Magnetic moments of isomeric bandheads in transitional nuclei: 119I and 192Tl

Nuclear g-factors of isomeric bandheads in the transition nuclei ¹¹⁹I and ¹⁹²Tl have been measured to be $\text{g[}{}^{119}\text{I}\text{(}\text{9}\text{2}{}^{\mathrm{+}}\text{)] = 1.20(3)}$ and $\text{g[}{}^{192}\text{Tl}\text{(8}{}^{\mathrm{?}}\text{)] = 0.207(5)}$. These values are in agreement with a model of one or two quasiparticles coupled to a deformed core. This interpretation is also supported by a preliminary quadrupole moment determination of $\text{Q[}{}^{192}\text{Tl}\text{(8}{}^{\mathrm{?}}\text{)] = 45(9)}\text{fm}{}^2$. The lifetimes were remeasured to be $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 34.6(5)}\text{ns}$ and $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 296(5)}\text{ns}$ for the ¹¹⁹I and the ¹⁹²Tl isomers, respectively.     

Magnetic dipole moments near Sn: Measurement on isomeric 11/2 states in odd-A Te and Te by NMR/ON

On-line low temperature nuclear orientation (OLNO) experiments have been performed on the odd-A Te isotopes ¹³¹Te and ¹³³Te using the technique of nuclear magnetic resonance on oriented nuclei (NMR/ON). The magnetic moments of the isomeric 11/2⁻ states have been measured extending the known data on these states in the Te isotopes up to the neutron shell closure at N = 82. The contribution to the 11/2⁻ magnetic moment in ¹³³Te due to core polarisation is calculated using an RPA shell model as well as corrections to the magnetic dipole operator caused by mesonic exchange currents. The neutron number dependence of the magnetic moments of the 11/2⁻ isomers in heavy Te isotopes is discussed in terms of particle-core coupling model (PCM) calculations.     

On the static quadrupole moments of the 21 states in Te and Te

The reorientation effect in Coulomb excitation was used to measure the static quadrupole moments of the first 2⁺ states in ¹²⁶Te and ¹²⁸Te. The particle-γ coincidence technique using a large NaI(Tl) crystal was employed to measure relative excitation probabilities at backward and forward projectile scattering angles. The Winther-de Boer multiple Coulomb excitation program was used to analyze the data. The influence of the deorientation effect was also determined. For positive interference via the second 2⁺ state the extracted quadrupole moments of the first 2⁺ states are; −0.20±0.09 b and -0.24±0.08 b for ¹²⁶Te and ¹²⁸Te respectively. The quadrupole moments of the first 2⁺ states of^{122,124,126,128,130}Te determined by different techniques are in excellent agreement with one another. The values are compared with recent theoretical calculations.     

Properties of the 3/2~-[521] band in the odd-N rare-earth nuclei

High-spin states in 161Er have been studied experimentally via the 150Nd(16O, 5n) reaction at a beam energy of 86 MeV. Three rotational bands built on the 5/2+[642], 3/2-[521], and 11/2-[505] configurations have been extended up to high-spin states, and particularly, the α = -1/2 branch of the ground state 3/2-[521] band has been revised significantly. It is found that signature inversion occurs in the 3/2-[521] band after the band crossing in 161Er. The systematics of the signature inversion associated wit...     

Magnetic moments of proton drip-line nuclei13O and9C

The magnetic moments of the proton drip-line nuclei¹³O(I = 3/2^–,T _1/2 = 8.6 ms) and 9C(I = 3/2^–,T _1/2 = 126 ms) have been determined for the first time through the combined techniques of polarized radioactive nuclear beams and-NMR detection. The observed magnetic moments are ¦(¹³O)¦ = 1.3891 ±0.0003 _N and ¦(⁹C)¦ = 1.3914 ±0.0005 _N. Spin expectation values are deduced to be 0.76 and 1.44 for¹³O and⁹C, respectively. While the of¹³O is consistent with the systematics from isospinT= 1/2 mirror pairs, the of⁹C is unusually large, even far larger than the single particle value, = 1.     

Magnetic moments of spherical nuclei: Status of the problem and unsolved issues

Dipole magnetic moments of more than 100 odd spherical nuclei are calculated within the theory of finite Fermi systems. For the effective interaction of nucleons within the theory of finite Fermi systems, use is made of a version that takes into account nuclear-medium-modified amplitudes for the exchange of one pion and one rho meson. A new tensor local charge ζ _t is incorporated in the theory of finite Fermi systems in addition to the known orbital (ζ _l ) and spin (ζ _s ) local charges. Good agreement with experimental data, at a level of 0.1 to 0.2μ _N , is obtained for the overwhelming majority of the nuclei considered here. Several cases of a significant discrepancy with experimental data, at a level of 0.3 to 0.5μ _N , are revealed. Possibilities for removing these discrepancies are discussed. A detailed comparison with known results obtained within the multiparticle shell model is performed for 2p-to 1f-shell nuclei. Cases where the standard theory of finite Fermi systems must be extended by taking into account multiparticle configurations are found. Magnetic moments are analyzed for a number of long isotopic chains. Several new experimental values of magnetic moments for copper isotopes far from the beta-stability valleys are known. For the example of the copper-isotope chain, it is shown how the emergence of a deformation in the ground state of a nucleus can be revealed on the basis of a systematic analysis of magnetic moments.     

Evidence for the existence of the [2 0 2]3/2 deformed band in mirror nuclei 25Mg and 25Al

After 50 years of its prediction, the highest-lying [2 0 2]3/2 orbit among the six Nilsson single-particle orbits originating from the sd shells in prolately deformed nuclei and the rotational band on this orbit were identified. The band members were observed in 25Al at excitation energies of 6-7.5 MeV in a high-resolution 25Mg(3He,t) charge-exchange reaction at 0 degrees having a strong selectivity for Gamow-Teller transitions. In the comparison with the analogous M1 transitions in 25Mg, the J(pi)=3/2(+) bandhead state and the excited 5/2(+) and 7/2(+) members were clearly assigned.     

Microscopic calculations for the two 5/2 − resonances of the nuclei 7Li and 7Be

Calculations for the two 5/2 ? resonances of the mirror nuclei ⁷Li and ⁷Be are performed within the framework of cluster representations of nuclei. Using the same microscopic forces for both nuclei, their phase-shift and resonance width differences in the energy region of the 5/2 ? resonances are shown to be mainly due to effects produced by the Coulomb interaction.     

Magnetic moments and structure of the nuclei3H,3He and of baryons

From a solution of the problem of magnetic moments of the nuclei³H and³He, two properties are obtained: - These nuclei have mixed orbital ground states. - These states are not charge symmetric. The first property is expected to hold also for baryons in the quark model, on account of recently measured magnetic moments. Supporting evidence and implications for baryon structure are discussed.     

Magnetic moments of high-spin states above the rotational band of 168Hf and 172Hf

The transient magnetic field IMPAC technique was used to measure the magnetic moments of high-spin states above the rotational band of ¹⁶⁸Hf and ¹⁷²Hf, populated in the reactions ^{156, 160}Gd(¹⁶O, 4n). The average g-factors of these prerotational feeding states were deduced to be 0.07 ± 0.04 and 0.14 ± 0.04 for ¹⁶⁸Hf and ¹⁷²Hf, respectively. These results are in agreement with a reduction of the collective g-factors due to a neutron phase transition.     

A tunneling spectroscopy study of the temperature dependence of the forbidden band in Bi2Te3 and Sb2Te3

Tunneling measurements of dI/dV, d ² I/dV ², and d ³ I/dV ³ were formed along the C ₃ axis (normally to layers) for Bi₂Te₃ and Sb₂Te₃ layered semiconductors in the temperature range 4.2<T>29 5 K. Temperature dependences of the forbidden band energy E _g were obtained. The forbidden band energy in Bi₂Te₃ was 0.20 eV at room temperature and increased to 0.24 eV at T=4.2 K. The E _g value for Sb₂Te₃ was 0.25 eV at 295 K and 0.26 eV at 4.2 K. The distance between the top of the higher valence band of light holes and the top of the valence band of heavy holes situated lower was found to be ΔE _V≈19 meV in Bi₂Te₃; this distance was independent of temperature. The conduction bands of Bi₂Te₃ and Sb₂Te₃ each contain two extrema with distances between them of ΔE _c≈25 and 30 meV, respectively.     

Masses of nuclei of the 1f 7/2 subshell

Binding and one-nucleon separation energies are calculated for nuclei with 20 ≤ Z, N ≤ 28, where both protons and neutrons occupy the 1f _7/2 valence subshells. To this aim, two different methods are applied. The first method employs the self-consistent approach with the effective Skyrme forces and pairing interaction, while the second one makes use of the semiempicial multiparticle shell model with the effective two-body matrix elements of the interaction defined from the empirical data. The intercomparison between the two methods is carried out. The text was submitted by the authors in English.     

Magnetic State of Layered Cobalt Chalcogenides Co7Se8 and Co7Te8

JETP Letters - The structural and magnetic properties of the Co7Te8 layered compound have been studied for the first time using X-ray diffraction, measurements of the magnetic susceptibility, and...     

Interpretation of (h11/2)2 isomers in the N≈76 region of transitional nuclei

The E2 hindrance factors of high spin isomers involving (h_11/2)² excitations in the N ≈ 76 and Z ≈ 76 regions of transitional and deformed nuclei are compared. Using the correlation with the product of the valence nucléon numbers N_pN_n, a systematic picture of the weakly K-forbidden decays is presented.     

Optical properties and electronic band structure of CdGa2Te4

Optical properties of a defect-chalcopyrite-type semiconductor CdGa₂Te₄ have been studied by optical absorption, spectroscopic ellipsometry (SE), and electroreflectance (ER) measurements. Optical absorption measurements suggest that CdGa₂Te₄ is a direct-gap semiconductor having the band gap of ∼1.36 eV at 300 K. The complex dielectric-function spectra, ε(E)=ε₁(E)+iε₂(E), measured by SE reveal distinct structures at energies of the critical points (CP's) in the Brillouin zone. ER spectrum facilitates the precision determination of the CP parameters (energy position, strength, and broadening). By performing the band-structure calculation, these CP's are successfully assigned to specific points in the Brillouin zone.     

Theoretical and experimental investigations of the properties of Ge2Sb2Te5 and indium-doped Ge2Sb2Te5 phase change material

We have carried out comprehensive computational and experimental study on the face-centered cubic Ge₂Sb₂Te₅ (GST) and indium (In)-doped GST phase change materials. Structural calculations, total density of states and crystal orbital Hamilton population have been calculated using first-principle calculation. 5 at.% doping of In weakens the Ge–Te, Sb–Te and Te–Te bond lengths. In element substitutes Sb to form In–Te-like structure in the GST system. In–Te has a weaker bond strength compared with the Sb–Te bond. However, both GST and doped alloy remain in rock salt structure. It is more favorable to replace Sb with In than with any other atomic position. X-ray diffraction (XRD) analysis has been carried out on thin film of In-doped GST phase change materials. XRD graph reveals that In-doped phase change materials have rock salt structure with the formation of In₂Te₃ crystallites in the material. Temperature dependence of impedance spectra has been calculated for thin films of GST and doped material. Thickness of the as-deposited films is calculated from Swanepoel method. Absorption coefficient (α) has been calculated for amorphous and crystalline thin films of the alloys. The optical gap (indirect band gap) energy of the amorphous and crystalline thin films has also been calculated by the equation \( \alpha h\nu = \beta (h\nu - E_{\text{g }} )^{2} \) . Optical contrast (C) of pure and doped phase change materials have also been calculated. Sufficient optical contrast has been found for pure and doped phase change materials.     

Signal enhancement in 5QMAS spectra of spin-5/2 quadrupolar nuclei

5QMAS experiments on spin-5/2 systems display a low sensitivity compared with their 3QMAS counterparts. Nevertheless, the superior resolution of 5QMAS over 3QMAS makes these experiments a favorable choice for many materials. We report an enhancement scheme for the 5QMAS experiment, using an improved five-quantum excitation pulse scheme combined with a FAM-II conversion pulse. The results are verified experimentally on a polycrystalline sample of gamma-(27)Al(2)O(3), showing an enhancement factor of 2.4 over the simple two-pulse (CW) 5QMAS scheme. Numerical computations of the efficiency parameter epsilon support these results.     

Lifetimes in the ground-state band and the structure of 118Te

Lifetimes of excited states in ¹¹⁸Te have been measured using the Doppler Shift Attenuation (DSA) and Recoil Distance (RD) methods in the ¹⁰⁹Ag(¹³C, p3n) reaction at a beam energy of 54 MeV. Lifetime values of the ground-state band levels with spins I ^π = 2⁺-16⁺ have been obtained. The excitation energies and B(E2) values are interpreted in the framework of a version of IBFM ( IBM + 2qp) with the maximum boson number exceeding its standard value. A satisfactory agreement with experimental level scheme and B(E2) values for the ground-state band is achieved. Received: 7 June 2001 / Accepted: 7 February 2002     

Magnetic susceptibility and band structure of intercalation compounds of 2H-TaS2

A universal correlation is reported between the magnetic susceptibility of the TaS₂ layers at 300 K and the population (1 to 2 e^-/TaS₂) of the TaS₂ conduction d-band in intercalation compounds of 2H-TaS₂. From this curve, the variation in the density of states at the Fermi level D(E_F) with E_F was derived; good agreement with the variation predicted by band structure calculations for 2H-TaS₂ was found.