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The reflection of protons from a partially cesiated tungsten surface is studied in the energy domain between 100 and 2000 eV and in the angular domain between 75° and 85° with respect to the surface normal. The study is performed by measuring the angular and energy distribution of the scattered negative ions. The reflection can take place along two paths. One path is reflection from the cesium surface layer, the other one is reflection from the tungsten substrate. A dependence of the final charge state on the path is observed. It is inferred that this phenomenon is due to incomplete neutralization of the protons scattered from the cesium layer. The energy loss of the reflected ions cannot be accounted for by using only the binary collision model. Also the electronic stopping of the atoms by the metal electrons is shown to be an important energy loss mechanism. Total conversion measurements of H+ to H- combined with the measurements of the negatively charged fraction of the scattered particles, as reported in the proceeding paper, yield the particle reflection coefficient as a function of the angle of incidence. These reflection coefficients show that for angles of incidence less than 75° already more than 50% of the particles do not reflect from the surface. Total conversion efficiency measurements with H- ions as primary ions show that the influence of the initial charge state on the total conversion is very small.  相似文献   

3.
Scattering from rough surfaces is studied using a perturbative treatment of the Ewald-Oseen extinction theorem. Expressions for the first and second order fields in the roughness parameter are presented for arbitrary incident fields and used for the calculation of scattering and extinction cross sections. The cross sections are shown to have contributions from diffuse scattering as well as from surface polariton emission and include the hitherto studied effects such as Smith-Purcell radiation, Wood anomalies and reflectance drops at rough surfaces.  相似文献   

4.
The formation of negative hydrogen ions by scattering protons from a metal surface is described with two models: a probability model and an amplitude model. In both models the electron motion is described quantum mechanically and the nuclear motion classically. However, in the probability model the time evolution of the ionization probability is considered, while in the amplitude model the time evolution of the corresponding wave function amplitude is considered. The electron affinity level of an atom close to the metal is lowered by means of image forces and broadened due to resonant transition of an electron between te conduction band of the metal and the valence shell of the atom. The calculated position of the affinity level and the transition rate in both models give rise to maximum negative ionization efficiencies of 4% on W(110), 40% on cesiated tungsten and 15% on cesium.  相似文献   

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Molecular beam scattering from surfaces offers a unique method for studying elementary gas-solid collisions. Recent technological advances have made it possible to study elastic and inelastic scattering from clean surfaces characterized by LEED and Auger spectroscopy. These experiments have provided information on surface structures, with and without adsorbed gases, on the gas-surface interaction potential, and on inelastic collisions involving phonon annihilation and creation. These recent measurements are reviewed and discussed in terms of the latest theoretical work.  相似文献   

7.
Alkali atoms have been shown previously to have only unstable binding states inside liquid4He. We calculate the equilibrium configurations and binding energies of single alkali atoms near the liquid-vapor interface of4He and3He. A simple interface model is used to predict the surface deformation due to the presence of the atoms. A more realistic density functional model yields somewhat higher energies in the case of4He. For all alkali atoms, we find the surface binding energies to be around 10 to 20 K. A similar analysis with atom-H2 interactions finds that alkali atoms tend to submerge into liquid H2, with the exception of Li.  相似文献   

8.
B.F. Mason  B.R. Williams 《Surface science》1987,180(2-3):L134-L140
Three diverse rough surfaces have been studied using inelastic He scattering. The first is an ion bombarded Ag(110) surface where a broadened specular peak remains visible but scattering remains entirely elastic as viewed by the incoherent component. The second is a cleaved Te(10 ) surface composed of helical chains where the roughness originates from thermal oscillations and scattering is almost entirely inelastic. Thirdly, a glass (7740) disc is shown to be physically rough but the surface is sufficiently rigid to yield largely elastic incoherent scattering.  相似文献   

9.
Hiromu Asada 《Surface science》1981,110(2):270-286
Scattering of linear molecules, which are internally deactivated initially, from solid surfaces is investigated classical mechanically. The solid is modeled with a three-dimensional isotropic Debye solid whose surface is essentially flat but thermally roughened by lattice vibration, and the molecule is described as a rigid body, which interacts with the solid via an exponential potential wall and a stationary attractive potential well. A variation in the interaction energy due to thermal roughening of the surface and due to nonsphericity of the molecule being regarded as perturbations on the system, a second order perturbation theory is developed to construct a Gaussian velocity distribution function of molecules scattered off the exponential wall and still moving inside the potential well. Among the molecules in the distribution, those with sufficient energy to escape from the potential well are regarded as being scattered into the free space. This model shows that the major differences between the scattering of monatomic molecules and that of linear ones result from less normal momentum transfer to the linear molecules than to the monatomic ones.  相似文献   

10.
Coupled channels problem for kaonic hydrogen is solved using nonlocal potentials + Coulomb potential. It is applied for model and realistic problem for KH andKHe.Presented at the symposium Mesons and Light Nuclei, Bechyne, Czechoslovakia, May 27–June 1,1985.Supported in part by the DOE, Contract No. DE-ATO6-79ER10405.  相似文献   

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Differential cross sections for negative pion scattering on 4He have been measured at five pion kinetic energies between 110 and 260 MeV in the angular range from 5° to 180°. Total cross sections have also been measured at eleven energies between 67 and 285 MeV. The differential cross sections have been fitted with a phenomenological expression for the nuclear scattering amplitude. Conventional phase shifts have been reconstructed starting from the parameters of the fits.  相似文献   

13.
Abstract

Reflection and scattering of waves from plane and statistically rough interfaces between nonlinear media are studied theoretically. New hysteresis-type dependences of the reflection and transmission coefficients on the amplitude of the incident wave and on the angle of incidence are predicted. Scattering diagrams for diffusely reflected and transmitted fields are calculated. It is found that when the dielectric constant is a steep function of the incident amplitude, nonlinearity suppresses the Bragg resonant scattering mechanism. Smooth roughness of the boundary is shown to enhance the penetration of evanescent waves into nonlinear media.  相似文献   

14.
Scattering of potassium atomic beams from cleaved surfaces of LiF, KCl and mica were studied. The observed spatial distributions follow the cosine distribution in most cases. At large incident angles the distributions from LiF and KCl deviate from the cosine and show apparent backscatterings. A simple model is proposed to interpret the backscattering in terms of macroscopic roughness of cleaved surfaces. The sticking coefficient S (t) is defined and the mass balance between the incident and outgoing atoms is examined. Mass balance holds within the limits of errors on the surfaces of LiF and KCl at temperatures above 400 K. On a mica surface deposition of potassium atoms is observed even at temperatures higher than room temperature. It is shown from the change of the sticking coefficient that the deposition does not proceed linearly in the initial period.  相似文献   

15.
We have developed an experimental method based on the visibility factor of light-scattering minima to obtain size-polydispersity information from contaminants upon a flat substrate. We verify the method by using double-interaction-model calculations and use this technique to examine experimentally the radial variation of a micrometer-sized fiber and the size polydispersity of spherical particles upon a substrate.  相似文献   

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Total and differential cross sections for simultaneous excitation of H(2s), H(3s) and He(1s 2s) by electron impact in the presence of a photon field have been calculated in second-order perturbation theory. The characteristics of the results are interpreted in terms of their physical origin. The off-shell excitation cross section for the He(1s 2s) state is found to be one order of magnitude smaller than that for excitation of the H(2s) state. This is consistent with our expection that atoms with higher dipole-polarisability should favour larger off-shell cross sections for transitions betweens-states.  相似文献   

18.
D. Viel 《Il Nuovo Cimento D》1991,13(11):1361-1367
Summary The scattering of μp atoms in the 1S state from gold atoms was calculated using semi-classical methods. The results were used to write a Monte Carlo program simulating backscattering from a gold surface. For isotropically incident μp of kinetic energy (0.035–10) eV it was found that approximately 5% escape from the surface. The fraction backscattered showed little dependence on the initial μp kinetic energy but increased greatly with incident angle from the normal to the surface.  相似文献   

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This paper deals with the scattering of a TM plane wave from conductive periodic random surfaces. By means of the stochastic functional approach, the scattered field is expressed in terms of a harmonic series representation, in which the coefficients are homogeneous random functions and are given by Wiener-Hermite expansions. An approximate solution for the Wiener kernels is obtained up to the second order. Several anomalies appear in the angular distribution of the incoherent scattering because of combinations of scattering due to surface randomness and diffraction due to surface periodicity. These are incoherent Wood's anomalies associated with guided surface waves propagating along the surface, enhanced backscattering and diffracted backscattering enhancement. The physical reasons for these anomalies and numerical results are discussed.  相似文献   

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