Megawatt peak power, 1 kHz, 266 nm sub nanosecond laser source based on single-crystal fiber amplifier

We report the realization of a UV source based on the fourth harmonic generation with LBO/BBO of a Nd:YAG passively Q-switched oscillator amplified in a single-crystal fiber. With careful optimization of the nonlinear components and parameters, we obtain 530 mW average power at 266 nm with pulses of 540 ps at the repetition rate of 1 kHz, which represents a 22.7 % total conversion efficiency from IR to UV and nearly 1 MW peak power. The beam quality M ² is measured to be below 2.     

Absolute frequency measurements of wavelength standards 532 nm, 543 nm, 633 nm and 1540 nm

This paper describes the results of absolute frequency measurements of primary wavelength standards 633 nm, 543 nm, 532 nm, (iodine stabilized) and 1540 nm (acetylene stabilized) in CMI. The values obtained with Menlo Systems femtosecond frequency comb in CMI are compared with previous measurements of the same standards in BIPM, BEV and MPQ. Measured sub-Doppler linewidths and relative intensities of several hyperfine spectral components of iodine molecule are also presented.     

Sub-10 nm writing: focused electron beam-induced deposition in perspective

Over the past decade, focused electron beam-induced deposition has become a mature necessary part of the tool box engineers and scientists. This review presents the current state of the art in sub-10 nm focused electron beam deposition and describes the dominant mechanisms that have been found so far for this regime. Several questions regarding patterning at the highest resolution are addressed. What do our findings mean for using sub-10 nm focused electron beam deposition for industrial applications? And which fundamental issues remain to be solved? The overview shows that low-energy secondary electrons dominate the deposition process. As a result, the highest obtainable spatial resolution (averaged over many deposits) is limited by the mean free path of those electrons. Therefore, the only route to improve the resolution beyond the current appears to be using complexes that are sensitive to the high-energy electrons in the incident beam, rather than to the secondaries. Focused electron beam-induced deposition is compared to related techniques. It is on par with resist-based sub-10 nm electron beam lithography, showing similar spatial resolutions at similar electron doses. Regarding ion beam lithography, there are several distinguishing issues. Sub-10 nm writing has yet to be demonstrated for ion deposition, and although the deposition rate is relatively low when writing with electrons, electrons do not induce damage to the sample. The latter is a crucial advantage for focused electron beam-induced deposition. Finally, the main challenges regarding the applicability of sub-10 nm focused electron beam-induced deposition are discussed.     

Femtosecond diode laser MOPA system at 920 nm based on asymmetric colliding pulse mode-locking

We report on the generation of 267 fs long pulses with a peak power of 661 W emitted by an InGaAs diode laser master-oscillator power-amplifier (MOPA) system with an external grating compressor. The oscillator emits strongly chirped picosecond pulses with several nanometer of bandwidth, which can be amplified without significant phase modulation and are compressed to femtosecond pulses after leaving the amplifier. We used a diode laser module for asymmetric colliding pulse mode-locking and optimized the collision point and the relative intensity of the counter-propagation pulses.     

Effect of metals on UV-excited plasmonic lithography for sub-50 nm periodic feature fabrication

This paper describes and compares the effect of metal films, such as aluminum (Al) and silver (Ag) on UV-excited two-beam surface plasmon interference nanolithography. A planar four-layer configuration has been employed to study the light intensity distribution on the recording medium. It is observed that high-density sub-50 nm periodic structures were achievable by employing the above-mentioned metal films when interrogated with p-polarized, 364 nm illumination wavelength source. It is found that the obtained periodic feature shows good exposure depth and high contrast when Al is used as a metal film. The initial experimental result of planar four-layer configuration is also presented.     

Sub-30 nm lithography with near-field scanning optical microscope combined with femtosecond laser

We report direct laser writing of lithography patterns with a feature width of 20±5 nm on thin photoresist film by combining a double-frequency femtosecond laser and a near-field scanning optical microscope. The obtained feature size is much smaller than the laser wavelength () and the aperture diameter (d) with a resolution of /20 and d/2, respectively. The lithography patterns were analyzed with an atomic force microscope and a scanning electron microscope. The effects of laser energy and writing speed on the feature size were investigated. The underlying physical mechanism was also discussed. PACS 07.79.Fc; 07.79.Lh; 42.70.Jk; 68.37.Hk; 81.16.Nd     

Measurements of cavitation bubble dynamics based on a beam-deflection probe

We present an optodynamic measurement of a laser-induced cavitation bubble and its oscillations based on a scanning technique using a laser beam-deflection probe. The deflection of the beam was detected with a fast quadrant photodiode which was built into the optical probe. The applied experimental setup enabled us to carry out one- or two-dimensional scanning of the cavitation bubble, automatic control of the experiment, data acquisition and data processing. Shadow photography was used as a comparative method during the experiments.     

Narrowband, mid-infrared, seeded optical parametric generator based on non-critical CdSiP2 pumped by 120-ps, single longitudinal mode 1,064 nm pulses

In this work, we present low-threshold, efficient optical parametric generation in CdSiP₂ pumping at 1,064 nm with 120-ps-long, single longitudinal and transverse mode pulses at 230-kHz repetition rate provided by a microchip passively Q-switched master-oscillator power amplifier laser system. Seeding at the signal wavelength with a laser diode, we generated bandwidth-limited idler pulses at 6,100 nm.     

High-gain Al2O3:Nd3+ channel waveguide amplifiers at 880 nm, 1060 nm, and 1330 nm

Neodymium-doped aluminum oxide films with a range of Nd³⁺ concentrations are deposited on silicon wafers by reactive co-sputtering, and single-mode channel waveguides with various lengths are fabricated by reactive ion etching. Photoluminescence at 880, 1060, and 1330 nm from the Nd³⁺ ions with a lifetime of 325 μs is observed. Internal net gain at 845–945 nm, 1064, and 1330 nm is experimentally and theoretically investigated under continuous-wave excitation at 802 nm. Net optical gain of 6.3 dB/cm at 1064 nm and 1.93 dB/cm at 1330 nm is obtained in a 1.4-cm-long waveguide with a Nd³⁺ concentration of 1.68×10²⁰ cm^?3 when launching 45 mW of pump power. In longer waveguides a maximum gain of 14.4 dB and 5.1 dB is obtained at these wavelengths, respectively. Net optical gain is also observed in the range 865–930 nm and a peak gain of 1.57 dB/cm in a short and 3.0 dB in a 4.1-cm-long waveguide is obtained at 880 nm with a Nd³⁺ concentration of 0.65×10²⁰ cm^?3. By use of a rate-equation model, the gain on these three transitions is calculated, and the macroscopic parameter of energy-transfer upconversion as a function of Nd³⁺ concentration is derived. The high internal net gain indicates that Al₂O₃:Nd³⁺ channel waveguide amplifiers are suitable for providing gain in many integrated optical devices.     

Wide-band semi-reflection/transmission film based on diluted Drude metal

We investigate the electromagnetic response of a composite structure consisting of two diluted Drude metal layers with sub-wavelength spacing at microwave frequencies. Simulations show that our structure can be considered as two equivalent thin films with different permittivity layered together so as to effectively tune the transmission T(ω) and reflection R(ω) in a frequency band. We demonstrate a wide band between 5.98 GHz to 8.15 GHz where T(ω) and R(ω) are tuned within 50% ± 2%. Parametric explorations show that the working band can be further shifted by geometric scaling. Our structure has potential to construct a metamaterial-based beam splitter which can be applied in a microwave or even terahertz system.     

Ultra-narrow-linewidth continuous-wave THz sources based on multiplier chains

We demonstrate two different sources at 1.3 THz based on multiplier chains (72nd harmonic generation), which exhibit linewidths at the level of 2×10⁻¹² in relative units. The multiplication processes are shown not to contribute significantly to this linewidth. The phase noise of one of the sources and the fractional power in the carrier (76%) were determined. The application of these sources as references for quantum cascade THz lasers and for spectroscopy of ultracold molecules is suggested. Thus, rotational spectroscopy with few Hz resolution at 1.3 THz is possible with the present easy-to-use sources. An approach for reducing the linewidth by a factor on the order of 10³ to the 1×10⁻¹⁵ level using optical technology is proposed.     

Hierarchy in optical near-fields based on compositions of nanomaterials

Optical near-field interactions exhibit hierarchical responses in the nanometer scale allowing unique functions in nanophotonic systems. Such hierarchical properties in optical near-fields originate various physical entities in the nanometer scale. Engineering nanomaterial compositions, while maintaining geometrically equivalent conditions, leads to characteristic hierarchical responses. We experimentally demonstrate such material-dependent optical near-field hierarchy using core–shell-type nanostructures composed of gold and silver.     

Terahertz subwavelength filters based on a 2D lattice of metal wires

The filtering properties of a 2D square lattice made of metallic wires are investigated through the band structures and transmission spectra by the finite-difference time-domain method. All the results show that the transmission can be affected by factors such as wave polarization, incidence direction, and wire radius. It is found that the Γ–M direction and smaller radius of metal wires are preferable for a high-frequency-pass filter for TE waves, while the Γ–X direction and comparatively greater radius of metal wires are suitable for a low-frequency-pass and a wide stop-band filter for TM waves. Band edges of the filters can be tuned by adjusting the radius of wires and lattice constant. The key features of the band structure and the corresponding transmission spectrum are strongly correlated. Our work demonstrates that detailed band maps can help understanding the transmission properties, which are essential for designing wave filters.     

Femtosecond OPO based on LBO pumped by a frequency-doubled Yb-fiber laser-amplifier system for CARS spectroscopy

We present detailed investigations of a femtosecond green-pumped optical parametric oscillator (OPO) based on lithium triborate. As pump source, a frequency-doubled Yb-fiber laser-amplifier system is used. The OPO generates signal pulses tunable over a spectral range from 780 to 940 nm and idler pulses tunable from 1630 to 1190 nm. More than 250 mW are generated in the signal beam and more than 300 mW in the idler beam. Without dispersion compensation chirped signal pulses with a pulse duration between 100 and 250 fs are measured. Using this system for coherent anti-Stokes Raman scattering spectroscopy, vibrational resonances between 1110 and 6760 cm⁻¹ can be excited. Due to the chirped pulses, a spectral resolution of 100 cm⁻¹ is achieved, which is 2.5 times higher compared to an excitation with time-bandwidth limited pulses.     

Ozone concentration-monitoring photoacoustic system based on a frequency-quadrupled Nd:YAG laser

A novel type of system based on a frequency-quadrupled Nd:YAG laser light source at 266 nm and a dual-cell photoacoustic detection unit was developed, and its applicability for ozone-concentration measurement with a minimum detectable ozone concentration of about 100 pptV was demonstrated. The instrument was calibrated against an ozone generator, and it was installed at a regional environmental monitoring station to be operated in parallel with a commercial UV-absorption photometry based ozone-monitoring instrument. While good agreement between the readings of the two systems was found, the photoacoustic system outperformed its optical absorption based counterpart as far as minimum detectable concentration and measurement accuracy is concerned.     

A new polarimeter based on optical non-reciprocity in gratings with two-dimensional chirality

We have studied the optical transmission properties of a number of different dielectric diffraction gratings that each exhibit two-dimensional chirality in their grating elements. We have found that the diffracted beams transmitted through these structures exhibit large anisotropic polarization changes and polarization-dependent intensity modulations even though the chiral elements are arranged in square grating arrays. The strength and functional form of both of these effects differ for each diffracted beam. They are also dependent on the chirality of the surface patterning and the thickness of the patterned dielectric film. We show how these properties could be exploited to provide a new and more versatile form of polarimeter, and how the operation of such a device is inherently dependent on the optical non-reciprocity of these chiral gratings.     

Linewidth studies on Cd+ 636.0 nm and 537.8 nm lines excited in a He-Cd hollow cathode discharge

Hollow cathode (HC) lasers usually operate in a single axial mode without any optical selection. This is attributed to the large homogeneous linewidth of the gain curve due to the relatively high filling pressure of these lasers. Collisional and Doppler broadening (Δν_C and Δν_D) of the Cd⁺ 636 nm and Cd⁺ 538 nm lines (laser transitions of the HeCd⁺ laser) excited in a HC discharge tube were determined using a Fabry–Perot interferometer technique. It was found that in the pressure range 7–25 mbar Δν_D was nearly constant, while, as expected, Δν_C increased linearly with pressure. The broadening constants were α(636 nm)= (47±2) MHz/mbarand α(538 nm)=(11.8±0.5) MHz/mbar. The first constant is large enough to explain single-mode operation of the red HeCd⁺ laser; but in the case of the green laser, the exact reason for the single-mode operation remained unclear. Received: 23 November 2000 / Revised version: 30 March 2001 / Published online: 7 June 2001