Dipole blockade at Förster resonances in high resolution laser excitation of Rydberg states of cesium atoms

High resolution laser excitation of np Rydberg states of cesium atoms shows a dipole blockade at F?rster resonances corresponding to the resonant dipole-dipole energy transfer of the np+np --> ns+(n+1)s reaction. The dipole-dipole interaction can be tuned on and off by the Stark effect, and such a process, observed for relatively low n(25-41), is promising for quantum gate devices. Both Penning ionization and saturation in the laser excitation can limit the range of observation of the dipole blockade.     

磁性薄膜原子层数对极化方向的影响

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Energy Mechanism of Charges Analyzed in Real Current Environment

We analyze in this work the energy transfer process of accelerated charges, the mass fluctuations accompanying this process, and their inertial properties. Based on a previous work, we use here the dipole antenna, which is a very convenient framework for such analysis, for analyzing those characteristics. We show that the radiation process can be viewed by two energy transfer processes: one from the energy source to the charges and the second from the charges into the surrounding space. Those processes, not being in phase, result in mass fluctuations. The same principle is true during absorption. We show that in a transient period between absorption and radiation the dipole antenna gains mass according to the amount of absorbed energy and loses this mass as radiated energy. We rigorously prove that the gain of mass, resulting from electrical interaction has inertial properties in the sense of Newton's third low. We arrive to this result by modeling the reacting spacetime region by an electric dipole.     

Model for photosynthetic light harvesting system: Energy transfer in anthracene- and biphenyl-cholorophyll derivatives

An intramolecular energy transfer from the ultraviolet absorbing donor to the pyro-pheophorbide a moiety occurs with high efficiency in model antenna compounds composed of 4-phenylbenzoic acid or anthracenecarboxylic acid and pyropheophorbide a. The energy transfer mechanism involves a Förster tyoe dipole-dipole coupling between the donor transition dipole(s) and the acceptor transition dipole(s) represented by the Soret band of the pyropheophorbide a moiety.     

Oscillations of echo amplitude in glasses in a magnetic field induced by nuclear dipole-dipole interaction

The influence of a magnetic field on the dipole echo amplitude in glasses (at temperatures of about 10 mK) induced by the dipole-dipole interaction of nuclear spins has been theoretically studied. It has been shown that a change in the mutual position of nuclear spins at tunneling and the Zeeman energy E _H of their interaction with the external magnetic field lead to a nonmonotonic magnetic-field dependence of the dipole echo amplitude. The approximation that the nuclear dipole-dipole interaction energy E _d is much smaller than the Zeeman energy has been found to be valid in the experimentally important cases. It has been shown that the dipole echo amplitude in this approximation may be described by a simple universal analytic function independent of the microscopic structure of the two-level systems. An excellent agreement of the theory with the experimental data has been obtained without fitting parameters (except for the unknown echo amplitude).     

Ferromagnetic to antiferromagnetic transition of one-dimensional spinor Bose gases with spin-orbit coupling

The effect of the interatomic dipole-dipole interaction on the single-photon transmission spectrum is investigated theoretically in the single-mode optical waveguide containing a pair of dipole interaction two-level atoms and the incident photon, respectively. The results show that the interatomic dipole-dipole interaction can induce a remarkable change in the photon-atom on-resonance frequency in the single-photon transmission spectrum compared with the nonexistence of the interatomic dipole-dipole interaction. As a consequence, the original zero transmission probability at the original photon-atom resonant frequency increases to one directly thanks to the appropriately-chosen dipole-dipole interaction strength. Consequently, this characteristic reveals that the interatomic dipole-dipole interaction treated as an important internal physical mechanism can perform as a functional quantum switching to manipulate the photon’s transmission in the optical waveguide. The corresponding interpretations responsible for this phenomenon are presented.     

Effective field theory for spinor dipolar Bose Einstein condensates

We show that the effective theory of long wavelength low energy behavior of a dipolar Bose-Einstein condensate(BEC) with large dipole moments (treated as a classical spin) can be modeled using an extended non-linear sigma model (NLSM) like energy functional with an additional non-local term that represents long ranged anisotropic dipole-dipole interaction. Minimizing this effective energy functional we calculate the density and spin-profile of the dipolar Bose-Einstein condensate in the mean-field regime for various trapping geometries. The resulting configurations show strong intertwining between the spin and mass density of the condensate, transfer between spin and orbital angular momentum in the form of Einstein-de Hass effect, and novel topological properties. We have also described the theoretical framework in which the collective excitations around these mean field solutions can be studied and discuss some examples qualitatively.     

Effect of dipole forces on the structure of the liquid phases of DNA

The dipole-dipole contribution to the energy of the pair interaction between DNA molecules has been calculated and analyzed. Rigid fragments of DNA, i.e., of a length of about the persistent length, which have discrete dipole moments of base pairs, are considered. For a given distance between the centers of mass of molecules, the energy of the dipole-dipole interaction is a function of three angular variables; the angles ?₁ and ?₂ between the central dipoles of both molecules and the z axis passing through the centers of the molecules, as well as the angle ξ between long axes of the molecules, are taken as these variables. It is shown that the dipole energy has minima when the mutual orientation of the molecules satisfies one of the following conditions: (i) ?₁ = ?₂ = 0 or (ii) ?₁ = ?₂ = π. The cholesteric twist angle ξ can be both positive and negative in dependence on the type of the minimum. For realistic cholesteric dispersion parameters, the dipole energy is only slightly lower than the experimentally known binding energy of the molecules in dispersion. The results allow the assumption that the dipole forces significantly affect the structure and other properties of DNA suspensions; in particular, they can lead to nontrivial texture phenomena, biaxial correlation, and multistability.     

Elastic interaction of two atoms adsorbed on a solid surface

The long-range interaction of two adsorbed atoms mediated by the elastic distortion of the substrate is calculated classically for an elastically isotropic substrate. For identical atoms, the interaction is repulsive; for different atoms, it can be repulsive or attractive. It varies as ρ^?3 with the distance ρ between the two adsorbed atoms. This is the same spatial dependence as for the dipole - dipole interaction between two adsorbed atoms. For two xenon atoms adsorbed on gold, the elastic interaction is somewhat smaller than the dipole-dipole interaction. The interaction energy is inversely proportional to the shear modulus of the substrate, so that it may become quite large near a distortive phase transition.     

Re-evaluation of some lithium dipole properties and dipole-dipole and dipole-quadrupole van der Waals constants

Our previous one-centre pseudo-state results for some ground-state Li atom dipole oscillator strength sums, the dipole-dipole dispersion energy constants for the Li-Li, Li-H and Li-He ground-state interactions and the dipole-quadrupole dispersion energy constant for the Li-Li interaction are re-evaluated in the light of a more reliable selection for the resonance dipole oscillator strength of the Li atom. These and some of our previous lithium pseudo-state results are compared with corresponding literature values.     

Collective oscillations of the magnetic moments of a chain of spherical magnetic nanoparticles with uniaxial magnetic anisotropy

Magnetic particles moving freely in a fluid can organize dense phases (3D clusters or linear chains). We analyze the spectrum of magnetic oscillations of a chain of spherical magnetic particles taking into account the magnetic anisotropy of an individual particle for an arbitrary relation between the anisotropy energy and the energy of the dipole interaction of particles. For any relation between these energies, the spectrum contains three branches of collective oscillations: a high-frequency branch and a weakly split doublet of low-frequency branches. The frequency of the high-frequency branch is determined by a stronger interaction, while the frequencies of the low-frequency branches are determined by the weakest interaction. Accordingly, the dispersion is maximal for oscillations formed by the dipole-dipole interaction of particles, which have high frequencies in the case of a strong dipole interaction or low frequencies in the case of a strong anisotropy.     

Electronic states of dysprosium submonolayer films adsorbed on the W(100) surface

The unfilled electronic states of dysprosium submonolayer films absorbed on the W(100) surface are investigated using angle-resolved inverse photoelectron spectroscopy. It is shown that the energy position of the peak at 1.7 eV is independent of the angle of incidence of electrons onto the crystal surface. This specific feature is associated with electron transitions to the Dy 4f state located above the Fermi level. A correlation between the change in the energy position of this peak and the change in the work function with an increase in the absorbed dysprosium coverage suggests that the dipole moment of adatoms is affected by the dipole-dipole interaction.     

Cherenkov terahertz radiation from Dirac semimetals surface plasmon polaritons excited by an electron beam

We demonstrate a physical mechanism for terahertz(THz) generation from surface plasmon polaritons(SPPs). In a structure with a bulk Dirac semimetals(BDSs) film deposited on a dielectric substrate, the energy of the asymmetric SPP mode can be significantly enhanced to cross the light line of the substrate due to the SPP-coupling between the interfaces of the film. Therefore, the SPPs can be immediately transformed into Cherenkov radiation without removing the wavevector mismatch. Additionally, the symmetric SPP mode can also be dramatically lifted to cross the substrate light line when a buffer layer with low permittivity relative to the substrate is introduced. In this case, dual-frequency THz radiation from the two SPP modes can be generated simultaneously. The radiation intensity is significantly enhanced by over two orders due to the field enhancement of the SPPs. The radiation frequency can be tuned in the THz frequency regime by adjusting the beam energy and the chemical potential of the BDSs. Our results could find potential applications in developing room temperature, tunable, coherent, and intense THz radiation sources to cover the entire THz band.     

金属光栅对表面等离子体波的辐射抑制研究

对金属光栅进行严格耦合波理论计算, 得到了780和1500 nm波长入射光条件下不同光栅调制深度(20-80 nm)对应的反射谱. 根据Fano理论推导了描述反射谱线的经验公式, 最后应用有限元法计算光栅表面近场电场分布, 验证了公式的正确性. 反射谱线公式反映出光栅耦合表面等离子体的各个物理效应, 其中最重要的是反映出光栅在某一调制深度下对表面等离子体反耦合的抑制作用, 这一发现为设计光栅能量约束器件提供了物理依据.     

Resonance intermolecular energy transfer near semiconductor nanoparticles

The problem of the resonance dipole-dipole interaction between two molecules near a spherical semiconductor nanoparticle is considered. It is shown that the presence of the nanoparticle results in the additional interaction between the molecules, which, under certain conditions, can significantly exceed the direct dipole-dipole interaction. This occurs in the case when the ground-state energy of an exciton is in a close resonance with the energies of molecular transitions. The effect of the additional interaction on the probability of intermolecular resonance energy transfer is especially important at large distances between molecules. The matrix elements of the interaction are estimated for nanoparticles of semiconductor materials CuCl and GaAs.     

Stark shift contribution to field statistics in a generalized Jaynes-Cummings model

The nonlinear and multiphoton interaction between a single two-level atom and two modes of radiation is studied in a generalized Jaynes-Cummings model. An intensity-dependent level shift is considered. The time evolution operator is obtained. The detuning has a photon number dependence. Different statistical aspects pertaining to either the atom or the fields are calculated. The dipole moment, the dipole-dipole correlation function, as well as the transient spectrum are obtained.     

The interaction of transverse domain walls

The interaction between transverse domain walls is calculated analytically using a multipole expansion up to third order. Starting from an analytical expression for the magnetization in the wall, the monopole, dipole, and quadrupole moments are derived and their impact on the interaction is investigated using the surface and volume charges. The surface charges are important for the dipole moment while the volume charges constitute the monopole and quadrupole moments. For domain walls that are situated in different wires it is found that there is a strong deviation from the interaction of two monopoles. This deviation is caused by the interaction of the monopole of the wall in the first wire with the dipole of the wall in the second wire and vice versa. The dipole-dipole and the quadrupole-monopole interactions are found to be also of considerable size and non-negligible. A comparison with micromagnetic simulations shows a good agreement.     

Physical model and the associative memory of a cytoskeleton microtubule as a system of dipoles

A physical model of the conformational degrees of freedom of a cytoskeleton microtubule represented as a system of interacting dipoles is elaborated, characteristic physical quantities are estimated, and a phase diagram of the ferroelectric state of the microtubule at T = 0 is constructed. The presence of frustrated couplings J _ij between the dipoles appears to be the most important feature of the disordered dipole system of the microtubule, owing to which the ground state of the dipole system splits into a large number of lower energy states. The dynamics of the dipole system is determined by the relaxation of the dipole-dipole interaction energy. After the dipole system has evolved to its final state, the input image is associated with one of reference images stored earlier; hence, the dipole system of a microtubule can be viewed as a distributed system with associative memory.     

有机分子多层LB膜中聚集体理论和实验研究H

文中采用经典偶极相互作用模型讨论了多层Z型LB膜中分子聚集体的类型 ,给出了分子偶极相互作用能的表达式;并对理论结果与紫外可见吸收光谱的实验值进行了比较,理论结果和实验值符合较好.     

Damping of the giant dipole resonance in hot,strongly rotating nuclei

The isovector dipole density-density response of hot rotating nuclei is calculated applying a cranked deformed Nilsson potential together with a separable dipole-dipole residual interaction. The transformation of the response function from the internal rotating coordinate frame to the laboratory frame is discussed and illustrated by classical results for a charged particle moving in a harmonic-oscillator potential. Calculations for ¹⁰⁸Sn, ¹⁵²Dy and ¹⁹⁶Pb are presented. For ¹⁰⁸Sn at high excitation energy thermal fluctuations of the shape gives rise to a rather structureless strength function with a considerable width. For ¹⁵²Dy and ¹⁹⁶Pb superdeformed minima of the potential surface are predicted. The coupling of the giant dipole resonance to the shape degrees of freedom of superdeformed nuclei can split the vibration by ≈ 10 MeV, the lowest peak being expected at an excitation energy of ≈ 7–8 MeV and carrying ≈ 30% of the energy-weighted sum rule.