Field-induced neutron depolarization in amorphous RE-TM spin glasses

Neutron depolarization induced by an applied magnetic field is reported for the amorphous spin glass compositions DyCu, GdAl₂ and NdFe₂. The different field-cooled behavior observed in the first two compositions is attributed to the different mechanisms (exchange fluctuations and random crystal field anisotropy) believed to stabilize the spin glass state in the two cases.     

Zero field muon spin relaxation in simple magnets and spin glasses

A theory is developed for the calculation of zero field muon spin relaxation function for classical simple magnets (Ising, XY, and Heisenberg) in D(=1,2,3) dimensions. The results are different from the Kubo-Toyabe theory, except for Heisenberg system in three dimension. Relation between the relaxation function and random field distribution is dicussed and a new method of analysing experimental data is suggested and discussed in the context of spin glasses.     

Nonequilibrium properties of re-entrant spin glasses in a magnetic field

In this paper the authors discuss how the re-entrant spin-glass state arises in the disordered alloys Ni_100−x Mn_x (x=19, 21, 23), along with the nonequilibrium magnetic properties of these alloys. It is shown that near the Gabay-Toulouse phase line the time it takes the system to reach equilibrium is comparable to times required to perform static experiments (10¹–10⁴ s); cooling the sample into the region of crossover with the de Almeida-Thouless line causes these times to increase to astronomical values of more than 10¹⁶ s. A method is proposed for constructing magnetic phase diagrams of systems of this type in “magnetic field-temperature” coordinates. Fiz. Tverd. Tela (St. Petersburg) 41, 2028–2033 (November 1999)     

Order parameters forn-vector spin glasses ind dimensions

We report Monte Carlo simulations of the time-dependent behavior of Edwards-Anderson spin glasses with Gaussian nearest-neighbor exchange, for both spin dimensionalityn and space dimensionalityd from 2 up to 6. A (nearly) logarithmic decay of the Edwards-Anderson order parameter with time is observed for alln and alld, similar to earlier studies forn=1. But the Monte Carlo data forn>1 suggest stronger than those forn=1 that all order parameters considered vanish in thermal equilibrium for nonzero temperature, because the decay forn>1 is faster at the temperatures of interest. For Heisenberg spins (n=3) no significant dependence of the Edwards-Anderson order parameterq on the size of the lattice was observed ford=2,3 and 4, whereas ford=5 and 6,q was smaller for smaller systems (in contrast to thed=5 Ising case). These results are the first Monte Carlo indication of a change in the bulk behavior of Heisenberg spin glasses at dimensionalityd=4. Quenching the system to zero temperature and then applying a field we find that the order parameter , measuring the alignment with respect to the state at zero field, is destroyed by a sufficiently strong magnetic field, for all observedn andd.Sonderforschungsbereich 125 Aachen-Jülich-Köln, FRG     

Field-induced anisotropy in concentrated systems of rigid particles and macromolecules

This paper presents experimental results on the use of spectroscopic optical polarimetry to study structure in dense systems of rigid particles and rigid polymer liquid crystals. These measurements probe microstructural anisotropy induced by the application of electric fields in the case of dense suspensions of rigid spheres, or flow fields in the case of polymer liquid crystals. It is demonstrated that conservative linear dichroism can measure moments of the particle pair distribution function in dense suspensions. In liquid crystals, the dichroism is a result of field-induced anisotropy in the defect structure of the material.     

Field-induced negative differential spin lifetime in silicon

We show that the electric-field-induced thermal asymmetry between the electron and lattice systems in pure silicon substantially impacts the identity of the dominant spin relaxation mechanism. Comparison of empirical results from long-distance spin transport devices with detailed Monte?Carlo simulations confirms a strong spin depolarization beyond what is expected from the standard Elliott-Yafet theory even at low temperatures. The enhanced spin-flip mechanism is attributed to phonon emission processes during which electrons are scattered between conduction band valleys that reside on different crystal axes. This leads to anomalous behavior, where (beyond a critical field) reduction of the transit time between spin-injector and spin-detector is accompanied by a counterintuitive reduction in spin polarization and an apparent negative spin lifetime.     

Field-induced structural aging in glasses at ultralow temperatures

In nonequilibrium experiments on the glasses Mylar and BK7, we measured the excess dielectric response after the temporary application of a strong electric bias field at millikelvin temperatures. A model recently developed describes the observed long time decays qualitatively for Mylar [Phys. Rev. Lett. 90, 105501(2003)]], but fails for BK7. In contrast, our results on both samples can be described by including an additional mechanism to the mentioned model with temperature independent decay times of the excess dielectric response. As the origin of this novel process beyond the "tunneling model" we suggest bias field induced structural rearrangements of "tunneling states" that decay by quantum mechanical tunneling.     

Frustrated percolation,spin glasses and glasses

Summary The static and dynamic properties of the frustrated percolation model are investigated. This model, which contains frustration as an essential ingredient, exhibits two transitions: a percolation transition at a temperatureT _p with critical exponents of the ferromagnetic (s=1/2)-state Potts model, and a second transition at a lower temperatureT _g in the same universality class of the Ising spin glass model. AboveT _p the time-dependent autocorrelation function is characterized by a single exponential, while forT _p>T>T _g preliminary numerical results show a broad shoulder or plateau typical of a structural glass transition. BelowT _g the system is in glassy state with an infinitely long relaxation time. Paper presented at the I International Conference on Scaling Concepts and Complex Fluids, Copanello, Italy, July 4–8, 1994.     

Insulating spin glasses

The possibility of obtaining spin glasses by addition of impurities in an antiferromagnetic insulator is examined. Dipolar interactions are briefly considered but the attention is focussed on Heisenberg systems. Equivalence with the Edwards-Anderson model is derived in a theoretical case. Experimental realisations, such as quasi-one dimensional systems, and spinels, are reviewed. A weak concentration of non-magnetic impurities can give rise to a new state that we call semi spin glass, in which a ferromagnetic component coexists with a transverse, spin glass component. An important case is when the pure system has a high ground state degeneracy (cooperative paramagnet). Non-magnetic impurities or other forms of disorder can transform it into a spin glass.     

Thermopower of spin glasses

We calculate the thermopowerS _d(T) of spin glasses on the basis of thesd exchange model with additional interactions between the impurity spins by means of time dependent perturbation theory. Similarly to the Kondo effect, the observed giant thermopower can only be explained if one also takes into account the spin independent interactionV between the magnetic impurities and the conduction electrons. We obtain a Kondo termS _d ⁽¹⁾ (T) (which reduces for vanishing spin interactions to the thermopower of Kondo systems) and in addition a resonance termS _d ⁽²⁾ (T) of opposite sign which vanishes for vanishing interactions. The superposition of both terms leads to an additional extremum of the total thermopower and to a change of sign at a temperatureT ₀ which depends on the Kondo temperature and on the magnetic excitations of the spin glass and therewith on the freezing temperatureT _f. We obtain at low temperatures for oscillating and relaxing spin glass modesS _d ⁽¹⁾ T² andS _d ⁽²⁾ T. At high temperaturesS _d ⁽¹⁾ (T) decreases as |lnT|^–3 andS _d ⁽²⁾ asT ^–1. A close relationship between the temperature dependent resistivity in Born approximation andS _d ⁽¹⁾ (T) is pointed out.SFB 125 Aachen-Jülich-Köln     

Superconductivity of spin glasses

The coexistence of superconducting and spin glass phases is investigated. The dependence of the phase transition temperature in the spin glass state both on the impurity concentration and the superconductivity state is given. The influence of the spin glass phase on the renormalized frequency and the order parameter of the conduction electrons is determined.     

Field-induced three- and two-dimensional freezing in a quantum spin liquid

Field-induced commensurate transverse magnetic ordering is observed in the Haldane-gap compound Ni(C(5)D(14)N(2))2N(3)(PF(6)) by means of neutron diffraction. Depending on the direction of applied field, the high-field phase is shown to be either a three-dimensional ordered Néel state or a short-range ordered state with dominant two-dimensional spin correlations. The structure of the high-field phase is determined, and properties of the observed quantum phase transition are discussed.     

Localized spin excitations in magnets with triangular spin ordering

Some types of localized spin excitations in hexagonal antiferromagnets with triangular spin ordering are investigated. The character of relaxation of these spin excitations is studied.