Electronic structure,magnetic exchange,and electrical transport properties of the magnetic compounds EuS,GdS and GdP

Optical reflectivity measurements between 0.03 eV and 12 eV have been performed on the isomorphic compounds EuS, GdP and GdS. A Kramers-Kronig analysis of these data permits the evaluation of intra- and interband transitions and the derivation of the electronic structure. The conducting behavior changes from semiconducting for undoped EuS to metallic for Eu_0.99Gd_0.01S and GdS; also GdP exhibits metal-like conductivity. In GdP and GdS the stoichiometry can be varied while keeping the phase purity. In these compounds the concentration of free carriers depends on the stoichiometry just as does the mobility, which in addition depends also on temperature. Large scattering anomalies are observed near the magnetic ordering temperatures for all compounds. In spite of the same spectroscopic ground state ${}^8\text{S}\text{7}\text{2}$ for EuS, GdP and GdS only EuS is ferromagnetic, the others being antiferromagnetic. In the alloy system GdPGdS the free carrier concentration could be varied over nearly two orders of magnitude and the superexchange and free carrier contribution to the total exchange interaction could be separated. Clearly the free carriers contribute a RKKY interaction.An attempt is made to correlate and explain the different physical properties of the related compounds EuS, GdP and GdS by their specific electronic structure.     

Magnetic field dependence of the 31P longitudinal nuclear-spin relaxation time in GdP at high temperatures

The magnetic field dependence of the longitudinal nuclear-spin relaxation time for ³¹P nuclei in paramagnetic GdP is expressed in terms of a wavevector frequency-dependent relaxation-shape function. A Gaussian representation of the memory function associated with the spin-velocity relaxation function is chosen that satisfies the first six frequency moments. The results are compared with the experimental data of Myers and Narath.     

Measurements of the HCN ν3 band broadened by N2

N₂-broadened halfwidths have been measured for 51 absorption lines belonging to the ν₃ fundamental band of hydrogen cyanide (¹H¹²C¹⁴N) near 3311 cm^?1. The data were recorded at room temperature using a Fourier transform spectrometer with a nominal resolution of 0.06 cm^?1. A nonlinear least-squares spectral-fitting procedure was used to obtain both line intensities and collision-broadened halfwidths from scans recorded at several different pressures. The N₂-broadened halfwidths, determined for all lines with J ≤ 25 in both the P and R branches of the band, show the expected distribution with J for broadening by a nonpolar gas. The halfwidth values range from approximately 0.17 cm^?1 atm^?1 near the band center to 0.11 cm^?1 atm^?1 for high-J lines. The band intensity for the ν₃ fundamental derived from these measurements is 236.2 ± 9.5 cm^?2 atm^?1 at 296 K, and empirical coefficients for the vibration-rotation interaction F-factor were also determined.     

Effect of M+2 ions on the luminescence of Pb+2 in NaCl

The effect of additional doping with M⁺² ions on the luminescence of NaCl:Pb⁺² has been systematically investigated. The data show that the same two emissions at 310 and 380 nm are observed for mixed Pb⁺²-M⁺² clusters as for Pb⁺² aggregates. Moreover, the presence of a M⁺² ion associated to a Pb⁺² ion in a mixed cluster shifts the 310 nm emission (predominantly observed for free Pb⁺²-vacancy dipoles) to 380 nm. The results are consistent with the Fukuda's model, involving an emission at 310 nm from tetragonal (T) minima in the adiabatic potential energy surface (APES) and another one from less symmetry (X) minima at 380 nm. The data for NaCl:Pb⁺²:Mn⁺², show that an excitation transfer is taking place from the X minima of the ³T_1u state of Pb⁺² to Mn⁺².     

Electron scattering from 70Ge and 72Ge

Cross sections have been measured for the elastic and inelastic scattering of electrons from ⁷⁰Ge and ⁷²Ge for momentum transfers from 0.65 to 1.14 fm^?1. Values for the parameters of a Fermi type ground-state charge distribution were obtained from a phase shift analysis of the elastic cross sections. The rms charge radius corresponding to these parameters is 4.07±0.02 fm for ⁷⁰Ge and 4.05±0.03 fm for ⁷²Ge. Using DWBA analysis the reduced transition probabilities for the electroexcitation of the 2₁⁺ and 3₁^? states were found to be: B(E2, ω)↑ = 19.7±1.2, 26.8±2.0 W.u.; B(E3, ω)↑ = 36±5, 37±7 W.u. for ⁷⁰Ge and ⁷²Ge respectively. The J^π = 3^? assignments for the state at 2.562 MeV in ⁷⁰Ge and 2.515 MeV in ⁷²Ge are confirmed.     

Coulomb excitation of230Th with32S,84Kr and142Nd projectiles

The Coulomb excitation measurements for the²³⁰Th nucleus with³²S,⁸⁴Kr and¹⁴²Nd projectiles are presented. The use of different projectiles allowed us to get information in the ground-state band and side bands. The energy spectrum of the ground-state band and of the lowest negative-parity band have been investigated up to the spin valueI=24⁺ andI=19^?(21), respectively. Five side bands (K ^π=0⁺, 2 ₁ ⁺ , 2 ₂ ⁺ , 1^?, 2^?) were observed also. The branching ratios for a large number of transitions in the spin regionI≦10 for π=+1 andI≦9 for π=? 1 are analysed. The full set of experimental data contains information on the mixing of the adiabatic states and on the nuclear response to the electromagnetic field ofγ-radiation. It is shown that the experimental data may be explained taking into account the coupling of the ground-β- and twoγ-bands and also of theK ^π=0^?, 1^? and 2^? negative-parity bands. An enhancement of the transitions from theγ-to theβ-band in respect to the transitions from theγ to the ground band and from theβ- to the ground band is reported. The mixing of the negative-parity bands is found to be typical for the alignment of the octupole-vibrational angular momentum. The strong spin dependence of the intrinsic matrix elements of the electric-dipole operator follows from the branching ratios of inter- and intra-band transitions from theK ^π=0^? states.     

Measurement of the polarization parameter of the reactionsπ− p → π0n and ηn at 5 and 8 GeV/c

Measurements of the polarization parameter of the reactions π^?p → π⁰n and π^?p → ηn at 4.90 and 7.85 GeV/c and for a squared four-momentum transfer ?t ranging from 0.1 to 2.0 (GeV/c)² have been achieved by using a butanol polarized proton target and detecting only the two γ's from the neutral meson decay. The background due to events involving bound protons has been separately measured and subtracted out. A large positive polarization has been found for the reaction π^?p → π⁰n. It is consistent with other pion-nucleon scattering data connected by isospin conservation. The polarization for the reaction π^?p → ηn is not significantly different from zero within the large experimental errors.     

Diffusion of sulfur in nickel oxide single crystals

The diffusion of sulfur in nickel oxide single crystals has been investigated over the temperature range from 1000 to 1250°C. The measured data were found to deviate markedly from the error function complement dependence for diffusion from a constant source. The deviation is attributed to the migration of sulfur by the “double mode simultaneous diffusion mechanism.” The faster mode diffusion is suggested to be via nickel vacancies, and the slower mode diffusion is suggested to be via oxygen vacancies. The diffusivities for faster mode are given by D_f = 2.94 exp[? 86.6 kcal/RT] cm² sec^?1 and, the slower mode, D_s = 1.08 × 10^?9 exp [?32.8 kcal/RT]cm²sec^?1.     

Gain studies on a uranine-damc dye mixture laser under nitrogen laser pumping

The radiative and Forster type of energy transfer processes in a dye mixture laser of 7-diethylamino-4-methyl coumarin (donor) and fluorescein disodium salt (acceptor) under nitrogen laser pumping were investigated. The Forster transfer rate calculated from the absorption and emission spectra of acceptor and donor is 1.3 × 10¹¹ liter mole^?1sec^?1. The gain of acceptor at 550 nm was measured for acceptor concentrations N_A from 10^?3M to 3 × 10^?3M for a fixed ratio F = 1 of donor to acceptor concentrations at different pump powers. The results agreed with the rate equation model proposed for the dye mixture laser. The radiative rate constant calculated from these results is 3.1 × 10¹⁰ liter mole^?1sec^?1. Numerical simulation of the rate equations showed that the acceptor reaches peak emission with a time lag of 3 ns with respect to the donor peak emission for F = 0.998, N_A = 10^?5M. This time lag decreases with increasing N_A and becomes zero for N_A = 10^?1M, F = 0.048.     

Approximation of the electron excitation cross sections for triplet states excited from the 23 S 1 metastable state in helium

The method of approximated four-parameter representation of the electron-impact cross sections for a helium atom excited from the 2³ S ₁ metastable state into higher triplet states is applied and discussed. The approximation consists in interpolation over the whole set of the cross section values for each helium atomic level measured in our experiments and reported by other researchers. The approximation parameters and the cross sections calculated using these parameters for the maxima of the corresponding excitation functions are presented for 19 triplet levels of the S, P, and D HeI series with n=2–10. The interpolated values are compared to the theoretical cross sections. The serial regularities were investigated for the S, P, and D levels studied and a decrease in the cross sections for excitation from the given metastable state within each series, described by the approximate law Q=Cn ^?5, was revealed. Validity of the similarity relationship and the Bethe approximation for cross sections in the 2³ S?n ³ P series was verified. It is shown that the cross sections for a triplet level excitation from the 2³ S ₁ metastable state exceed the corresponding values for excitation from the ground state of helium by a factor of approximately 10³ for n=2 and 3 and 10 2 for the higher levels. It is concluded that the proposed method of representation of the cross sections for the electron-impact excitation of triplet levels from the metastable state increases accuracy and more importantly, reliability of the final results.     

Depolarization in proton inclusive inelastic scattering and in the (d,p) reaction on medium-weight nuclei

The energy-averaged depolarization parameter K_y^y′ has been measured for the inelastic scattering of 18 MeV protons from ⁵⁴Fe, ⁶³Cu and ⁹²Mo at 45°, 90° and 135°, and for 14.35 MeV protons from ⁶³Cu at 45° and 135°. In all cases K_y^y′ varies from approximately unity for scattering with low energy loss to approximately zero for inelastic scattering to high excitation energies. The change from one of these values to the other occurs over a region ≈ 6 MeV wide centered at about 5 MeV excitation. A simple two-component model fits both the K_y^y′ and inelastic crosssection data. K_y^y′ has also been measured for the ⁵⁴Fe($\text{d}$, $\text{p}$)Fe reaction with 16 MeV deuterons incident. Here K_y^y′ changes from approximately the maximum possible value, $\text{2}\text{3}$, to about zero in a 6 MeV region centered at roughly 13 MeV excitation. The ($\text{d}$,$\text{p}$) data can be fitted by an extension of the model used for the proton scattering data.     

Jet-cooled laser-induced fluorescence spectroscopy of B2Σ+–X2Σ+ system of scandium monoxide: Improved molecular constants at equilibrium

The investigation on B²Σ⁺–X²Σ⁺ system of ScO was extended to higher vibrational levels by laser-induced fluorescence (LIF) spectroscopy in a free-jet. We have observed rotationally resolved excitation spectra for (4,0), (3,0), (2,0), and (1,2) bands in addition to the previously observed (0,0) and (1,0) bands. The wavenumbers of these bands were fitted to a Hamiltonian matrix to determine the molecular constants for the vibrational levels up to ν′=4 of the B²Σ⁺ state and ν″=2 of the X²Σ⁺ state. In addition, the vibration constants of the ground states were determined from the dispersed fluorescence wavenumbers between B²Σ⁺ (ν′=0–4) and X²Σ⁺ (ν″=0–8) transitions. The equilibrium molecular constants, derived from the extensive set of molecular constants for individual vibrational levels, were used to construct RKR potential energy curves for both the electronic states. The Franck–Condon factors were also calculated for the B²Σ⁺–X²Σ⁺ transition.     

Elastic scattering of deuterons by 14C from Ed = 4 to 10 MeV

Angular distributions for the elastic scattering of deuterons by ¹⁴C were measured at nine energies between E_d = 4.2 and 10 MeV. Excitation functions were taken in 50 keV steps from E_d = 4 to 10 MeV. A resonance was observed at E_d = 4.5 MeV, which corresponds to an excitation energy of 14.41 MeV in ¹⁶N. An analysis using an optical model plus a single-level formula derived from the R-matrix formalism yields an l-value assignment of l = 4 for this resonance. Of the three J^π values allowed for l = 4 (J^π = 3⁺, 4⁺, 5⁺), the value of J_π = 3⁺ is found to be slightly preferred. Possible identification of this resonance with an analog in ¹⁶O is discussed. The angular distributions measured at off-resonance energies were analyzed with an optical-model potential which has a surface-peaked imaginary well. The energy dependence of the real and imaginary well depths are explicitly determined in the present work for E_d = 4 to 10 MeV. The best-fit optical-model parameters obtained from the present study are compared to those from the ¹⁴N(d, d)¹⁴N work.     

Single-pion production in antineutrino-induced neutral-current interactions

Results are presented on antineutrino-induced processes in which a single π⁰or π^? is produced. The raw data come from analysis of film from Gargamelle filled with a propane-freon mixture. Comparison of the neutral-current production rates for π⁰and π^?, after correction for nuclear effects, indicates that pure isoscalar or pure isovector transitions are not favoured. The ratio of the neutral-to-charged-current single-π⁰ production rates is found to be compatible with the static model for Δ³³ resonance production in the framework of the Weinberg-Salam theory, yielding values for sin²θ_W in the range 0.15–0.52.     

Seeking and investigating isospin-two narrow dibaryon resonances in neutron-proton interactions at P n =5.20±0.13 Gev/c

The results are presented that are obtained from searches for and an investigation of isospin-two narrow resonances in the effective-mass spectrum of ppπ⁺ combinations originating from the reaction np → ppπ⁺π^?π^? induced by P _n =5.20±0.13 GeV/c neutrons. Data subjected to our analysis come from the 1-m hydrogen bubble chamber installed at the Laboratory for High Energies, Joint Institute for Nuclear Research (Dubna), and exposed to a beam of quasimonochromatic neutrons. Narrow structures in the effective-mass spectrum of ppπ⁺ combinations are found at 2175, 2221, 2321, 2398, 2471, 2525, 2596, and 2709 MeV/c ². The experimental widths of the resonances are determined primarily by the instrumental resolution. The branching fractions for various channels through which the 2596-MeV/c ² resonance decays are determined to be (83±23)% for the Δ ₃₃ ⁺⁺ p channel, (10±3)% for the (BB) ₂₀₉₅ ⁺⁺ π⁺ channel, and (7 _?7 ⁺¹⁵ for the ppπ⁺ channel; here, (BB) ₂₀₉₅ ⁺⁺ is a dibaryon in the two-proton system with a mass around 2095 MeV/c ². A qualitative analysis of the spins of the 2596-and 2709-MeV/c ² resonances is performed.     

An experimental test of exchange degeneracy in the hyperchange exchange reactions π+p→K+Σ+and K−→π−Σ+

For the first time, the line reversed reactions π⁺p→K⁺Σ⁺and K^?p→π^?Σ⁺ have been studied in the same apparatus. We present the differential cross sections and polarizations over a large t range and at two momenta, 7.0 and 10.1 GeV/c. The differential cross sections as a function of t are shown for the first time to cross over. Going from the lower to the higher momentum, the differences in cross section between the two reactions diminish at low |t| by about a factor 2. We find large polarizations of opposite sign for the two reactions. The momentum dependence, presented in the form of α_eff(t) for the t range 0 to ?2 (GeV/c)², is compared with the expectations from the K¹?K⁷ trajectory.     

Inclusive production of Σ±(1385) in pp interactions at 12 and 24 GeV/c

The inclusive production of Σ^±(1385) is studied in pp interactions at 12 and 24 GeV/c. In this energy range, the inclusive cross sections for Σ⁺(1385) and Σ^?(1385) rise from 0.20 ± 0.03 mb to 0.28 ± 0.03 mb and from 0.07 ± 0.02 mb to 0.12 ± 0.02 mb. The decays of Σ^±(1385) account for ～20% of all observed Λ hyperons. The p_T² distributions are compatible with an exponential decrease and the slopes are in agreement with a common value of B ～ 3 (GeV/c)^?2. The longitudinal spectra are significantly different: Σ^?(1385) is mainly produced in the central region, whereas proton fragmentation contributes strongly to Σ⁺(1385) production.     

The reaction π−p → K0Σ0 up to 2375 MeV/c

Differential cross-section and polarization measurements for the reaction π^?p → K⁰Σ⁰ are presented from 1395 to 2375 MeV/c incident beam momentum. The polarization data from an earlier experiment, from thershold to 1334 MeV/c, have been re-analysed by an improved method leading to a substantial reduction in the errors.     

A study of 80,82,84Sr by (α, 2nγ) reactions

The ^AKr(α, 2nγ)^A+2Sr reactions have been studied by in-beam γ-ray spectroscopy for A = 78, 80, and 82. States with spins up to 10⁺ in ^82,84Sr and 6⁺ in ⁸⁰Sr are identified. The Sr nuclei undergo a transition from spherical to deformed ground states as neutrons are removed from the N = 50 shell. The systematics of these nuclei are compared with calculations based upon the shell model and interacting boson model.     

Pion-nucleus inelastic scattering and charge exchange

Using a separable fixed scatterer pion-nucleon interaction and the distorted wave impulse approximation we have made predictions for medium energy pion inelastic scattering from ¹⁶O and (π^?, π⁰) charge exchange from ⁴⁸Ca. An optical potential based on the pion-nucleon interaction adopted in this work has been shown previously to provide good fits to pion-nucleus elastic scattering. After a discussion of the basic formulae, we present results of calculations for pion inelastic scattering from ¹⁶O for initial pion lab kinetic energies of 70 and 180 MeV. Because of the strong energy dependence of the pion-nucleon interaction there are qualitative differences between the predictions for the nuclear response in the momentum transfer, energy loss plane for T_π^lab = 70 and 180 MeV. At these energies, states not prominently excited by other probes are predicted to be observable. In particular, J^π = 3^? and 4^?, T = 0 states appear prominently in the excitation spectrum region at large momentum transfer. A comparison of π^? and π⁺ scattering showing the effects of the Coulomb interaction is presented. The predictions for pion single-charge exchange on ⁴⁸Ca indicate that this interaction would be useful for studying the location of the T_> states arising from the splitting of the giant dipole resonance in T ≠ 0 nuclei.