Study of Fission Barrier Heights of Uranium Isotopes by the Macroscopic-Microscopic Method

Potential energy surfaces of uranium nuclei in the range of mass numbers 229 through 244 are investigated in the framework of the macroscopic-microscopic model and the heights of static fission barriers are obtained in terms of a double-humped structure. The macroscopic part of the nuclear energy is calculated according to Lublin–Strasbourg-drop(LSD) model. Shell and pairing corrections as the microscopic part are calculated with a folded-Yukawa single-particle potential. The calculation is carried out in a five-dimensional parameter space of the generalized Lawrence shapes. In order to extract saddle points on the potential energy surface, a new algorithm which can effectively find an optimal fission path leading from the ground state to the scission point is developed. The comparison of our results with available experimental data and others' theoretical results confirms the reliability of our calculations.     

Study of Fission Barrier Heights of Uranium Isotopes by the Macroscopic-Microscopic Method

Potential energy surfaces of uranium nuclei in the range of mass numbers 229 through 244 are investigated in the framework of the macroscopic-microscopic model and the heights of static fission barriers are obtained in terms of a double-humped structure. The macroscopic part of the nuclear energy is calculated according to Lublin-Strasbourg-drop (LSD) model. Shell and pairing corrections as the microscopic part are calculated with a folded-Yukawa single-particle potential. The calculation is carried out in a five-dimensional parameter space of the generalized Lawrence shapes. In order to extract saddle points on the potential energy surface, a new algorithm which can effectively find an optimal fission path leading from the ground state to the scission point is developed. The comparison of our results with available experimental data and others' theoretical results confirms the reliability of our calculations.     

Marked Advance in Widths and Heights of Harmonic Plateau

We propose a scheme to simultaneously widen and heighten the high-order harmonic plateau on a large scale. More specifically, by adopting a united two-atom system with a suitable inter-nuclear separation instead of a single-atom, the harmonic plateau is widened from I_p + 3.2U_p to I_p + 8.5U_p; further, by adopting the combined pulse, the extended plateau (harmonics near I_p + 5.6U_p) is selectively heightened in excess of 4 orders of magnitudecompared with the case of the low-frequency pulse alone. By means ofthe wavelet transform for the induced dipole of these harmonics, asingle x-ray pulse as short as 210 asec is achieved.     

The Higher-Order Approximation in General Theory of Self-consistent Field Beyond Hartree-Fock

In this paper, the higher-order approximation in the general theory of self-consistent field is presented by the Wick's theorem, and the solution of equations is discussed.     

裂变位垒参数的推荐和裂变位垒参数库

通过分析和计算锕系核裂变截面和全套中子反应截面获取了一组锕系核的裂变位垒参数.Fm)在此基础上,广泛收集实验裂变位垒参数,通过比对和评价,推荐了本组的129个核素(109Cd—255的实验裂变位垒参数.此外,对收集的不同裂变位垒参数作了分析与评价,推荐了7组实验和1组模型计算的裂变位垒参数,并组建了中国评价核参数库裂变位垒参数子库(CENPL FBPL). The fission barrier parameters for actinide nuclei were obtained by analysis and calculations of fission cross-sections and complete neutron reaction cross sections. A lot of experimental fission barrier parameters from different authors were collected. A set of fission barrier parameters for 129 nuclei ranging from~(109)Cd~( ) to~(255)Fm were recommended after performing comparisons, evaluations and systematics extrapolations for these extracted fission barrier parameters in model calculations of fissi...     

光谱学方法研究介质阻挡沿面放电辉光模式的电场分布

利用介质阻挡沿面放电装置,在低气压空气中实现了辉光放电模式。利用光电倍增管对放电发光信号进行检测,发现外加电压每半周期出现一个发光脉冲,并且正负半周期的光脉冲是不对称的。利用Photoshop软件处理放电的照片,研究发现平行于高压电极不同位置的发光强度基本相同,然而距离高压电极越远,发光强度减小。放电中总电场由外加电场和电介质积累的壁电荷电场共同决定,确定该电场具有重要意义。通过分析放电的发射光谱中N+₂(B 2Σ+_u→X 2Σ+_g)谱线391.4 nm和N₂的第二正带系(C 3Π_u→B 3Π_g)谱线337.1 nm的比值,可以定性地说明电场的分布。研究发现电场在高压电极附近较大而远离高压电极处较小。这些研究结果对沿面放电的数值模拟和工业应用具有重要的价值。     

石墨烯过渡层对金属/SiC接触肖特基势垒调控的第一性原理研究

由于SiC禁带宽度大,在金属/SiC接触界面难以形成较低的势垒,制备良好的欧姆接触是目前SiC器件研制中的关键技术难题,因此,研究如何降低金属/SiC接触界面的肖特基势垒高度(SBH)非常重要.本文基于密度泛函理论的第一性原理赝势平面波方法,结合平均静电势和局域态密度计算方法,研究了石墨烯作为过渡层对不同金属(Ag,Ti,Cu,Pd,Ni,Pt)/SiC接触的SBH的影响.计算结果表明,单层石墨烯可使金属/SiC接触的SBH降低;当石墨烯为2层时,SBH进一步降低且Ni,Ti接触体系的SBH呈现负值,说明接触界面形成了良好的欧姆接触;当石墨烯层数继续增加,SBH不再有明显变化.通过分析接触界面的差分电荷密度以及局域态密度,SBH降低的机理可能主要是石墨烯C原子饱和了SiC表面的悬挂键并降低了金属诱生能隙态对界面的影响,并且接触界面的石墨烯及其与金属相互作用形成的混合相具有较低的功函数.此外,SiC/石墨烯界面形成的电偶极层也可能有助于势垒降低.     

石墨烯过渡层对金属/SiC接触肖特基势垒调控的第一性原理研究

由于SiC禁带宽度大,在金属/SiC接触界面难以形成较低的势垒,制备良好的欧姆接触是目前SiC器件研制中的关键技术难题,因此,研究如何降低金属/SiC接触界面的肖特基势垒高度(SBH)非常重要.本文基于密度泛函理论的第一性原理赝势平面波方法,结合平均静电势和局域态密度计算方法,研究了石墨烯作为过渡层对不同金属(Ag,Ti,Cu,Pd,Ni,Pt)/SiC接触的SBH的影响.计算结果表明,单层石墨烯可使金属/SiC接触的SBH降低;当石墨烯为2层时,SBH进一步降低且Ni,Ti接触体系的SBH呈现负值,说明接触界面形成了良好的欧姆接触;当石墨烯层数继续增加,SBH不再有明显变化.通过分析接触界面的差分电荷密度以及局域态密度,SBH降低的机理可能主要是石墨烯C原子饱和了SiC表面的悬挂键并降低了金属诱生能隙态对界面的影响,并且接触界面的石墨烯及其与金属相互作用形成的混合相具有较低的功函数.此外,SiC/石墨烯界面形成的电偶极层也可能有助于势垒降低.     

改进WKB近似的新方法

利用转移矩阵理论，在考虑层间一次反射和转折点处实际相移的基础上，导出了改进的ＷＫＢ公式，数值计算的结果表明本文所得公式的精度远优于传统的ＷＫＢ近似，而且能适用于接近于截止的模式和变化剧烈的折射率分布。     

N2介质阻挡放电中有效电场的光谱测定

采用蒙特卡罗方法，模拟了N2非平衡态直流放电等离子体过程。计算了不同E／N条件下电子在氮气中的漂移速度，结果与实验数据符合得很好。模拟了电子激发态粒子数随E／N的变化关系。提出在介质阻挡放电研究和应用中，通过监测两条紫外谱线145和201nm强度之比来监测有效电场的方法。     

On the Role of Capacitance Determination Accuracy for the Electrical Characterization of Pulsed Driven Dielectric Barrier Discharges

A dielectric barrier discharge (DBD) of coaxial geometry has been investigated. The discharge cell was filled by 100 mbar of argon and driven by positive square voltage pulses with a rise time of 20 ns and 75 ns. The internal discharge characteristics such as the discharge current, the gas gap voltage, the instantaneous power and energy have been determined from measured current and voltage waveforms. The peculiarities of the experimental evaluation of the discharge parameters are discussed in detail. Special attention is paid to the accurate experimental determination of the key capacitance values of the DBD, namely the capacitance of the reactor cell C_cell and the capacitance of the dielectric barriers C_d. The influence of the capacitance value accuracy on precision of electrical characterization is demonstrated and it is shown that a small uncertainty in the C_d value leads to large errors in the evaluation of the gas gap voltage. Nevertheless, the obtained accuracy of the capacitance values allows the reliable comparison of the electrical DBD parameters. These are sensitive to the mode of discharge excitation. The shortening of the voltage rise time leads to the increase of the total and instantaneous energy as well as the peak power dissipated into the discharge. (© 2013 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)     

夸克—介子耦合模型中介质相关参数的自洽确定

通过建立夸克－介子耦合（ＱＭＣ）模型与量子强子动力学（ＱＨＤ）模型的等价性条件,自渝地定出了介质相关的ＱＭＣ模型参数,数值计算表明,ＱＭＣ模型袋参数及核子袋半产大,而零点运动参数则不受影响。     

Fission fragment mass yields of Th to Rf even-even nuclei

Fission properties of the actinide nuclei are deduced from theoretical analysis. We investigate potential energy surfaces and fission barriers and predict the fission fragment mass yields of actinide isotopes. The results are compared with experimental data where available. The calculations were performed in the macroscopic-microscopic approximation with the Lublin-Strasbourg Drop (LSD) for the macroscopic part, and the microscopic energy corrections were evaluated in the Yukawa-folded potential. The Fourier nuclear shape parametrization is used to describe the nuclear shape, including the non-axial degree of freedom. The fission fragment mass yields of the nuclei considered are evaluated within a 3D collective model using the Born-Oppenheimer approximation.     

Potential energy surfaces and fission fragment mass yields of even-even superheavy nuclei

Potential energy surfaces and fission barriers of superheavy nuclei are analyzed in a macroscopic-microscopic model. The Lublin-Strasbourg Drop (LSD) model is used to obtain the macroscopic part of the energy, whereas the shell and pairing energy corrections are evaluated using the Yukawa-folded potential; a standard flooding technique is utilized to determine barrier heights. A Fourier shape parametrization containing only three deformation parameters is shown to effectively reproduce the nuclear shapes of nuclei approaching fission. In addition, a non-axial degree of freedom is taken into account to better describe the structure of nuclei around the ground state and in the saddle region. In addition to the symmetric fission valley, a new highly asymmetric fission mode is predicted in most superheavy nuclei. The fission fragment mass distributions of the considered nuclei are obtained by solving 3D Langevin equations.     

Gauge Invariance of a Time-Dependent Harmonic Oscillator in Magnetic Dipole Approximation

A manifestly gauge-invariant formulation of non-relativistic quantum mechanics is applied to the case of time-dependent harmonic oscillator in the magnetic dipole approximation. A general equation for obtaining gauge-invariant transition probability amplitudes is derived.     

Torsional analysis of 2-butynol

The microwave spectrum of 2-butynol, CH₃CCCH₂OH, has been investigated in the frequency range of 6-26.5 GHz. The spectra of the A and E torsional states were observed using Fourier transform microwave spectroscopy. Due to the presence of the cylindrically symmetric CC “spacer” between the methyl group and the rest of the molecule, the barrier to internal rotation, V₃, is only 7 cm⁻¹. One conformer of 2-butynol was observed and assigned. The spectrum was analyzed with the ρ-axis method using a very flexible Hamiltonian which gives a fit an order of magnitude better than that obtained with more standard code for internal rotation. The spectroscopic constants are: 23744.(18), 2093.429(1), 1966.358(1), and −400.34(2) MHz for A, B, C, and D_ab; 0.48(1) kHz, −30.3(4) kHz, and 4.5(5) MHz for Δ_J, Δ_JK, and Δ_K; and 0.1406(6), 6.93(9) cm⁻¹, −33.4(7) kHz, and 192.0(9) GHz for ρ, V₃, L_V, and F, respectively. The root mean squared error of the fit is 14 kHz. The angles between the internal rotor axis and principal axes are θ_a=12°, θ_b=78°, with θ_c held fixed at 90°.     

自由立体显示器中锯齿状交错狭缝光栅的设计

光栅式自由立体显示由于易存在莫尔条纹和串扰的问题而影响其显示效果.利用斜光栅可减轻莫尔条纹但增加了视点间的串扰.本文提出一种减轻莫尔条纹的光栅设计方法,同时对可视区域影响较小.设计中对光栅进行分段,并将相邻两段狭缝错开一定距离.该方法能减小通过同一狭缝看到两相邻子像素之间的黑条的比例,获得较宽且较淡的莫尔条纹,从而减轻了视觉干扰.仿真结果表明该光栅相比传统垂直光栅,莫尔条纹亮度下降了108.1%,而可视区域仅减小32.8%,具有较高的实用价值.     

圆柱形介质阻挡放电等离子体光谱诊断

在350~1150 nm范围内对开放空间Ar气介质阻挡放电等离子体的发射光谱进行测量,表明Ar发射谱线主要集中在680 nm~950 nm,且都为Ar原子谱线。采用发射光谱相对强度对比法,选取相距较近且有相同下能级的727.29 nm(2P2-1S4),738.40 nm(2P3-1S4)和751.47 nm(2P5-1S4)三条光谱测量电子温度。通过对在Ar气和空气中放电谱线的对比和分析,得出发射光谱相对强度与电源功率的关系。最终得出若要便于工业应用和光谱测量,需要选择特定的气体流量和电源功率。     

自由立体显示器中锯齿状交错狭缝光栅的设计

光栅式自由立体显示由于易存在莫尔条纹和串扰的问题而影响其显示效果.利用斜光栅可减轻莫尔条纹但增加了视点间的串扰.本文提出一种减轻莫尔条纹的光栅设计方法,同时对可视区域影响较小.设计中对光栅进行分段,并将相邻两段狭缝错开一定距离.该方法能减小通过同一狭缝看到两相邻子像素之间的黑条的比例,获得较宽且较淡的莫尔条纹,从而减轻了视觉干扰.仿真结果表明该光栅相比传统垂直光栅,莫尔条纹亮度下降了108.1％,而可视区域仅减小32.8％,具有较高的实用价值.     

Quantum Barrier Penetration Studies with Oriented Nuclei: Proton and Neutron Emission from Exotic Isotopes

We report a programme of novel experiments involving direct proton emission and β-delayed proton and neutron emission for exotic nuclei oriented at low temperatures. Full modelling of the quantum tunneling and angular distribution has been made for the first time for these processes. Their study has application in many fields of natural science. The study of barrier effects involving angular momentum and non-spherical deformation can be approached more directly via single-particle emission than via alpha decay, which suffers from complications relating to preformation of the alpha particle. Using the new formalism, predictions are presented for angular distributions of β-delayed neutrons from oriented ¹³⁷I and of direct proton emission from oriented ¹⁴⁷Tm. This revised version was published online in September 2006 with corrections to the Cover Date.