共查询到20条相似文献,搜索用时 15 毫秒
1.
《中国科学:物理学 力学 天文学(英文版)》2010,(7)
In order to experimentally probe into the complicated interaction between charge ordering and spin ordering in manganites,two sets of samples Nd0.5Sr0.5Mn1-xGaxO3(NSMGO) and Nd 0.5Sr0.5Mn1-y CryO3(NSMCO)(0.0 x,y 0.075),have been studied by means of electrical transport,magnetization,electron spin resonance and transmission electron microscopy analysis.By comparing the influence of Cr-doping and Ga-doping in the Nd0.5Sr0.5MnO3(NSMO) system,large difference between the evolution of charge ordering temperature T co in the Cr-doping and the Ga-doping cases is found.In the NSMCO system,the CE-type antiferromagnetic(AFM)/charge ordering(CO) phase disappears with only 2.5 percent Cr doping;but in the NSMGO system,the CE-type AFM/CO phase always exists.This phenomenon indicates that the charge ordering formation is dominated by the spin ordering.As a result,it is experimentally proved that there is strong coupling interaction between charge ordering and spin ordering in NSMO system. 相似文献
2.
M. Yu. Kagan K. I. Kugel D. I. Khomskii 《Journal of Experimental and Theoretical Physics》2001,93(2):415-423
A simple model of charge ordering is considered. It is explicitly shown that at any deviation from half-filling (n≠1/2), the system is unstable with respect to the phase separation into the charge ordered regions with n=1/2 and the metallic regions with a smaller electron or hole density. A possible structure of this phase-separated state (metallic droplets in a charge ordered matrix) is discussed. The model is extended to account for the strong Hund-rule onsite coupling and the weaker intersite antiferromagnetic exchange. The analysis of this extended model allows us to determine the magnetic structure of the phase-separated state and to reveal the characteristic features of the manganites and other substances with charge ordering. 相似文献
3.
Litong Jiang 《中国物理 B》2021,30(11):117106-117106
The first-principles calculations were used to explore the tunable electronic structure in DyNiO3 (DNO) under the effects of the biaxial compressive and tensile strains. We explored how the biaxial strain tunes the orbital hybridization and influences the charge and orbital ordering states. We found that breathing mode and Jahn-Teller distortion play a primary role in charge ordering state and orbital ordering state, respectively. Additionally, the calculated results revealed that the biaxial strain has the ability to manipulate the phase competition between the two states. A phase transition point has been found under tensile train. If the biaxial train is larger than the point, the system favors orbital ordering state. If the strain is smaller than the point, the system is in charge ordering state favorably. 相似文献
4.
We present a spring-defect model in 3-dimensions to describe the connection between elastic distortion and interstitial carbon
ordering associated with phase transition from a body centred cubic (BCC) to body centered tetragonal (BCT) structure in BCC
metals such as α-iron. The presence or the absence of the carbon is modelled in terms of a pseudo spinŝ=+1or -l.An Ising interaction between carbon atoms is recovered after eliminating the lattice degrees of freedom, which is
longranged. The coupling between the spin and lattice degrees of freedom allows for a systematic study of ferroelasticity
and the variation of the lattice parameter with carbon concentration. The mean field results for the paraelastic to ferroelastic
transition, lattice parameter and static compliance are presented. The significant feature of this calculation is not only
a derivation of the defect-defect interaction, but also an explicit calculation of the strain dipole tensor associated with
each defect, from a microscopic model. 相似文献
5.
The spring-defect model developed by us in the accompanying paper I to discuss ferroelasticity, exhibited in the BCT phase
of α-iron (BCC metals), is used to analyse anelastic relaxation across the paraelastic to ferroelastic phase transition. The
kinetics of the underlying Hamiltonian representing strain-strain interactions is treated within mean-field theory. The relaxation-response
relation of the linear response theory is employed to derive explicit expressions for the anelastic strain, the frequency-dependent
compliance and the internal friction in terms of the basic parameters of the spring-defect model. 相似文献
6.
7.
《Solid State Communications》1987,62(4):213-220
Interchain electron hopping t⊥ in conducting polymers with the small confinement parameter γ leads to the antiferromagnetic (AB) 3-d ordering of the dimerization pattern only at 2t2γ >γΔ2 (2Δ being the Peierls gap), otherwise the ferromagnetic (AA) one occurs. Polarons (Ps, υ = 1) and bipolarons (BPs, υ = 2) stability areas: t⊥/Δ<tc (υ,γ) are found in the phase plane “t⊥ vs γ” with critical tc being larger in the AB phase and for BPs. At the AA-AB transition interface, “deconfinement” of kink-solitons is possible. Photogeneration of Ps and BPs may proceed via metastable free states separated by the self-trapping barriers (STBs) which are also different in AA and AB (in the latter STBs exist even in 2-d systems) and are lower for BPs. 相似文献
8.
Eugene R. Speer 《Journal of statistical physics》1986,42(5-6):895-920
We show that, for neutral systems of particles of arbitrary charges in two dimensions, with hard cores, coefficients of the Mayer series for the pressure exist in the thermodynamic limit below certain thresholds in the temperature. Our methods apply also to correlation functions and yield bounds on the asymptotic behavior of their Mayer coefficients. 相似文献
9.
M. Hervieu A. Barnabé C. Martin A. Maignan F. Damay B. Raveau 《The European Physical Journal B - Condensed Matter and Complex Systems》1999,8(1):31-41
Charge ordering phenomena in the manganites Ca1-xSmxMnO3 have been studied for , using electron diffraction and lattice imaging, completed by magnetic and transport measurements. Three domains can be distinguished,
depending on the nature of the structural transitions with temperature. For , the structural transition from a pseudo-tetragonal to a monoclinic form, with decreasing temperature, coincides with the
competition between ferromagnetism and antiferromagnetism that is characterized by the temperature Tpeak on the M
(
T
) curves; short-range charge ordering is observed for manganites. For the second domain, , a structural transition from an orthorhombic to a long-range charge ordered state is clearly observed with decreasing temperature.
The corresponding temperature TCO coincides with the temperature Tpeak deduced from magnetic measurements. This long range charge ordering, which appears along a, is either commensurate or incommensurate depending on the x value, with a modulation vector, q being close to x. These modulated superstructures correspond to a stacking of single Mn3+ stripes with multiple Mn4+ stripes along a, either in a commensurate or in an incommensurate manner. The third domain , is characterized by a transition to a charge ordered state with commensurate superstructure at low temperature. The latter
can be described as a “partially” charge ordered state in which single “Mn3+” stripes alternate with mixed “Mn3+/Mn4+” stripes.
Received 17 June 1998 相似文献
10.
We discuss a new mechanism of orbital ordering, which in charge transfer insulators is more important than the usual exchange interactions and which can make the very type of the ground state of a charge transfer insulator, i.e., its orbital and magnetic ordering, different from that of a Mott-Hubbard insulator. This purely electronic mechanism allows us to explain why orbitals in Jahn-Teller materials typically order at higher temperatures than spins, and to understand the type of orbital ordering in a number of materials, e.g., K2CuF4, without invoking the electron-lattice interaction. 相似文献
11.
I. P. Kogutyuk P. P. Kogutyuk L. F. Pryadko M. D. Smolin 《Russian Physics Journal》1985,28(2):109-112
Using a generalized Hubbard model within the framework of Kubo formalism, the concentration and temperature dependences of thermo-emf () in materials with charge ordering are calculated. It is shown that in a charge-ordered state a threefold inversion of the sign of a occurs with change in charge carrier concentration (n). Temperature reduction leads to a phase transition of the crystal into a charge-ordered state, which at certain values of n also causes a change in the sign of .Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika. No. 2, pp. 26–29, February, 1985. 相似文献
12.
A. M. Finkel'stein 《Zeitschrift für Physik B Condensed Matter》1984,56(3):189-196
Interacting electrons, diffusing in a two-dimensional (2d) disordered system, are studied. The renormalization group equations, including both localization effects and Coulomb correlations, are derived. We encounter a qualitatively new situation: the constants describing electron interaction diverge as a result of the renormalization when a certain scale is achieved, whereas the resistence proves to be finite. Calculation of the spin density correlation function reveals that the system exhibits a tendency for spin density rearrangement. 相似文献
13.
Jean-Paul Pouget 《Physica B: Condensed Matter》2012,407(11):1762-1770
We review 35 years of structural studies of quasi-1D organic conductors during which the concepts of 2kF and 4kF BOW and CDW have been elaborated. In strongly correlated quarter filled band systems these instabilities give rise to SP, DM and CO ground states. We relate these structural features to the instabilities of the 1D electron gas. To stabilize the different ground states the nature of the electron-phonon coupling has to be considered together with the coupling of the organic stacks with the anion sublattice. New results concerning the classification of the SP phase in connection with the adiabatic or antiadiabatic phonon field and its competition with the CO are also introduced. 相似文献
14.
T. K. Rebane 《Physics of Atomic Nuclei》2012,75(4):455-463
The problem of boundness of a
+
b
+
c
−
d
− four-particle Coulomb systems (quadrions) is studied versus the masses of the particles involved. Inequalities that make
it possible to deduce that, if some reference quadrions form a bound state, the same is true for a large number of quadrions
formed by particles having various masses were derived. A compendium of calculations for energies of reference systems that
possess various symmetries [positronium molecules (e
+
e
+
e
−
e
−) and quadrions of the a
+
b
+
b
−
b
−, a
+
b
+
a
−
b
−, and a
+
a
+
b
−
c
− types] is given, and groups of bound asymmetric quadrions corresponding to them are determined. An inequality for kinetic
energies of particles that makes it possible to find out, by using asymmetric reference systems, whether specific quadrions
are bound is obtained. It is shown that the boundness of many quadrions is ensured by the boundness of respective three-particle
systems. The entire body of the present results permits proving that, of the total number of 406 quadrions containing electrons,
muons, pions, kaons, protons, deuterons, and tritons and their antiparticles, 227 quadrions are bound. 相似文献
15.
We study the spin ordering within the three-leg ladders present in the oxyborate Fe3O2BO3 consisting of localized classical spins interacting with conduction electrons (one electron per rung). We also consider the competition with antiferromagnetic superexchange interactions to determine the magnetic phase diagram. Besides a ferromagnetic phase we find (i) a phase with ferromagnetic rungs ordered antiferromagnetically and (ii) a zigzag canted spin ordering along the legs. We also determine the induced charge ordering within the different phases and the interplay with lattice instability. Our model is discussed in connection with the lattice dimerization transition observed in this system, emphasizing the role of the magnetic structure. 相似文献
16.
Luo W Franceschetti A Varela M Tao J Pennycook SJ Pantelides ST 《Physical review letters》2007,99(3):036402
The structural, electronic, and magnetic properties of mixed-valence compounds are believed to be governed by strong electron correlations. Here we report benchmark density-functional calculations in the spin-polarized generalized-gradient approximation (GGA) for the ground-state properties of doped CaMnO(3). We find excellent agreement with all available data, while inclusion of strong correlations in the GGA+U scheme impairs this agreement. We demonstrate that formal oxidation states reflect only orbital occupancies, not charge transfer, and resolve outstanding controversies about charge ordering. 相似文献
17.
18.
We analyse the behaviour of 2-order parameter systems (where one subsystem is superconducting) in constant external ordering fields and find the spatial distribution of the order parameters.The authors would like to thank Prof. B. T.Matthias and Prof. T. L.Birman for useful discussions. 相似文献
19.
We study the interplay of topological excitations in stripe phases: charge dislocations, charge loops, and spin vortices. In two dimensions these defects interact logarithmically on large distances. Using a renormalization-group analysis in the Coulomb-gas representation of these defects, we calculate the phase diagram and the critical properties of the transitions. Depending on the interaction parameters, spin and charge order can disappear at a single transition or in a sequence of two transitions (spin-charge separation). These transitions are nonuniversal with continuously varying critical exponents. We also determine the nature of the points where three phases coexist. 相似文献
20.
Feng Y Jaramillo R Srajer G Lang JC Islam Z Somayazulu MS Shpyrko OG Pluth JJ Mao HK Isaacs ED Aeppli G Rosenbaum TF 《Physical review letters》2007,99(13):137201
Elemental chromium orders antiferromagnetically near room temperature, but the ordering temperature can be driven to zero by applying large pressures. We combine diamond anvil cell and synchrotron x-ray diffraction techniques to measure directly the spin and charge order in the pure metal at the approach to its quantum critical point. Both spin and charge order are suppressed exponentially with pressure, well beyond the region where disorder cuts off such a simple evolution, and they maintain a harmonic scaling relationship over decades in scattering intensity. By comparing the development of the order parameter with that of the magnetic wave vector, it is possible to ascribe the destruction of antiferromagnetism to the growth in electron kinetic energy relative to the underlying magnetic exchange interaction. 相似文献