Broadly tunable femtosecond Cr:LiSAF laser

We demonstrate wavelength tunability of femtosecond pulses over a range of more than 50 nm from a diode-pumped Cr:LiSAF laser. The mode-locking mechanism can be explained by soliton mode locking that is started and stabilized by a broadband semiconductor saturable-absorber mirror designed for low loss over the full reflection bandwidth of the underlying Bragg mirrors, which ultimately limits tunability. We obtain 45-fs pulses at 105-mW average output power and a maximum mode-locked average output power of 125 mW with 60-fs pulses.     

Efficient generation of narrow-bandwidth picosecond pulses by frequency doubling of femtosecond chirped pulses

We demonstrate efficient generation of picosecond narrow-bandwidth pulses by frequency mixing of broadband opposite chirped pulses in a type I doubling crystal. This procedure allows us to produce picosecond pulses that are perfectly synchronized with femtosecond pulses. The experiment shows a decrease of the initial bandwidth by a factor of more than 30, while a high conversion efficiency is maintained.     

Long-term optical phase locking between femtosecond Ti:sapphire and Cr:forsterite lasers

Long-term optical phase-coherent two-color femtosecond pulses were generated by use of passively timing-synchronized Ti:sapphire and Cr:forsterite lasers. The relative carrier-envelope phase relation was fixed by an active feedback loop. The accumulated phase noise from 10 mHz to 1 MHz of the locked beat note was 0.43 rad, showing tight phase locking. The optical frequency fluctuation between two femtosecond combs was submillihertz, with a 1 s averaged counter measurement over 3400 s, leading to a long-term femtosecond frequency-comb connection.     

Implementation of the direct locking method for long-term carrier-envelope-phase stabilization of a grating-based kHz femtosecond laser

We have stabilized the carrier-envelope phase (CEP) of amplified femtosecond laser pulses from a grating-based chirped-pulse amplification femtosecond laser by the direct locking method. Long-term CEP stabilization in the oscillator was achieved by employing a double-feedback loop to control both the pumping power and the cavity dispersion. Large CEP drift, induced during amplification, was compensated by adjusting the grating separation in the pulse compressor, and the CEP stabilization was maintained for four hours with a phase jitter of about 180 mrad. After pulse compression to 5.5-fs pulses in a filamentation pulse compressor, CEP-stabilized laser pulses were applied for high-harmonic generation to confirm the CEP stabilization.     

与794nm飞秒激光精确同步的无直流背底的1064nm脉冲光的产生

基于非共线光参量放大(NOPA)，以宽带794nm飞秒激光的倍频光为抽运光，以连续的He-Ne激光为信号光，产生了与宽带794nm飞秒激光精确同步的无直流背底的1064nm的脉冲光.实验结果显示该1064nm的光脉冲可作为光参量啁啾脉冲放大系统的抽运激光链的种子光，从而实现用全光学方法实现OPCPA系统抽运光和信号光的精确同步.还将非共线光参量放大器置于经特殊设计的He-Ne激光腔内，也同样成功得到了无直流背底的1064nm的光脉冲.经一次光参量放大后所得到的1064nm光的光谱和空间啁啾特性与非共线光参量放大器置于He-Ne激光腔外时得到的1064nm的光脉冲相同，而其单脉冲能量约为腔外NOPA的10倍. 关键词： 非线性光参量放大 光参量啁啾脉冲放大 时间同步     

Spectral filtering of femtosecond laser pulses by interference filters

Phase properties of optical thin film interference filters are discussed from the aspect of their usage for phase-error free wavelength separation of broadband femtosecond laser pulses. It is shown that both transmissive or reflective interference filters with high contrast ratios exhibit high cubic phase shifts on transmission or reflection, respectively, causing intolerable distortion in the temporal pulse shape. We show, however, that high efficiency wavelength separation of broadband femtosecond laser pulses can be achieved by using low contrast, properly designed reflective optical interference filters directly built into the cavity of the broad spectrum, femtosecond pulse lasers or parametric oscillators. For demonstrative purposes, we implemented the idea for a Kerr-lens mode-locked Ti:sapphire laser, and obtained two-color, inherently synchronized, unchirped, femtosecond pulse outputs from a single laser oscillator.     

飞秒钛宝石放大激光脉冲的载波包络相位测量与控制

通过对重复频率为1 kHz的放大飞秒激光脉冲的光谱干涉实验,结合傅里叶变换进行了载波包络相位漂移的实验研究.在此基础上利用锁相环反馈控制技术实现了对载波包络相位的精密锁定,锁定后的激光脉冲稳态相位均方根误差小于80mrad,锁定时间超过3h.同时在理论上分析了光谱干涉测量放大激光脉冲载波包络相位的原理,给出了光谱干涉信号与载波包络相位的关系. 关键词： 飞秒钛宝石放大器 载波包络相位 光谱干涉 超连续     

Efficient and tunable diode-pumped femtosecond Yb:glass lasers

Diode-pumped Yb:phosphate and Yb:silicate glass lasers have been passively mode locked for the first time to the authors' knowledge. Reliable self-starting mode locking without critical cavity alignment has been achieved with intracavity semiconductor saturable-absorber mirrors and soliton mode locking. We generated pulses as short as 58 fs with the Yb:phosphate laser and 61 fs with the Yb:silicate laser at average output powers of 65 and 53 mW, respectively. The pulse repetition rate was 112 MHz. Additionally, we demonstrated tunability of femtosecond pulses from 1025 to 1065 nm for the Yb:phosphate and from 1030 to 1082 nm for the Yb:silicate glasses. The highest mode-locked output power was 405 mW, with 183-fs pulses from the phosphate glass. The diode pump power was 1.68 W, corresponding to 24% optical-to-optical efficiency. The highest cw output power was 510 mW at the same incident pump power.     

Wavelength-tunable multicolored femtosecond laser pulse generation in a fused silica glass plate

We obtained an array of multicolored femtosecond laser pulses with as many as 17 different colors that are spatially isolated. The mechanism of generation was proved to be cascaded four-wave mixing and with the following procedure. The output beam from a femtosecond laser was split into two. One of the two beams was pulse-compressed with a hollow core fiber and the intensity of the other was reduced. The two beams were synchronized and combined with a small crossing angle in a plate of fused silica glass plate. The wavelengths of the sidebands are continuously tunable from near-ultraviolet to near-infrared. The pulse duration, spatial mode, spectrum, and energy stability of the sidebands were studied. As many as fifteen spectral up-shifted pulses and two spectral downshifted pulses were obtained with spectral bandwidths broader than 1.8 octaves. Properties such as pulse energy as high as 1 μmJ, 45 fs pulse duration, smaller than 1.1 times of the diffraction limit Gaussian spatial profile, and better than 2% RMS power stability of the generated sidebands make it can be used in various experiments. The characterization showed that the sidebands have sufficiently good qualities to enable application to for various multicolor femtosecond laser experiments, for example, a multicolor pump-probe experiment.     

采用飞秒光纤激光同步泵浦的自启动锁模钛宝石激光研究

针对常规连续激光泵浦钛宝石激光振荡器不能自启动锁模的缺点,采用倍频飞秒光纤激光同步泵浦,通过调节振荡器腔长与泵浦腔长匹配,实现了飞秒钛宝石激光的自启动锁模。实验中采用3.4 W的倍频掺镱光纤激光同步泵浦钛宝石激光振荡器,获得了平均功率大于130 mW、重复频率75 MHz、光谱宽度大于47 nm、脉冲宽度17 fs的锁模脉冲输出,不仅能够稳定可靠地实现自启动锁模,解决了常规钛宝石激光振荡器锁模启动的困难,而且还具有同步输出1040,800,520 nm三束飞秒激光的特点,为进一步开展飞秒激光相干合成以及光参量放大等研究提供了优势基础。     

Stretched-pulse mode-locking synchronously triggered by a femtosecond master laser at sub-megahertz repetition rate

A stretched-pulse mode-locked ytterbium-doped fiber laser was passively synchronized to a femtosecond Ti:sapphire laser at a low repetition rate of 240 kHz through large cross absorption modulation along additional 1-m-long erbium-doped fiber. The synchronous fiber laser with an ultra-long fiber cavity could produce not only nanosecond flat-top pulses with tunable pulse duration but also Gaussian-shape stretched pulses with its minimum pulse duration of ∼450 ps as confirmed by cross-correlation measurement. When operating in the stretched pulse regime, the sub-nanosecond fiber laser could be synchronously triggered by the master injection with the cavity-length mismatch tolerance up to ∼7.8 cm and timing jitter less than 400 fs, confirming that the stretched-pulse mode-locking of the ultra-long slave fiber laser could be robustly controlled by cross absorption modulation effects in the erbium-doped fiber with appropriate femtosecond master injection.     

Flexible and rapidly configurable femtosecond pulse generation in the mid-IR

We demonstrate a new experimental approach for flexible femtosecond pulse generation in the mid-IR by use of difference-frequency generation from two tightly synchronized Ti:sapphire lasers. The resultant mid-IR pulse train can be easily tuned, with an adjustable repetition frequency up to 100 MHz, a pulse energy of approximately 1.5 x 10(-13) J, and an intensity noise similar to that of the Ti:sapphire. Rapid switching of the mid-IR wavelength and programmable amplitude modulation are achieved by precision setting of the time delay between two original pulses.     

Synchronized retroreflection-pumped femtosecond optical parametric oscillator

We report a flexible technique for threshold reduction and output power enhancement in synchronously pumped optical parametric oscillators (SPOPOs) based on synchronized retroreflection of the undepleted pump using a collimating system and a delay line, which allows easy and independent adjustment of the spatial and temporal overlap of the retroreflected beam in the nonlinear crystal. The method permits initial synchronization of the forward and retroreflected pump by interferometry, providing threshold reduction before oscillation is initiated. We demonstrate the technique in a femtosecond SPOPO based on BiB3O6, where a threshold reduction of 22% and an output power enhancement of 70% are achieved compared with single-pass pumping, with no detrimental effect on the spectral and temporal characteristics of the output pulses.     

飞秒激光烧蚀硅表面产生微纳结构过程中激光脉冲数目的影响

为了研究飞秒激光脉冲数目与硅表面形貌之间的关系,在相同的SF6气体氛围下,改变照射硅表面的飞秒激光脉冲数,发现在飞秒激光照射下由硅表面形成的微型锥状尖峰的高度与飞秒激光脉冲数呈现一种非线性关系.通过对该关系的研究有利于找出在制造具有较高吸收效率的高微型锥状尖峰的"黑硅"的实验条件,有利于基于"黑硅"材料的光电器件转化效...     

Talbot effect under illumination of double femtosecond laser pulses

The Talbot effect under illumination of double femtosecond laser pulses has been reported. Spectrums of double femtosecond laser pulses with phase differences are quite different from that of one single femtosecond laser pulse. Therefore, the Talbot images of the double femtosecond laser pulses with phase differences are different from that of one single femtosecond laser pulse. Specifically, for the phase difference corresponding to π, the Talbot image shows the largest difference from that of one single pulse. Experimental results are in good agreement with the theoretical analysis. The behaviors of Talbot images under double femtosecond laser pulses illumination cannot be obtained under one femtosecond laser pulse, monochromatic or polychromatic light illumination. Therefore, it is a new interesting optical phenomenon for the Talbot effect which should have potential applications.     

16.2-W average power from a diode-pumped femtosecond Yb:YAG thin disk laser

We demonstrate a power-scalable concept for high-power all-solid-state femtosecond lasers, based on passive mode locking of Yb:YAG thin disk lasers with semiconductor saturable-absorber mirrors. We obtained 16.2 W of average output power in pulses with 730-fs duration, 0.47-muJ pulse energy, and 560-kW peak power. This is to our knowledge the highest average power reported for a laser oscillator in the subpicosecond regime. Single-pass frequency doubling through a 5-mm-long lithium triborate crystal (LBO) yields 8-W average output power of 515-nm radiation.     

Tunable, high-repetition-rate, femtosecond pulse generation in the ultraviolet

We report efficient generation of tunable femtosecond pulses in the ultraviolet (UV) by intracavity doubling of a visible femtosecond optical parametric oscillator (OPO). The OPO, based on a 400 microm BiB3O6 crystal and pumped at 415 nm in the blue, can provide visible femtosecond signal pulses across 500-710 nm. Using a 500 microm crystal of beta-BaB2O4 internal to the OPO cavity, efficient frequency doubling of the signal pulses into the UV is achieved, providing tunable femtosecond pulses across 250-355 nm with up to 225 mW of average power at 76 MHz. Cross-correlation measurements result in UV pulses with durations down to 132 fs for 180 fs blue pump pulses.     

飞秒激光脉冲与金属光阴极相互作用

本文从理论上分析了飞秒激光与光阴极相互作用过程，采用双温模型分析了飞秒激光脉冲辐照下金属薄膜的温度效应。通过建立一个简单的光电效应模型，获得了最佳的金属光阴极厚度，通过该模型可以发现，产生的光电流对在飞秒激光脉冲辐照下的电子温度和晶格温度有着很大的依赖关系。     

Generation of femtosecond vacuum-ultraviolet pulses

High power femtosecond pulses in the Vacuum Ultra Violet (VUV) have been generated through the nonlinear interaction of femtosecond KrF pulses with xenon and argon gas. Under near resonant two photon excitation of xenon by a femtosecond KrF laser, parametric four wave mixing processes lead to VUV pulses at 147 and 108 nm with pulse energies in the 10 µJ range. Tuning is demonstrated by mixing the KrF pulse with a 500 fs dye laser pulse at 497 nm, resulting in 165 nm emission. In argon, a three photon resonance leads to third harmonic generation at 83 nm and micro joule level pulses near 127 nm generated by a six wave mixing process. Since the spectra of the VUV pulses show an ionization-induced blue shift with increasing KrF laser intensity, the VUV pulses can be shown to have temporal duration less than the pulse width (450 fs) of the KrF laser. Blue shifting of the third harmonic of the KrF laser in argon is dominated by a reduction in the neutral gas density rather than by an increase in the electron density.     

Long-distance femtosecond laser filaments in air

This paper reviews the recent studies of filamentation of femtosecond lasers pulses in air in the Institute of Physics, Chinese Academy of Sciences. The filamentation mechanisms of free propagated femtosecond laser pulses, effect of air turbulence on the filamentation, interaction between filaments are presented.