and ratio of the level density parameter in fission to neutron emission. The analysis has been performed for both the positive and negative pions as the projectile at 80, 100 and 150 MeV energies. The computed cross sections satisfactorily reproduced the experimental findings when compared with the available experimental data in the literature. We observed a smooth dependence at 150 MeV, and a sharper dependence at 80 and 100 MeV pion energy, in the fissility region above 29.44.     

Cascade-exciton model analysis of level density parameter dependence in proton induced fission cross sections of some sub-actinide nuclei

Fission cross sections strongly depend on the ratio of the level density parameter in fission to neutron emission, a_f/a_n. In this work, a cascade-exciton model implemented in the code CEM95 has been used to observe this effect for proton induced fission cross sections of tungsten, lead and bismuth. The method was employed using different level density parameter ratios for each fission cross section calculation. The calculated fission cross sections are compared with the available experimental data in the literature. It has been observed that a change of the ratio of the level density parameter, a_f/a_n, is necessary with the incident energy of the proton, to best estimate the fission cross sections in CEM95.     

Calculation of prompt fission neutron spectrum for 233U（n,f）reaction by the semi-empirical method~

The prompt fission neutron spectra for the neutron-induced fission of ²³³U for low energy neutrons (below 6 MeV) are calculated using nuclear evaporation theory with a semi-empirical method, in which the partition of the total excitation energy between the fission fragments for the n_th+²³³U fission reactions is determined by the available experimental and evaluation data. The calculated prompt fission neutron spectra agree well with the experimental data. The proportions of high-energy neutrons of prompt fission neutron spectrum versus incident neutron energies are investigated with the theoretical spectra, and the results are consistent with the systematics. The semi-empirical method could be a useful tool for the prompt evaluation of fission neutron spectra.     

Analysis of Neutron Double-Differential Cross Sections for n ＋ ^12 C Reaction Below 30 MeV

Based on the light nucleus reaction model （Nucl. Sci. Eng. 133 （1999） 218）, four aspects （neutron incident energy region, reaction channel analysis, the renewed level schemes and the optical model parameters） of n＋ ^12 C reaction are improved to calculate total outgoing neutron double-dilferential cross sections with modified LUNF code below 30 MeV. The calculated results agree fairly well with the experimental data at En = 14.1 MeV and 18 MeV. The analysis shows that the pre-equilibrium mechanism, which is exactly considered the conservation of energy, momentum and parity, dominates the whole reaction process. The contribution of the neutron emission from 5He to total energy- angular spectra is also considered properly. This modified LUNF code will be a useful tool to set up the file of neutron double-differential crass sections below 30 Me V in the neutron evaluation nuclear data library.     

Calculation of prompt fission neutron spectrum for 233U（n,f） reaction by the semi-empirical method

The prompt fission neutron spectra for the neutron-induced fission of 233U for low energy neutrons （below 6 MeV） are calculated using nuclear evaporation theory with a semi-empirical method, in which the partition of the total excitation energy between the fission fragments for the nth＋233U fission reactions is determined by the available experimental and evaluation data. The calculated prompt fission neutron spectra agree well with the experimental data. The proportions of high-energy neutrons of prompt fission neutron spectrum versus incident neutron energies are investigated with the theoretical spectra, and the results are consistent with the systematics. The semi-empirical method could be a useful tool for the prompt evaluation of fission neutron spectra.     

Research on the prompt neutron multiplicity of fission fragments for 235U（n,f）

According to some experimental and evaluated data,the total excitation energy partitioning way between both of the fission fragments was given with a semi-empirical method. With the calculated energy partitioning way,the prompt neutron multiplicity as a function of fragment mass,（A） ,for neutron-induced fission of 235U at En=0.0253 eV,3 MeV,and 5 MeV was calculated. The results are checked with the total average prompt neutron multiplicities  and compared with the experimental and evaluated data.     

Systematical law of (n, γ) reaction cross sections of even-even nuclei

We have derived a formula for the neutron radiative capture cross section in the framework of a statistical model approach to nuclear reactions. Based on this formula, new systematics are established between the (n, γ) reaction cross section and the energy level density of a compound nucleus or a relative neutron excess of an even-even target nucleus for neutron incident energy above the resonance region to MeV. Good agreement with experimental data suggests that this new systematical law is helpful to analyze the experimental data.     

Multi-modal analysis for low energy neutron-induced fission of 235U

Low energy neutron induced fission of 235U is studied in the framework of the multi-modal fission model. The fission fragment properties, such as the yields, the average total kinetic energy distribution and the average neutron separation energy, are investigated for incident neutron energies from thermal to 6.0 MeV. The multi-modal fission approach is also used to evaluate the prompt fission neutron multiplicity and spectra for the neutron-induced fission of 235U with an improved version of the Los Alamos model for incident neutrons below the （n, nf） threshold. The three most dominant fission modes are taken into account. The model parameters are determined on the basis of experimental data. The calculated results are in good agreement with the experimental data.     

Calculation of prompt fission neutron spectra for 235U(n,f)

The prompt fission neutron spectra for the neutron-induced fission of ²³⁵U at E_n < 5 MeV are calculated using nuclear evaporation theory with a semi-empirical model, in which the nonconstant and constant temperatures related to the Fermi gas model are taken into account. The calculated prompt fission neutron spectra reproduce the experimental data well. For the n(thermal)+²³⁵U reaction, the average nuclear temperature of the fission fragment, and the probability distribution of the nuclear temperature, are discussed and compared with the Los Alamos model. The energy carried away by γ rays emitted from each fragment is also obtained and the results are in good agreement with the existing experimental data.     

Further Analysis of Neutron Double-Differential Cross Section of n ＋ ^16O at 14.1 MeV and 18 MeV

By using a new reaction model for light nuclei, the double-differential cross section of total outgoing neutron with LUNF code for n＋^16O reactions at En=14.1 MeV and 18 MeV have been calculated and analyzed. In this paper the opened reaction channels, which have contribution to emitting the neutrons, are listed in detail. To improve the fitting results the direct inelastic scattering mechanism is involved. The calculating results agree fairly well with the experimental data at E,~ = 14.1 MeV and the deviation from calculated results and experimental data in low energy region at En= 18 MeV has been analyzed. Since the possibility of 5He has been affirmed theoretically [J.S. Zhang, Sci. Chin. G 47 （2004） 137], so 5He emission from n＋ ^16O reaction is taken into account, which plays an important role at the region of the outgoing neutron energy εn〈3 MeV in total outgoing neutron energy-angular spectrum. The calculated results indicate that the pre-equilibrium mechanism dominates the whole reaction processes, and the recoil effect in light nuclear reactions is essentially important.     

Measurement of(n,α)and(n,2n)reaction cross sections at a neutron energy of 14.92±0.02 MeV for potassium and copper with uncertainty propagation

Experimentally measured neutron activation cross sections are presented for the ⁶⁵Cu(n,0)^62mCu,⁴¹ K(n,a)^38Cl,and ⁶⁵Cu(n.2n)⁶⁴Cu reactions with detailed uncertainty propagation.The neutron cross secions were measured at an incident energy of 14.92±0.02 MeV,and the neutrons were based on the(d,n)a fusion reaction.The ²⁷ Al(n,a)²⁴Na reaction was used as a reference reaction for the normalization of the neutron flux.The pre-calib-rated lead-shielded HPGe detector was used to detect the residues'γ-ray spetra.The data from the measured cross sections are compared to the previously measured cross sections from the EXFOR database,theoretically calculated cross sections using the TALYS and EMPIRE codes,and evaluated nuclear data.     

高激发核相继裂变的限制

高温核衰变是当前中能重离子核物理中研究最热烈的课题.理论上对高温核的衰变进行了各种预言,相继裂变就是其中之一.本文从有关核裂变的时间尺度、裂前中子发射、裂变截面等随激发能的变化和多重碎裂的实验结果以及复杂碎片发射时间的实验结果分析了对高温核相继裂变的限制,提出了从复杂粒子蒸发向多重碎裂过渡的可能性. Sequential fission is one of the several kinds of theoratical production for hot nucleus de-cay.By analysing relevant experimental results such as fission time scale,prescission neutron emission,fission cross sections and their variation with excitation energy,the results of multifragmentation andthe time scale of complex fragment emission,a limit to the sequential fission of the hot nucleus is sug-gested in this paper.A transition from intermediate mass fragment evaporation to..     

Dependence of Nucleon and Pion-Induced Fission Cross Sections on the Level Density Parameter in the Cascade-Exciton Model

A new method is used to compute the fission cross sections in which a change of the ratio of the level density parameter in fission to neutron emission channels is taken into account with the change of the incident energy of the projectile. It is shown that fission cross sections induced by nucleons and pions depend on the ratio of the level density parameter in the fission and evaporation modes, i,e. af /an, respectively. We are unable to describe well the cross sections for fission without using this new method. The computed values exhibit reasonable agreement with the experimental data found in the literature across a wide range of beam energies.     

中子源有源法核查技术研究

用有源 (主动 )方法研究了贫化铀组合系统的中子诱发裂变缓发中子探测技术 .在不同屏蔽和组合等条件下测量和比较了贫化铀系统的缓发裂变中子分布 ,进一步研究了实验系统的可核查性 .探讨了区分核与非核系统的方法. The technique for detecting the delayed neutrons from neutron induced fission in uranium systems was studied by using an active method with 3He proportional counting tube array and a 14 MeV D T neutron source. Under the conditions of different shielding and combination, the distributions of delayed fission neutrons from depleted uranium systems were measured and the reliability of the systems was studied. The method to distinguish a nuclear system from a non nuclear one was discussed.     

LS301快中子探测器的效率刻度

主要介绍了利用252Cf标准裂变中子能谱刻度快脉冲LS301型液闪中子探测器的探测效率的实验方法和结果, 简要介绍了实验数据的处理过程, 得到了阈值分别为0.5, 0.7, 1.0和1.6 MeV, 以及中子能量在10 MeV以下的探测器效率, 并对测量结果进行了误差分析。同时为了检验实验结果的准确性, 将实验结果与理论计算结果进行比较, 两者在不确定度范围内符合得很好。Neutron detection efficiency of LS301 fast neutron detector was calibrated by measuring the neutron energy spectrum of 252Cf source, which has a standard fission neutron spectrum. A low mass, fast ionization chamber is used as the fission fragments detector in the time of flight(TOF) spectrometer and afforded the start signal of neutron flight. The stop signal was offered by the anode of LS301. A measured TOF spectrum was turned to the neutron energy spectrum which will be compared with the standard one. Consequently, the fast neutron detection efficiency of LS301 was obtained. Calibration procedures of experimental and data processing was given. Relative detection efficiencies were obtained separately for threshold settings of 0.5, 0.7, 1.0 and 1.6 MeV for neutron energies under 10 MeV. Experimental results accorded with theoretical efficiency curves which were calculated with the Monte Carlo code NEFF50.     

超重核合成的同位素依赖探讨

利用二参量Smoluchowski方程计算了54Fe+204Pb,56Fe+206Pb,58Fe+208Pb冷熔合和32,34,36S+238U热熔合的复合核形成截面和蒸发残余截面, 结果清楚地显示出超重核合成截面随同位素的变化。 由于较低的入射道库仑位垒、 较低的不对称裂变谷中的条件鞍点和较小的中子分离能, 一般地说, 丰中子同位素的超重核形成截面明显增强。 The cross sections of the compound nucleus formation and e vaporation residue for the 54Fe+204Pb, 56Fe+206Pb, 58Fe+208Pb cold fusion and 32,34, 36S+238U hot fusion have been calculated by using a two parameter Smoluchowski equation. Our results clearly show the isotope dependence of superheavy nucleus production. The formation cross sections of the neutron rich isotope are, generally speaking, obviously enhanced due to the lower Coloumb barrier , lower height of the conditional saddle point, and smaller neutron separation energy.     

基于ImIQMD模型对近垒重系统准裂变反应的研究

利用改进的同位旋相关的量子分子动力学(ImIQMD)模型程序,对能量在库仑位垒附近的48Ca+208Pb反应系统进行了模拟。 计算得到的俘获截面、 准裂变截面和碎片分布及其发生的时间分布等结果与实验数据符合较好。 同时还得到了准裂变过程中发射第三个较大碎片的截面, 并简单讨论了它们的发射机制。Based on the improved isospin dependent quantum molecular dynamics (ImIQMD) model,the reaction of 48Ca+208Pb at energies near the Coulomb barrier was investigated systematically. The capture cross section,the quasi fission cross section, the mass distribution of the quasi fission fragments and the time for quasi fission happened were obtained. According to the comparison with experimental data,the calculated capture cross sections and the fragment distributions of the quasi fission were reasonable. Additionally,we got the cross sections of the third largest fragment,and the emission mechanism was also discussed briefly.     

2.8MeV中子诱发238U裂变的瞬发中子谱高能段实验测量

在中国原子能科学研究院的高压倍加器上利用中子飞行时间方法测量了2.8 MeV中子引起238U裂变的瞬发中子能谱,通过增大样品量和设计合适的屏蔽体提高了效应/本底比,使得测量数据的不确定度满足预期目标（在5.5～14 MeV能区内,能量间隔为0.5 MeV条件下能谱的不确定度小于10%）。将实验几何、中子源能量分布及角分布、探测效率、束流的时间结构等实验条件输入到MCNP程序里,模拟了出射的中子谱,模拟结果与测量结果在不确定度范围内一致,验证了在入射中子能量较低时238>U的裂变瞬发中子谱评价数据的可靠性。The Prompt Fission Neutron Spectrum (PFNS) of 238U induced by 2.8 MeV neutron was measured using the Cockcroft-Walton accelerator in China Institute of Atomic Energy (CIAE). The signal/background ratio was improved by increasing the amount of sample mass and using an appropriate shielding system. The final uncertainty of neutron energy spectrum in 5.5～14 MeV region is less than 10% with a bin size of 0.5 MeV which has reached this project's anticipation. The experimental geometry, the angular distribution and energy distribution of neutron source, the detection efficiency and time structure of deuteron beam were inputted into the MCNP code to simulate the outgoing neutron spectrum. The simulated results agree with the experimental ones within the uncertainty. The result indicates that the evaluated PFNS for 238U at low neutron energy is reliable.     

用中子晕弹核探寻同位旋非对称核物质状态方程

总结和评述了用中子晕弹核探寻同位旋非对称核物质状态方程。 在具有同位旋和动量依赖的同位旋相关量子分子动力学框架内, 采用对比中子晕弹核和相等质量稳定弹核在完全相同入射道条件下物理观测量的差别, 来突出中子晕核明显的同位旋效应和加强物理观测量对于同位旋的灵敏性, 从而提取核物质状态方程。 例如, 与稳定弹核碰撞系统相比, 中子晕弹核明显提高了发射核子的中子\|质子比和增加了它对于对称势的灵敏性, 这两点特征非常有利于提取对称势。 同样, 由于中子晕弹核碰撞系统在低能区（E<60 MeV）由于内部松散结构减弱了核子碰撞力度和动量耗散, 与稳定核碰撞系统相比, 明显提高了原子核阻止; 而在高能区由于两体碰撞同位旋效应的增加, 从而明显提高了原子核阻止。 利用这些特征可以提取核子\|核子碰撞截面的介质效应和同位旋依赖性。 Based on the isospin and momentum dependent quantum molecular dynamics, we use the comparison for the differences between observables in the reactions induced by the halo\|neutron projectile and stable projectile with the same mass under complete same incident channel condition to protrude the isospin effect of halo\|neutron projectile and strengthen the sensitivity of observable on the isospin for extracting the information for the equation of state. For example, the halo\|neutron projectile increases the emitted neutron\|proton ratio and then enhances its sensitivity on the symmetrical potential. Two points above are more favorable than the normal neutron\|rich and neutron\|poor projectiles for extracting the symmetry potential. We also found that the neutron\|halo projectile induces the decrease of nuclear stopping in lower beam energy region and the increase in higher beam energy region, compared to corresponding same mass stable projectile under the same incident channel condition, so that we can use these properties to extract the information for the medium effect and isospin effect of in\|medium nucleon\|nucleon cross section.