Nd-Fe(Co,Nb)-B交换耦合磁体的磁性

用熔体快淬法结合热处理制备了高性能纳米复合永磁合金Nd₉Fe_85.5-xCo_xNb₁B_4.5(0≤x≤16).最佳磁性能对应的成分为Nd₉Fe_81.5Nb₁B_4.5,其永磁性能如下：最大磁能积(BH)_max＝156kJ/m³,剩磁J_r＝1.11T 关键词：     

纳米晶复合永磁材料的交换耦合相互作用和磁性能

本介绍了纳米磁性材料晶粒交换耦合相互作用的有关理论。采用不同模型讨论了晶粒交换耦合相互作用对纳米单相软磁材料、永磁材料及双相复合永磁材料磁性能的影响。简述了用δM（H）曲线和不可逆磁导率的变化研究晶粒交换耦合相互作用及反磁化过程的方法。讨论了合金分配比、添加元素、制备及热处理工艺对磁体硬磁性能的影响。从理论和实验两方面分析、研究了纳米复合永磁材料的反磁化过程和矫顽力机制。     

纳米晶复合永磁材料的交换耦合相互作用和磁性能

本文介绍了纳米磁性材料晶粒交换耦合相互作用的有关理论。采用不同模型讨论了晶粒交换耦合相互作用对纳米单相软磁材料、永磁材料及双相复合永磁材料磁性能的影响。简述了用δM(H)曲线和不可逆磁导率的变化研究晶粒交换耦合相互作用及反磁化过程的方法。讨论了合金成分配比、添加元素、制备及热处理工艺对磁体硬磁性能的影响。从理论和实验两方面分析、研究了纳米复合永磁材料的反磁化过程和矫顽力机制。     

反铁磁耦合硬磁-软磁-硬磁三层膜体系的不可逆交换弹性反磁化过程

采用一维原子链模型研究了反铁磁耦合的硬磁/软磁/硬磁三层膜体系的反磁化过程. 研究结果表明,当考虑了软磁层的磁晶各向异性能后,软磁层厚度和界面交换耦合强度的改变都有可能导致软磁层的交换弹性反磁化过程由可逆过程转变为不可逆过程. 对软磁层很薄的体系,其反磁化过程是典型的可逆交换弹性反磁化过程. 然而,当软磁层厚度超过某一临界厚度t_c时,反磁化过程转变为不可逆的交换弹性反磁化过程. 软磁-硬磁界面交换耦合强度A_sh对反磁化行为也有很大的影响. 对于软磁层厚度小于临界厚度t_c的体系,也存在一个临界界面交换耦合强度A_sh^c. 当A_sh大于A_sh^c时,软磁层的反磁化过程是可逆的交换弹性反磁化过程;而当A_sh小于A_sh^c时,这一过程变为不可逆. 给出了体系的可逆与不可逆交换弹性反磁化过程随软磁层厚度和界面交换耦合强度变化的磁相图. 同时还研究了偏转场随软磁层厚度的变化关系. 关键词： 反铁磁耦合三层膜 交换弹性反磁化过程 反磁化机理 磁相图     

自旋1/2铁磁模型的相互作用淬灭

本文设想了一个相互作用淬灭后在t=0时刻开启的海森堡反铁磁模型,并对其进行了解析分析.在低温近似下,通过求解海森堡方程给出该系统随时间演化的自旋算符的解析形式.文中主要推算并讨论了自旋传播子,通过对传播子的讨论发现这个新体系的自旋波谱发生了变化.文末对此现象进行了讨论.     

自旋1/2铁磁模型的相互作用淬火

本文设想了一个相互作用淬火后在 时刻开启的海森堡反铁磁模型,并对其进行了解析分析.在低温近似下,通过求解海森堡方程给出该系统随时间演化的自旋算符的解析形式.主要推算并讨论了自旋传播子,通过对传播子的讨论发现这个新体系的自旋波谱发生了变化.文末对此现象进行了讨论.     

Nd-Fe-B/FeCo多层纳米复合膜的结构和磁性

制备了Nd₂₈Fe₆₆B₆/Fe₅₀Co₅₀多层纳米复合磁性薄膜，对溅射态和650℃退火处理15 min试样的相成分分析和微结构的观察显示，溅射态薄膜呈非晶态，经650℃退火处理15 min后，薄膜主要相成分为硬磁性Nd₂Fe₁₄B相和软磁性相FeCo(110)相.Nd₂Fe₁₄B相呈柱状，其易磁化c轴垂直于膜面，尺寸约10 nm.在硬磁性相和软磁性相之间存在少量富Nd相和非晶态，富Nd相大小约7 nm.磁性测量和分析表明，1)该系列薄膜退火态具有垂直于膜面的磁晶各向异性.2)对于固定厚度(10 nm)层Nd-Fe-B和不同厚度(t_FeCo=1—100 nm)层FeCo多层纳米复合膜,剩磁随软磁相FeCo 厚度的增加快速增加，而矫顽力则减小.当t_FeCo=5 nm时，最大磁能积达到200 kJ/m³. 3)硬磁相Nd-Fe-B层和软磁相FeCo层之间交换耦合导致剩磁和磁能积增强. 关键词： Nd-Fe-B/FeCo多层纳米复合膜 交换耦合 磁各向异性     

基于Stoner-Wohlfarth 模型磁性纳米颗粒的磁化反转

纳米磁性材料由于其特殊的磁学性能,近年来,在许多领域受到了广泛的应用。在基础理 论研究中,人们提出了各种描述纳米磁性材料的理论;另一方面,计算机计算能力以及实验手段 的提高,使得应用计算机进行材料设计以及探测单个纳米颗粒的磁学特性成为可能。这使得人们 对纳米磁性材料的理解更加深入。本篇论文介绍了磁性纳米颗粒的磁化反转机制的基本理论与实 验研究的最新进展。本文首先从磁性材料中基本的相互作用入手说明这些相互作用在纳米尺度下 的表现形式,随后详细介绍了基于Stoner-Wohlfarth 模型计算机模拟方法,最后简单介绍两种 可以用来研究单个纳米颗粒磁化反转实验手段以及相关的实验结果。     

纳米复合永磁材料中软磁性相交换硬化的研究

本文就纳米复合永磁材料中软磁相被交换硬化问题,从一维模型和三维模拟计算进行了分析研究. 一维和三维各向异性样品研究表明,在相同微结构下,当硬磁相的各向异性降低时,除矫顽力降低外,在磁矩全部反转之前退磁曲线是一样的. 因此,硬磁相各向异性的降低不会导致最大磁能积(BH)_max增大和剩磁增加. 对于三维各向同性样品的模拟计算表明,降低硬磁相的各向异性会使剩磁和(BH)_max都明显降低. 因此,增强硬磁相的各向异性并增大硬磁相晶粒尺寸是提高 关键词： 纳米复合永磁 矫顽力 剩磁 磁能积     

磁性纳米颗粒系统偶极相互作用的Monte Carlo研究

采用局域Monte Carlo方法模拟不同易轴分布的简单立方排列单分散单畴Fe纳米颗粒系统的ZFC-FC曲线及磁滞回线.结果表明：随着偶极相互作用的增强，系统的阻塞温度T_B逐渐增大，且ZFC曲线的峰变宽.说明偶极相互作用使得系统的有效能垒提高，分布宽度增加.研究FC曲线磁化强度的倒数与温度关系，发现偶极相互作用系统中存在反铁磁有序.系统的阻塞态及超顺磁态的磁滞回线表明，极低低温下，随着偶极相互作用的增强，系统的矫顽力和剩磁减小，偶极相互作用阻碍系统的磁化；系统处于超顺磁态，各向异性作用及偶极相互作用使得系统的磁化曲线偏离Langevin曲线且偶极相互作用展现出退磁相互作用效应.偶极相互作用增强，系统磁化曲线与Langevin曲线偏差量的最大值向低场移动.在偶极相互作用下，易轴与外场夹角为45°的磁性纳米颗粒系统的平均有效能垒和有效能垒分布宽度较易轴随机分布系统的大.     

Interfacial roughness and temperature effects on exchange bias properties in coupled ferromagnetic/antiferromagnetic bilayers

Monte Carlo simulations have been used to study the relationship between the exchange bias properties and the interface roughness in coupled ferromagnetic/antiferromagnetic (FM/AFM) films of classical Heisenberg spins. It is shown that the variation of the exchange bias field versus the AFM anisotropy strongly depends on the FM/AFM interface. Unlike the flat interface, a non-monotonic dependence is observed for the roughest FM/AFM interface. This is explained by canted magnetic configurations at the FM/AFM interface, which appear after the first reversal due to the magnetic frustration. The temperature dependence of the exchange field is also dependent on the roughness. While the exchange field is roughly constant for the flat interface, a decrease is observed for the roughest interface as the temperature increases. This has been interpreted as a significant decrease of the effective coupling between the FM and the AFM due to the disordering of the moments at the FM/AFM interface because of the combination of magnetic frustration and temperature activation.     

Computational studies on magnetism and ferroelectricity

Magnetics, ferroelectrics, and multiferroics have attracted great attentions because they are not only extremely important for investigating fundamental physics, but also have important applications in information technology. Here, recent computational studies on magnetism and ferroelectricity are reviewed. We first give a brief introduction to magnets, ferroelectrics, and multiferroics. Then, theoretical models and corresponding computational methods for investigating these materials are presented. In particular, a new method for computing the linear magnetoelectric coupling tensor without applying an external field in the first principle calculations is proposed for the first time. The functionalities of our home-made Property Analysis and Simulation Package for materials (PASP) and its applications in the field of magnetism and ferroelectricity are discussed. Finally, we summarize this review and give a perspective on possible directions of future computational studies on magnetism and ferroelectricity.     

A Monte Carlo study of the thermodynamic properties of a quasi-one-dimensional organic polymer ferromagnet

The thermodynamic properties of a quasi-one-dimensional organic ferromagnet at different temperatures and in different applied magnetic fields have been investigated by means of the Heisenberg model combined with the Monte Carlo method. The results indicate that a peak in the magnetic susceptibility is obtained at low temperatures. Furthermore, the effect of dimerization on the magnetic properties has also been studied. We find that the dimerization suppresses the magnetization in this model. The ferromagnetic couplings between the side-free radicals stabilize the ferromagnetism and increase the apparent Curie temperature.     

耦合同轴磁绝缘传输线的低阻抗大面积轫致辐射二极管设计

为了设计与前端低阻抗同轴磁绝缘传输线耦合的大面积轫致辐射二极管,提出了一种利用锥形磁绝缘传输线（MITL）结合阴极开孔结构来对电子输运进行调节的二极管设计方案。该结构的主要特点是在不外加电子输运调控装置的前提下,利用大角度的入射电子产生轫致辐射,在靠近二极管出射窗附近形成大面积准均匀辐射区。采用二维粒子模拟与蒙特卡罗模拟（MCNP 4C）相结合的数值模拟方法对二极管进行了模拟和分析,对于如何构建更好反映角向均匀的MCNP源提出了新的想法。模拟结果表明,该设计方案可以实现在不外加电子输运调控装置的情况下,在二极管后端得到均匀大面积轫致辐射区。     

Interface motion in a two-dimensional Ising model with a field

We determine by Monte Carlo simulations the width of an interface between the stable phase and the metastable phase in a two-dimensional Ising model with a magnetic field, in the case of nonconversed order parameter (Glauber dynamics). At zero temperature, the width increases ast with–1/3, as predicted by earlier theories. As temperature increases, the value of the effective exponent that we measure decreases toward the value 1/4, which is the value in the absence of magnetic field.     

Monte Carlo investigation of the correlation between magnetic and chemical ordering in NiFe alloys

The Ni_xFe_1−x alloys close to the stoichiometric Ni₃Fe composition are modeled by means of Monte Carlo simulations. To describe the atomic and magnetic configurations, the Ising and Heisenberg models with nearest-neighbor interactions have been used, respectively. The pairwise interactions have been fitted to the experimentally measured Curie and Kurnakov temperatures, the Fe-Fe magnetic exchange interaction has been considered antiferromagnetic. The mutual influence of the magnetic and chemical ordering is evidenced and a good agreement with the phase diagram is obtained. Our numerical results show that the magnetic order is able to increase the Kurnakov temperature and, reciprocally, the chemical order is responsible for a rise in the Curie temperature. Also, the influence of the applied magnetic field on the chemical order is investigated and an increase of the Kurnakov temperature with the external field is observed.     

二元合金表面偏析的Monte Carlo方法模拟

详细介绍了二元合金表面偏析的Monte Carlo模拟方法,并应用改进的分析型嵌入原子模型结合Monte Carlo方法模拟研究了Pd-Au合金表面成分及其剖面成分分布,发现Au在表面偏析,并同已有实验结果进行了比较.     

Monte Carlo study on bilayer thin films magnetic properties dependence with discontinouos anisotropy parameters

In the last few years there has been significant interest in the field of thin films, due to numerous specific phenomena related to the low dimension of these systems, and to the large opportunities in development of high technologies based on their specific magnetic and electronic properties. When dealing with systems of reduced dimensionality it is important to take into account the influence of magnetic anisotropies. In this paper we investigate the magnetic properties of bilayer thin film. This behavior is modeled using Monte Carlo simulations, in the Extended Anisotropic Heisenberg Model. The magnetization, out-of-plane and in-plane magnetic susceptibilities, and also the specific heat bearings according to temperature are investigated in order to find the potential magnetic ordering phases and the critical temperatures, for two sets parameter assignments. For quasi-uniform anisotropy parameters of the film we detect the ferromagnetism-paramagnetism transition and then, by changing the model parameters values, we relieve a short range ferromagnetic ordering phase arising from the antiferromagnetic base layer coupling influence and from easy-plane anisotropy discontinuity on the layers interface.      

Nano-graphene monolayer with higher-order exchange couplings: Monte Carlo study

We have used the Monte Carlo simulation to study the phase diagrams and the magnetic properties of a single nano-graphene layer with next-nearest neighbors coupling $J_2$ and four-spin interaction $J_4$. Interesting behaviors have been found. In particular, the nanographene can present tricritical and triple points for appropriate system parameters.