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The B-spline expansion technique and the time-dependent multilevel approach (TDMA) are used to study the interaction between microwave field and sodium atoms. The Rydberg sodium atom energy levels of p states in zero field are calculated, and the results are in good agreement with the other theoretical ones. The time evolutions during the population transfers of the five states from n=75 to n=79 in different microwave fields are obtained. The results show that the coherent control of the population transfer from the lower states to the higher ones can be accomplished by optimizing the microwave pulse parameters. 相似文献
3.
The time-dependent multilevel approach(TDMA) and B-spline expansion technique are used to study the coherent population transfer between the quantum states of a potassium atom by a single frequency-chirped microwave pulse.The Rydberg potassium atom energy levels of n=6-15,l=0-5 states in zero field are calculated and the results are in good agreement with other theoretical values.The time evolutions of the population transfer of the six states from n=70 to n=75 in different microwave fields are obtained.The results show that the coherent control of the population transfer from the lower states to the higher ones can be accomplished by optimizing the microwave pulse parameters. 相似文献
4.
贾光瑞 《原子与分子物理学报》2014,31(6)
采用含时多态展开方法研究了太赫兹场中里德堡铷原子布居数迁移的动力学过程,计算了一个太赫兹脉冲序列与三能级里德堡铷原子系统相互作用后的布居数分布,以及多脉冲序列对多量子态里德堡铷原子系统的相干操控,给出了同一主量子数n中不同角量子数l态布居数的含时演化过程.结果表明:通过优化太赫兹脉冲序列参数,铷原子布居数可由初态被抽运到较高的目标态,在太赫兹频率范围实现里德堡原子的操纵与控制. 相似文献
5.
采用含时多态展开方法研究了太赫兹场中里德堡铷原子布居数迁移的动力学过程,计算了一个太赫兹脉冲序列与三能级里德堡铷原子系统相互作用后的布居数分布,以及多脉冲序列对多量子态里德堡铷原子系统的相干操控,给出了同一主量子数n中不同角量子数l态布居数的含时演化过程.结果表明:通过优化太赫兹脉冲序列参数,铷原子布居数可由初态被抽运到较高的目标态,在太赫兹频率范围实现里德堡原子的操纵与控制. 相似文献
6.
Using a time-dependent multilevel approach, we demonstrate
that lithium atoms can be transferred to states of lower principle
quantum number by exposing them to a frequency chirped microwave
pulse. The population transfer from n = 79 to n = 70 states of
lithium atoms with more than 80% efficiency is achieved by means
of the sequential two-photon Δ n = - 1 transitions. It is
shown that the coherent control of the population transfer can be
accomplished by the optimization of the chirping parameters and
microwave field strength. The calculation results agree well with
the experimental ones and novel explanations have been given to
understand the experimental results. 相似文献
7.
运用含时多态展开方法和B-样条函数研究了啁啾频率微波场中里德伯钠原子的量子态之间的布居数迁移.计算了里德伯钠原子n=70-77的开普勒频率.计算了在不同的微波场中六个态的布居数从n=70到n=77随时间的迁移,布居数跃迁到最终态n=77达到了98%,这可以通过连续的单光子跃迁来实现.结果表明,通过优化微波脉冲参数可以实现从低态到较高态的布居跃迁的相干控制. 相似文献
8.
We present a theoretical study of dynamics of Rydberg states of lithium using ultra short chirped laser pulse having a Gaussian
envelope. The population transfer probabilities are calculated of different Rydberg states on chirped laser factors. The calculations
are performed by direct numerical integration of Schr?dinger equation using fourth order Runge-Kutta method. The behavior
of dynamics of Rydberg states for these factors is of great significance. These results are of potential interest in coherent
quantum control, quantum computation and in many physical and chemical processes. 相似文献
9.
H. Rinneberg J. Neukammer A. König K. Vietzke H. Hieronymus M. Kohl H. -J. Grabka G. Jönsson 《Hyperfine Interactions》1987,38(1-4):515-530
The purpose of the present paper is to illustrate some selected aspects of high resolution laser spectroscopy of Rydberg atoms,
rather than giving an extensive review of the state of the art. The following topics will be discussed: (i) Excitation and
detection of Ba Rydberg atoms with principal quantum numbers up ton≲300; (ii) Stark effect and atomic diamagnetism of high-n Ba Rydberg states in thel-mixing region, (iii) Resonance in singlet-triplet mixing of 6snp1P1 and 6snd1D2 Ba Rydberg states deduced from hyperfine structure measurements. 相似文献
10.
I. I. Beterov I. I. Ryabtsev D. B. Tretyakov N. N. Bezuglov A. Ékers 《Journal of Experimental and Theoretical Physics》2008,107(1):20-27
The results of theoretical calculations of the blackbody ionization rates of lithium, potassium, and cesium atoms residing in Rydberg states are presented. The calculations are performed for nS, nP, and nD states in a wide range of principal quantum numbers, n = 8?65, for blackbody radiation temperatures T = 77, 300, and 600 K. The calculations are performed using the known quasi-classical formulas for the photoionization cross sections and for the radial matrix elements of transitions in the discrete spectrum. The effect of the blackbody-radiation-induced population redistribution between Rydberg states on the blackbody ionization rates measured under laboratory conditions is quantitatively analyzed. Simple analytical formulas that approximate the numerical results and that can be used to estimate the blackbody ionization rates of Rydberg atoms are presented. For the S series of lithium, the rate of population of high-lying Rydberg levels by blackbody radiation is found to anomalously behave as a function of n. This anomaly is similar to the occurrence of the Cooper minimum in the discrete spectrum. 相似文献
11.
The dynamics of hydrogen atom in the presence of a strong radiation field of the titanium-sapphire laser is studied for the Keldysh parameters γ ≥ 1 and γ ≤ 1. It is demonstrated that the ionization is supplemented with the effective population of the excited states with the principal quantum numbers n = 5–10 in the entire range of variation in the Keldysh parameter. The population of the excited Rydberg states can be interpreted as a consequence of the multiphoton resonance involving the initial 1s state and a group of excited states in the vicinity of the continuum boundary with the simultaneous repopulation of these states by Λ-type Raman transitions under the action of the laser field. The resulting coherent Rydberg packet appears to be stable with respect to ionization, so that the ionization of the atomic system in the presence of strong electromagnetic field is suppressed. Physical reasons for the stabilization are discussed. An interpretation of the effective population of the Rydberg states in the recent experiments on the ionization of atomic helium by the titanium-sapphire laser is proposed. 相似文献
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David R. Herrick 《Molecular physics》2013,111(5):1211-1219
The impact parameter method is applied to high Rydberg atoms for estimating Δn=0 dipole transition cross sections. Values for high-l states are determined in large part by polarization and relativistic fine-structure contributions to energy levels. Computed cross sections for low-l helium atoms show good agreement with angular momentum transfer cross sections from electron impact experiments over the range 20<n<80. 相似文献
14.
Single colour three photon resonant ionization (2 + 1) is observed in atomic potassium vapour in a heat pipe oven using an
excimer laser pumped dye laser. Using wavelengths between 570 nm and 603 nm various2S and2D Rydberg states are populated by two photon excitation. Third photon of the same wavelength ionizes the atoms. Rydberg states
up ton ⋍ 50 are observed. Electric field as low as 1 V/cm causes extensive Stark mixing of the states. This results in progressively
higher three photon ionization signals via the perturbed2P and2F Rydberg states. The three photon ionization process is studied using both linearly and circularly polarized incident light.
The experiment shows qualitatively that the2P Rydberg states are perturbed primarily by the2D states in the prescence of an external electric field and to a much smaller extent by2S states. This is also explained theoretically by calculating the Stark mixing coefficients under the Bates and Daamgard (1949)
approximation. Implication for a similar effect in other alkali elements is discussed. 相似文献
15.
S. Westermann T. Amthor A. L. de Oliveira J. Deiglmayr M. Reetz-Lamour M. Weidemüller 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2006,40(1):37-43
We investigate excitation transfer and migration
processes in a cold gas of rubidium Rydberg atoms.
Density-dependent measurements of the resonant population exchange
for atoms initially excited into the 32P3/2(|mJ|=3/2) state
are compared with a Monte Carlo model for coherent energy
transfer. The model is based on simulations of small atom
subensembles involving up to ten atoms interacting via coherent
pair processes. The role of interatomic mechanical forces due to the
resonant dipole-dipole interaction is investigated.
Good agreement is found between the experimental data and the
predictions of the model, from which we infer that atomic motion
has negligible influence on the energy transfer up to Rydberg
densities of 108 cm-3, that the system has to be described in terms
of many-body dynamics, and that the energy transfer
preserves coherence on microsecond timescales. 相似文献
16.
A. Wetzels A. Gürtler H.G. Muller L.D. Noordam 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2001,14(2):157-165
An optically excited Rydberg wavepacket can be generated by exciting the electron from a low-lying state to a coherent superposition
of high-lying states with a short broadband optical pulse. A special kind of Rydberg wavepacket is generated in the case of
a interaction of a weak THz half cycle pulse with a stationary Rydberg state, called the THz wavepacket. This THz wavepacket
is a coherent superposition of the initial Rydberg state and its neighbouring states. We have investigated the time evolution
of THz wavepackets by measuring the impact of two in time delayed half cycle pulses ( ≈ 200 V cm-1) on the population of a stationary (n = 40) Rydberg state in rubidium. The first half cycle pulse creates the THz wavepacket and the second half cycle pulse probes
the dynamics of the THz wavepacket. We support our experimental data by numerically solving the Schr?dinger equation and with
a semi-classical picture. Whereas an optically excited wavepacket is initially localized, a THz wavepacket is initially delocalized
and becomes localized after half a revival time.
Received 23 August 2000 and Received in final form 27 March 2001 相似文献
17.
M. G. Giammarchi 《Hyperfine Interactions》2009,193(1-3):321-327
Antihydrogen production by charge exchange reaction between positronium (Ps) and antiprotons requires an efficient excitation of Ps atoms up to high-n levels (Rydberg levels). We propose a two-step laser light excitation, the first from ground to n?=?3 and the second from this level to a Rydberg level n?>?15. In this study it is assumed that a Ps cloud is produced by positrons hitting a target converter located in a Penning-Malmberg trap within a uniform ~ 1 T magnetic field. We model the optical transition structure by taking into account Doppler and motional Stark effects. The predicted efficiency for population deposition in high n states is of ~30%. 相似文献
18.
The autoionization mechanisms of dense nP3/2 (n = 20–97) Rydberg gases of 87Rb atoms in the spontaneous evolution were investigated for the first time. By observing the characteristic time of the electrons generated through autoionization process, the dependence of autoionization mechanisms (black-body radiation, electron–Rydberg collision, and Penning ionization) on the principal quantum number n of initial nP states was demonstrated. The dependence on the number n in nP Rydberg atoms is similar to those in nD Rydberg atoms. 相似文献
19.
The B-spline expansion technique and the time-dependent multilevel approach (TDMA) are used to study the interaction between a microwave field and sodium atoms. The Rydberg sodium atom energy levels of p states in zero field are calculated, and the results are in good agreement with the other theoretical ones. The time evolutions during the population transfers of the five states from n = 75 to n = 79 in different microwave fields are obtained. The results show that the coherent control of the population transfer from the lower states to the higher ones can be accomplished by optimizing the microwave pulse parameters. 相似文献
20.
利用电热法将含金物质加热,产生Au原子束,再以两束UV脉冲激光垂直照射,将处于基态的Au原子共振激发至高Rydberg态。滞后于激光脉冲200ns的高压脉冲电场(6500V/cm)加到反应区,使处于Rydberg态的Au原子电离。激光波长在一定范围内扫描,共测出了Au原子的n2D3/2(n=18—38)和n2S1/2(n=21—34;36—38)两通道的38条能级的位置。用参数拟合得到2D3/2和2S1/2两系列的极限分别为:ED=74409.8(3)cm-1,ES=74410.0(2)cm-1,计算了每条能级的量子亏损。我们的实验还证明了场电离是一种十分有效的电离手段,比用通常的激光光电离效率要高得多。这在共振电离谱学(RIS)的研究中是一种很有效的方法。
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