An advanced LIF-PLV system for analysing the hydrodynamics in a laboratory bubble column at higher void fractions

Bubble columns are widely used in the chemical industry and biotechnology. Flow and turbulence in such an apparatus are induced by the bubble rise, and the bubble behaviour is strongly affected by swarm effects (i.e. the interaction between bubbles). For analysing the bubble swarm behaviour and simultaneously evaluating the flow structure and bubble-induced turbulence, a bubble column of 140 mm diameter and a height of 650 mm or 1,400 mm (initial water level) were considered. The bubble column was aerated with relatively fine bubbles having a mean size between about 0.5 and 4.0 mm. The gas hold-up was varied in the range between 0.5 and 19%. A two-phase pulsed-light velocimetry (PLV) system was developed to evaluate instantaneous flow fields of both rising bubbles and the continuous phase. The measurement of the liquid velocities in the bubble swarm was achieved by adding fluorescing seed particles. Images of bubbles and fluorescing tracer particles were acquired by two CCD cameras. Hence, the images from tracers and bubbles were easily separated by optical interference filters with a bandwidth corresponding to the emitting wavelength of the fluorescing tracer particles and the wavelength of the applied Nd-YAG pulsed laser, respectively. To improve the phase separation of the system, the CCD cameras were additionally placed in a non-perpendicular arrangement with respect to the light sheet. The acquired images were evaluated with the minimum-quadratic-difference algorithm. The potential of this technique for the analysis of bubbly flows with higher void fraction was explored. In order to obtain averaged velocity maps of bubble and fluid within the entire column, about 1,000 image pairs were recorded and evaluated for each phase. In addition, turbulence intensities of the fluid were deduced from the measurements. The turbulence properties were used to characterise bubble-induced turbulence for various bubble mean diameters and gas hold-ups. Moreover, the determination of the average bubble slip velocity within the bubble swarm was possible.     

Slip velocity measurements in an upward bubbly flow by combined LDA and electrodiffusional techniques

 An experimental technique for the measurement of the local slip velocity of spherical bubbles is reported. It is based on the measurement of the local liquid velocity by an electrodiffusional method, and the bubble velocity by a specially adapted LDA (Laser Doppler anemometer) with a short measuring volume. The bubble velocity is measured taking into account the shift between the bubble centre and the centre of the LDA measuring volume. The slip velocity is obtained by subtracting the liquid velocity from the bubble velocity at the point corresponding to the bubble centre. The technique is applicable for flows with high velocity gradients. Results of the slip velocity measurements in an upward bubbly flow at laminar pipe Reynolds numbers are presented. Received: 25 July 1996/Accepted: 13 April 1998     

Bubbly jets in stagnant water

Air–water bubbly jets are studied experimentally in a relatively large water tank with a gas volume fraction, C_o, of up to 80% and nozzle Reynolds number, Re, ranging from 3500 to 17,700. Measurements of bubble properties and mean axial water velocity are obtained and two groups of experiments are identified, one with relatively uniform bubble sizes and another with large and irregular bubbles. For the first group, dimensionless relationships are obtained to describe bubble properties and mean liquid flow structure as functions of C_o and Re. Measurements of bubble slip velocity and estimates of the drag coefficient are also provided and compared to those for isolated bubbles from the literature. The study confirms the importance of bubble interactions to the dynamics of bubbly flows. Bubble breakup processes are also investigated for bubbly jets. It was found that a nozzle Reynolds number larger than 8000 is needed to cause breakup of larger bubbles into smaller bubbles and to produce a more uniform bubble size distribution. Moreover, the Weber number based on the mean water velocity appears to be a better criteria than the Weber number based on the bubble slip velocity to describe the onset of bubble breakup away from the nozzle, which occurs at a Weber number larger than 25.     

Turbulent shear stress profiles in a bubbly channel flow assessed by particle tracking velocimetry

Particle tracking velocimetry (PTV) is applied to a bubbly two-phase turbulent flow in a horizontal channel at Re = 2 × 10⁴ to investigate the turbulent shear stress profile which had been altered by the presence of bubbles. Streamwise and vertical velocity components of liquid phase are obtained using a shallow focus imaging method under backlight photography. The size of bubbles injected through a porous plate in the channel ranged from 0.3 to 1.5 mm diameter, and the bubbles show a significant backward slip velocity relative to liquid flow. After bubbles and tracer particles are identified by binarizing the image, velocity of each phase and void fraction are profiled in a downstream region. The turbulent shear stress, which consists of three components in the bubbly two-phase flow, is computed by analysis of PTV data. The result shows that the fluctuation correlation between local void fraction and vertical liquid velocity provides a negative shear stress component which promotes frictional drag reduction in the bubbly two-phase layer. The paper also deals with the source of the negative shear stress considering bubble’s relative motion to liquid.     

Interfacial area concentration in gas–liquid bubbly to churn flow regimes in large diameter pipes

This study performed a survey on existing correlations for interfacial area concentration (IAC) prediction and collected an IAC experimental database of two-phase flows taken under various flow conditions in large diameter pipes. Although some of these existing correlations were developed by partly using the IAC databases taken in the low-void-fraction two-phase flows in large diameter pipes, no correlation can satisfactorily predict the IAC in the two-phase flows changing from bubbly, cap bubbly to churn flow in the collected database of large diameter pipes. So this study presented a systematic way to predict the IAC for the bubbly-to-churn flows in large diameter pipes by categorizing bubbles into two groups (group 1: spherical or distorted bubble, group 2: cap bubble). A correlation was developed to predict the group 1 void fraction by using the void fraction for all bubble. The group 1 bubble IAC and bubble diameter were modeled by using the key parameters such as group 1 void fraction and bubble Reynolds number based on the analysis of Hibiki and Ishii (2001, 2002) using one-dimensional bubble number density and interfacial area transport equations. The correlations of IAC and bubble diameter for group 2 cap bubbles were developed by taking into account the characteristics of the representative bubbles among the group 2 bubbles and the comparison between a newly-derived drift velocity correlation for large diameter pipes and the existing drift velocity correlation of Kataoka and Ishii (1987) for large diameter pipes. The predictions from the newly-developed two-group IAC correlation were compared with the collected experimental data in gas–liquid bubbly to churn flow regimes in large diameter pipes and their mean absolute relative deviations were obtained to be 28.1%, 54.4% and 29.6% for group 1, group 2 and all bubbles respectively.     

Prediction of bubble concentration profiles in vertical turbulent two-phase flow

In vertical bubbly flow, the bubbles are not distributed evenly across the flow section. Several investigators have observed a wall-skewed bubble concentration profile in a vertical upward flow. This paper presents an analysis that predicts this type of bubble distribution by incorporating into the equation of motion a lateral force due to the relative velocity of the two phases and the eddy diffusivity of the liquid. Comparison of analysis and experiment shows good agreement.     

Study of periodically excited bubbly jets by PIV and double optical sensors

Interactions between large coherent structures and bubbles in two-phase flow can be systematically observed in a periodically excited bubbly jet. Controlled excitation at fixed frequency causes large eddy structures to develop at regular intervals. Thus, interactions between large vortices and bubbles can be studied with PIV and double optical sensors (DOS) using phase-averaging techniques. A number of results on the time and space dependence of velocities and void fractions are presented revealing physical interactions between the liquid flow field and bubble movement as well as feedbacks from bubble agglomeration on the development of flow structures. A clear indication of bubble trapping inside the vortex ring is the generation of a bubble ring that travels with the same velocity as the vortex ring. The DOS results indicate clustering of the bubbles in coherent vortex structures, with a periodic variation of void fraction during the excitation period.     

Bubble and liquid turbulence characteristics of bubbly flow in a large diameter vertical pipe

The bubble and liquid turbulence characteristics of air–water bubbly flow in a 200 mm diameter vertical pipe was experimentally investigated. The bubble characteristics were measured using a dual optical probe, while the liquid-phase turbulence was measured using hot-film anemometry. Measurements were performed at six liquid superficial velocities in the range of 0.2–0.68 m/s and gas superficial velocity from 0.005 to 0.18 m/s, corresponding to an area average void fraction from 1.2% to 15.4%. At low void fraction flow, the radial void fraction distribution showed a wall peak which changed to a core peak profile as the void fraction was increased. The liquid average velocity and the turbulence intensities were less uniform in the core region of the pipe as the void fraction profile changed from a wall to a core peak. In general, there is an increase in the turbulence intensities when the bubbles are introduced into the flow. However, a turbulence suppression was observed close to the wall at high liquid superficial velocities for low void fractions up to about 1.6%. The net radial interfacial force on the bubbles was estimated from the momentum equations using the measured profiles. The radial migration of the bubbles in the core region of the pipe, which determines the shape of the void profile, was related to the balance between the turbulent dispersion and the lift forces. The ratio between these forces was characterized by a dimensionless group that includes the area averaged Eötvös number, slip ratio, and the ratio between the apparent added kinetic energy to the actual kinetic energy of the liquid. A non-dimensional map based on this dimensionless group and the force ratio is proposed to distinguish the conditions under which a wall or core peak void profile occurs in bubbly flows.     

The Fokker–Planck Equation for Bubbly Flows and the Motion of Gas Bubble Pairs

A method is proposed to calculate the bubble distribution function in a bubbly flow. First a review is given of the equations of motion and the dynamic behaviour of a pair of bubbles moving through a liquid at moderate Reynolds number. Subsequently, a Fokker–Planck type transport equation is derived for the bubble distribution function. It is assumed that the interaction is primarily by frequent and binary encounters, each with weak hydrodynamic interaction between the bubbles. The bubble collision cross-section, which needs to be known for the transport coefficients, is presented. A comparison with PDF-methods for fluid particles in turbulent reacting flows is made.     

A DNS study of laminar bubbly flows in a vertical channel

Direct numerical simulations are used to examine laminar bubbly flows in vertical channels. For equal size nearly spherical bubbles the results show that at steady state the number density of bubbles in the center of the channel is always such that the fluid mixture there is in hydrostatic equilibrium. For upflow, excess bubbles are pushed to the walls, forming a bubble rich wall-layer, one bubble diameter thick. For downflow, bubbles are drawn into the channel center, leading to a wall-layer devoid of bubbles, of a thickness determined by how much the void fraction in the center of the channel must be increased to reach hydrostatic equilibrium. The void fraction profile can be predicted analytically using a very simple model and the model also gives the velocity profile for the downflow case. For the upflow, however, the velocity increase across the wall-layer must be obtained from the simulations. The slip velocity of the bubbles in the channel core and the velocity fluctuations are predicted reasonably well by results for homogeneous flows.     

Order and disorder in particle–liquid flows in a pipe

The spherical expanded polystyrene particle–oil two-phase flow in a vertical pipe was used to simulate the dispersed phase distribution in laminar bubbly flows. A three-dimensional particle image tracking technique was used to track the particles in the flow to study the ordered structure of dispersed phase distribution and its transition to disorder. The ordered structures behaved as particle strings aligned in the flow direction as induced by the flow shear. The structures were quite durable in high liquid velocity flows and dispersed gradually as the liquid velocity decreased. In lower velocity flows, the particles tended to form clusters in the horizontal direction, as predicted by potential theory for spherical bubbles rising in a quiescent inviscid liquid and as observed in experiments on non-shear bubbly water flows.     

Rising behavior of single bubble in infinite stagnant non-Newtonian liquids

This work is an experimental study of the rising behavior of single air bubbles in infinite stagnant non-Newtonian liquids. Aqueous solutions of carboxymethyl cellulose (CMC) are selected to study the effect of rheological properties. The high speed photography is employed to record the bubble motion in CMC solutions. The bubble size, rising trajectory, bubble shape and velocities are determined by digital image processing technique. As expected, the rheological properties have great influence on the rising behavior of single bubble. In the less concentrated CMC solutions, the bubble rising process can be divided into three stages according to spatial evolution of bubble shape. The deformation changes the trajectories of rising bubbles and bubble hydrodynamics. As the solution concentration increases, the transitional stage gradually disappears. In the most concentrated CMC solution, the first continuous shape flattening stage is directly followed by a rising process with bubble shape basically constant, the rectilinear path and constant rising velocity. Dimensional analysis is performed to formulate a general dimensionless correlation for the deformation and motion of bubbles in infinite liquids by considering the rheological properties.     

Interaction between Taylor bubbles rising in stagnant non-Newtonian fluids

The interaction between Taylor bubbles rising in stagnant non-Newtonian solutions was studied. Aqueous solutions of carboxymethylcellulose (CMC) and polyacrylamide (PAA) polymers were used to study the effect of different rheological properties: shear viscosity and viscoelasticity. The solutions studied covered a range of Reynolds numbers between 10 and 714, and Deborah numbers up to 14. The study was performed with pairs of Taylor bubbles rising in a vertical column (0.032 m internal diameter) filled with stagnant liquid. The velocities of the leading and trailing bubbles were measured by sets of laser diodes/photocells placed along the column. The velocity of the trailing bubble was analysed together with the liquid velocity profile in the wake of a single rising bubble (Particle Image Velocimetry data obtained from the literature). For the less concentrated CMC solutions, with moderate shear viscosity and low viscoelasticity, the interaction between Taylor bubbles was similar to that found in Newtonian fluids. For the most concentrated CMC solution, which has high shear viscosity and moderate viscoelasticity, a negative wake forms behind the Taylor bubbles, inhibiting coalescence since the bubbles maintain a minimum distance of about 1D between them. For the PAA solutions, with moderate shear viscosity but higher viscoelasticity than the CMC solutions, longer wake lengths are seen, which are responsible for trailing bubble acceleration at greater distances from the leading bubble. Also in the PAA solutions, the long time needed for the fluid to recover its initial shear viscosity after the passage of the first bubble makes the fluid less resistant to the trailing bubble flow. Hence, the trailing bubble can travel at a higher velocity than the leading bubble, even at distances above 90D.     

Characterization of bubble mobility in channel flow with fibrous porous media walls

In composites processing, resin is introduced into a fibrous domain to cover all the empty spaces between the fibers. It is important to extract air bubbles from the domain before the resin solidifies. Failure to do so will entrap these voids in the final part, which is detrimental to its performance. Hence, there is a need to understand bubble motion in a fibrous porous domain in which the bubbles move with the resin in channels surrounded by fibrous walls. A rising bubble model is presented that consists of a single spherical void in a cylindrical axisymmetric two-phase domain of resin and air surrounded by porous media boundaries. The motion of a bubble in a channel flow with porous boundaries is modeled by replacing the walls with a slip velocity. Focus is on how the porous media permeability influences the bubble motion. A parameter called bubble mobility is defined as the ratio of bubble rise velocity to the resin free surface velocity. Results suggest that fabric permeability and fluid properties can be optimized to increase bubble mobility and ultimately lead to reduction in void content during composites processing.     

An experimental study of plane bubbles rising at inclination

The characteristics of bubbles rising in two-dimensional tanks is investigated. It is found that the influence of fluid properties, while negligible for vertically rising bubbles, measurably affects the inclined bubble rise velocity. The measured increase in the rise velocity at inclination relative to the vertical value is explained qualitatively. In addition, a comparison is made between the wave analogy correlation of Maneri & Mendelson and vertical rise velocity data. The comparisons show that the correlation predicts the three-dimensional effects of tank spacing when the data are reduced on an equivalent bubble radius basis.     

Fluctuation characteristics of bubbly liquid flow in converging-diverging nozzle

The pressure fluctuation characteristics in bubbly liquid flow in a converging-diverging nozzle are interpreted on the basis of the previous theoretical results concerning the possible wave modes in bubbly liquid flow and their properties. The experiment is performed in a visual blowdown facility using water and nitrogen gas. The intensity and power spectrum density of the pressure fluctuations are measured, as well as the velocities of liquid and bubbles, the void fraction and the chord length of bubbles. All the fluctuation characteristics and their relation with the main stream condition are compatible with the theoretical predictions. The instability of the convection mode in the presence of the velocity slip and the cut off of the propagation modes in moderate frequency are demonstrated.     

A numerical scheme for Euler–Lagrange simulation of bubbly flows in complex systems

An Eulerian–Lagrangian approach is developed for the simulation of turbulent bubbly flows in complex systems. The liquid phase is treated as a continuum and the Navier–Stokes equations are solved in an unstructured grid, finite volume framework for turbulent flows. The dynamics of the disperse phase is modeled in a Lagrangian frame and includes models for the motion of each individual bubble, bubble size variations due to the local pressure changes, and interactions among the bubbles and with boundaries. The bubble growth/collapse is modeled by the Rayleigh–Plesset (RP) equation. Three modeling approaches are considered: (a) one‐way coupling, where the influence of the bubble on the fluid flow is neglected, (b) two‐way coupling, where the momentum‐exchange between the fluid and the bubbles is modeled, and (c) volumetric coupling, where the volumetric displacement of the fluid by the bubble motion and the momentum‐exchange are modeled. A novel adaptive time‐stepping scheme based on stability‐analysis of the non‐linear bubble dynamics equations is developed. The numerical approach is verified for various single bubble test cases to show second‐order accuracy. Interactions of multiple bubbles with vortical flows are simulated to study the effectiveness of the volumetric coupling approach in predicting the flow features observed experimentally. Finally, the numerical approach is used to perform a large‐eddy simulation in two configurations: (i) flow over a cavity to predict small‐scale cavitation and inception and (ii) a rising dense bubble plume in a stationary water column. The results show good predictive capability of the numerical algorithm in capturing complex flow features. Copyright © 2010 John Wiley & Sons, Ltd.