Nuclear Reactions under Irradiation of Deuterated Structures by X Rays

Measurements of emission from nuclear reaction products (neutrons and protons) have been carried out appearing in the deuterated structures of textured CVD diamond, palladium, titanium, and zirconium under irradiation with a beam of X rays using independent methods (neutron detector based on He-3 counters, Si surface-barrier semiconductor detectors and CR-39 track detector). The possibility of enhancement of both DD reaction and multi-particle deuterium fusion by the beam of X rays with energy ranging 20–30 keV in solid deuterated targets has been established. Analysis of X-ray fluorescence spectra of the target bombarded by beams of ions has revealed “additional” peaks, the occurrence of which cannot be related to any of the known elements, and requires separate study.

     

Performance of CVD diamond alpha particle detectors

The inherent properties of diamond can, in principle, make it an ideal material for radiation detectors with interesting capabilities. We have fabricated a particle detector using a free-standing CVD diamond film with a thickness of 300 μm and area of 2 cm×2 cm and measured 5.5 MeV α spectra from an ²⁴¹Am source. The I-V characteristics indicate that a fine Ohmic contact is formed between the CVD diamond and electrode. At the external electric field 10 kV/cm, the collection efficiency reaches an average value of 41%, corresponding to a charge collection distance (CCD) of about 259 μm and the energy resolution achieves 4.3%.     

Monte Carlo simulations of multiplexed electronic grade CVD diamond for neutron detection

A novel and evolutionary multiplexing technique is introduced in this work where electronic grade single crystal chemical vapor deposition (CVD) diamond plates are multiplexed together in both a series and parallel configuration, sending electronic signals from each diamond plate to a single electronic acquisition system. Modeling of this novel multiplexing technique consisted of MCNPX simulations and significant post processing. The model developed allowed for the characterization of charge collection efficiency corrections to the location of charge creation to determine the effect of increasing detection medium size with respect to charge collection direction on the measured pulse height spectrum. This work was conducted to show that this technique is theoretically capable of replacing a single crystal diamond plate of similar size for use in neutron detection without the immediate need of advancing CVD diamond growth technologies. Further, this work indicates the expected pulse height evolution from a singular large single crystal diamond if such a crystal is produced in the future. The results of this work indicate that a 14.1 MeV neutron induced energy pulse of 8.4 MeV (due to the ¹²C(n,α_o)⁹Be reaction) in the pulse height spectrum has its energy resolution broadened by a factor of two to a total value of 0.225 percent for a multiplexed array with a thickness from 0.05 to 1 cm and an intrinsic detection efficiency of 25.4 percent for a 1 cm thick diamond crystal. It is also qualitatively discussed that the number of secondary neutron interactions with the diamond detector array may be about 5 percent. The results of this work indicate the capability of multiplexing diamond plates together for spectroscopic neutron detection with a combined intrinsic detection efficiency and energy resolution greater than any other diamond-based neutron detection system reported to date.     

Detecting neutrons by forward recoil protons at the Energy & Transmutation facility: Detector development and calibration with 14.1-MeV neutrons

As part of the Energy & Transmutation project, we are developing a detector for neutrons with energies in the 10–100 MeV range emitted from the target irradiated by a charged-particle beam. The neutron is detected by measuring the time-of-flight and total kinetic energy of the forward-going recoil proton [1] knocked out at a small angle from a thin layer of plastic scintillator, which has to be selected against an intense background created by γ quanta, scattered neutrons, and charged particles. On the other hand, neutron energy has to be measured over the full range with no extra tuning of the detector operation regime. Initial measurements with a source of 14.1-MeV neutrons are reported.     

Measuring high-energy γ-ray emission accompanying the spontaneous fission of <Superscript>252</Superscript>Cf nuclei

The probability of high-energy γ-ray emission accompanying the spontaneous fission of ²⁵²Cf nuclei in the energy range of 5–60 MeV was measured experimentally. The γ rays were detected by a BGO detector with a size of ∅7.6 × 7.6 cm in coincidence with neutrons detected by an organic polystyrene-based scintillator with a size of ∅6.0 × 2.0 cm. To reject events associated with the cosmic background, we propose an original method that combines rapid digitizing of the pulse shape and the time-of-flight method.     

Experimental neutron flux measurements with a diamond detector at the QUINTA setup

The operational capability of a diamond detector used to measure the neutron spectrum by the response function on the QUINTA setup [1] installed at the proton beam of the phasotron [2] (Laboratory of Nuclear Problems, Joint Institute for Nuclear Research) was demonstrated in the energy interval of 2.1–20 MeV. The neutron-flux count rate was measured. The energy of neutrons was estimated at 7.4–25.7 MeV based on the diamond-detector response spectrum. The dependence of the diamond-detector response spectra on the angle between the proton beam and the line going through the detector and the center of the QUINTA setup was investigated. The angular anisotropy of the neutron flux was demonstrated. Measurements at different distances from the detector to the QUINTA setup were performed.     

Survey meter combining CVD diamond and silicon detectors for wide range of dose rates and high accumulated doses

We have developed a prototype of a survey meter combining a CVD diamond detector and silicon detectors to appropriately take temporal measurements of γ-ray radiations over a wide range of the dose rates and to measure high accumulated doses of γ-ray radiations. In order to carry out this, at first, we have studied the radiation hardness of diamond detectors suitably fabricated with high-quality single-crystalline CVD diamond films to confirm that such CVD diamond detectors have greatly superior radiation hardness, compared with commercially available silicon detectors. It is evidenced that the performance of the CVD diamond detector did not significantly change even after heavy γ-ray irradiation of 0.7 MGy while the silicon detectors have a remarkable increase in the dark current, a detection peak shift to the low energy side, and a decrease in detection counts for 5.486-MeV α particles. Due to a size limitation of the CVD diamond detector, such a CVD diamond detector was combined with six commercially available silicon detectors to fabricate a survey meter which can appropriately work under severe irradiation conditions, or, at accumulated doses larger than at least 0.5 MGy and which can cover a wide range of the dose rates from 1 μGy/h to at least 1 kGy/h. The prototype survey meter had a practically useful linearity in this dose rate range. Thus, we have confirmed that such a diamond-Si combined survey meter can be put into practical use.     

化学气相沉积金刚石薄膜探测器对α粒子的电荷收集效率

 实验测量了自行研制的三明治电极结构化学气相沉积(CVD)金刚石薄膜探测器在室温下对241Am, 243Am 与244Cm α粒子的能谱响应,得到了其α粒子响应电荷收集效率随偏压的变化关系;获得了不同偏压下其相对平均电荷收集效率及响应谱下降沿10%处的相对电荷收集效率。结果表明：所研制的CVD金刚石薄膜探测器性能稳定,对α粒子响应的电荷收集效率随偏压的增加而趋于饱和,对α粒子平均电荷收集效率达33.5%,谱下降沿10%处的电荷收集效率达57%。     

Influence of Bonner sphere response functions above 20 MeV on unfolded neutron spectra and doses

Monte Carlo (MC) codes for neutron transport calculations such as MCNP, MCNPX, FLUKA, PHITS, and GEANT4, crucially rely on cross sections that describe the interaction of neutrons with nuclei. For neutron energies below 20 MeV, evaluated cross sections are available that are validated against experimental data. In contrast, for high energies (above 20 MeV) experimental data are scarce and, for this reason, every neutron transport code is based on theoretical nuclear models to describe interactions of neutrons with nuclei in matter. Here we report on the calculation of a complete set of response functions for a Bonner spheres spectrometer (BSS), by means of GEANT4 using the Bertini and Binary Intranuclear Cascade (INC) models for energies above 20 MeV. The recent results were compared with those calculated by MCNP/LAHET and MCNP/HADRON MC codes. It turns out that, whatever code used, the response functions were rather similar for neutron energies below 20 MeV, for all 16 detector/moderator combinations of the considered BSS system. For higher energies, however, differences of more than a factor of 2 were observed, depending on neutron energy, detector/moderator combination, MC code, and nuclear model used. These differences are discussed in terms of neutron fluence rates measured at the environmental research station (UFS), “Schneefernerhaus”, (Zugspitze mountain, Germany, 2650 m a.s.l.) for energies below 0.4 eV (thermal neutrons), between 0.4 eV and 100 keV (epithermal neutrons), between 100 keV and 20 MeV (evaporation neutrons), and above 20 MeV (cascade neutrons). In terms of total neutron fluence rates, relative differences of up to 4% were obtained when compared to the standard MCNP/LAHET results, while in terms of total ambient dose equivalent, relative differences of up to 8% were obtained. Both the GEANT4 Binary INC and Bertini INC gave somewhat larger fluence and dose rates in the epithermal region. Most relevant for dose, however, those response functions calculated with the GEANT4 Bertini INC model provided about 18% less neutrons in the cascade region, which led to a roughly 13% smaller contribution of these neutrons to ambient dose equivalent. It is concluded that doses from secondary neutrons from cosmic radiation as deduced from BSS measurements are uncertain by about 10%, simply because of some differences in nuclear models used by various neutron transport codes.     

A CVD diamond film detector for pulsed proton detection

A chemical vapour deposition （CVD） diamond film detector was prepared and the main characteristics for pulsed proton detection were studied at Beijing Tandem Accelerator. The result shows that the charge collection efficiency of the detector increases with increasing electric field intensity and reaches to 9.44% at 5 V/μm with the charge collection distance of 15.9 μm. The relationship between the sensitivity of the detector and proton energy is consistent with the Monte Carlo （MC） simulation result. Its plasma time for a pulse with 4.85×10^5 protons is 1l.2ns. The dose threshold for onset of damage under 9MeV proton irradiation in the detector is about 10^13 cm^-2. All of the results show that a CVD diamond detector has fast time response and high radiation hardness, and can be used in pulsed proton detection.     

用于质子和伽马射线探测的金刚石薄膜探测器的辐照性能

 研制出CVD金刚石薄膜探测器,在国家串列加速器和⁶⁰Co稳态辐射源上分别完成了该探测器对9 MeV质子束流和1.25 MeV γ射线的辐照性能研究。结果表明:该探测器在9 MeV质子照射累积强度达到10¹³ cm^-2时,探测器信号电荷收集效率减小量低于3.5%,辐照前后探测器暗电流没有明显变化。计算得到9 MeV质子对该探测器的损伤系数为1.3×10^-16 μm^-1·cm²。由于γ射线与金刚石作用产生的电子起到了填补缺陷的作用,探测器信号电荷收集效率随γ射线照射剂量的增加略有增加,在γ射线累积照射量达到10.32 C/kg时,其增幅小于0.7%。说明金刚石薄膜探测器具有较高耐辐照强度,适用于高强度辐射测量领域。     

Development of a segmented fast neutron spectrometer

We discuss the development of a spectrometer based on full energy absorption using liquid scintillator doped with enriched ⁶Li. Of specific interest, the spectrometer is expected to have good pulse height resolution, estimated to lie in the range 10–15% for 14-MeV neutrons. It should be sensitive to flux rates from 10⁻⁶ cm⁻² s⁻¹ to 10⁶ cm⁻² s⁻¹ above a threshold of 500 keV in an uncorrelated γ background of up to 10⁴ s⁻¹. We have constructed a pilot version of the detector using undoped liquid scintillator, and we report its present status. The detector’s efficiency is determined by the volume of the scintillator (∼1.21) and is estimated to be 0.2–0.5% for 3-MeV neutrons. The good pulse height resolution is achieved by compensation of the nonlinear light yield of the scintillator due to the use of optically separated segments, which collect scintillations from each recoil proton separately. We demonstrate here the response of the detector to neutrons from a Pu-α-Be source, whose energies range up to 10 MeV. Initial testing indicates a low threshold (≈600 keV) and good spectral response after requiring a multiplicity of three segments. Such a spectrometer has applications for low-background experiments in fundamental physics research, characterizations of neutron flux in space, and the health physics community. The text was submitted by the authors in English.     

Evolution of nuclear spectroscopy at Saha Institute of Nuclear Physics

Experimental studies of nuclear excitations have been an important subject from the earliest days when the institute was established. The construction of 4 MeV proton cyclotron was mainly aimed to achieve this goal. Early experiments in nuclear spectroscopy were done with radioactive nuclei with the help of beta and gamma ray spectrometers. Small NaI(Tl) detectors were used for gamma-gamma coincidence, angular correlation and life time measurements. The excited states nuclear magnetic moments were measured in perturbed gamma-gamma angular correlation experiments. A high transmission magnetic beta ray spectrometer was used to measure internal conversion coefficients and beta-gamma coincidence studies. A large number of significant contributions were made during 1950–59 using these facilities. Proton beam in the cyclotron was made available in the late 1950’s and together with 14 MeV neutrons obtained from a C-W generator a large number of short-lived nuclei were investigated during 1960’s and 1970’s. The introduction of high resolution Ge gamma detectors and the improved electronics helped to extend the spectroscopic work which include on-line (p ₇ p′γ) and (p ₇ nγ) reaction studies. Nuclear spectroscopic studies entered a new phase in the 1980’s with the availability of 40–80 MeV alpha beam from the variable energy cyclotron at VECC, Calcutta. A number of experimental groups were formed in the institute to study nuclear level schemes with (α ₇ xnγ) reactions. Initially only two unsuppressed Ge detectors were used for coincidence studies. Later in 1989 five Ge detectors with a large six segmented NaI(Tl) multiplicitysum detector system were successfully used to select various channels in (α ₇ xnγ) reactions. From 1990 to date a variety of medium energy heavy ions were made available from the BARC-TIFR Pelletron and the Nuclear Science Centre Pelletron. The state of the art gamma detector arrays in these centres enabled the Saha Institute groups to undertake more sophisticated experiments. Front line nuclear spectroscopy works are now being done and new informations are obtained for a large number of nuclei over a wide mass range. Currently Saha Institute is building a multi-element gamma heavy ion neutron array detector (MEGHNAD), which will have six high efficiency clover Ge detector together with charged particle ball and other accessories. The system is expected to be usable in 2002 and will be used in experiments using high energy heavy ions from VECC.     

Measurement of peak fluence of neutron beams using Bi-fission detectors

Fission fragments and other charged particles leave tracks of permanent damage in most of the insulating solids. Damage track detectors are useful for personal dosimeters and for flux/dose determination of high-energy particles from accelerators or cosmic rays. A detector that has its principal response at nucleon energy above 50 MeV is provided by the fission of Bi-209. Neutrons produce the largest percentage of hadron dose in most high-energy radiation fields. In these fields, the neutron spectrum is typically formed by low-energy neutrons (evaporation spectrum) and high-energy neutrons (knock-on spectrum). We used Bi-fission detectors to measure neutron peak fluence and compared the result with the calculated value of neutron peak fluence. For the exposure to 100 MeV we have used the iThemba Facility in South Africa.     

Response of a Si-diode-based device to fast neutrons

Semiconductor devices based on a Si-detector are frequently used for charged particle's detection; one application being in the investigation of cosmic radiation fields. From the spectra of energy deposition events in such devices, the total energy deposited by the radiation in silicon can be derived. This contribution presents the results of studies concerning the response of this type of detector to fast neutrons. First, the spectrum of energy deposition was established in fast neutron radiation fields with average energies from 0.5 to 50 MeV. It was found that these spectra vary significantly with the neutron energy. The comparison with the spectra registered in photon beams permitted an estimation of the part of energy deposited that could be attributed to neutrons. It was found that this part increases rapidly with neutron energy. The possibilities to use this type of detector for neutron detection and dosimetry for radiation protection are analysed and discussed.     

Energy calibration of a Δ<Emphasis Type="Italic">E</Emphasis>-<Emphasis Type="Italic">E</Emphasis> scintillation telescope in (α, p) reaction

A procedure for and the results from the energy calibration of a ΔE-E scintillation telescope used in experiments performed at the INR to study the nd-breakup reaction are described. The telescope was calibrated using a beam of α particles with an energy of 30 MeV of the U-120 cyclotron (INP). Secondary protons from the ^10,11B(α, p) reaction were recorded by the ΔE-E telescope at several recording angles and with the application of different absorbing foils. The calibration results from the ΔE-E telescope were obtained over the interval E _p = 10–30 MeV, allowing us to measure the energies of secondary protons in the ndbreakup reaction when the energy of primary neutrons is 20–60 MeV.     

Bismuth-fission detectors for high energy nucleons: II. Proton and neutron responses

A critical requirement for the ²⁰⁹Bi-fission detector is the knowledge of its response as a function of energy for both neutrons and protons. For this reason, stacks of ²⁰⁹Bi-fission detectors have been exposed to proton beams of 100 and 150 MeV at the Paul Sherrer Institute. Similar stacks have been exposed to neutron beams of 100 and 160 MeV at the Svedberg Laboratory from Uppsala University. The calibrations data with neutrons have been compared with those obtained with protons of the same energies. This comparison has proved that the response of ²⁰⁹Bi-fission detector for neutrons is two to three times smaller than that for protons at least in the range of nucleon energy up to 150 MeV.     

Energetic neutrons and gamma rays measured on the Aryabhata satellite

An experiment to measure energetic neutrons and gamma rays in space was launched in the first Indian scientific satellite,Aryobhata, on April 19, 1975. From this experiment, the first measurements in space of the Earth’s albedo fiux of neutrons of energy between 20 and 500 MeV have been made; the values obtained for two mean geomagnetic vertical cut-off rigidities of 5.6 and 17.0 GV are (6.3±0.4)×10⁻² and (1.4±0.3)×10⁻² neutrons cm⁻² sec⁻¹ respectively. These measurements confirm that protons arising from cosmic ray albedo neutron decay, can adequately account for the protons in the inner radiation belt. Observations on gamma rays of energy between 0.2 and 24 MeV have enabled the determination of the total background gamma ray flux in space as a function of latitude. This in turn has permitted useful information on the diffuse cosmic gamma rays. We have also observed four events that showed sudden increases in the gamma ray counting rates between 0.2 and 4.0 MeV. Observational details of these events are given.     

Response of chemical vapor deposition diamond detectors to X-ray

The outstanding properties of diamond, such as radiation hardness, high carrier mobility, high band gap and breakdown field, distinguish it as a good candidate for radiation detectors. The detector's performance is strongly limited by the concentration of defects (grain boundaries and/or impurities) in chemical vapor deposition (CVD) diamond. We report the response of free-standing CVD diamond with a thickness of 300 μm and area of 2×2 cm², synthesized by a hot filament chemical vapor deposition (HFCVD) technique, to 5.9 keV X-ray radiation from a ⁵⁵Fe source. The linear I-V characteristics indicate that CVD diamond has good ohmic contacts. This detector also shows good results such as dark-current of 10⁻⁸ A, photocurrent of 10⁻⁶ A, energy resolution <0.4%, and a high ratio of signal to noise.     

A multi NaI(Tl) detector array for medium energyγ-ray spectroscopy

An array of seven hexagonal NaI(Tl) detectors has been set up for measuringγ-ray spectra in the energy region 5 MeV ≤E _γ ≤ 40 MeV with good accuracy. This is in contrast to earlier set ups which mostly used one large sized (about 10 inchesφ × 15 inches long)NaI(Tl) detector. This set up has been made for the study ofγ decay of GDR based on high spin states and ultra-dipole radiations. The array has been provided with the following features: a) TOF discrimination against neutrons, b) pile up detection and elimination, c) active and passive shielding to cut down background and d) an array of trigger counters for multiplicity dependence measurements. The well known program EGS4 has been used to determine the response of the array forγ-rays in the energy region 5–40 MeV and several test measurements have been carried out to confirm the validity of the calculated response functions. Some typicalγ-ray spectra fromα and¹⁶O induced reactions measured at VECC, Calcutta and Pelletron accelerator at TIFR are also shown.