Fiber-laser-based green-pumped continuous-wave singly-resonant optical parametric oscillator

Stable, high-power, second-harmonic-generation (SHG) of a compact CW Ytterbium (Yb) fiber laser at 1064 nm into the green and its use as a pump source for CW singly-resonant optical parametric oscillator (SRO) is demonstrated. Using a simple single-pass SHG configuration in MgO:sPPLT, as much as 9.6 W of single-frequency green radiation at 532 nm is generated from 30 W of fundamental power at a conversion efficiency of 32.7% in a Gaussian spatial profile with a beam quality factor of M ² < 1.3. Thermal effects have been investigated at different fundamental power levels and various thermal management schemes are employed to maximize the second-harmonic power. The green source is successfully deployed to pump a CW SRO tunable over 855–1408 nm, generating up to 2.1 W of idler at 1168 nm. The peak-to-peak idler power stability is better than 10.7% over 40 min, with beam quality factor M ² < 1.26 for the idler and M ² < 1.52 for the signal.     

Non-collinear nanosecond optical parametric oscillator based on periodically poled LN with tilted domain walls

We report on a non-collinear, 1064 nm pumped, 10 kHz repetition rate ns-OPO which consists of a 13 mm long periodically poled lithium niobate (PPLN) crystal in a hemispherical optical cavity. The non-collinear phase-matching is achieved by tilting the domains by 60° with respect to the pump beam. This phase-matching avoids back conversion of signal and idler radiation into pump radiation and thus improves the spatial quality of the generated OPO radiation considerably. At a pump power of 5.5 W the OPO provided a conversion efficiency of up to 34%. The generated OPO pulses with a total power of up to 1.85 W were emitted in an almost diffraction limited beam with a M²-value of 1.1. The beam quality did not change when the pump power was varied in the range of 2–5 W. PACS 42.65.-k; 42.65.Yj     

High-power mid-infrared tunable optical parametric oscillator based on 3-mm-thick PPMgCLN

The experimental results of a high-power tunable mid-IR laser are presented. The optical parametric oscillator (OPO) with a 3-mm-thick PPMgCLN crystal was pumped by a 1.064 μm pulse laser. When the pump power of the 1.064 μm laser was 151 W at 10 kHz, and the operating temperature of the PPMgCLN with 5% MgO doping was 100°C, average output power of 23.7 W at 3.91 μm was obtained with a slope efficiency of 18.2% for the idler resonant OPO. The variation of the 3.91 μm output power was about ±4% in 10 min continuous operation. The beam quality factor M ² was less than 2.6. The average output power of 27.4 W at 3.91 μm was also obtained with 151 W pump power and the slope efficiency of 20.9% for the signal resonant OPO by changing the coating parameters of the OPO cavity mirrors. The mid-IR wavelength tunability of 3.7–4.0 μm can be achieved by adjusting the temperature of a 29 μm period PPMgCLN crystal from 200 to 30°C.     

Optimally-output-coupled, 17.5 W,fiber-laser-pumped continuous-wave optical parametric oscillator

We present a stable, high-power, fiber-laser-pumped, continuous-wave (cw), singly resonant optical parametric oscillator (SRO) for the mid-infrared in an output-coupled (OC) configuration, providing 17.5 W of total output power at 61% extraction efficiency. Using a single-frequency, cw Yb fiber laser at 1064 nm and a 50-mm-long MgO:PPLN crystal, through optimization of signal output coupling we generate up to 9.8 W of signal power in the near-infrared together with 7.7 W of idler power for 28.6 W of pump, while in the absence of output coupling, 8.6 W of idler power is generated for the same pump power at 30% efficiency. The SRO is tunable over 360 nm in the idler range. The deployment of signal output coupling results in a total tuning of 513 nm (120 nm of signal, 393 nm of idler) over which watt-level output power can be extracted. Through careful control of thermal effects we achieve a long-term peak-to-peak idler power stability of 5% over 14 hours near room temperature. The output beams have TEM₀₀ spatial profile with M ²<1.28 for the idler and M ²<1.37 for the signal.     

High-power,high-quality ZGP OPO pumped by a Tm,Ho:GdVO<Subscript>4</Subscript> laser

We report a ZGP OPO system capable of producing >6 W at a signal wavelength of 3.80 μm and an idler wavelength of 4.45 μm. The pumping source is the Tm,Ho:GdVO₄ laser operated at 2.049 μm with an M ² of 1.07. The ZGP OPO generated a total combined output power of 6.1 W at signal wavelength and idler wavelength under pumping power of 18.3 W, and an M ² of 1.7 for OPO output was obtained.     

Few‐cycle,broadband, mid‐infrared optical parametric oscillator pumped by a 20‐fs Ti:sapphire laser

A few‐cycle, broadband, singly‐resonant optical parametric oscillator (OPO) for the mid‐infrared based on MgO‐doped periodically‐poled LiNbO₃ (MgO:PPLN), synchronously pumped by a 20‐fs Ti:sapphire laser is reported. By using crystal interaction lengths as short as 250 µm, and careful dispersion management of input pump pulses and the OPO resonator, near‐transform‐limited, few‐cycle idler pulses tunable across the mid‐infrared have been generated, with as few as 3.7 optical cycles at 2682 nm. The OPO can be continuously tuned over 2179‐3732 nm (4589‐2680 cm^‐1) by cavity delay tuning, providing up to 33 mW of output power at 3723 nm. The idler spectra exhibit stable broadband profiles with bandwidths spanning over 422 nm (FWHM) recorded at 3732 nm. The effect of crystal length on spectral bandwidth and pulse duration is investigated at a fixed wavelength, confirming near‐transform‐limited idler pulses for all grating interaction lengths. By locking the repetition frequency of the pump laser to a radio‐frequency reference, and without active stabilization of the OPO cavity length, an idler power stability better than 1.6% rms over >2.75 hours is obtained when operating at maximum output power, in excellent spatial beam quality with TEM₀₀ mode profile. Photograph shows a multigrating MgO:PPLN crystal used as a nonlinear gain medium in the few‐cycle femtosecond mid‐IR OPO. The visible light is the result of non‐phase‐matched sum‐frequency mixing between the interacting beams.     

Boosting quantum efficiency using multi-stage parametric amplification

We develop a numerical simulation to demonstrate increased quantum efficiency that can be achieved by using a second stage, phase matched crystal to convert signal energy to the idler wavelength. A pair of ZnGeP₂ crystals with walkoff and pump absorption were simulated leading to a tripling of the idler output energy. The output beam characteristics are close to a Gaussian beam with an M² around 1.1.     

Numerical analysis of the spatial behaviour of nanosecond optical parametric oscillators of beta-barium borate

We report on a numerical analysis of the temporal and spatial beam properties of nanosecond optical parametric oscillators (OPOs). The analysis is performed for a 355-nm-pumped critically phase-matched OPO of beta-barium borate. The calculations provide detailed information on the dependence of the OPO beam quality (measured by the quality factor M ²) on pump energy. An important result is the strong increase of the M ² value for pump energies exceeding 1–2 times the energy at threshold. Furthermore, a temporal analysis of single OPO pulses indicates that the M ² value strongly increases during the first few nanoseconds of the OPO oscillation. This increase is understood by considering the temporal dynamics of the spatial profiles of the OPO signal beam and the depleted pump radiation. Received: 1 April 1999 / Revised version: 26 July 1999 / Published online: 20 October 1999     

Efficient, single frequency, high repetition rate, PPLN OPO pumped by a prelase Q-switched diode-pumped Nd:YAG laser

Single axial mode operation (<200 MHz optical bandwidth) of a high repetition rate periodically poled lithium niobate optical parametric oscillator (OPO) has been obtained at signal wavelengths between 1.46 μm and 1.64 μm. OPO signal slope efficiencies of 35% have been measured for repetition rates of 5–20 kHz. Single mode operation required spectral narrowing of both the pump laser and the OPO. A simple technique of prelase Q-switching was implemented to reduce the optical bandwidth of the cw diode-pumped Nd:YAG pump laser to <1 GHz. A single intracavity étalon was then sufficient to ensure single frequency oscillation of the OPO signal. The OPO output was stable with a smooth spatial profile and an M ² value of 1.3. Received: 29 September 1999 / Published online: 27 January 2000     

Investigation of the spatial beam quality of pulsed ns-OPOs

This paper reports on an experimental investigation of the spatial beam quality of a pulsed nanosecond optical parametric oscillator (OPO). The OPO is a 355 nm pumped type-I BBO-OPO. The spatial quality of the OPO output is characterized by the M²-parameter in dependence of other experimental parameters such as resonator length, pump-beam diameter, pump-pulse duration and pump energy. The results obtained indicate, that an appropriate choice of these parameters substantially improves the spatial beam quality of the OPO output. Received: 19 November 2002 / Revised version: 3 February 2003 / Published online: 5 May 2003 RID="*" ID="*"Corresponding author. Fax: +49-631/205-3906, E-mail: anstett@rhrk.uni-kl.de     

Low-threshold singly-resonant continuous-wave optical parametric oscillator based on MgO-doped PPLN

We present a 532 nm-pumped singly-resonant cw optical parametric oscillator based on MgO-doped PPLN with a minimum threshold pump power of 0.3 W. The OPO with a two-mirror standing-wave cavity is optimized by using a tunable diode laser on the path of the resonant signal beam. The maximum output power is 200 mW at an idler wavelength near 1330 nm at a pump power of 2 W. We report the degradation of the output power and beam characteristics at high pump power indicating a strong thermal lensing in the crystal. The continuous tuning range of the OPO is measured to be 800 MHz which is close to 90% of the free spectral range of the OPO cavity.     

Femtosecond OPO based on LBO pumped by a frequency-doubled Yb-fiber laser-amplifier system for CARS spectroscopy

We present detailed investigations of a femtosecond green-pumped optical parametric oscillator (OPO) based on lithium triborate. As pump source, a frequency-doubled Yb-fiber laser-amplifier system is used. The OPO generates signal pulses tunable over a spectral range from 780 to 940 nm and idler pulses tunable from 1630 to 1190 nm. More than 250 mW are generated in the signal beam and more than 300 mW in the idler beam. Without dispersion compensation chirped signal pulses with a pulse duration between 100 and 250 fs are measured. Using this system for coherent anti-Stokes Raman scattering spectroscopy, vibrational resonances between 1110 and 6760 cm⁻¹ can be excited. Due to the chirped pulses, a spectral resolution of 100 cm⁻¹ is achieved, which is 2.5 times higher compared to an excitation with time-bandwidth limited pulses.     

Development of injection-seeded, pulsed optical parametric generator/oscillator systems for high-resolution spectroscopy

We report the development and application of pulsed optical parametric generator (OPG) and optical parametric oscillator (OPO) systems that are injection seeded with near-infrared distributed feedback diode lasers. The OPG is injection seeded at the idler wavelength without the use of a resonant cavity. Two counter-rotating, beta-barium-borate (β-BBO) crystals are used in the OPG. These crystals are pumped by the third harmonic, 355-nm output of an injection-seeded Nd:YAG laser. An OPO version of the system has also been developed by placing two flat mirrors around the two β-BBO crystals to form a feedback cavity at the signal wavelength. The OPO cavity length is not actively controlled. The output signal beam from the OPG or OPO is amplified using an optical parametric amplifier (OPA) stage with four β-BBO crystals. The frequency bandwidths of the signal and idler laser radiation from OPG/OPA and OPO/OPA systems have been determined to be slightly greater than 200 MHz. The temporal pulses from each system are smooth and near-Gaussian. High-resolution optical absorption measurements of acetylene (C₂H₂) were performed as another check of the frequency spectrum of the idler beam. The frequency-doubled signal output of the OPO/OPA system was used to perform high-resolution, single-photon, laser-induced fluorescence (LIF) spectroscopic studies of the (0,0) vibrational band of the A ²Σ⁺−X ²Π electronic transition of nitric oxide (NO) at low pressure. Excellent agreement was obtained between the theory and the experiment. The signal output of the OPG/OPA system was also used for sub-Doppler, two-photon LIF spectroscopic studies of the same vibration–rotation manifold of NO.This revised version was published online in August 2005 with a corrected cover date.     

Enhanced beam quality for medical applications at 6.45 μm by using a RISTRA ZGP OPO

A high-average power ZGP OPO with a nonplanar ring RISTRA cavity, pumped by a Ho³⁺:LLF MOPA is presented. A maximum pulse energy at 100 Hz repetition rate of 5.67 mJ at 6.45 ??m with a M² = 1.8 was achieved. The slope efficiency was 16% and the emission spectrum is shown. With a repetition rate of 200 Hz an average output power of 0.95 W at 6.45 ??m was reached.     

Theoretical and experimental studies on passively Q-switched KTiOAsO4 optical parametric oscillator

A passively Q-switched intracavity optical parametric oscillator based on KTiOAsO₄ (KTA) crystal is studied theoretically and experimentally. The rate-equation-based theoretical model is established to describe the time evolutions of the population inversion density of the laser crystal, ground-state population density of the saturable absorber, fundamental photon density, signal photon density and the idler photon density. In the experiment, a laser diode-end pumped, passively Q-switched Nd:YAG/KTA IOPO with a Cr⁴⁺:YAG crystal as the saturable absorber is realized to verify this model. The characteristics including the output power, the pulse repetition rate, the pulse width and the beam quality were investigated for this OPO. The experimental results for the output power and the repetition rate agree with the theory well. And both results show that with same pumping level the idler pulse width is shorter than the signal one.     

High-power synchronously pumped AgGaS(2) optical parametric oscillator

Greater than 2 W of average power was generated in the infrared region by a AgGaS(2) optical parametric oscillator (OPO). A Q -switched mode-locked laser was used to pump the OPO synchronously. Tunability from 1.4 to 1.9mum and a maximum output power of 750 mW at 1.44mum were achieved with a standing-wave cavity. Redesigning the cavity into a ring configuration allowed the depleted pump, signal, and idler beams to be extracted efficiently through separate mirrors. This design generated signal and idler beams of high spatial quality at respective power levels of 1.5 and 620 mW at a pulse repetition rate of 2 kHz.     

High repetition rate mid-infrared generation with singly resonant optical parametric oscillator using multi-grating periodically poled MgO:LiNbO3

A high repetition rate mid-infrared singly resonant optical parametric oscillator (OPO) using MgO-doped multi-grating periodically poled LiNbO₃ (MgO:PPLN) is demonstrated. A 1064 nm Q-switched Nd:YVO₄ laser at 10 kHz repetition rate and pulse width of 17.8 ns was used to pump the OPO. The period of the quasi-phase matched (QPM) grating in the multi-grating MgO:PPLN chip varied from 25.5 to 31.5 μm in steps of 0.5 μm. This corresponds to the generation of a signal beam from 1.37 to 1.64 μm and an idler beam from 3.0 to 4.8 μm, respectively. A maximum signal power of 250 mW and idler power of 140 mW has been obtained with an input pump beam of power 1.92 W, for a grating period of 30.5 μm. A maximum optic-optic conversion efficiency of 20% and 7.4% in the idler has been observed. It has been observed that the output power increases as the period of the grating increases.     

Idler-resonant optical parametric oscillator based on KTiOAsO4

An idler-resonant KTiOAsO₄ (KTA) optical parametric oscillator is demonstrated within a diode-end-pumped acousto-optically Q-switched Nd:YAG laser. With an X-cut KTA crystal, idler wave at 3467 nm and signal wave at 1535 nm are generated. Under an incident diode pump power of 15.4 W, the idler output power of 105 mW and signal power of 720 mW are obtained at a pulse repetition rate of 40 kHz. The pulse widths of the idler and signal waves are 7.2 and 3.1 ns, respectively. The beam quality factors (M²) of the idler wave are within 1.2 in both horizontal and vertical directions.     

Efficient Nd:YAG pumped mid-IR laser based on cascaded KTP and ZGP optical parametric oscillators and a ZGP parametric amplifier

Efficient conversion into the mid-IR of a low pulse-energy (2.5 mJ) Nd:YAG laser is achieved by cascaded KTiOPO₄ (KTP) and ZnGeP₂ (ZGP) optical parametric oscillators followed by a ZGP optical parametric amplifier. The first stage 2.13 μm degenerate KTP OPO uses four KTP crystals in a walk-off compensated geometry and an elliptical pump beam focal geometry to produce up to 2.2 W from 6.3 W incident. The 2.13 μm e-ray pumps a Type-I ZGP OPO, which produces 0.5 W of light in the 3.8-4.8 μm spectral region that in turn is amplified by a 2.13 μm o-ray pumped optical parametric amplifier generating 0.84 W with an M² of <2.     

Mid-infrared ZGP OPO pumped by near-degenerate narrowband type-I PPKTP parametric oscillator

The total pulse energy of the signal and idler in a near-degenerate type-I periodically poled KTiOPO₄ (PPKTP) optical parametrical oscillator (OPO) was spectrally confined within a 2 nm spectral bandwidth at 2.13 μm. This was achieved by using a volume Bragg grating as the output coupler. Both the signal and the idler from the PPKTP OPO were then simultaneously used to pump a mid-infrared ZnGeP₂ (ZGP) OPO. The 2 nm bandwidth was narrower than the ZGP crystal acceptance bandwidth and, thus, made efficient conversion in the second OPO possible. A total slope efficiency of 10% from 1.06 μm to the 3.5–5 μm region was demonstrated, generating 250 μJ in the mid-IR with only 3.6 mJ of 1.06 μm pump energy. This corresponds to a Nd:YAG pump to mid-IR conversion efficiency of 7%. PACS 42.65.Yj; 42.72.Ai; 42.40.Eq