Ac-cotunneling through an interacting quantum dot in a magnetic field

We analyze inelastic cotunneling through an interacting quantum dot subject to an ambient magnetic field in the weak tunneling regime under a non-adiabatic time-dependent bias-voltage. Our results clearly exhibit photon-assisted satellites and an overall suppression of differential conductance with increasing driving amplitude, which is consistent with experiments. We also predict a zero-anomaly in differential conductance under an appropriate driving frequency.     

Cotunneling current through a two-level quantum dot coupled to magnetic leads: the role of exchange interaction

The cotunneling current through a two-level quantum dot weakly coupled to ferromagnetic leads is studied in the Coulomb blockade regime. The cotunneling current is calculated analytically under simple but realistic assumptions as follows: (i)?the quantum dot is described by the universal Hamiltonian, (ii)?it is doubly occupied, and (iii)?it displays a fast spin relaxation. We find that the dependence of the differential conductance on the bias voltage is significantly affected by the exchange interaction on the quantum dot. In particular, for antiparallel magnetic configurations in the leads, the exchange interaction results in the appearance of interference-type contributions from the inelastic processes to the cotunneling current. Such dependence of the cotunneling current on the tunneling amplitude phases should also occur in multi-level quantum dots weakly coupled to ferromagnetic leads near the mesoscopic Stoner instabilities.     

Cotunneling through a quantum dot coupled to ferromagnetic leads with noncollinear magnetizations

Spin-dependent electronic transport through a quantum dot has been analyzed theoretically in the cotunneling regime by means of the second-order perturbation theory. The system is described by the impurity Anderson Hamiltonian with arbitrary Coulomb correlation parameter U. It is assumed that the dot level is intrinsically spin-split due to an effective molecular field exerted by a magnetic substrate. The dot is coupled to two ferromagnetic leads whose magnetic moments are noncollinear. The angular dependence of electric current, tunnel magnetoresistance, and differential conductance are presented and discussed. The evolution of a cotunneling gap with the angle between magnetic moments and with the splitting of the dot level is also demonstrated.     

Mesoscopic fluctuations of tunneling and cotunneling in quantum dots

Recent measurements of mesoscopic tunneling and cotunneling fluctuations in Coulomb blockaded ballistic quantum dots are presented. The statistics and parametric fluctuations (as a function of magnetic field) of Coulomb blockade peak heights are found to be consistent with random-matrix-theory predictions. Mesoscopic fluctuations of elastic cotunneling, measured in the valleys between blockade peaks, are also presented along with a semiclassical explanation of the observed enhancement of the magnetic field scale of cotunneling fluctuations compared to resonant tunneling fluctuations.     

Electronic transport spectroscopy of carbon nanotubes in a magnetic field

We report magnetic field spectroscopy measurements in carbon nanotube quantum dots exhibiting fourfold shell structure in the energy level spectrum. The magnetic field induces a large splitting between the two orbital states of each shell, demonstrating their opposite magnetic moment and determining transitions in the spin and orbital configuration of the quantum dot ground state. We use inelastic cotunneling spectroscopy to accurately resolve the spin and orbital contributions to the magnetic moment. A small coupling is found between orbitals with opposite magnetic moment leading to anticrossing behavior at zero field.     

Interplay of magneto-elastic and polaronic effects in electronic transport through suspended carbon-nanotube quantum dots

We investigate the electronic transport through a suspended carbon-nanotube quantum dot. In the presence of a magnetic field perpendicular to the nanotube and a nearby metallic gate, two forces act on the electrons: the Laplace and the electrostatic force. They both induce coupling between the electrons and the mechanical transverse oscillation modes. We find that the difference between the two mechanisms appears in the cotunneling current.     

Coherent probing of excited quantum dot states in an interferometer

Measurements of elastic and inelastic cotunneling currents are presented on a two-terminal Aharonov-Bohm interferometer with a Coulomb-blockaded quantum dot embedded in each arm. Coherent current contributions, even in a magnetic field, are found in the nonlinear regime of inelastic cotunneling at a finite-bias voltage. The phase of the Aharonov-Bohm oscillations in the current exhibits phase jumps of pi at the onsets of inelastic processes. We suggest that additional coherent elastic processes occur via the excited state. Our measurement technique allows the detection of such processes on a background of other inelastic current contributions and contains qualitative information about the ratio of transport and inelastic relaxation rates.     

Use of quantum dots as a switch for single-electron transfer free from cotunneling

Based on symmetry constraint that leads to the appearance of nodes in the wave functions of 3-electron systems at regular triangle configurations, it was found that, if the parameters of confinement are skillfully chosen and if a magnetic field is tuned around the first critical point of the single-triplet transition, a 2-electron quantum dot can be used as a switch for single-electron transport free from cotunneling.     

Measurements of Kondo and spin splitting in single-electron transistors

We measure the spin splitting in a magnetic field B of localized states in single-electron transistors using a new method, inelastic spin-flip cotunneling. Because it involves only internal excitations, this technique gives the most precise value of the Zeeman energy Delta=/g/mu(B)B. In the same devices we also measure the splitting with B of the Kondo peak in differential conductance. The Kondo splitting appears only above a threshold field as predicted by theory. However, the magnitude of the Kondo splitting at high fields exceeds 2/g/mu(B)B in disagreement with theory.     

Magnetic-field dependence of tunnel couplings in carbon nanotube quantum dots

By means of sequential and cotunneling spectroscopy, we study the tunnel couplings between metallic leads and individual levels in a carbon nanotube quantum dot. The levels are ordered in shells consisting of two doublets with strong- and weak-tunnel couplings, leading to gate-dependent level renormalization. By comparison to a one- and two-shell model, this is shown to be a consequence of disorder-induced valley mixing in the nanotube. Moreover, a parallel magnetic field is shown to reduce this mixing and thus suppress the effects of tunnel renormalization.     

Cotunneling spectroscopy in few-electron quantum dots

Few-electron quantum dots are investigated in the regime of strong tunneling to the leads. Inelastic cotunneling is used to measure the two-electron singlet-triplet splitting above and below a magnetic field driven singlet-triplet transition. Evidence for a nonequilibrium two-electron singlet-triplet Kondo effect is presented. Cotunneling allows orbital correlations and parameters characterizing entanglement of the two-electron singlet ground state to be extracted from dc transport.     

Nonequilibrium transport through a spinful quantum dot with superconducting leads

We study the nonlinear cotunneling current through a spinful quantum dot contacted by two superconducting leads. Applying a general nonequilibrium Green function formalism to an effective Kondo model, we study the rich variation in the IV characteristics with varying asymmetry in the tunnel coupling to source and drain electrodes. The current is found to be carried, respectively, by multiple Andreev reflections in the symmetric limit, and by spin-induced Yu-Shiba-Rusinov bound states in the strongly asymmetric limit. The interplay between these two mechanisms leads to qualitatively different IV characteristics in the crossover regime of intermediate symmetry, consistent with recent experimental observations of negative differential conductance and repositioned conductance peaks in subgap cotunneling spectroscopy.     

Josephson current in carbon nanotubes with spin-orbit interaction

We demonstrate that curvature-induced spin-orbit coupling induces a 0-π transition in the Josephson current through a carbon nanotube quantum dot coupled to superconducting leads. In the noninteracting regime, the transition can be tuned by applying a parallel magnetic field near the critical field where orbital states become degenerate. Moreover, the interplay between charging and spin-orbit effects in the Coulomb blockade and cotunneling regimes leads to a rich phase diagram with well-defined (analytical) boundaries in parameter space. Finally, the 0 phase always prevails in the Kondo regime. Our calculations are relevant in view of recent experimental advances in transport through ultraclean carbon nanotubes.     

A study of the ultrafast optical response of magnetized GaAs/AlGaAs quantum wire structures

We have studied analytically the ultrafast optical response of GaAs/AlGaAs quantum wire subjected to a moderately strong transverse magnetic field. The energy dispersion relations have been numerically calculated and show a significant deviation from parabolic behaviour as the magnetic field is increased. The effective semiconductor Bloch equation technique is used to calculate the induced polarization and differential transmission spectra in the quantum wire. The calculated induced polarization is used to study the optical coherent transient phenomenon of optical nutation. The analysis demonstrates that the magnetic field effectively alters the optical response of the semiconductor quantum wire nanostructures. It is observed that the nutating signal frequency enhances with an increasing magnetic field. The results are useful to explain magnetic field effects on the transient optical properties of semiconductor nanostructures.     

Magnetic Field Effects on Quantum-Dot Spin Valves

We study the magnetic field effects on the spin-polarized transport of the quantum dot (QD) spin valve in the sequential tunneling regime. A set of generalized master equation is derived. Based on that, we discuss the collinear and noncollinear magnetic field effects, respectively. In the collinear magnetic field case,we find that the Zeeman splitting can induce a negative differential conductance (NDC), which is quite different from the one found in previous studies. It has a critical polarization in the parallel arrangement and will disappear in the antiparallelconfiguration. In the noncollinear magnetic field case, the current shows two plateaus and their angular dependence is analyzed. Although sometimes the two current plateaus have similar angular dependence, their mechanisms are different. Our formalism is also suitable for calculating the transport in magnetic molecules, in which the spin splitting is induced not by a magnetic field but by the intrinsic magnetization.     

Cotunneling current and shot noise in quantum dots

We derive general expressions for the current and the shot noise, taking into account non-Markovian memory effects. In generalization of previous approaches, our theory is valid for an arbitrary Coulomb interaction and coupling strength and is applicable to quantum dots and more complex systems such as molecules. A fully consistent diagrammatic expansion up to second order in the coupling strength, taking into account cotunneling processes, allows for a study of transport in an intermediate coupling strength regime relevant to many current experiments. We discuss a single-level quantum dot as a first example, focusing on the Coulomb-blockade regime where the cotunneling processes dominate. We find super-Poissonian shot noise due to inelastic spin-flip cotunneling processes at an energy scale different from the one expected from first-order calculations.     

Violation of the Wiedemann-Franz law in a single-electron transistor

We study the influence of Coulomb interaction on the thermoelectric transport coefficients for a metallic single-electron transistor. By performing a perturbation expansion up to second order in the tunnel-barrier conductance, we include sequential and cotunneling processes as well as quantum fluctuations that renormalize the charging energy and the tunnel conductance. We find that Coulomb interaction leads to a strong violation of the Wiedemann-Franz law: the Lorenz ratio becomes gate-voltage dependent for sequential tunneling, and is increased by a factor 9/5 in the cotunneling regime. Finally, we suggest a measurement scheme for an experimental realization.     

Cotunneling-mediated transport through excited states in the Coulomb-blockade regime

We present finite-bias transport measurements on a few-electron quantum dot. In the Coulomb-blockade regime, strong signatures of inelastic cotunneling occur which can directly be assigned to excited states observed in the nonblockaded regime. In addition, we observe structures related to sequential tunneling through the dot, occurring after it has been excited by an inelastic cotunneling process. We explain our findings using transport calculations within the real-time Green's function approach, including diagrams up to fourth order in the tunneling matrix elements.     

Double-dot charge qubit and transport via dissipative cotunneling

We investigate transport through an exotic charge qubit composed of two strongly capacitively coupled quantum dots, each being independently connected to a side gate which in general exhibits a fluctuating electrostatic field (i.e., Johnson-Nyquist noise). Two quantum phases are found: the "Kondo" phase where an orbital-Kondo entanglement emerges and a "local moment" phase in which the noise destroys the Kondo effect leaving the orbital spin unscreened and resulting in a clear suppression of the conductance. In the Kondo realm, the transfer of charge across the setting is accompanied by zero-point charge fluctuations in the two dissipative environments and then the I-V characteristics are governed by what we call "dissipative cotunneling."