An irradiation chamber for experimental studies on SSNTD response to alpha particles

An irradiation apparatus was designed in our laboratory to study the detection efficiency dependence of SSNTDs (CR-39, LR115, Makrofol) on alpha particles of different energy and incident angle. The system was designed to irradiate up to nine detectors in a short time, allowing to obtain reproducible conditions on many detectors and therefore to reduce random variations of the results. The system is composed of a pressure-controlled stainless-steel chamber containing a ²⁴¹Am source and a circular rotating table with 10 detector holders, one of which is devoted to an ion-implanted silicon detector for irradiation energy monitoring. The table rotation is controlled electronically via a photodiode-based system, so that the position of the detectors under the source is known with a maximum uncertainty of 0.5 mm. The detector holders allow to change the detector (both passive and active) to source inclination angle continuously and with an uncertainty better than 1. The source-to-detector distance is controlled electronically and can be varied from 5 to 30 cm with an uncertainty of about 0.1 mm. Some simulations, obtained using the transport code TRIM, to project the irradiation chamber and its main characteristics are reported and discussed.     

Stopping power measurements of Si in polycarbonate detectors

The rate of energy loss of the impinging ion as it passes through succeeding layers of the target material gives information regarding the nature of the material and helps to calculate the range of the ions in a thick target in which the ions are stopped. In the present work, the range of 118 MeV ²⁸Si was measured in different types of polycarbonates, viz. Makrofol-N, Makrofol-G and Makrofol-KG, using the nuclear track technique. Polyallyldiglycol carbonate (PADC) was used as the backing detector. The experimental values of range and energy-loss rate are compared with the theoretical values obtained from different computer codes, viz. BENTON, HUBERT, RANGE, TRIM’98 and SRIM’03.     

Alpha-particle calibration of CR-39 using a beehive collimator

A device to determine the detection efficiency of CR-39 for alpha particles is presented. A beehive collimator restricted the angle of incidence of alpha particles on a CR-39 sheet, such that the total number of alpha emitters could be determined. This makes it possible to obtain the critical angle of incidence, Θ_C, and the maximum angle of incidence resulting in round (diameter ratio <1.100) etch pits, Θ_max. In this work, these angles were determined for incidence energies around 7.5 MeV (more specifically 6.1 and 8.8 MeV).     

Study on the etching conditions of polycarbonate detectors for particle analysis of safeguards environmental samples

The fission track technique was applied to the particle analysis for safeguards environmental samples to obtain information about the isotope ratio of nuclear materials in individual particles. To detect the particles containing nuclear material with high detection efficiency and less particle loss, the influence of uranium enrichments on etching conditions of a fission track detector made of polycarbonate was investigated. It was shown that the increase in uranium enrichment shortened the suitable etching time both for particle detection and for less particle loss. From the results obtained, it was suggested that the screening of the uranium particles according to the enrichment is possible by controlling the etching time of the detector.     

Study of the response of silicon detectors for alpha particles

Numerous radon measurements are carried out using silicon detectors directly in the environment. This new kind of alpha radiation measurement has been developed because the reduced cost makes it possible to replace the usual plastic track detectors. At our laboratory, an alpha particle detector has been designed from a commercial silicon photodiode. This type of detector can determine the device response perfectly in any kind of environment. Different spectrum analyses have been conducted in the laboratory and field to define the exact origin of counted alpha particles. We studied the response for different radon and thoron concentration levels and observed the energy of the detected alpha particles. We carried out some of these experiments with gas flux, and some without, to show the effects of interactions with surfaces to obtain thermodynamic equilibrium in the detection chamber. Finally, the silicon diodes that we tested measure the alpha particles of the decay products (polonium) from the radon and the thoron, but very weakly from the gases themselves. Thus, it is possible to make mistakes when measuring the radon if the count of alpha particles is performed without spectrum analysis. One reason for this is that the decay progenies of the radon are solid radio-elements with thermodynamic proprieties different from gases.     

Bremsstrahlung of fast charged particles on clusters in a wide spectral range

Within the framework of the first Born approximation and a simple model of the structural factor, the bremsstrahlung of fast charged particles on polyatomic clusters is calculated and analyzed with regard to the polarization mechanism in a wide spectral range including a domain of high frequencies. The role of cooperative phenomena in the static and polarization channels of bremsstrahlung is investigated. It is established that these phenomena, being negligible for static bremsstrahlung, substantially influence the polarization bremsstrahlung. It is shown that the constructive interference between the contributions of the atoms of a cluster to the polarization bremsstrahlung substantially increases its intensity and changes its dependence on the basic parameters of the problem compared with the case of bremsstrahlung on an isolated atom.     

Determination of the range of alpha particles in SSNTD by optical density method

A technique based on the optical density (D) measurement of the etched track is useful for charged particles spectroscopy using SSNTD. It was shown that the stopping power of alpha particles in CR-39 is proportional to D. We measured the optical density and derived an expression to estimate the range of alpha particles in CR-39 detector as a function of the bulk etching rate and etching time. The relation between the etching time, track parameters (depth, radius) and D for different alpha particles energy and etching conditions were studied. A relation describing D as a function of track size is proposed.     

Radiography of biological specimens with alpha particles and the CR-39 SSNTD

This work studies the alpha particle radiography technique in conjunction with the CR-39 SSNTD. The irradiations were made in the CV-28 cyclotron at IEN/CNEN/RJ using a 7 MeV/nucleon alpha particle beam. The best etch time to obtain radiographs was determined as six hours. A calibration curve was obtained, so to allow a quantitative interpretation of the images to be performed. Its behavior was checked by several experiments with other energy degrading materials. Several radiographs of “in-vitro” biological specimens were obtained. The results showed the potential capability of this technique for studies in paleontology.     

Helium ion distributions in a 4 kJ plasma focus device by 1 mm-thick large-size polycarbonate detectors

Helium ion beam profile, angular and iso-ion beam distributions in 4 kJ Amirkabir plasma focus (APF) device were effectively observed by the unaided eyes and studied in single 1 mm-thick large-diameter (20 cm) polycarbonate track detectors (PCTD). The PCTDs were processed by 50 Hz–HV electrochemical etching using a large-size ECE chamber. The results show that helium ions produced in the APF device have a ring-shaped angular distribution peaked at an angle of ∼±60°$\sim \pm 60\mathrm{°}$ with respect to the top of the anode. Some information on the helium ion energy and distributions is also provided. The method is highly effective for ion beam studies.     

Factors affecting the registration and counting of alpha tracks in solid state nuclear track detectors

In view of the fact that the radon progeny contribute the highest to the natural radiation dose to general populations, large scale and long-term measurements of radon and its progeny in the houses have been receiving considerable attention. Solid State Nuclear Track Detector (SSNTD) based systems, being the best suited for large scale passive monitoring, have been widely used for the radon gas (using a cup closed with a semi-permeable membrane) and to a limited extent, for the measurement of radon progeny (using bare mode in conjunction with the cup). These have been employed for radon mapping and indoor radon epidemiological studies with good results. In this technique, alpha tracks recorded on SSNTD films are converted to radon/thoron concentrations using corresponding conversion factors obtained from calibration experiments carried out in controlled environments. The detector response to alpha particles depends mainly on the registration efficiency of the alpha tracks on the detector films and the subsequent counting efficiency. While the former depends on the exposure design, the latter depends on the protocols followed for developing and counting of the tracks. The paper discusses on parameters like etchant temperature, stirring of the etchant and duration of etching and their influence on the etching rates on LR-115 films. Concept of break down thickness of the SSNTD film in spark counting technique is discussed with experimental results. Error estimates on measurement results as a function of background tracks of the films are also discussed in the paper.      

The method of simultaneous size and activity measurement of alpha emitting hot particles using multiple track analysis of solid state nuclear track detectors

Current work is concentrated upon the detection and analysis of hot particles from contaminated ground. Simultaneous measurement of parameters as activity and size of radioactive particle would have immense value for many applications in radiation protection and control of the environment. The algorithm and performance of multiple alpha track analysis is discussed.     

Study of bubble damage detectors for neutron detection

Bubble damage detectors have been prepared by using polyacrylamide as detector solid and freon as detector liquid. Tests show that the prepared detectors are sensitive to fast neutrons and have proportionality between bubble number and neutron fluence within a certain range of neutron fluence. Therefore, it can be used as a fast neutron detector and a dosimeter. Our experiments also show that the sensitivity of the detector increases with temperature.     

Verification of Mason and Smythe equations for electrical treeing breakdown at the tip of charged particle tracks in ECE polycarbonate detectors

There are two different equations to describe enhancement of field strength at the track tip in ECE polycarbonate detectors: Mason and Smythe equations. In order to evaluate the equations, PC detectors with different thicknesses were exposed to 1 MeV alpha and/or fast neutron. The response of the detectors was studied as a function of applied voltage and average field strength. The ratio of critical voltages for different detectors was estimated experimentally and compared with calculated values. The experimental results are in good agreement with Smythe's equation. The results show that the track density and mean track diameter in the different detectors have the same behaviour, when the macroscopic field strength increases, and also that the field strength at the tip of tracks is proportional to macroscopic field strength.     

Stilbene composite scintillators as detectors of fast neutrons emitted by a 252Cf source

The results of the measurements are presented of the relative efficiency ε for ²⁵²Cf fast neutron detection by composite detectors based on stilbene crystalline grains. The effects of the grain size and height of the composite detector on its scintillation properties were studied. It is shown that the efficiency of fast neutron detection of stilbene composite scintillators ranges up to 60% of that of bulk single crystals. The results are also presented for relative light output measurements of stilbene composite detectors irradiated by gamma photons of ¹³⁷Cs, as well as transmittance data of samples in the range of their transparency absorption.     

System for calibration of track detectors used in gaseous and solid alpha radionuclides monitoring

A laboratory system for the calibration of track detectors and charcoal detectors used in monitoring of radon and its decay products/their aerosols in air, is proposed. The system consists of three main components: (i) the alpha exposure chambers, including alpha monitoring devices and the connection with the ²²⁶Ra radioactive source. The CR-39 track detectors are mounted in the monitoring devices pre-equipped or not with paper filter; (ii) the calibrated  ²²⁶Ra source. Among the three tested sources: ²²²Rn, ²²⁶Ra+²²²Rn and ²²⁶Ra, the ²²⁶Ra source is considered the most appropriate radon source for our calibration system. It is kept into an airtight flat bottom flask, the radionuclide ²²⁶Ra being always in the radioactive equilibrium with their descendants. In the alpha exposure chambers, the source assures the radon at a constant rate; (iii) the ALFAUURASE program for the computation of radioactive accumulation of the alpha ²²⁶Ra descendants. For any initial mass of the parent, the amount and the activity of each alpha decay product and of all the decay products can be calculated by this computation program. Each component of the calibration system is described in the paper. The use of the system for the calibration of CR-39 track detectors in radon measurements is tested.     

An alpha particle detector based on a GPS mosaic scintillator plate for continuous air monitoring in plutonium handling facilities

An alpha particle detector was developed for continuous air monitoring of radioactive contamination in working chambers at plutonium handling facilities. A 5-cm-square Gd₂Si₂O₇:Ce (cerium-doped gadolinium pyro-silicate, GPS:Ce) mosaic scintillator plate for alpha particle measurements was fabricated from GPS single-crystal grains of around 550 μm diameter; the GPS grains were made of a GPS polycrystalline body grown using a top seeded solution method. The scintillator layer thickness was approximately 100 μm. The surface filling rate of the GPS grains was ca. 62%. To suppress the influence of non-uniformity of pulse heights of a photomultiplier tube, a central part of ∅ 40 mm of a 76-mm-diameter photomultiplier tube was used. In addition, 3 mm thick high-transmission glass was used as a substrate of the scintillator plate. The detector achieved energy resolution of 13% for 5.5 MeV alpha particles, detection efficiency of 61% and a radon progeny nuclide reduction ratio of 64.5%. A new alpha particle detector was developed to achieve a high radon progeny nuclide reduction ratio approaching that of a silicon semiconductor detector, with high resistance to electromagnetic noise and corrosion.     

Fission cross section and fragment angular distribution in gold fission induced by 55 MeV alpha particles using solid state nuclear track detectors

The angular distribution of fission fragments in alpha induced fission has been studied at an incident energy of 55 MeV in¹⁹⁷Au target. The relative differential fission cross sections were measured at different angles between 10° and 170° and the resulting angular distributions fitted by least squares method with Legendre polynomials. In the present work, a correction for the self-scattering and self-absorption of fission fragments in the target itself was applied and a target of 3 mg/cm² was used to get good statistics. The anisotropy for 55 MeV alpha induced fission of gold was 2·83±0·43 and the fission cross section calculated by integrating the measured angular distributions over all the solid angles was 5·2±1.0 mb, confirming the value of 4·0±0·05 mb reported by Burnettet al but contrary to the high value of 10±3 mb reported by Ralarosyet al.     

Analysis of energy distribution in a loaded quantum anharmonic oscillator in a wide temperature range

Analysis of the energy distribution in an ensemble of quantum anharmonic oscillators loaded by an external force in a wide temperature range (from T = 0) is carried out using a general approach based on the virial theorem. At T = 0, anharmonic effects are observed: a linear variation of zero-point energy of an oscillator under loading (energy decrease during extension and increase under compression) and a linear variation of the average kinetic and potential energy components. At high temperatures, at which the dynamics of the oscillators becomes classical, the anharmonic effects are manifested in a linear variation in the vibrational energy and a linear variation in the average kinetic and potential energy components upon an increase in force. Mutually compensating variation in the average kinetic and potential energy components of the internal dynamic energy of an oscillator (energy redistribution upon loading) takes place both at low and high temperatures.