Generation of soliton-like wave packets and wave packets with linear phase modulation in gaining optical wave-guides with saturable nonlinearity

We have considered the dynamics of soliton-like pulses and stable frequency-modulated self-similar pulses in an active medium with saturable nonlinearity and a parabolic refractive-index profile. We show that, based on gaining gradient fibers with a parabolic distribution of the refractive index and saturable nonlinearity, it is possible to create complexes that ensure generation of laser pulses with a high (above 1 TW) peak power.     

Navigating localized wave packets in phase space

The ability to localize and to steer Rydberg wave packets in phase space using tailored sequences of half-cycle pulses is demonstrated. Classical phase-space portraits are used to explain the method and to illustrate the level of control that can be achieved. This is confirmed experimentally by positioning a phase-space-localized wave packet at the center of a stable island or navigating it around its periphery. This work provides a valuable starting point for further engineering of electronic wave functions.     

Recovery time in quantum dynamics of wave packets

A wave packet formed by a linear superposition of bound states with an arbitrary energy spectrum returns arbitrarily close to the initial state after a quite long time. A method in which quantum recovery times are calculated exactly is developed. In particular, an exact analytic expression is derived for the recovery time in the limiting case of a two-level system. In the general case, the reciprocal recovery time is proportional to the Gauss distribution that depends on two parameters (mean value and variance of the return probability). The dependence of the recovery time on the mean excitation level of the system is established. The recovery time is the longest for the maximal excitation level.     

Amplitude and phase reconstruction of electron wave packets for probing ultrafast photoionization dynamics

Ultrafast atomic processes, such as excitation and ionization occurring on the femtosecond or shorter time scale, were explored by employing attosecond high-harmonic pulses. With the absorption of a suitable high-harmonic photon a He atom was ionized, or resonantly excited with further ionization by absorbing a number of infrared photons. The electron wave packets liberated by the two processes generated an interference containing the information on ultrafast atomic dynamics. The attosecond electron wave packet, including the phase, from the ground state was reconstructed first and, subsequently, that from the 1s3p state was retrieved by applying the holographic technique to the photoelectron spectra comprising the interference between the two ionization paths. The reconstructed electron wave packet revealed details of the ultrafast photoionization dynamics, such as the instantaneous two-photon ionization rate.     

Formation of ground-state vibrational wave packets in intense ultrashort laser pulses

The formation of coherent vibrational wave packets in the electronic ground state of neutral molecules in intense ultrashort laser pulses and their subsequent detection by means of recently developed pump-probe experiments are discussed. The wave packet formation is due to the pronounced dependence of the strong-field ionization rate on the internuclear distance. This leads to a deformation of the initial wave function due to an internuclear-distance dependent depletion. The phenomenon is demonstrated with a time-dependent wave packet study for molecular hydrogen.     

Nonlinear space-time dynamics of ultrashort wave packets in water

We have monitored the space-time transformation of a 150-fs pulse undergoing self-focusing and filamentation in water, by means of the nonlinear gating technique. We have observed that pulse splitting and subsequent recombination apply to axial temporal intensity only, whereas the space-integrated pulse profile preserves its original shape.     

Controlling high harmonic generation with molecular wave packets

We show that, by controlling the alignment of molecules, we can influence the high harmonic generation process. We observed strong intensity modulation and spectral shaping of high harmonics produced with a rotational wave packet in a low-density gas of N2 or O2. In N2, where the highest occupied molecular orbital (HOMO) has sigma(g) symmetry, the maximum signal occurs when the molecules are aligned along the laser polarization while the minimum occurs when it is perpendicular. In O2, where the HOMO has pi(g) symmetry, the harmonics are enhanced when the molecules are aligned around 45 degrees to the laser polarization. The symmetry of the molecular orbital can be read by harmonics. Molecular wave packets offer a means of shaping attosecond pulses.     

Nondispersive wave packets as solitonic solutions of level dynamics

We discuss the analogy between nondispersive wave packets in periodically driven hydrogen atoms and solitons as solitary wave solutions of nonlinear dynamical systems. Whereas the wave packet eigenstates should not be considered as solitons propagating in real space, they are shown to display the essential features of solitonic solutions as they propagate through the irregular lattice of quasienergy levels evolving with a fictitious time like the strength or the frequency of the driving force.     

Optical control of the quantum-state distribution of vibrational wave packets using trains of phase-locked pulses

An intuitive scheme for controlling the quantum state composition of one-coordinate molecular wave packets is developed. The accumulated phase difference between the various components of the molecular wave packet is determined, and then a sequence of phase-locked optical pulses is employed to selectively enhance or depopulate specific vibrational states, or sets of vibrational states. The quantum state composition of the resulting wave packet, and the efficiency of the control scheme, is determined by calculating the multi-pulse response of the time-dependent vibrational state populations.     

Holography of wave packets

We describe the principles of holographic storage and reconstruction of ultrashort light pulses using spectrally nonselective media. This can be achieved by the application of a 3-D recording medium and by the holography of waves produced by spatial spectral decomposition of light pulses. We also describe various transformations of optical temporal signals based on holographic spectral filtering and nonlinear interaction of spectral decomposition waves.     

On the theory of wave packets

In this paper we discuss some aspects of the theory of wave packets. We consider a popular noncovariant Gaussian model used in various applications and show that it predicts too slow a longitudinal dispersion rate for relativistic particles. We revise this approach by considering a covariant model of Gaussian wave packets, and examine our results by inspecting a wave packet of arbitrary form. A general formula for the time dependence of the dispersion of a wave packet of arbitrary form is found. Finally, we give a transparent interpretation of the disappearance of the wave function over time due to the dispersion—a feature often considered undesirable, but which is unavoidable for wave packets. We find, starting from simple examples, proceeding with their generalizations and finally by considering the continuity equation, that the integral over time of both the flux and probability densities are asymptotically proportional to the factor 1/|x|² in the rest frame of the wave packet, just as in the case of an ensemble of classical particles.     

Conservation of molecular alignment for cyclic rotational wave packets in periodic pulse trains

The existence of states for which molecular alignment can be maintained for long periods of time is shown. These states, consisting of coherent superpositions of rotational states, are found among cyclic states of the generalized Floquet operator corresponding to a molecule in a short nonresonant laser pulse. For a single pulse alignment can be maintained, in some cases, for more than 40 times the pulse duration. Because of the special properties of these coherent states, arbitrarily long alignment can be achieved by using well-timed pulse trains.     

Cyclotron dynamics of electron wave packets in topological insulators in an external magnetic field

The evolution of electron wave packets formed from surface states in topological insulators located in an external magnetic field is studied. The electron and spin densities of the wave packets under consideration are calculated analytically and are visualized. The influence of the main characteristics of the wave packets (the spin polarization) on the splitting and the change in their forms with time is considered.     

Three-dimensional molecular wave packets: Calculation of revival times from periodic orbits

We present a theoretical analysis of revivals and fractional revivals of three-dimensional wave packets, which describe the coupled vibrational motion of phosphaethyne (HCP) in its ground electronic state. The wave packets studied are chosen to evolve along the periodic orbits, which quantize the states in the three fundamental progressions. The revival times T_rev are found to depend strongly on the particular mode excited and on the mean excitation energy. Based on a semiclassical analysis, T_rev is shown to be determined by the dependence of the period of the orbits on the classical action along them.     

Theory of cross phase modulation for the vibrational modes of trapped ions

We analyze nonlinear coupling between individual vibrational quanta for trapped ions. The nonlinear Coulomb interaction causes a Kerr-type Hamiltonian, for which we derive an analytical expression for the coupling constant χ. In contrast to a previously published formula [C.F. Roos, T. Monz, K. Kim, M. Riebe, H. Häffner, D.F.V. James, R. Blatt, Phys. Rev. A 77 (2008) 040302(R)], our result is in close agreement with experimental data.