Dependence of the lidar signal depolarization on the receiver’s field of view in the sounding of fog and clouds

We report an experimental study of the lidar signal depolarization as a function of the relative contribution of the multiple scattering in case of optically dense objects in the atmospheric planetary boundary layer. Results of the observation of fog and stratus clouds are presented, as well as those obtained by sounding of stratocumulus clouds during a snowfall. The lidar data point to a rise of the depolarization coefficient as the influence of the multiple scattering increases in consequence of both viewing angle enlargement and penetration into the object sounded. The variations of the depolarization coefficient are studied as a function of the field of view. In the case of fog, this dependence is approximated by a three-parameter exponential law; it is found that the depolarization increases steeply when the viewing angle is increased from 9 mrad to 12.5 mrad. The relationships between the approximation parameters and the microphysical characteristics of the scattering medium are considered. The experimentally determined size of the area where multiple scattering occurs is in good agreement with that calculated according to the diffusion model. The results obtained on the multiple scattering effect on the depolarization can also be employed in determining the extinction coefficient profiles in optically dense objects, as well as in evaluating the characteristic size of the scattering particles. Received: 6 September 1999 / Revised version: 7 February 2000 / Published online: 6 September 2000     

Study of atmospheric water in gaseous and. liquid state by using combined elastic–Raman. depolarization lidar

A combined elastic–Raman lidar system based on a tripled Nd:YAG laser is used for the separate detection of elastic backscatter and Raman signals from atmospheric nitrogen, water vapor and liquid water and for their depolarization measurement. Vertical profiles of water-vapor and liquid-water content measured under clear-sky conditions behave differently: inside the boundary layer the ratio of liquid-water to water-vapor Raman backscatters rises with altitude. The depolarization measurements bring additional information about atmospheric scattering. The observed depolarization ratio of the water-vapor Raman signal is about 14%, while for liquid water this ratio varies in the 30–75% range, which exceeds the depolarization of bulk water and is attributed to the water-aerosol effects. Raman contours of water vapor and liquid water are partially overlapped, and bleed-through of liquid-water Raman backscatter leads to enhancement of depolarization of the water-vapor Raman signal. This parameter may be used as a convenient indicator of liquid-water interference in water-vapor measurements. Received: 12 December 2000 / Revised version: 27 September 2001 / Published online: 7 November 2001     

New method of elaboration of the lidar signal

In lidar measurements noise and fluctuations strongly affect the results. The reason is a rapid decrease of the signal-to-noise ratio with an increase of distance. The differential absorption lidar (DIAL) is particularly sensitive to the signal instabilities. In this paper we present a method of the signal acquisition that is suitable for registration of both large light fluxes and single photons. We also present new method of solution of the DIAL equations. Compared to the traditional algorithm used for signal elaboration our procedures are much more stable and they are able to increase the effective range of lidar measurements. Received: 2 February 1999 / Revised version: 30 June 1999 / Published online: 16 September 1999     

Multiply scattered component of lidar returns

The results of statistical simulation of the spatiotemporal structure of the multiply scattered component of lidar returns by the Monte Carlo method are discussed for the case of monostatic sensing geometry. The spatial characteristics of the region of the medium where occurs the last scattering of photon before arriving at the reciever. This region of the medium is called the instantaneous brightness body of multiply scattered radiation. It is demonstrated that the instantaneous brightness body of multiply scattered radiation that propagates toward the receiver may occupy a large volume that does not necessarily coincide with the region of formation of the singly scattered component. The main factors influencing the spatial and brightness characteristics of this volume source are established. The effect of scattering order on the spatiotemporal structure of lidar returns is analyzed for the case of sensing of aerosol haze and advective and radiative fogs with optical thickness 2<τ<8. Received: 2 August 2001 / Revised version: 7 January 2002 / Published online: 25 September 2002 RID="*" ID="*"Corresponding author. Fax: +7-38/2225-8026, E-mail: belov@iao.ru     

An algorithm to determine cirrus properties from analysis of multiple-scattering influence on lidar signals

A Monte Carlo-based evaluation of the multiple-scattering influence on ground-based Raman lidar measurements is presented. The lidar returns from cirrus clouds are analyzed in order to evaluate vertical profiles of the extinction and backscattering coefficients. Results show that for the typical cirrus cloud, the presence of the multiple scattering can lead to an underestimation of the extinction coefficient by as large as 200% whereas the backscattering coefficient is almost unaffected for the Raman lidar technique. An algorithm to select one or a set of phase functions which fit to the lidar data is also presented. It is an iterative procedure based on Monte Carlo scattering simulation. By comparison of the experimental value of the lidar ratio, corrected for the multiple scattering influence, and the phase function used in the Monte Carlo simulation, one can determine a suitable phase function. The validity and sensitivity of the algorithm have been demonstrated by applying it to simulated cases. The application to some real cases indicates that our procedure allows for the establishing of a practical scattering model for the cirrus clouds.     

Application of lidar in ultraviolet,visible and infrared ranges for early forest fire detection

The efficiencies of direct lidars operating at 355, 532, 1064 and 1540-nm radiation wavelengths for early forest fire detection were compared. For each wavelength, the range for reliable smoke-plume detection was estimated on the basis of a computer simulation plume using a one-dimensional “top-hat” gas dynamic model for the calculation of the backscattering and extinction-coefficient profiles within the plume. The agreement between the predicted signal-to-noise ratio (SNR) and experimental results for 532 and 1064-nm wavelength radiation is good. The decrease of the signal-to-noise ratio with distance is maximum for 355 nm and minimum for 1064 nm. At 1540 nm, the decay of SNR with distance is slightly faster, but the SNR is higher than for other wavelengths, leading to the highest detection efficiency for the same energy of the probing laser pulse. For a burning rate of 2 kg/s and a laser beam divergence of 2.5 mr, the maximum distance for reliable detection varies between 6 and 12 km, depending on the wavelength. Received: 15 May 2002 / Revised version: 13 September 2002 / Published online: 22 January 2003 RID="*" ID="*"Corresponding author. Fax: +351-21/841-8120, E-mail: rui.vilar@ist.utl.pt     

Deconvolution filtering of ground-based LIDAR returns from tropospheric aerosols

A deconvolution filtering model of multiple scattering in ground-based single field of view (SFOV) LIDAR returns is described. It is based on time series deconvolution techniques. The contribution of multiply scattered photons in SFOV LIDAR returns can be numerically modeled by processing LIDAR signals without additional information about aerosol properties and measurement geometry. Deconvolution results are in good agreement with those performed by Monte Carlo calculations, showing that the significance of multiply scattered photons is strongly correlated with aerosol concentration. It is found that, for ground-based LIDAR, the contribution of multiply scattered photons to LIDAR signals is typically below 5% in a clear urban atmosphere, and up to 14% in a very dirty urban atmosphere in Hong Kong during winter seasons. Received: 8 October 2002 / Revised version: 29 January 2003 / Published online: 22 May 2003 RID="*" ID="*"Corresponding author. Fax: +81-298/51-8229, E-mail: gao@proteo.gr.jp RID="**" ID="**"Present address: Preteomics Lab., Amakubo 1-16-1, Tsukuba 305-0005, Japan     

A LIDAR technique to measure the filament length generated by a high-peak power femtosecond laser pulse in air

We demonstrate a new method for measuring the length of a femtosecond laser pulse induced filament in air using a LIDAR (LIght Detection And Ranging) technique. The LIDAR involves a detector with a fast response time. The back-scattered multiphoton induced fluorescence from nitrogen molecules excited inside the filament is measured, from which the length of the filament can be determined. We find good agreement between the measured filament length and the length estimated from burn patterns on paper. In addition, good qualitative agreement between the experimental measurement and numerical simulations is obtained for the signal features of the filament. We propose that this new method can be used to quantitatively determine filamentation at longer distances. Received: 11 June 2002 / Revised version: 21 October 2002 / Published online: 5 February 2003 RID="*" ID="*"Corresponding author. Fax: +1-418/656-2623, E-mail: aiwasaki@phy.ulaval.ca     

Estimation of required parameters for detection of small smoke plumes by lidar at 1.54 μm

Parameters of eyesafe lidar at 1.54 μm for detection of small plumes of smoke from burning wood or oil have been evaluated. It was assumed that a diode-pumped solid-state Er:glass laser at 1.54 μm or a Nd:YAG laser with a Raman cell or optical-parametric oscillator is used as a light source and that detection of backscattered light is performed with an avalanche photodiode. Ash and soot particle size distributions were taken from experiments. A backscattering coefficient at 1.54 μm for various source of smoke was estimated. In computing the laser energy, range between lidar and smoke, receiver optics diameter, fuel mass burned in unit time, fire source radius, laser pulse duration and visibility were varied. Results of the computations enabled estimation of the required laser energy, which ranges from 0.05 to 1400 mJ depending on the parameters. Received: 5 January 2000 / Revised version: 3 March 2000 / Published online: 11 May 2000     

Detection of small forest fires by lidar

The possibility of detecting small forest fires with the help of a simple and cheap lidar operating at 0.532-μm wavelength up to distances of about 6.5 km is demonstrated. The values of the signal-to-noise ratio (SNR) achieved in the experiments are consistent with theoretical estimations obtained by computational modeling of the lidar detection process, including simulation of the smoke-plume shape and of the laser beam–plume interaction. This model was used to assess the potential of the lidar technique for fire surveillance in large forest areas. In particular, the upper limiting range for effective detection (SNR>5) of small localized fires in dry- and clear-weather conditions is estimated at 7–15 km depending on operation mode, burning rate, and observation geometry. Received: 29 August 2001 / Published online: 29 November 2001     

Analysis of lidar measurements using nonparametric kernel regression methods

The lidar technique is an efficient tool for remote monitoring of the distribution of a number of atmospheric species. We study measurements of sulphur dioxide emitted from the Italian volcano Mt. Etna. This study is focused on the treatment of data and on the procedure to evaluate range-resolved concentrations. In order to make an in-depth analysis, the lidar system was prepared to store measurements of individual backscattered laser pulses. Utilizing these repeated measurements a comparison of three different methods to average the returned signals is made. In the evaluation process we use local polynomial regression to estimate the range-resolved concentrations. Here we calculate optimal bandwidths based on the empirical-bias bandwidth selector. We also compare two different variance estimators for the path-integrated curves: local polynomial variance estimation and variance estimation based on Taylor approximations. Results show that the method performs well. An advantage compared to previous methods for evaluation of lidar measurements is that an estimate of the mean squared error of the estimated concentration can be calculated. Received: 9 July 2001 / Revised version: 15 November 2001 / Published online: 17 January 2002     

Current state-of-the-art of LIDAR inversion methods for atmospheres of arbitrary optical density

It is the intention of this paper to report on the currently used methods to solve the different LIDAR signal inversion problems for molecular atmospheres, aerosols and clouds. Apart from more traditional approaches, we shall present a recent one using multiple scattering effects rather than avoiding them, which is useful especially for dense clouds.     

Plasma-based nitrogen tail pulse shutter for CO2-TEA lidar dial systems

This paper presents the construction, use and characterisation of a laser-induced sealed plasma shutter to clip off the nitrogen pulse tail of a CO₂-TEA laser-based lidar dial system. Investigation of the optimum gas filling pressure, temporal profile of the clipped pulse, and the laser threshold power intensities to achieve ionisation growth and breakdown in helium, argon, and nitrogen are also presented. Values of these power density thresholds lie between 3×10¹¹ W cm^-2–5×10¹² W cm^-2, 2×10¹¹ W cm^-2–2×10¹² W cm^-2 and 3×10¹³ W cm^-2–2×10¹⁴ W cm^-2 for helium, argon, and nitrogen, respectively. The range resolution attainable with the present clipped pulses is 15 m, which is 30 times better than that readily obtained with the nitrogen-tailed pulses. Field measurements of the lidar returns with the clipped pulse from a co-operative target are presented. Received: 27 December 1999 / Revised version: 11 February 2000 / Published online: 27 April 2000     

The LITE correlative measurements campaign in southern Italy: preliminary results

A,355 and R_A,532); the two data sets appearing to be highly correlated. LITE vs. Potenza LIDAR measurements of R_A,355 and R_A,532 display a correlation coefficient of 0.72 and 0.86, respectively. Stratospheric aerosol dimensional characteristics are determined starting from the measured values of the ?ngstrom coefficient. Received: 24 May 1996/Revised version: 8 October 1996     

Measurement of filament length generated by an intense femtosecond laser pulse using electromagnetic radiation detection

We present a new method to measure the length of a filament induced by the propagation of intense femtosecond laser pulses in air. We used an antenna to detect electromagnetic pulses radiated from multipole moments inside the filament oscillating at the plasma frequency. The results are compared with the values detected from the backscattered fluorescence induced by multiphoton ionization of nitrogen molecules excited inside the filament. The values are found to be in good agreement. Received: 6 November 2002 / Revised version: 27 January 2003 / Published online: 24 April 2003 RID="*" ID="*"Corresponding author. Fax: +1-418/656-2623, E-mail: shosseini@phy.ulaval.ca     

Quantitative wavelength-modulation spectroscopy without certified gas mixtures

We study the quantification of signal strength in wavelength-modulation spectroscopy, and present algorithms which allow for the quantitative analysis of second-harmonic spectra for arbitrary combinations of line width and modulation depth. The algorithms are validated through measurements on CO lines in the 0 ? 3 overtone band. They can be used for measuring the line strength of lines that are too weak to allow direct absorbance measurements, and for quantifying the response from monitors applying wavelength-modulation under conditions where calibration with certified gases is not feasible. Received: 20 August 1999 / Revised version: 2 September 1999 / Published online: 30 November 1999     

Diode-laser-seeded optical parametric oscillator for airborne water vapor DIAL application in the upper troposphere and lower stratosphere

Received: 4 May 1998/Revised version: 17 July 1998     

Silver-island films probed by hyper-Rayleigh scattering and atomic force microscopy

Incoherent second-harmonic generation, or hyper-Rayleigh scattering (HRS), and atomic force microscopy (AFM) are proposed as a combined probe of nonlinear optical and structural properties of silver-island films. HRS and linear (Rayleigh) scattering indicatrices are measured. The correlation function, deduced from the HRS indicatrices and characterising spatial fluctuations of the total polarisation at second-harmonic frequency, has a length scale significantly larger than that of the correlation functions that are obtained from the AFM data and characterise spatial fluctuations of quadratic optical susceptibilities of the dipole and quadrupole types. This difference is interpreted as indicating that the HRS indicatrix shape is determined by the long-range fluctuations of the local-field factors. Received: 16 October 2001 / Revised version: 16 April 2002 / Published online: 6 June 2002     

The application of quasi-phase-matched parametric light sources to practical infrared chemical sensing systems

Quasi-phase-matched (QPM) materials allow the generation of spectroscopically useful infrared radiation in an efficient and broadly tunable format. Here, we describe several applications of QPM-based light sources to remote and local chemical sensing. The remote systems are gas imagers that employ a fiber-pumped continuous-wave optical parametric oscillator or a microlaser-pumped, diode-seeded optical parametric amplifier as the illumination source. Technology described for local sensing includes a cavity ring down spectrometer that employs a novel optical parametric generator–amplifier to achieve ≥350 cm^-1 of contiguous tuning and a long-wave infrared light source based on QPM GaAs. In each case the use of QPM materials in conjunction with effective pump sources instills simplicity and ruggedness into the sensing systems. Received: 15 April 2002 / Revised version: 6 June 2002 / Published online: 12 September 2002 RID="*" ID="*"Corresponding author. Fax: +1-925/294-2595, E-mail: tjkulp@sandia.gov RID="**" ID="**"Present address: Corning Inc., Corning, NY 14831, USA RID="*" ID="*"Present address: Corning Inc., Corning, NY 14831, USA RID="**" ID="**"Present address: Blue Leaf Networks, Sunnyvale, CA 94086, USA RID="***" ID="***"Present address: Sandia National Laboratories, Albuquerque, NM 87185, USA     

LIDAR mapping of ozone-episode dynamics in Paris and intercomparison with spot analyzers Supplementary material available at http://link.springer.de/journals/apb

Continuous mapping of an ozone episode in Paris in June 1999 has been performed using a differential absorption lidar system. The 2D ozone concentration vertical maps recorded over 33 h at the Champ de Mars are compiled in a video clip that gives access to local photochemical dynamics with unprecedented precision. The lidar data are compared over the whole period with point monitors located at 0-, 50-, and 300-m altitudes on the Eiffel Tower. Very good agreement is found when spatial resolution, acquisition time, and required concentration accuracy are optimized. Sensitivity to these parameters for successful intercomparison in urban areas is discussed. Received: 11 February 2002 / Published online: 14 March 2002