Tuning the Kondo effect with a mechanically controllable break junction

We study electron transport through C(60) molecules in the Kondo regime using a mechanically controllable break junction. By varying the electrode spacing, we are able to change both the width and the height of the Kondo resonance, indicating modification of the Kondo temperature and the relative strength of coupling to the two electrodes. The linear conductance as a function of T/T(K) agrees with the scaling function expected for the spin-1/2 Kondo problem. We are also able to tune finite-bias Kondo features which appear at the energy of the first C(60) intracage vibrational mode.     

Kondo effect in quantum dots at high voltage: universality and scaling

We examine the properties of a dc-biased quantum dot in the Coulomb blockade regime. For voltages V that are large compared to the Kondo temperature T(K), the physics is governed by the scales V and gamma, where gamma approximately V/ln(2)(V/T(K)) is the nonequilibrium decoherence rate induced by the voltage-driven current. Based on scaling arguments, self-consistent perturbation theory, and perturbative renormalization group, we argue that due to the large gamma the system can be described by renormalized perturbation theory in 1/ln(V/T(K))<1. However, in certain variants of the Kondo problem, two-channel Kondo physics is induced by a large voltage V.     

Kondo universal scaling for a quantum dot coupled to superconducting leads

We study competition between the Kondo effect and superconductivity in a single self-assembled InAs quantum dot contacted with Al lateral electrodes. Because of Kondo enhancement of Andreev reflections, the zero-bias anomaly develops side peaks, separated by the superconducting gap energy Delta. For ten valleys of different Kondo temperature T(K) we tune the gap Delta with an external magnetic field. We find that the zero-bias conductance in each case collapses onto a single curve with Delta/k(B)T(K) as the only relevant energy scale, providing experimental evidence for universal scaling in this system.     

Measurement of quantum noise in a carbon nanotube quantum dot in the Kondo regime

The current emission noise of a carbon nanotube quantum dot in the Kondo regime is measured at frequencies ν of the order or higher than the frequency associated with the Kondo effect k(B)T (K)/h, with TK the Kondo temperature. The carbon nanotube is coupled via an on-chip resonant circuit to a quantum noise detector, a superconductor-insulator-superconductor junction. We find for hν ≈ k(B)T(K) a Kondo effect related singularity at a voltage bias eV ≈ hν, and a strong reduction of this singularity for hν ≈ 3k(B)T(K), in good agreement with theory. Our experiment constitutes a new original tool for the investigation of the nonequilibrium dynamics of many-body phenomena in nanoscale devices.     

Quantum dots with even number of electrons: kondo effect in a finite magnetic field

We show that the Kondo effect can be induced by an external magnetic field in quantum dots with an even number of electrons. If the Zeeman energy B is close to the single-particle level spacing Delta in the dot, the scattering of the conduction electrons from the dot is dominated by an anisotropic exchange interaction. A Kondo resonance then occurs despite the fact that B exceeds by far the Kondo temperature T(K). As a result, at low temperatures T相似文献   

Current-induced decoherence in the multichannel Kondo problem

The properties of a local spin S=1/2 coupled to K independent wires is studied in the presence of bias voltages which drive the system out of thermal equilibrium. For K?1, a perturbative renormalization group approach is employed to construct the voltage-dependent scaling function for the conductance and the T matrix. In contrast to the single-channel case, the Kondo resonance is split even by bias voltages small compared to the Kondo temperature T(K), V?T(K). Besides the applied voltage V, the current-induced decoherence rate Γ?V controls the physical properties of the system. While the presence of V changes the structure of the renormalization group considerably, decoherence turns out to be very effective in prohibiting the flow towards new nonequilibrium fixed points even in variants of the Kondo model where currents are partially suppressed.     

Even-odd effect in Andreev transport through a carbon nanotube quantum dot

We have measured the current (I)-voltage (V) characteristics of a single-wall carbon nanotube quantum dot coupled to superconducting source and drain contacts in the intermediate coupling regime. Whereas the enhanced differential conductance dI/dV due to the Kondo resonance is observed in the normal state, this feature around zero-bias voltage is absent in the superconducting state. Nonetheless, a pronounced even-odd effect appears at finite bias in the dI/dV subgap structure caused by Andreev reflection. The first-order Andreev peak appearing around V=Delta/e is markedly enhanced in gate-voltage regions, in which the charge state of the quantum dot is odd. This enhancement is explained by a "hidden" Kondo resonance, pinned to one contact only. A comparison with a single-impurity Anderson model, which is solved numerically in a slave-boson mean-field approach, yields good agreement with the experiment.     

Kondo model for the "0.7 anomaly" in transport through a quantum point contact

Experiments on quantum point contacts have highlighted an anomalous conductance plateau around 0.7(2e(2)/h), with features suggestive of the Kondo effect. Here, an Anderson model for transport through a point contact analyzed in the Kondo limit. Hybridization to the band increases abruptly with energy but decreases with valence, so that the background conductance and the Kondo temperature T(K) are dominated by different valence transitions. This accounts for the high residual conductance above T(K). The model explains the observed gate-voltage, temperature, magnetic field, and bias-voltage dependences. A spin-polarized current is predicted even for low magnetic fields.     

Universality of the Kondo effect in quantum dots with ferromagnetic leads

We investigate quantum dots in clean single-wall carbon nanotubes with ferromagnetic PdNi-leads in the Kondo regime. Most of the Kondo resonances exhibit a splitting, which depends on the tunnel coupling to the leads and an external magnetic field B, but only weakly on the gate voltage. Using numerical renormalization group calculations, we demonstrate that all salient features of the data can be understood using a simple model for the magnetic properties of the leads. The magnetoconductance at zero bias and low temperature depends in a universal way on gμ(B)(B-B(c))/k(B)T(K), where T(K) is the Kondo temperature and B(c) the external field compensating the splitting.     

Climbing the entropy barrier: driving the single- towards the multichannel Kondo effect by a weak coulomb blockade of the leads

We study a model proposed recently in which a small quantum dot is coupled symmetrically to several large quantum dots characterized by a charging energy E(c). Even if E(c) is much smaller than the Kondo temperature T(K), the long-ranged interactions destabilize the single-channel Kondo effect and induce a flow towards a multichannel Kondo fixed point associated with a rise of the impurity entropy with decreasing temperature. Such an "uphill flow" implies a negative impurity specific heat, in contrast with all systems with local interactions. An exact solution found for a large number of channels allows us to capture this physics and to predict transport properties.     

Evidence for charge Kondo effect in superconducting Tl-doped PbTe

We report results of low-temperature thermodynamic and transport measurements of Pb1-xTlxTe single crystals for Tl concentrations up to the solubility limit of approximately x=1.5%. For all doped samples, we observe a low-temperature resistivity upturn that scales in magnitude with the Tl concentration. The temperature and field dependence of this upturn are consistent with a charge Kondo effect involving degenerate Tl valence states differing by two electrons, with a characteristic Kondo temperature T(K) approximately 6 K. The observation of such an effect supports an electronic pairing mechanism for superconductivity in this material and may account for the anomalously high T(c) values.     

Mesoscopic Kondo screening effect in a single-electron transistor embedded in a metallic ring.

We study the Kondo screening effect generated by a single-electron transistor or quantum dot embedded in a small metallic ring. When the ring circumference L becomes comparable to the fundamental length scale xi(0)(K) = Planck's constant over upsilon(F)/T(0)(K) associated with the bulk Kondo temperature, the Kondo resonance is strongly affected, depending on the total number of electrons (mod4) and magnetic flux threading the ring. The resulting Kondo-assisted persistent currents are also calculated in both Kondo and mixed-valence regimes, and the maximum values are found in the crossover region.     

Critical Kondo destruction in a pseudogap Anderson model: scaling and relaxational dynamics

We study the pseudogap Anderson model as a prototype system for critical Kondo destruction. We obtain finite-temperature (T) scaling functions near its quantum-critical point, by using a continuous-time quantum Monte Carlo method and also considering a dynamical large-N limit. We are able to determine the behavior of the scaling functions in the typically difficult to access quantum-relaxational regime (?ω相似文献   

Kondo effect in a magnetic field and the magnetoresistivity of kondo alloys

The effect of a magnetic field on the spectral density of a S = 1/2 Kondo impurity is investigated at zero and finite temperatures by using Wilson's numerical renormalization group method. A splitting of the total spectral density is found for fields larger than a critical value H(c)(T = 0) approximately 0.5T(K), where T(K) is the Kondo scale. The splitting correlates with a peak in the magnetoresistivity of dilute magnetic alloys which we calculate and compare with the experiments on CexLa1-xAl2,x = 0.0063. The linear magnetoconductance of quantum dots exhibiting the Kondo effect is also calculated.     

Temperature dependence of a single Kondo impurity

Recent advances in scanning tunneling microscopy have allowed the observation of the Kondo effect for individual magnetic atoms. One hallmark of the Kondo effect is a strong temperature-induced broadening of the Kondo resonance. In order to test this prediction for individual impurities, we have investigated the temperature dependent electronic structure of isolated Ti atoms on Ag(100). We find that the Kondo resonance is strongly broadened in the temperature range T = 6.8 K to T = 49.0 K. These results are in good agreement with theoretical predictions for Kondo impurities in the Fermi liquid regime, and confirm the role of electron-electron scattering as the main thermal broadening mechanism.     

Specific heat of Ce0.8La0.2Al3 in magnetic fields: a test of the anisotropic Kondo picture

The specific heat C of Ce0.8La0.2Al3 has been measured as a function of temperature T in magnetic fields up to 14 T. A large peak in C at 2.3 K has recently been ascribed to an anisotropic Kondo effect in this compound. A 14-T field depresses the temperature of the peak by only 0.2 K, but strongly reduces its height. The corresponding peak in C/T shifts from 2.1 K at zero field to 1.7 K at 14 T. The extrapolated specific heat coefficient gamma = lim as T --> 0 of C/T increases with field over the range studied. We show that these trends are inconsistent with the anisotropic Kondo model.     

Divergence at low bias and down-mixing of the current noise in a diffusive superconductor-normal-metal-superconductor junction

We present current noise measurements in a long diffusive superconductor-normal-metal-superconductor junction in the low voltage regime, in which transport can be partially described in terms of coherent multiple Andreev reflections. We show that, when decreasing voltage, the current noise exhibits a strong divergence together with a broad peak. We ascribe this peak to the mixing between the ac-Josephson current and the noise of the junction itself. We show that the junction noise corresponds to the thermal noise of a nonlinear resistor 4k B T/R with R=V/I(V) and no adjustable parameters.     

Experimental test of the numerical renormalization-group theory for inelastic scattering from magnetic impurities

We present measurements of the phase coherence time taupsi in quasi-one-dimensional Au/Fe Kondo wires and compare the temperature dependence taupsi of with a recent theory of inelastic scattering from magnetic impurities [Phys. Rev. Lett. 93, 107204 (2004)10.1103/PhysRevLett.93.107204]. A very good agreement is obtained for temperatures down to 0.2T(K). Below the Kondo temperature T(K), the inverse of the phase coherence time varies linearly with temperature over almost one decade in temperature.     

Universal scaling in nonequilibrium transport through a single channel Kondo dot

Scaling laws and universality play an important role in our understanding of critical phenomena and the Kondo effect. We present measurements of nonequilibrium transport through a single-channel Kondo quantum dot at low temperature and bias. We find that the low-energy Kondo conductance is consistent with universality between temperature and bias and is characterized by a quadratic scaling exponent, as expected for the spin-1/2 Kondo effect. We show that the nonequilibrium Kondo transport measurements are well described by a universal scaling function with two scaling parameters.     

Kondo state for a compact Cr trimer on a metallic surface

The ground state of a Cr trimer supported on the Au(111) surface is investigated by means of a variational approach to the Coqblin-Schrieffer Hamiltonian. The temperature of Kondo-resonance formation (T(K)) for equilateral trimers increases drastically as compared to T(K) for a single Cr adatom. The Kondo state of a Cr trimer proves to be very sensitive to geometry and a small shift of any atom from the symmetrical position leads to a rapid decrease in T(K). These results are in good agreement with recent observations of the Kondo response of a single antiferromagnetic chromium trimer [T. Jamneala, Phys. Rev. Lett. 87, 256804 (2001)]].