Spin dynamics of the electron-doped high-T(c) superconducting cuprates

We show that a basic difference between the electron- and hole-doped cuprates is their proximity to two different quantum critical points in a 2D free fermion system on a square lattice and that the spin dynamics observed recently for the first time in the electron-doped Nd2-xCexCuO4, very different from that in the hole-doped cuprates, can be understood as a consequence of this effect.     

Modeling study of peak-dip-hump structure in tunneling spectraof high-temperature superconducting cuprates

We propose new specific model for quasiparticle (QP) tunneling across thesuperconductor-insulator-normal metal (SIN) junction based on two mechanisms. Origin ofthe many features of the tunneling spectra, such as peak-dip-hump (PDH) structure, U- andV-shapes, temperature dependence of differential tunneling conductance, asymmetricconductance peaks, zero-bias conductance, subgap feature and gap inhomogeneity have beenexplained by the proposed model. We show that the energy scales of the binding energies oflarge polarons and polaronic Cooper pairs are identified by pseudogap (PG) crossovertemperature on the cuprate phase diagram.     

Single-particle spectrum in the electron-doped cuprates

We study the evolution of the single-particle spectrum with electron doping in a scheme which adds multiple exchange of transverse spin excitations to the mean-field antiferromagnetic insulator. Away from half-filling small Fermi surface pockets appear first around the X points, and simultaneously new spectral weight grows in the insulating gap. With further doping the in-gap states develop the character of a renormalized quasiparticle band near the chemical potential. The essential features in momentum-energy space agree well with recent studies using angle-resolved photoemission spectroscopy on electron-doped cuprates. We interpret the origins and the nature of the in-gap states using a simple variational wave function.     

Nuclear magnetic resonance study of langatate

A langatate crystal was studied using the nuclear magnetic resonance method. The temperature dependence of the spin-lattice relaxation rate of ⁷¹Ga nuclei was measured in a single-crystal sample in the range 294–500 K. It was shown that the relaxation rate depends linearly on the square of the temperature. The shape of the powder spectrum obtained under static conditions was found to correspond to large values of the quadrupole coupling constant of gallium nuclei. The measurements of the powder spectra obtained upon magic-angle spinning made it possible to estimate the quadrupole coupling constant for gallium in the tetrahedral and octahedral oxygen coordinations.     

Local magnetooptical study of magnetic structures in high-temperature superconducting composites

The results from magnetooptical investigations of the remagnitization processes in composite film structures based on high-temperature superconductors in the temperature range of 4 to 80 K are presented. It is shown that the remagnetization of structures is due to the formation and propagation of wave of magnetic flux annihilation (areas with zero magnetic induction). The relationship between the penetration depth of annihilation front and the external magnetic field at different ambient temperatures, and the temperature dependence of the rate of motion of the front of magnetic flux annihilation, are found. The experimental data qualitatively fit the results from numerical calculations performed using the Monte Carlo method.     

Nuclear magnetic resonance measurement station in SECUF using hybrid superconducting magnets

Nuclear magnetic resonance(NMR) is one of the most powerful tools to explore new quantum states of condensed matter induced by high magnetic fields at a microscopic level. High magnetic field enhances the intensity of the NMR signal, and more importantly, can induce novel phenomena. In this article, examples are given on the field-induced charge density wave(CDW) in high-Tc superconductors and on the studies of quantum spin liquids. We provide a brief introduction to the high magnetic field NMR platform, the station 4 of the Synergetic Extreme Condition User Facility(SECUF), being built at Huairou, Beijing.     

Metal-insulator crossover in superconducting cuprates in strong magnetic fields

The metal-insulator crossover of the in-plane resistivity upon temperature decrease, recently observed in several classes of cuprate superconductors, when a strong magnetic field suppresses the superconductivity, is explained using the U(1)xSU(2) Chern-Simons gauge field theory. The origin of this crossover is the same as that for a similar phenomenon observed in heavily underdoped cuprates without magnetic field. It is due to the interplay between the diffusive motion of the charge carriers and the "peculiar" localization effect due to short-range antiferromagnetic order. We also calculate the in-plane transverse magnetoresistance which is in fairly good agreement with available experimental data.     

Tuning the resonance in high-temperature superconducting terahertz metamaterials

In this Letter, we present resonance properties in terahertz metamaterials consisting of a split-ring resonator array made from high-temperature superconducting films. By varying the temperature, we observe efficient metamaterial resonance switching and frequency tuning. The results are well reproduced by numerical simulations of metamaterial resonance using the experimentally measured complex conductivity of the superconducting film. We develop a theoretical model that explains the tuning features, which takes into account the resistive resonance damping and additional split-ring inductance contributed from both the real and imaginary parts of the temperature-dependent complex conductivity. The theoretical model further predicts more efficient resonance tuning in metamaterials consisting of a thinner superconducting split-ring resonator array, which are also verified in subsequent experiments.     

NMR study of magnetic moments arising in superconducting cuprates under electron/neutron irradiation

The measurements of direct-current magnetic susceptibility and nuclear magnetic resonance (NMR) were performed in the superconducting cuprates YBa₂Cu₃O_6.9 (⁸⁹Y,⁶³Cu), Tl₂Ba₂CaCu₂O₈ (¹⁷O,²⁰⁵Tl), irradiated by fast neutrons (E _n = 1 MeV) and electrons (E _e = 5 MeV). The influence of the radiation-induced structural disorder on the spin susceptibility and magnetic state of atoms in the CuO₂ layer is considered. The possible effect onT _c of the spin-exchange scattering of carriers by localized moments arising under irradiation was estimated following the Abrikosov-Gorkov approach and its contribution was found to be too small in comparison with the real suppression ofT _c under irradiation.     

Effect of temperature on phonon contribution to Green function of high-temperature superconducting cuprates

The phonon contribution to the nodal electron Green function in cuprates is considered. It is shown that the temperature dependence of the real part of the self-energy component of the Green function for cuprates with a hole doping level close to optimal is described by the electron-phonon interaction in the framework of the extended Eliashberg model.     

Nuclear magnetic resonance study of potassium dihydrophosphate

A powder sample of potassium dihydrophosphate KH₂PO₄ has been studied by the ³¹P NMR method in a wide temperature range covering the ferroelectric phase transition. Changes in the position and shape of the resonance line at the transition to the ferroelectric phase have been revealed. The parameters of the chemical shift tensor of ³¹P (isotropic shift, anisotropy, and asymmetry) in the ferroelectric phase have been calculated from the experimental data. A sharp increase in the anisotropy of the tensor at the phase transition has been demonstrated. Dielectric measurements have also been carried out to verify the transition temperature.     

Nuclear magnetic resonance study of ultrananocrystalline diamonds

We report on a nuclear magnetic resonance (NMR) study of ultrananocrystalline diamond (UNCD) materials produced by detonation technique. Analysis of the ¹³C and ¹H NMR spectra, spin-spin and spin-lattice relaxation times in purified UNCD samples is presented. Our measurements show that UNCD particles consist of a diamond core that is partially covered by a sp ²-carbon fullerene-like shell. The uncovered part of outer diamond surface comprises a number of hydrocarbon groups that saturate the dangling bonds. Our findings are discussed along with recent calculations of the UNCD structure. Significant increase in the spin-lattice relaxation rate (in comparison with that of natural diamond), as well as stretched exponential character of the magnetization recovery, are attributed to the interaction of nuclear spins with paramagnetic centers which are likely fabrication-driven dangling bonds with unpaired electrons. We show that these centers are located mainly at the interface between the diamond core and shell.     

Nuclear magnetic resonance study of strongly correlated superconductors

This paper introduces nuclear magnetic resonance works in the strongly correlated super-conductors: heavy-Fermion, high-T _C superconductors and Sr₂RuO₄. The analyses strongly support the spin-fluctuation-mediated superconductivity model in a high-T _C superconductor.     

Models of bands and Fermi surfaces for electron-doped cuprates

The properties of Fermi surfaces and electron bands in electron-doped cuprates have been studied. The possible origins of a hole pocket in the nodal direction and a pseudogap at hot spots are discussed, including stripe phases and double bands in an antiferromagnetically correlated Fermi liquid. Within the framework of the mean field method, it is shown that both t-t′-t″-U Hubbard model solutions with a homogeneous antifer-romagnetic spin structure and those with a diagonal stripe structure can reproduce the fragmentar character of the Fermi surface. The appearance of hole pockets in various structures is related either to states in the lower Hubbard band or to states localized on domain walls. The behavior of a gap at the leading edge of the energy distribution of photoelectrons and its dependence on oxygen removal in the course of annealing are considered.     

On the phase transition of superconducting cuprates in zero and non-zero magnetic fields

We present the results of measurements of the magnetizationM(T) and the specific heatC _p (T) of YBa₂Cu₃O_6.9 and Bi₂Sr₂CaCu₂O₈ in the vicinity of their respective critical temperature and in magnetic fields between 0 and 5 T. From these data we calculate the temperature- and magnetic field derivatives ofM andC _p . Both these measured and calculated quantities are used for testing theoretical predictions concerning the universality class of the transitions and to verify the influence of fluctuations accompanying the transitions.     

Pattern of the induced magnetic field in high-temperature superconducting ceramics

Our experiments performed earlier have shown that, when an external magnetic field is absent, the transport critical current in 3-d superconducting ceramics is a homogeneous function of the sample transverse sizes. The transport critical current density and magnetic field induced by the current are homogeneous functions of a point on the sample cross-section. Using these experimental results equations describing the induced magnetic field pattern in ceramic sample have been derived. The distributions of the transport critical current density and induced magnetic field in the samples having polygonal, diamond-shaped cross-sections illustrate the results.     

Nano-scale complexities in the superconducting cuprates

Underdoped cuprates are characterized by nano-scale complexity with strong spatial variation in the electronic properties, including superconductivity. It is often assumed that the stripe order underlies this spatial complexity, but the evidence of local stripe order in the superconducting phase is weak. We propose an alternative idea of electronically driven two-dimensional local order that leads to phase separation in the reciprocal space, which could be the basis for two-component superconductivity.     

Local measurements of magnetic characteristics of high-temperature superconducting films

A new experimental technique for measuring magnetic characteristics of high-temperature superconducting (HTS) films is described. The measurement system includes a laser providing for local measurements. The measured magnetic characteristics of the HTS films are of scientific and practical interest.