Project of the ultracold and cold neutron source at the WWR-M reactor with superfluid helium as a moderator

The WWR-M reactor of the Petersburg Nuclear Physics Institute provides a unique opportunity for creating conditions of low radiative heat release (～4 × 10^?3 W/g) at a sufficiently high neutron flux (～3 × 10¹² neutrons/(cm² s)). This opportunity can be implemented in the reactor thermal column, which represents a 1-m-diameter channel adjacent to the reactor core. This diameter of the channel allows the arrangement of the core gamma shielding made of bismuth (15 cm thick), a graphite premoderator (300 dm³) at a temperature of 20 K, and a converter with superfluid helium (35 dm³) at a temperature of 1.2 K. Calculations show that the heat release in the source (20 W) can be removed by pumping helium vapor, and the density of ultracold neutrons in an experimental trap will be ～10⁴ neutrons/cm³, which is higher than that of existing sources of ultracold neutrons by two to three orders of magnitude.     

Program of Fundamental-Interaction Research for the Ultracold-Neutron Source at the the WWR-M Reactor

The use of ultracold neutrons opens unique possibilities for studying fundamental interactions in particles physics. Searches for the neutron electric dipole moment are aimed at testing models of CP violation. A precise measurement of the neutron lifetime is of paramount importance for cosmology and astrophysics. Considerable advances in these realms can be made with the aid of a new ultracold-neutron (UCN) supersource presently under construction at Petersburg Nuclear Physics Institute. With this source, it would be possible to obtain an UCN density approximately 100 times as high as that at currently the best UCN source at the high-flux reactor of the Institute Laue–Langevin (ILL, Grenoble, France). To date, the design and basic elements of the source have been prepared, tests of a full-scale source model have been performed, and the research program has been developed. It is planned to improve accuracy in measuring the neutron electric dipole moment by one order of magnitude to a level of 10^?27 to 10^?28e cm. This is of crucial importance for particle physics. The accuracy in measuring the neutron lifetime can also be improved by one order of magnitude. Finally, experiments that would seek neutron–antineutron oscillations by employing ultracold neutrons will become possible upon reaching an UCN density of 10³ to 10⁴ cm^?3. The current status of the source and the proposed research program are discussed.     

散裂中子源耦合慢化器的中子学研究

利用蒙特－卡罗方法研究了散裂中子源中耦合慢化器的中子学特性。给出了冷中子与热中子慢化器的中子能谱。甲烷慢化器提供了性能非常好的冷中子，在低功率的散裂中子源中得到了应用。计算了慢中子引出的角分布。由于较低的氢密度，液态氢的漫化能力低于水与液态甲烷，但是可以通过增加预慢化器来弥补这一问题。2cm厚的水预慢化器层可以大约减少热量在低温慢化器中的热量沉积33％而不破坏中子特性。     

Inelastic p-He scattering at 141 MeV

Inelastic p-⁴He scattering at 141±2 MeV has been investigated with a high-pressure cloud chamber filled with helium. Results are presented for the total cross sections of each reaction channel and the neutron spectra for the p(⁴He, pn)³He reaction.     

PNPI differential EDM spectrometer and latest results of measurements of the neutron electric dipole moment

In this work, the double chamber magnetic resonance spectrometer of the Petersburg Nuclear Physics Institute (PNPI) designed to measure the neutron electric dipole moment (EDM) is briefly described. A method for long storage of polarized ultracold neutrons in a resonance space with a superposed electric field collinear to the leading magnetic field is used. The results of the measurements carried out on the ILL reactor (Grenoble, France) are interpreted as the upper limit of the value of neutron EDM |d_n| < 5.5 × 10^–26 e cm at the 90% confidence level.     

The energy release and temperature field in the ultracold neutron source of the WWR-M reactor at the Petersburg Nuclear Physics Institute

Results of calculations of energy releases and temperature fields in the ultracold neutron source under design at the WWR-M reactor are presented. It is shown that, with the reactor power of 18 MW, the power of energy release in the 40-L volume of the source with superfluid helium will amount to 28.5 W, while 356 W will be released in a liquid-deuterium premoderator. The lead shield between the reactor core and the source reduces the radiative heat release by an order of magnitude. A thermal power of 22 kW is released in it, which is removed by passage of water. The distribution of temperatures in all components of the vacuum structure is presented, and the temperature does not exceed 100°C at full reactor power. The calculations performed make it possible to go to design of the source.     

Spallation ultracold neutron source of superfluid helium below 1 K

For the production of high-density ultracold neutrons (UCNs), we placed 0.8 K superfluid helium in a cold neutron moderator. We resolved previous heat-load problems in the spallation neutron source that were particularly serious below 1 K. With a proton-beam power of 400 MeV×1 μA, a UCN production rate of 4 UCN cm(-3) s(-1) at the maximum UCN energy of E(c)=210 neV and a storage lifetime of 81 s were obtained. A cryogenic test showed that the production rate can be increased by a factor of 10 with the same storage lifetime by increasing the proton-beam power as well as (3)He pumping speed.     

Measurement of the quasi-isentropic compressibility of a helium plasma at a pressure of about 5000 GPa

The quasi-isentropic compressibility of a helium plasma has been measured using a spherical experimental chamber, as well as an X-ray diffraction complex consisting of three betatrons and a multichannel optoelectronic system for the detection of X-ray images. The density of the compressed helium plasma of about 8 g/cm³ has been obtained in the experiment at a pressure of 5000 GPa. Analysis of the data indicates that helium at the measured parameters is in a single ionized state.     

New gravitational experiment with ultracold neutrons

The results of a new neutron gravitation experiment are reported. The change in the energy of a neutron falling to a known height in the Earth’s gravitational field is compensated by an energy quantum ?Θ transferred to the neutron as a result of the phase modulation of the neutron wave. A phase diffraction grating moving across the direction of the propagation of the neutron wave is used as a modulator. The experiment has been carried out with ultracold neutrons Interference filters, neutron analogues of Fabry-Perot interferometers, are used for the spectrometry of ultracold neutrons. The force m _g g _n acting on the neutron in the Earth’s gravitational field has been measured with an accuracy of about 0.2%.     

Putting in operation a full-scale ultracold-neutron source model with superfluid helium

A project of the source of ultracold neutrons for the WWR-M reactor based on superfluid helium for ultracold-neutron production has been developed. The full-scale source model, including all required cryogenic and vacuum equipment, the cryostat, and the ultracold-neutron source model has been created. The superfluid helium temperature T = 1.08 K without a heat load and T = 1.371 K with a heat load on the simulator of P = 60 W has been achieved in experiments at a technological complex of the ultracold-neutron source. The result proves the feasibility of implementing the ultracold-neutron source at the WWR-M reactor and the possibility of applying superfluid helium in nuclear engineering.

     

Neutron diffraction study of polycrystalline 4He in a porous medium

The elastic (diffraction) component of the neutron scattering cross section, which carries information on the atomic structure of solid helium confined in silica aerogel, has been studied. Analysis of the crystalline structure of solid helium in a porous medium, which is determined from the existing neutron diffraction data, indicates that the superfluid phase is localized inside a hexagonal close-packed phase and is not present in a body-centered cubic crystal. It has also been revealed that the addition of the ³He isotope changes the structure of solid helium and hardly affects the formation of a superfluid phase.     

Neutron storage in a magnetic field

The motion of neutrons in magnetic traps is considered for various cases of neutron polarization. The results of implementing such traps in practice and special features of experiments studying magnetic neutron storage are discussed. The problem of neutron losses during injection via magnetic valves can be solved by conjoining a magnetic trap with a converter of cold neutrons into ultracold ones or with a source of ultracold neutrons. Prospects for expanding neutron-storage experiments by invoking a correlation analysis of neutron decay and by using the transport properties of charged particles in a nonuniform magnetic field are analyzed. In such an investigation, the recording of the storage time of neutrons proper can be supplemented with the detection of decay protons and electrons and with a parallel measurement of the asymmetries of proton and electron emission with respect to the magnetic field. A set of relative measurements permits improving the accuracy of an experimental determination of the neutron lifetime and combining this determination with the determination of correlation coefficients. On this basis, it is possible to find directly the ratio of the weak-interaction constants and the constants themselves. The application of the most advanced reactor and accelerator technologies to subcritical electric nuclear devices optimized for generating cold and ultracold neutrons, along with the use of solid deuterium and superfluid helium, creates preconditions for developing a neutron plant and for launching neutron studies at accelerators. Thus, the work that has been done as a development of V.V. Vladimirsky's proposals on magnetic neutron storage is analyzed, and the potential of a further use of ultracold neutrons and magnetic devices for deploying a full-scale precision experiment to study the beta decay of polarized neutrons is demonstrated.     

An apparatus of the NBC type and the physics results obtained

A nonbubble chamber (NBC) setup, especially designed to perform a series of experiments, is described. The setup consists of a neutron missing-mass spectrometer coupled with a system of large electromagnetic shower detectors. In spite of its large dimensions (the sensitive surface and volume are 2.16 × 10⁴ cm² and 7.8 × 10⁵ cm³, respectively), the neutron spectrometer has a time resolution of ±0.70 nsec FWHM, with ∼25% detection efficiency in the range (70–390 MeV) neutron kinetic energy. The time equalization between the various components of the neutron spectrometer has been established to within ±0.1 nsec. At present this is the most powerful and the most accurate high-energy neutron detector. The electromagnetic shower detector is based on the principle of simultaneous measurements of the spatial development of the electromagnetic cascade and of its energy release. This is obtained with nine elements of lead foil — spark chamber — plastic scintillator, all sandwiched together. The sensitive surface and volume of the electromagnetic shower detector are 1.45 × 10⁴ cm² and 7.2 × 10⁵ cm³, respectively.     

Ultracold neutron detector for the spectrometer of a neutron lifetime measuring

The gas-discharge detector is designed for the neutron lifetime spectrometer. The detector is intended for ultracold neutron flux monitoring in measurement cycles at the specrtometer (ILL, Grenoble, France). The detector has been successively tested with a Pu–Be neutron source under laboratory conditions and as a part of the spectrometer.     

Aus der Praxis Bestimmung der relativen Deuteriumhäufigkeit im Wasser mittels Dichtemessung

The track autoradiography according to the reaction ³He(n, p)³H has been used in both optical and electron microscopic investigations for the direct local nondestructive and quantitative analysis of the implanted He distribution in the material. The technique of the track autoradiogram replica production on a CN-85 detector is described for the tracks ca. 0.1 μm long. The autoradiograms of helium distribution are compared with the metallographic data on the welds of several steel grades. The track autoradiography has been applied to the determination of the helium evolution rate from the samples heated to 1200 K.     

Prospects for precision measurements of atomic helium using direct frequency comb spectroscopy

We analyze several possibilities for precisely measuring electronic transitions in atomic helium by the direct use of phase-stabilized femtosecond frequency combs. Because the comb is self-calibrating and can be shifted into the ultraviolet spectral region via harmonic generation, it offers the prospect of greatly improved accuracy for UV and far-UV transitions. To take advantage of this accuracy an ultracold helium sample is needed. For measurements of the triplet spectrum a magneto-optical trap (MOT) can be used to cool and trap metastable 2³S state atoms. We analyze schemes for measuring the two-photon 2³S →4³S interval, and for resonant two-photon excitation to high Rydberg states, 2³S →3³P →n³S, D. We also analyze experiments on the singlet-state spectrum. To accomplish this we propose schemes for producing and trapping ultracold helium in the 1¹S or 2¹S state via intercombination transitions. A particularly intriguing scenario is the possibility of measuring the 1¹S →2¹S transition with extremely high accuracy by use of two-photon excitation in a magic wavelength trap that operates identically for both states. We predict a “triple magic wavelength” at 412 nm that could facilitate numerous experiments on trapped helium atoms, because here the polarizabilities of the 1¹S, 2¹S and 2³S states are all similar, small, and positive.     

Effect of simultaneous helium implantation on the microstructure evolution of Inconel X-750 superalloy during dual-beam irradiation

This study focuses on investigation into the effect of helium implantation on microstructure evolution in Inconel X-750 superalloy during dual-beam (Ni⁺/He⁺) irradiation. The 1 MeV Ni⁺ ions with the damage rate of 10^?3 dpa/s as well as 15 keV He⁺ ions using rate of 200 appm/dpa were simultaneously employed to irradiate specimens at 400 °C to different doses. Microstructure characterization has been conducted using high-resolution analytical transmission electron microscopy (TEM). The TEM results show that simultaneous helium injection has significant influence on irradiation-induced microstructural changes. The disordering of γ′ (Ni₃ (Al, Ti)) precipitates shows noticeable delay in dose level compared to mono heavy ion irradiation, which is attributed to the effect of helium on promoting the dynamic reordering process. In contrast to previous studies on single-beam ion irradiation, in which no cavities were reported even at high doses, very small (2–5 nm) cavities were detected after irradiation to 5 dpa, which proved that helium plays crucial role in cavity formation. TEM characterization also indicates that the helium implantation affects the development of dislocation loops during irradiation. Large 1/3 〈1?1?1〉 Frank loops in the size of 10–20 nm developed during irradiation at 400 °C, whereas similar big loops detected at higher irradiation temperature (500 °C) during sole ion irradiation. This implies that the effect of helium on trapping the vacancies can help to develop the interstitial Frank loops at lower irradiation temperatures.     

Spectroscopic and chemical reactivity analysis of D-Myo-Inositol using quantum chemical approach and its experimental verification

Glow discharge conditioning (GDC) has long been accepted as one of the basic wall conditioning techniques for achieving ultrahigh vacuum in an unbaked chamber. As a part of this fundamental experimental study, a test chamber has been fabricated from stainless steel 304 L with its inner surface electropolished on which a detailed investigation has been carried out. Both helium and hydrogen gases have been employed as discharge cleaning medium. The discharge cleaning was carried out at 0.1 A /m ² current density with working pressure maintained at 1.0 × 10 ^-2 mbar. It was experimentally observed that the pump-down time to attain the base pressure ~10 ^-8 mbar was reduced by 62% compared to the unbaked chamber being pumped to this ultimate vacuum. The results were similar irrespective of whether the discharge cleaning medium is either hydrogen or helium. It was also experimentally established that a better ultimate vacuum could be achieved as compared to theoretically calculated ultimate vacuum with the help of discharge cleaning.     

Cold cesium molecules produced directly in a magneto-optical trap

We report on the observation of ultracold ground electric-state cesium molecules produced directly in a magneto- optical trap with a good signal-to-noise ratio. These molecules arise from the photoassociation of magneto-optical trap lasers and they are detected by resonantly enhanced multiphoton ionization technology. The production rate of ultracold cesium molecules is up to 4×10⁴ s^-1. We measure the characteristic time of the ground electric-state cesium molecules generated in the experiment and investigate the Cs₂⁺ molecular ion intensity as a function of the trapping laser intensity and the ionization pulse laser energy. We conclude that the production of cold cesium molecules may be enhanced by using appropriate experimental parameters, which is useful for future experiments involving the production and trapping of ultracold ground electric-state molecules.     

New measurements of the neutron electric dipole moment

We report a new measurement of the neutron electric dipole moment with the PNPI EDM spectrometer using the ultracold neutron source PF2 at the research reactor of the ILL. Its first results can be interpreted as a limit on the neutron electric dipole moment of |d _n | < 5.5 × 10^?26 e cm (90% confidence level).