Reinvestigation of the decay scheme of the short-lived isomeric states in112In

The two short-lived isomeric states in¹¹²In have been reinvestigated by means of the¹¹²Cd(d, 2n) and¹⁰⁹Ag (α, n) reactions. Measurements of delayed X- andγ-ray, lifetime and TDPAD spectra have been performed. A 6.32(3) keVγ-ray has been identified in the isomeric decay and anM1 multipolarity has been assigned to it on the basis of the measured internal conversion coefficients:α _L =196(39) andα _tot=231(35). TheE1+M2(δ =+0.24(4)) andE2 multipolarities have been determined for the 263 and 188 keV transitions deexciting the 8^?(T _1/2=2.82(2) μs) and 7⁺ (T _1/2=0.93(2) μs) isomeric states, respectively. A revised isomeric decay scheme is presented.     

The decay of 31 sec98Zr, 2.9 sec98Nb and 51 min98Nb

TheΒ- andγ-radiations of⁹⁸Zr and^{98m, g} Nb have been investigated employing scintillation and semiconductor spectrometers and coincidence techniques. Sources of⁹⁸Nb were produced by the⁹⁸Mo(n, p)⁹⁸Nb reaction, sources of⁹⁸Zr by fission of²³⁵U with thermal neutrons applying chemical separations. For⁹⁸Zr, a half-life of 30.7±0.4 sec and aQ _β-value of 2.3±0.2 MeV were obtained, for the⁹⁸Nb isomers, half-lives of 2.86±0.06 sec and 51.3±0.4 min, andQ _β-values of 4.8±0.2 MeV and 4.5±0.2 MeV, respectively. Noγ-rays were observed in the decay of⁹⁸Zr. The decay of 2.9 sec⁹⁸Nb was found to involve 11γ-ray transitions. In the decay of 51 min⁹⁸Nb, 54γ-transitions were detected. Spin and parity of 1⁺ and 4^? were deduced for the isomeric states of⁹⁸Nb.     

High-spin states in106Cd

Levels of¹⁰⁶Cd, populated by¹⁰⁴Pd(α, 2nγ)¹⁰⁶Cd have been studied measuring direct and delayedγ-ray spectra,γ-γ coincidences andγ-ray angular distributions. A decay level scheme is proposed including states up to 4659.8 keV. IntenseE2 transition cascades have been observed. The half-life of an isomeric level located at 4659.8 keV has been measured:T _1/2= 62±6ns. Nuclear Reactions ¹⁰⁴Pd(α, 2nγ),E _α=31MeV; measuredE _γ,I _γ,γ-γ coinc, σ(θ)T _1/2.¹⁰⁶Cd deduced levels,J, π, Enriched targets. Ge(Li) detectors.     

Decay characteristics of 0 2 + and 0 3 + states in112Cd and114Cd

Absolute rates ofE0 andE2 transitions depopulating 0 ₂ ⁺ and 0 ₃ ⁺ states in¹¹²Cd and¹¹⁴Cd have been determined using conversion-electron andγ-ray spectroscopy, and double Coulomb excitation. The collectivity of these states is established and discussed.     

Energy levels of 37K

Angular distributions have been measured for six ³⁶Ar(p,γ)³⁷K resonances in the E_p = 0.9−3.0 MeV energy region. These experiments yield spin- and parity assignments to seven excited states of ³⁷K, γ-ray branching ratios for each state, together with the multipolarity mixing ratios of most transitions. Lifetimes have been deduced from the same data with the DSA method.Excitation energies have been determined with a precision up to 20 eV. A resonance- and excitation-energy measurement at the E_p = 918keV resonance yields a ³⁶Ar(p, γ)³⁷K Q-value of Q = 1857.57 ± 0.09 keV.The ³⁶Ar(p, p₁γ) yield curve, measured in the E_p = 2.6–3.3 MeV region, yields additional information on resonance and excitation energies of ³⁷K states with a typical precision of 0.6 keV.The new data on ³⁷K levels allow a detailed comparison of the level schemes of the mirror nuclei ³⁷Ar and ³⁷K. The present experimental data agree quite well with the results of previous shell-model calculations.     

Multipolarity of some transitions in the96Zr(p,n γ e)96Nb reaction

The conversion electron andγ-ray spectra of the⁹⁶Zr(p, n γ)⁹⁶Nb reaction were measured with Ge(Li) and superconducting magnet transporter Si(Li) spectrometers respectively, at 4MeV bombarding proton energy. The multipolarities of some transitions were determined and conclusions were drawn on the spins and parities of the excited states of⁹⁶Nb.     

Anomalous behaviour of transition probabilities in75Kr

Two collective bands of⁷⁵Kr have been extended up to spin 21/2 using the compound reactions⁶⁴Zn(¹⁴N,p2n)⁷⁵Kr and⁵⁰Cr(²⁸Si, 2pn)⁷⁵Kr. Spins and parities were assigned from neutron-gatedγ-ray angular distributions and excitation functions using the OSIRIS anti-Compton spectrometer. The bands are interpreted to be built on the well-deformed Nilsson states: [442] 5/2 and [301] 3/2. Energies for both bands and the order of magnitude of the mixing ratios in thef _5/2 band can be reproduced within the single-particle-plus-rotor model, while the experimentalQ(I→I?1)/Q(I→I?2) ratios, deduced from mixing ratios and branching ratios, exhibit large deviations by a factor 4 to 6 from theoretical values (which are around one). An explanation of this effect may be found by treating the two rotational bands each as a result of mixing between rotational bands of oblate and prolate states; thus explaining the large difference between B(E2,I→I?1) andB(E2, I →I?2) in the bands of⁷⁵Kr.     

Band structures in73Se

Excited states of⁷³Se have been investigated up to spin, 21/2 using techniques of in-beamγ-ray spectroscopy in connection with the⁷⁰Ge(α, n) reaction. Mean lifetimes of 12 levels have been determined applying Doppler-shift andγ-RF-methods. Five different bands have been identified that reflect a variety of different excitation modes. The decoupled 9/2⁺ band is likely to correspond to an oblate deformation while the 5/2⁺ band is interpreted as a strongly coupled prolate band built on the Nilsson configuration [422] 5/2⁺. The 3/2^? band is a strongly coupled band built on the [301] 3/2^} configuration.Nuclear reactions:⁷⁰Ge(α,n),E=14, 16, 18, 19, 20MeV; measuredE _γ,I _γ,σ(E _γ,θ),γγ-coin, linear polarization, DSA,γ(t).⁷⁵Se deduced levels,I, π, τ, δ(E2/M1), B(σλ). Enriched targets, Ge detectors.     

In beam gamma spectroscopy of62Zn

The decay scheme of⁶²Zn has been investigated by studying the yield functions, angular distributions and coincidence relation-ships of theγ-rays emitted in the⁶³Cu(p, 2nγ) and⁶⁰Ni(α, 2nγ) reactions. Spins up to7? were assigned to the observed states. Nuclear Reactions ⁶⁰Ni(α, 2nγ)⁶²Zn,E _α=28–35 MeV and⁶³Cu(p, 2nγ)⁶²Zn,E _p = 22–31 MeV; measuredE _γ,I _γ(θ),I _γ(E _p , andI _γ,E _α-γ coincidences,⁶²Zn deduced decay scheme. Enriched target, Ge(Li) detectors.     

The decay scheme of the 3-s Isomer of100Nb and the properties of levels in100Mo

Theβ ^? decay of the longer-lived isomer in¹⁰⁰Nb has been studied at the fission-product separator JOSEF. Measurements ofγ-ray singles spectra, ofγ-γ coincidences and ofγ-γ angular correlations have been performed. A value oft _1/2=2.99(11)s has been determined for the isomer which probably hasI ^π=4⁺ or 5⁺. A scheme of the levels of¹⁰⁰Mo which are populated in the decay of this isomer has been established. Information on the spins of several states of¹⁰⁰Mo has been obtained. Thus,I=0 levels have been identified at 1,505, 2,038 and 2,087 keV. The mixing ratios have been determined for the 2₂ ⁺→2₁ ⁺ and 2₃ ⁺→2₁ ⁺ transitions. The results provide evidence for a vibrational structure of¹⁰⁰Mo with separate bands based on the ground state and on the first excited 0⁺ level.     

Sequential processes in the14N(τ,pα)12C* reaction

α-particle and proton spectra in coincidence with the 4.44 MeVγ-ray from the¹²C first excited state have been taken atE _τ MeV. Several states in¹³N and¹⁶O are seen to contribute to the decay sequenceα?p andp?α respectively. Estimates are given for the branching of these two decay modes and for a possible simultaneous break-up.     

Properties of isomeric states and the πd 3/2-vi 13/2 multiplet in194Au

The level structure of¹⁹⁴Au has been studied by observing prompt and delayedγ-rays following¹⁹⁴Pt(p,n) and¹⁹⁵Pt(p,2n) reactions. The conversion electron andγ-ray spectra from the decay of the 0.42s (10^?) and 0.60s (5⁺) isomers at 476 keV and 107.4 keV, respectively, have been measured using the He-jet method. The half-lives of the 6⁺ (278.2 keV, 1.1±0.4 ns), 7⁺ (224.6 keV, 2.6±0.2 ns) and 8⁺ (406.8 keV, 2.9±0.4 ns) members of theπd _3/2-vi _13/2 multiplet have been obtained from the time distributions between cyclotron beam pulses andγ-rays depopulating these levels. A calculation made assuming a pure two-particle configuration for the multiplet predicts very well theB(E2) values for the transitions between the levels of this multiplet but the calculatedB(M1) values are not in agreement with experimental results.     

High-spin states in89Nb,88Zr and88Nb with a shell-model description of theN=48 andN=47 nuclei

The reactions⁸⁹Y(α,4nγ),⁸⁹Y(α,p4nγ) and⁸⁹Y(α,5nγ) were used to populate high-spin states in, respectively,⁸⁹Nb,⁸⁸Zr and the previously unstudied nucleus⁸⁸Nb. These states were deduced via in-beam gamma-ray spectroscopy. The results of a shell-model study ofN=48⁸⁸Zr,⁹⁰Mo,⁸⁷Y,⁸⁹Nb andN=47⁸⁷Zr,⁸⁸Nb nuclei are compared to experiment.     

Level structure of 110in from the 110cd(p,nγ)110in reaction

γ-ray and γγ-coincidence spectra of the ¹¹⁰Cd(p, nγ)¹¹⁰In reaction were measured with Ge(Li), Ge(LEPS), and Ge(HP) spectrometers at 6 MeV bombarding proton energy. Energies (E_γ) and relative intensities (I_γ) of 95 ¹¹⁰In transitions (including 70 new ones) have been determined. The electron spectrum of the reaction was measured with a combined magnetic plus Si(Li) spectrometer at E_p = 6 MeV. Internal conversion coefficients of 41 transitions in ¹¹⁰In have been determined for the first time. The angular distribution of γ-rays was measured at 5.2, 5.6, and 6 MeV bombarding proton energies. A new, more complete level scheme of ¹¹⁰In has been deduced. On the basis of the internal conversion coefficients of transitions, Hauser-Feshbach analysis of (p, n) reaction cross sections, γ-ray angular distribution (and other) results unambiguous spin and parity assignments were made to 11 excited ¹¹⁰In levels. The energies of several ¹¹⁰In proton-neutron multiplets were calculated on the basis of the parabolic rule derived from the cluster-vibration model. The comparison of experimental and theoretical results provided identification of about 20 p-n multiplet states in ¹¹⁰In.     

Excited states of 96Nb from the 96Zr(p,nγ)96Nb reaction

The γ-ray spectra of the ⁹⁶Zi(p, nγ)⁹⁶Nb reaction have been measured with Ge(Li) detectors at different bombarding proton energies between 1.3 and 5.1 MeV. γγ coincidences were observed at E_p = 4.7 and 5.0 MeV. On the basis of experimental results a level scheme of ⁹⁶Nb was deduced, and γ-threshold energies and γ-branching ratios were determined. Computed Hauser-Feshbach (p, n′) cross sections have been compared with experimental data obtained from the γ-ray measurements, and level spins and parities have been determined. The energies of ⁹⁶Nb levels were calculated on the basis of the parabolic rule, derived from the cluster-vibration model. The Racah multipole decomposition method was used also for the theoretical interpretation of several ⁹⁶Nb multiplet states.     

Gamma deexcitation of the 180m Ta isomer

Vibrational states built on the K ^π = 9^? isomer and on the ground state (K ^π = 1⁺) in ¹⁸⁰Ta are calculated within the quasiparticle-phonon nuclear model using the ¹⁷⁸Hf nucleus as a core. A procedure for calculating the rates of K-allowed γ-ray transitions from vibrational states built on the isomer to those built on the ground state is presented. The probabilities of two-step processes consisting of a dipole excitation of the isomer and successive E1 and E2 transitions from them to vibrational states built on the ground state of the ¹⁸⁰Ta nucleus are calculated. Two-step transitions from the isomer to vibrational states below 2.7 MeV and to the vibrational states built on the ground state appear to be very weak. There are many E1 transitions from the vibrational states built on the isomer to the vibrational states built on the ground state. They are weak and cannot be responsible for the strong deexcitation of ^180m Ta in the relevant (γ, γ′) reaction. A decisive role is played by collective E2 transitions from dipole excitations in several excitation energy intervals ranging between 2.7 and 4.0 MeV. These highly intense K-allowed two-step γ-ray transitions can be responsible for the strong deexcitation of the ^180m Ta state in the (γ, γ′) reactions.     

Proton-neutron multiplet states in 114In

The γ-ray spectrum of the ¹¹⁴Cd(p, nγ)¹¹⁴In reaction was measured with Ge(Li) and Ge(HP) spectrometers at 4.8, 5.3, and 7.0 MeV bombarding proton energies. The energies (E_γ) and relative intensities (I_γ) of more than 170 γ-ray transitions in ¹¹⁴In have been determined. The electron spectrum of the reaction was measured with a combined magnetic plus Si(Li) spectrometer. Internal conversion coefficients of 38 transitions in ¹¹⁴In were determined for the first time. The level scheme of ¹¹⁴In, γ-ray branching ratios, multipolarity of transitions, level parity and spin values have been deduced. The energies of several ¹¹⁴In proton-neutron multiplets were calculated on the basis of the parabolic rule derived from the cluster-vibration model. The comparison of experimental and theoretical results provided classification of about 18 multiplet states in ¹¹⁴In. The experimental level scheme has also been compared with former theoretical calculations.     

Yrast and side bands in the odd-odd160, 162Tm nuclei

High-spin states in²⁰⁵Bi, populated in the²⁰⁵Tl(α, 4n) reaction with bombarding energies around 50 MeV have been studied usingγ-ray spectroscopic techniques. Spins and parities have been assigned on the basis of angular distribution andγ-ray linear polarization measurements. States with spins up to 39/2⁺ and excitation energies around 6 MeV have been identified. Calculations using the empirical shell model have been performed in order to assign configurations.     

Tentative level diagram of146Pm below 1.1 MeV

The level scheme of the doubly odd nucleus¹⁴⁶Pm was investigated by means of in-beam spectroscopy. The¹⁴⁶Nd(p, n) reaction in the 3.5–8 MeV proton energy interval on enriched targets has been used to populate the exited states of¹⁴⁶Pm. High resolutionγ-ray spectra using Ge(Li) and hyperpure Ge detectors and conversion electrons with a mini-orange spectrometer were measured. Withγ-exitation functions andnγ-coincidences usingnγ-discriminated NE231 neutron detectors transitions in¹⁴⁶Pm were identified,γγ-coincidences gave information aboutγ-cascades. With these data a level scheme of 38 levels below 1.1 MeV exitation energy has been deduced including 73 transitions. For 12 transitions experimental conversion coefficients have been evaluated, which agree with the expected values forM1/E2-transitions.     

High-spin states in108Sn

High spin states in¹⁰⁸Sn have been investigated using the⁹²Mo(¹⁹F,p2nγ)¹⁰⁸Sn reaction. In-beam measurements ofγ-γ-coincidences,γ-ray excitation functions andγ-ray angular distributions were performed with Ge(Li)-detectors, one of which had a Nal Compton suppression shield. A level scheme for¹⁰⁸Sn has been constructed up to anI ^π=(14^?) state.