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1.
We give a qualitative review of theoretical ideas and experimental work on laser-induced excitation of atomic Rydberg wave packets. Studying the motion of Rydberg wave packets with the help of short or intense laser pulses provides a bridge between quantum mechanics and the classical concept of the trajectory of an electron and corresponds to the real-time observation of atomic dynamics. 相似文献
2.
We present a quantitative semiclassical theory for the decay of nondispersive electronic wave packets in driven, ionizing Rydberg systems. Statistically robust quantities are extracted combining resonance-assisted tunneling with subsequent transport across chaotic phase space and a final ionization step. 相似文献
3.
本文采用激光短脉冲激发磁场中氢原子,研究氢里德堡波包在磁场中随时间的演化.结果证实氢里德堡波包在磁场中的运动也与闭合轨道密切相关.讨论了脉冲宽度τ对自动关联函数的影响以及不同初始态下的自动关联函数. 相似文献
4.
Mestayer JJ Wyker B Lancaster JC Dunning FB Reinhold CO Yoshida S Burgdörfer J 《Physical review letters》2008,100(24):243004
We demonstrate a protocol to create localized wave packets in very-high-n Rydberg states which travel in nearly circular orbits around the nucleus. Although these wave packets slowly dephase and eventually lose their localization, their motion can be monitored over several orbital periods. These wave packets represent the closest analog yet achieved to the original Bohr model of the hydrogen atom, i.e., an electron in a circular classical orbit around the nucleus. The possible extension of the approach to create "planetary atoms" in highly correlated stable multiply excited states is discussed. 相似文献
5.
Recent theoretical work on the dynamics of electronic Rydberg wave packets under the influence of laser-induced core transitions is reviewed. The discussion focuses on the intricate interplay between laser-modified electron correlation effects, radiative damping by the ionic core and the time evolution of electronic Rydberg wave packets. Via the stimulated light force this interplay manifests itself also in the atomic center of mass motion. A unified theoretical framework is provided by combining methods of quantum defect theory, stochastic techniques and semiclassical path expansions. 相似文献
6.
We explain the mechanism leading to directed chaotic transport in Hamiltonian systems with spatial and temporal periodicity. We show that a mixed phase space comprising both regular and chaotic motion is required and we derive a classical sum rule which allows one to predict the chaotic transport velocity from properties of regular phase-space components. Transport in quantum Hamiltonian ratchets arises by the same mechanism as long as uncertainty allows one to resolve the classical phase-space structure. We derive a quantum sum rule analogous to the classical one, based on the relation between quantum transport and band structure. 相似文献
7.
Photoelectron angular distributions of H ionization in low energy regime:Comparison between different potentials
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We theoretically investigate the low energy part of the photoelectron spectra in the tunneling ionization regime by numerically solving the time-dependent Schrdinger equation for different atomic potentials at various wavelengths.We find that the shift of the first above-threshold ionization(ATI) peak is closely related to the interferences between electron wave packets,which are controlled by the laser field and largely independent of the potential.By gradually changing the short-range potential to the long-range Coulomb potential,we show that the long-range potential's effect is mainly to focus the electrons along the laser's polarization and to generate the spider structure by enhancing the rescattering process with the parent ion.In addition,we find that the intermediate transitions and the Rydberg states have important influences on the number and the shape of the lobes near the threshold. 相似文献
8.
S.?Borbély K.?T?kési L.?Nagy 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2010,59(3):337-348
The ionization of the water molecule by intense ultrashort half-cycle electric pulses is studied theoretically. The formation
of the electron wave packets in the continuum was investigated by calculating ionization probability densities using classical
and quantum mechanical models. Single active electron and frozen core calculations were performed within the hydrogenic approximation.
Electrons from the highest occupied molecular orbital 1b11b_1 were considered. We found good agreement between the classical and quantum mechanical calculation at high intensities, where
the over-the-barrier ionization mechanism is dominant. 相似文献
9.
We study the ionization of helium Rydberg atoms in an electric field above the classical ionization threshold within the semiclassical theory.By introducing a fractal approach to describe the chaotic dynamical behavior of the ionization,we identify the fractal self-similarity structure of the escape time versus the distribution of the initial launch angles of electrons,and find that the self-similarity region shifts toward larger initial launch angles with a decrease in the scaled energy.We connect the fractal structure of the escape time plot to the escape dynamics of ionized electrons.Of particular note is that the fractal dimensions are sensitively controlled by the scaled energy and magnetic field,and exhibit excellent agreement with the chaotic extent of the ionization systems for both helium and hydrogen Rydberg atoms.It is shown that,besides the electric and magnetic fields,core scattering is a primary factor in the fractal dynamics. 相似文献
10.
This paper presents theoretical computations of the ionization rate of Rydberg lithium atom above the classical ionization threshold using semiclassical approximation. The yielded random pulse trains of the escape electrons are recorded as a function of emission time such that they can be related to the terms of the recurrence periods of the photoabsorption. This fact illustrates that it is ionic core scattering processes which give rise to chaos in autoionization dynamics and this is verified by comparison of our results with the hydrogen atom situation. In order to reveal the chaotic properties in detail, the sensitive dependence of the ionization rate upon the scaled energy is discussed for different scaled energies. This approach provides a simple explanation for the chaotic character in autoionization decay of Rydberg alkali-metal atoms. 相似文献
11.
Zhao W Mestayer JJ Lancaster JC Dunning FB Reinhold CO Yoshida S Burgdörfer J 《Physical review letters》2006,97(25):253003
The ability to localize and to steer Rydberg wave packets in phase space using tailored sequences of half-cycle pulses is demonstrated. Classical phase-space portraits are used to explain the method and to illustrate the level of control that can be achieved. This is confirmed experimentally by positioning a phase-space-localized wave packet at the center of a stable island or navigating it around its periphery. This work provides a valuable starting point for further engineering of electronic wave functions. 相似文献
12.
13.
Dehua Wang Kaiyun Huang Shenglu Lin 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2009,54(3):699-706
The ionization of Rydberg hydrogen atoms near a metal surface at different scaled energies above the classical saddle point
energy has been discussed by using the semiclassical method. The results show that the atoms ionize by emitting a train of
electron pulses. In order to reveal the chaotic and escape dynamical properties of this system in detail, the sensitive dependence
of the ionization rate upon the scaled energy is discussed. As the scaled energy is close to the saddle point energy, the
ionization process of the hydrogen atom is nearly the same as the case of hydrogen atom in an electric field. There is only
a single pulse of electrons, with an exponentially decaying tail. With the increase of the scaled energy, the ionization rates
are similar to the case of the hydrogen atom in parallel electric and magnetic field, a series of electron pulses appear in
the ionization process. This is caused by classical chaos, which occurs for the metal surface. Our studies also suggest that
the metal surface can play the role of both the electric and the magnetic fields. Our theoretical analysis will be useful
for guiding experimental studies of the ionization of atoms near the metal surface. 相似文献
14.
T. Prosen D. L. Shepelyansky 《The European Physical Journal B - Condensed Matter and Complex Systems》2005,46(4):515-518
We establish analogy between a microwave ionization of Rydberg
atoms and a charge transport through a chaotic quantum dot
induced by a monochromatic field in a regime with a potential
barrier between dot contacts.
We show that the quantum coherence leads to dynamical localization
of electron excitation in energy
so that only a finite number of photons is absorbed inside the dot.
The theory developed determines the dependence of localization length
on dot and microwave parameters showing that the microwave power
can switch the dot between metallic and insulating regimes.
ultiphoton ionization and excitation to highly excited states
(e.g., Rydberg states) 相似文献
15.
We have studied the ionization of Rydberg hydrogen atom near a metal surface with a semiclassical analysis of photoionization microscopy. Interference patterns of the electron radial distribution are calculated at different scaled energies above the classical saddle point and at various atom-surface distances. We find that different types of trajectories contribute predominantly to different manifolds in a certain interference pattern. As the scaled energy increases, the structure of the interference pattern evolves smoothly and more types of trajectories emerge. As the atom approaches the metal surface closer, there are more types of trajectories contributing to the interference pattern as well. When the Rydberg atom comes very close to the metal surface or the scaled energy approaches the zero field ionization energy, the potential induced by the metal surface will make atomic system chaotic. The results also show that atoms near a metal surface exhibit similar properties like the atoms in the parallel electric and magnetic fields. 相似文献
16.
We have observed multiphoton ionization of the 5s core electron from a 5snd radial Rydberg wave packet of Sr atoms using a short optical pulse. When the outer nd electron is at its outer turning point the inner 5s electron is removed from the atom, and the outer electron is left in a Sr+ Rydberg state, but when the outer electron is at the inner turning point this does not occur. Analysis of the final Sr+ Rydberg states shows that the two electrons interact as the inner electron leaves, so that the outer electron is not simply projected onto the Sr+ Rydberg states. 相似文献
17.
Johnsson P López-Martens R Kazamias S Mauritsson J Valentin C Remetter T Varjú K Gaarde MB Mairesse Y Wabnitz H Salières P Balcou P Schafer KJ L'Huillier A 《Physical review letters》2005,95(1):013001
We use a train of sub-200 attosecond extreme ultraviolet (XUV) pulses with energies just above the ionization threshold in argon to create a train of temporally localized electron wave packets. We study the energy transfer from a strong infrared (IR) laser field to the ionized electrons as a function of the delay between the XUV and IR fields. When the wave packets are born at the zero crossings of the IR field, a significant amount of energy (approximately 20 eV) is transferred from the field to the electrons. This results in dramatically enhanced above-threshold ionization in conditions where the IR field alone does not induce any significant ionization. Because both the energy and duration of the wave packets can be varied independently of the IR laser, they are valuable tools for studying and controlling strong-field processes. 相似文献
18.
A. Buchleitner K. Sacha D. Delande J. Zakrzewski 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》1999,5(2):145-157
We present a semiclassical analysis of the dynamics of Rydberg states of atomic hydrogen driven by a resonant microwave field
of linear polarization. The semiclassical quasienergies of the atom in the field are found to be in very good agreement with
the exact quantum solutions. The ionization rates of individual eigenstates of the atom dressed by the field reflect their
quasiclassical dynamics along classical periodic orbits in the near integrable regime, but exhibit a transition to nonspecific
rates when global chaos takes over in phase space. We concentrate both on the principal resonance where the unperturbed Kepler
frequency is equal to the driving field frequency and on the higher primary resonance The latter case allows for the construction of nondispersive wave packets which propagate along Kepler ellipses of intermediate
eccentricity.
Received: 23 June 1998 / Accepted: 10 November
1998 相似文献
19.
E. A. Shapiro 《Journal of Experimental and Theoretical Physics》2000,91(3):449-457
A graphic method for describing the localization of quantum wave packets in several dimensions is proposed. The method employs classical action-angle coordinates. Different kind of wave packets arising in the two-and three-dimensional Coulomb problems are described from a unified point of view. Specifically, a more precise interpretation of the structure of “angular” Rydberg wave packets is given. Certain additional features of the proposed approach are discussed. 相似文献
20.
We analyze the semiclassical evolution of Gaussian wave packets in chaotic systems. We show that after some short time a Gaussian wave packet becomes a primitive WKB state. From then on, the state can be propagated using the standard time-dependent WKB scheme. Complex trajectories are not necessary to account for the long-time propagation. The Wigner function of the evolving state develops the structure of a classical filament plus quantum oscillations, with phase and amplitude being determined by geometric properties of a classical manifold. 相似文献