Manifestation of anisotropic collisional generation of higher polarization moments in polarization of quadrupole emission

Direct observability of polarization moments of a higher order—octupole orientation of atomic angular momenta (κ=3) and their hexadecapole alignment (κ=4)—from polarization of quadrupole radiation is discussed. The case when atoms are excited through dipole absorption of light producing orientation or alignment of angular momenta with κ=1 or 2 and higher polarization moments are induced by collisions with a beam of particles is considered. It is shown that differences in the laws of transformation of polarization moments of various ranks κ in rotations of coordinate axes allow us to select the pure contribution of the higher polarization moment under study from the signal of polarization of quadrupole emission by excluding the contribution of orientation or alignment with κ=1 or 2. Optimum systems of coordinate axes for the observation of octupole orientation from circular polarization of light and for the observation of hexadecapole alignment from linear polarization of light, in which the pure contribution of the higher polarization moment under study to polarization of quadrupole emission reaches its maximum, are calculated.     

Contribution of hexadecapole alignment to the polarization of quadrupole emission under laser excitation conditions

The linear polarization of quadrupole emission by the J=2-J ₀=0 transition under conditions of laser excitation in a gas medium is studied. Cases of excitation through dipole and quadrupole absorption of monochromatic laser radiation are considered. Taking into account the anisotropy of collisional relaxation, the contributions of polarization moments of the second and fourth ranks, i.e., those with usual and hexadecapole alignments, to the signal of linear polarization of quadrupole emission are calculated. The dependence of this signal on the laser frequency, the density of the gas medium, and the angles determining the orientation of the system of axes of observation of light polarization relative to a laser ray is studied. The numerical calculations of contributions of usual and hexadecapole alignment to the signal of linear polarization are made for the magnetic quadrupole transition J=2-J ₀=0 between the states 2p ⁵(² P ₁ ^2/0 )3p′[3/2]₂ and 2p ⁵(² P ₁ ^2/0 )3s 3s′[1/2]⁰ of neon atoms in the xenon atmosphere.     

Core polarization corrections to magnetic dipole moments and transitions

Core polarization corrections to ground state magnetic dipole moments are calculated in first-order perturbation theory, with the use of Sussex matrix elements. These corrections are introduced in the particle-(hole-) core coupling model. It is shown that the need for effectiveg _s factors in the calculation of magnetic moments can be explained largely in terms of one-particle-one-hole polarization effects of the core. The influence of these effects on the reducedM1 transition probabilities forl-forbidden transition is also considered.     

Manifestation of higher polarization moments of the electronic shell of an atom in the collisional population transfer between the hyperfine-structure levels

The contributions of the relaxation of electronic polarization moments of various orders κ to the probabilities for the population transfer between the hyperfine-structure levels of an atom under the action of collisions are studied. It is shown that the contributions of higher electronic polarization moments with κ > 2 are comparable with the contributions of the orientation (κ=1) and the alignment (κ=2) or even exceed them in magnitude. This opens up the possibility of studying the collisional relaxation of higher polarization moments which are usually not observed and not involved in the emission and absorption of light under dipole transitions. The bounds for the allowable values of the rate constants for the collisional relaxation of higher polarization moments are obtained from the condition for nonnegativity of the total probabilities of population transfer between different hyperfine-structure levels under the action of collisions.     

Pair production and vacuum polarization of vector particles with electric dipole moments and anomalous magnetic moments

The matrix 8-component Dirac-like form of the P-odd equations for boson fields of spin 1 and 0 are obtained and the symmetry group of the equations is derived. We found exact solutions of the field equation for vector particles with arbitrary electric and magnetic moments in external constant and uniform electromagnetic fields. The differential probability of pair production of vector particles with electric dipole moments and anomalous magnetic moments by an external constant and uniform electromagnetic field has been found using exact solutions. We have calculated the imaginary and real parts of the electromagnetic field Lagrangian that takes into account the vacuum polarization of vector particles. Received: 14 April 2001 / Revised version: 13 July 2001 / Published online: 19 September 2001     

Influence of local excitation of octupolar Oligophenylenevinylenes on their dipole moments

Absorption and fluorescence spectra of octupolar centrosymmetric oligophenylenevinylene dyes (E,E)-bis[2-(4-hexyloxyphenyl)ethenyl]-(E,E)-3,6-bis-[2-(4-N,N-dipropylaminophenyl)ethenyl]pyrazine and (E,E,E,E)-2,3,5,6- tetra-[2-(4-hexyloxyphenyl)ethenyl]pyrazine were measured in various solvents. An electro-optical absorption method was used to determine their dipole moments as μ _g  = 6.1∙10^–30 and 3.4∙10^–30 C∙m in the equilibrium ground state and the increased values ∆ ^a μ = 11.9∙10^–30 and 8.2∙10^–30 C∙m upon excitation into a Franck–Condon state. Quantum-chemical calculations showed that the molecules had non-planar configurations. The π,π-conjugated system was localized on the most planar part of the molecule that was responsible for light absorption in the range 300–450 nm due to a change in the geometry of the molecules in the ground state. Localized excitation of the molecules caused their dipole moments ∆ ^a μ to change significantly.     

纳米银线波导中表面等离极化波激发和辐射的偏振特性研究术

在可见光波段（λ=750nm）,实验研究了在端面辅助情况下,细纳米银线波导中表面等离极化波激发和辐射的偏振特性．实验发现在细纳米银线中,不同偏振态的入射光对应的表面等离极化激元的激发和传输效率有明显不同,但对应的出射光始终为方向恒定的线偏振光．对于化学合成的纳米银线,端面的轴对称性普遍比较好,对此类纳米银线进行激发时,如果入射光偏振态与纳米线近似平行,则激发和传输表面等离极化激元的效率最高;如果正交,激发和传输效率则最低．对于某些端面轴对称性较差的纳米银线,如端面为尖端或类斜面,当入射光偏振态与纳米线有一定夹角时,激发和传输表面等离极化激元的效率最高．在入射光偏振改变的过程中出射光的偏振方向始终与纳米银线平行．最后结合有限元差分方法理论解释了纳米银线中这种偏振特性的物理机理．利用纳米银线中表面等离极化激元激发和辐射的偏振特性,可以在亚波长尺寸上实现对光强和偏振态的调控．     

各向异性量子点单光子发射的高偏振度特性

研究了线偏振脉冲光场激发下,单个各向异性InGaAs量子点的高偏振光发射. 给出其偏振因子与两个正交本征态之间的交叉弛豫之间的关系式. 分析表明，交叉弛豫随激发场强度增大，并导致偏振因子随激发场入射脉冲面积减小. 关键词： 量子点 单光子发射 偏振度     

Manifestation of the polarization incoherence of light in polarization self-action effects

On the basis of the beam tensor formalism proposed by F. I. Fedorov, the theory of polarization selfaction of radiation in isotropic resonant media is extended to the case of partial elliptic polarization of an electromagnetic wave. The influence of the degree of radiation polarization on the known polarization self-action effects is demonstrated and the self-polarization (depolarization) of light is predicted.     

Spontaneous and stimulated emission in GaSe under intense excitation

Emission spectra have been investigated in GaSe at 80 K under nitrogen laser excitation. In the case of intense excitation, an additional broad band appears at 5970 Å, and is considered to be due to an exciton-exciton collision process. This process leads to stimulated emission.     

Leptonic dipole moments in the left-right supersymmetric model

The observation of neutrino oscillations imposes a pattern of mixing in both the sneutrino and charged slepton sectors. On the other hand, the apparent 2.6 deviation of the anomalous magnetic moment of the muon from the standard model value favors a scenario beyond the standard model. We show that, in a supersymmetric model with left-right symmetry, which provides an explanation for both phenomena, the relationship between flavor conserving dipole moments, such as the magnetic and the electric dipole moments, and flavor violating dipole moments, such as and , is quite different from that in the MSSM. From general analytic considerations, we derive bounds on the fractional sneutrino mass splittings , and the fractional charged slepton splittings . For , the mixing is allowed to be maximal. We also comment on the magnitudes and correlations between CP-violating angles coming from electric dipole moments. We supplement the analytical considerations by detailed numerical calculations. Received: 6 September 2001 / Revised version: 30 October 2001 / Published online: 7 December 2001     

The influence of higher spatial harmonics of atomic polarization on the saturated absorption resonance upon excitation of open dipole transitions by a field of counterpropagating waves

The effect of a double structure of saturated absorption resonance in the field of counterpropagating light waves interacting with an atomic gas is studied. The experimental observation of this effect was first reported in 2011 in a work by our colleagues at the P.N. Lebedev Physical Institute of the Russian Academy of Sciences (Laboratory of Frequency Standards). The essence of the effect lies in the fact that, on exciting an open dipole transition, another, narrower, resonance of an opposite sign can be observed at the center of the ordinary saturated absorption resonance. A theoretical analysis of this effect has also been performed in this work in terms of a simple spectroscopic model of an atom with two nondegenerate energy levels without taking into account higher spatial harmonics of atomic polarization and polarizations of light waves (scalar model). The present work is devoted to the development of a theory of the formation of a central narrow resonance for the example of a real F _g = 1 → F _e = 1 atomic transition and to the study of its main characteristics (amplitude, width, contrast, and amplitude-to-width ratio). In addition, the theoretical results obtained without taking into account the influence of higher spatial harmonics and with inclusion of the influence of first higher harmonics are compared. This comparison shows that their influence on the parameters of the new nonlinear resonance is strong even in moderately intense light fields (R ~ γ, where R is the Rabi frequency). The results of this study can be of interest for quantum metrology, as well as for many experiments in which the laser-radiation frequency is stabilized by the saturated absorption resonance on open dipole transitions in atoms and molecules.     

Electric dipole moments in the limit of heavy superpartners

Supersymmetric loop corrections induce potentially large CP-violating couplings of the Higgs bosons to nucleons and electrons that do not vanish in the limit of heavy superpartners. The Higgs-mediated CP-odd four-fermion operators are enhanced by tan((3)beta and induce electric dipole moments of heavy atoms which exceed the current experimental bounds for the electroweak scale Higgs masses and tan(beta greater, similar 10. If only the first two sfermion generations are heavy, the Higgs-mediated contributions typically dominate over the Barr-Zee type two-loop diagrams at tan(beta>30.     

Vector polarization effect appearing in tensor polarized beams of nuclei under channeling conditions and during measurements of the quadrupole moments of unstable nuclei

General relations describing the spin dynamics of beams of nuclei with initial tensor and vector polarizations have been derived upon planar channeling in bent crystals. The performed analysis indicates that the vector polarization effect predicted by Baryshevsky and Sokolsky can be detected, occurring upon the planar channeling of a beam of nuclei with initial tensor polarization. The planar channeling of a beam of nuclei with initial tensor and vector polarizations can be used to determine the quadrupole moments of unstable nuclei with small lifetimes, up to 10⁻⁷ s. The quadrupole moments of nuclei with lifetimes of about 10⁻⁷ s cannot be measured via known methods, including optical methods.     

The microwave spectra and dipole moments of the cyanopyridines

Rotational transitions of 4-cyanopyridine, 3-cyanopyridine and 2-cyanopyridine have been observed and assigned. The values of the rotational constants for these three molecules are (in MHz):

$\text{4-cyanopyridine}\text{A=6000.}\text{B=1541.19}\text{C=1226.00}\text{3-cyanopyridine}\text{A=5823.01}\text{B=1571.34}\text{=1237.17}\text{2-cyanopyridine}\text{A=5835.756}\text{1598.219}\text{1254.460}$

The dipole moment components were also measured and are (in Debye):

$\text{4-cyanopyridine}\text{μ}{}_{\mathrm{a}}\text{=1.96}\text{μ}{}_{\mathrm{b}}\text{=0}\text{μ}{}_{\mathrm{total}}\text{=1.96}\text{3-cyanopyridine}\text{μ}{}_{\mathrm{a}}\text{=3.13}\text{μ}{}_{\mathrm{b}}\text{=1.90}\text{μ}{}_{\mathrm{total}}\text{=3.66}\text{2-cyanopyridine}\text{μ}{}_{\mathrm{a}}\text{=5.47}\text{μ}{}_{\mathrm{b}}\text{=1.87}\text{μ}{}_{\mathrm{total}}\text{=5.78}$

     

Spin resonance conditions for intrinsic and induced electric dipole moments of a spin-1 particle

We show that spin resonance caused by the tensor polarizability of a spin-1 particle rotating in a storage ring designed to measure the intrinsic electric dipole moment (EDM) is canceled on the average over time when conditions for the spin resonance caused by this EDM are precisely met. This solves the problem of a false EDM signal created by polarizability.