Flame-Flow Interaction in Premixed Turbulent Flames During Transient Head-On Quenching

This paper reports on experimental investigations of turbulent flame-wall interaction (FWI) during transient head-on quenching (HOQ) of premixed flames. The entire process, including flame-wall approach and flame quenching, was analyzed using high repetition rate particle image velocimetry (PIV) and simultaneous flame front tracking based on laser-induced fluorescence (LIF) of the OH molecule. The influence of convection upon flame structures and flow fields was analyzed qualitatively and quantitatively for the fuels methane (CH₄) and ethylene (C₂H₄) at ? = 1. For this transient FWI, flames were initialized by laser spark ignition 5 mm above the burner nozzle. Subsequently, flames propagated against a steel wall, located 32 mm above the burner nozzle, where they were eventually quenched in the HOQ regime due to enthalpy losses. Twenty ignition events were recorded and analyzed for each fuel. Quenching distances were 179 μm for CH₄ and 159 μm for C₂H₄, which lead by nondimensionalization with flame thickness to Peclet numbers of 3.1 and 5.5, respectively. Flame wrinkling and fresh gas velocity fluctuations proved flame and flow laminarization during wall approach. Velocity fluctuations cause flame wrinkling, which is higher for CH₄ than C₂H₄ despite lower velocity fluctuations. Lewis number effects explained this phenomenon. Results from flame propagation showed that convection dominates propagation far from the wall and differences in flame propagation are related to the different laminar flame speeds of the fuels. Close to the wall flames of both fuels propagate similarly, but experimental results clearly indicate a decrease in intrinsic flame speed. In general, the experimental results are in good agreement with other experimental studies and several numerical studies, which are mainly based on direct numerical simulations.     

LES-CMC Simulations of Different Auto-ignition Regimes of Hydrogen in a Hot Turbulent Air Co-flow

Large-Eddy Simulation (LES) results in combination with first-order Conditional Moment Closure (CMC) are presented for a hydrogen jet, diluted with nitrogen, issued into a turbulent co-flowing hot air stream. The fuel mixes with the co-flow air, ignites and forms a lifted-like flame. Global trends in the experimental observations are in general well reproduced: the auto-ignition length decreases with increase in co-flow temperature and increases with increase in co-flow velocity. In the experiments, the co-flow temperature was varied, so that different auto-ignition regimes, including low Damköhler number situations, were obtained (no ignition, random spots, flashback and lifted flame). All regimes are recovered in the simulations. Auto-ignition is found to be the stabilizing mechanism. The impact of different detailed chemistry mechanisms on the auto-ignition predictions is discussed. With increasing air temperature, the differences between the mechanisms considered diminish. The evolution of temperature, H₂O, H, HO₂ and OH from inert to burning conditions is discussed in mixture fraction space.     

An Experimental Investigation of the Turbulence Structure of a Lifted H2/N2 Jet Flame in a Vitiated Co-Flow

Measurements of mean velocity components, turbulent intensity, and Reynolds shear stress are presented in a turbulent lifted H₂/N₂ jet flame as well as non-reacting air jet issuing into a vitiated co-flow by laser doppler velocimetry (LDV) technique. The objectives of this paper are to obtain a velocity data base missing in the previous experiment data of the Dibble burner and so provide initial and flow field data for evaluating the validity of various numerical codes describing the turbulent partially premixed flames on this burner. It is found that the potential core is shortened due to the high ratio of jet density to co-flow density in the non-reacting cases. However, the existence of flame suppressed turbulence in the upstream region of the jet dominates the length of potential core in the reacting cases. At the centreline, the normalized axial velocities in the reacting cases are higher than the non-reacting cases, and the relative turbulent intensities of the reacting flow are smaller than in the non-reacting flow, where a self-preserving behaviour for the relative turbulent intensities exists at the downstream region. The profiles of mean axial velocity in the lifted flame distribute between the non-reacting jet and non-premixed flame both in the axial and radial distributions. The radial distributions of turbulent kinetic energy in the lifted flames exhibit a change in distributions indicating the difference of stabilisation mechanisms of the two lifted flame. The experimental results presented will guide the development of an improved modelling for such flames.     

Flamelet Based NO x -Radiation Integrated Modelling of Turbulent Non-premixed Flame using Reynolds-stress Closure

A methodology of extending laminar flamelet model in its adiabatic form to a non-adiabatic form which can account for radiative heat loss as well as its effect on NO _x pollutant has been developed. Coupling of radiation submodel with flamelet model is based on the enthalpy defect concept. Pollutant NO _x has been calculated from solution of its transport equation containing source term which is derived from flamelet calculations. Flamelet calculations adopted GRI 2.11 reaction mechanism which accounts for detailed carbon and NO _x chemistry. Depending on consideration of variation in scalar dissipation within flamelet calculations, the non-adiabatic form has been further divided into non-adiabatic model with single (NADS) and multiple scalar dissipation rates (NADM). Bluff-body stabilized CH₄/H₂ flame has been chosen as the test case to assess the capability of non-adiabatic models. Turbulence closure has been achieved with a Reynolds stress transport model. Calculations have also been carried out with a modified k-ε model for evaluation of relative performance of the two turbulence closures. Performance of non-adiabatic flamelet models in regard to the overall structure of the flame is reasonably good and the agreement is similar to that of the adiabatic flamelet model thereby indicating weakly radiating nature of the flame. However, the NADM model results in minor but encouraging improvement in NO mass fraction predictions by reducing the extent of overprediction observed with the adiabatic model. In contrast, the NADS model results in overprediction over and above the adiabatic predictions thereby showing that, it is imperative to consider variation in scalar dissipation rate in flamelet calculations to capture the effect of radiation on NO. The results also show that employing the modified k-ε model instead of the Reynolds stress transport model for turbulence closure in NADM calculations results in considerable overprediction in centerline NO mass fractions.     

LES Modeling of the Impact of Heat Losses and Differential Diffusion on Turbulent Stratified Flame Propagation: Application to the TU Darmstadt Stratified Flame

Common combustion chambers often exhibit turbulent flames propagating in partially-premixed mixtures. This propagation is generally governed by aerodynamics, unsteady mixing and chemical processes and may also be affected by conductive heat losses when the reactive zone develops close to the burner lips. The Filtered TAbulated Chemistry for Large Eddy Simulation (F-TACLES) model has been recently developed to include tabulated chemistry in Large Eddy Simulation (LES) of adiabatic stratified flames in flamelet regimes. The present article proposes a modeling approach to account for both differential diffusion and non-adiabatic effects on flame consumption speed following the F-TACLES formalism. The adiabatic F-TACLES model is first detailed using a generalized formalism for diffusive fluxes allowing either to account for differential diffusion or not. The F-TACLES model is then extended to non-adiabatic situations. A correction factor based on the non-adiabatic consumption rate is introduced to recover a realistic filtered flame consumption speed. The objective is here to tackle flame stabilization mechanisms when heat losses affect the reaction zone. The proposed approach is validated through the simulation of the unconfined stratified turbulent jet flame TSF-A for which stabilization process is affected by heat losses. Five simulations are performed for both adiabatic and non-adiabatic flow conditions comparing unity Lewis number and complex diffusion assumptions. The adiabatic F-TACLES model predicts a flame anchored at the burner lip disagreeing with experimental data. The non-adiabatic simulation exhibits local extinction due to heat losses near the burner exit. The flame is then lifted improving the comparison with experiments. Results also show a significant impact of molecular diffusion model on both mean flame consumption rate and angle.     

Measurement of adiabatic burning velocity in natural gas-like mixtures

Experimental measurements of the adiabatic burning velocities were carried out for natural gas-like mixtures burning in air over a range of equivalence ratios at atmospheric pressure. Effect of CO₂ dilution up to 60%, N₂ dilution up to 40% and 25% enrichment of ethane on burning velocity of methane–air flames were studied. Heat flux method with setup similar to that of [K.J. Bosschaart, L.P.H. de Goey, Detailed analysis of the heat flux method for measuring burning velocity, Combustion and Flame 132 (2003) 170–180] was used for measurement of burning velocities. Initially experiments were done for methane–air and ethane–air mixtures at various equivalence ratios and the results were in good agreement with published data in the literature. Computations were performed using PREMIX code with GRI 3.0 reaction mechanism for all the mixtures. Predicted flame structures were used to the explain the effect of N₂ and CO₂ dilution on burning velocity of methane–air flames. Peak burning velocity for CH₄/CO₂–air mixtures occur near to ϕ = 1.0.     

Influence of heat and mass transfer on the ignition and NOx formation in single droplet combustion

The effect of heat and mass transfer on the ignition, and in a second step on the nitrogen oxide (NO _x ) generation, of single burning droplets is examined in a numerical study. Spherical symmetry with no gravity and no forced convection is presumed; ambient temperature is set at 500 K, below the auto-ignition point. The essentials of a forced droplet ignition by an external energy source are introduced. Two methods are applied: heat introduction at a fixed radial position r and heat introduction at a fixed local equivalence ratio ϕ _r . This study’s distinctiveness compared to previous research is its focus on and its combination of partially pre-vaporized droplets and detailed chemistry, both being technically relevant in kerosene and diesel fuel combustion. The fuel of choice is n-decane (C₁₀H₂₂), and NO _x production is studied exemplarily as a representative group of pollutant emissions. The conducted simulations show a decrease of NO _x formation with an increase of the pre-vaporization rate \Uppsi. \Uppsi. This decrease is generally valid for both methods of heat introduction. However, results on flame stabilization and NO _x production reveal a high sensitivity to parameters of the ignition model. The burning behavior during the initial stages is dominated by the ignition position. Extracting heat from the exhaust gas region of burning droplets shows no impact on the flame position nor on the relative NO _x production. As a consequence, a well-founded modeling of the investigated droplet regime needs to resort to an iterative adaptation of the heat introduction parameters based on the findings of droplet burning and exhaust gas production.     

Turbulent Combustion of Hydrogen–CO Mixtures

Laminar and turbulent burning velocities were measured in a closed-volume fan-stirred vessel for H₂–CO mixtures using two independent methods of flame definition. It has been shown that the unsteady flame development is an important factor and it needs to be taken into account for comparison of the burning rates obtained in different experiments. For the atmospheric pressure flames, the mixtures with faster laminar flame velocities burnt faster in turbulent flow despite the fact that the lean flames exhibit cellular structures. However, even a modest increase of the initial pressure promotes strongly cellularity and causes a significant acceleration of a lean laminar flame. The same lean flame burns faster in turbulent flow as well and this increase in the rate of combustion is greater that can be deduced from variation of the molecular heat diffusivity and laminar flame speed.     

Nonpremixed bluff-body burner flow and flame imaging study

A nonpremixed bluff-body burner flow and flame have been studied using planar flow visualization and species concentration imaging techniques. The burner consists of a central jet of CH ₄ in a cylindrical bluff-body and an outer coflowing-air stream. Planar flow visualization, using Mie scattering from seed particles added to the fuel jet, Raman scattering from CH ₄ and laser-induced fluorescence of CH combined with Raman scattering of CH ₄ provided information on turbulent flow, mixing and combustion. The CH ₄ imaging system utilized two cameras, which enhanced the dynamic range of the diagnostic system by a factor of 10 over a single-camera system. It was observed that the fuel jet stagnated on the axis due to interaction with the high velocity air flow. The flow and mixing were found to have significant coherent and noncoherent, large-scale, time-varying structures. The detailed CH ₄ Raman and CH fluorescence measurements of an air-dominated bluff-body flame revealed that the stagnation zone governs mixing and flame stability. Through large-scale mixing, the stagnated jet feeds the recirculation zone and also creates a favorable condition to stabilize the flame detached from the bluff-body. The instantaneous flame zone, as defined by CH, was found to be narrow and concentrated in an envelope around the stagnation zone. This narrow flame characteristic is consistent with that observed for jet flames. Although the internal structure of the flame envelops have not yet been defined, these results suggest that this bluff-body flame can be modeled by a flame sheet type approach, where the reaction front is captured by the large-scale structures. This should simplify the development of modeling approaches for these flows since molecular mixing and chemical reaction, which occur within the flame sheet, can be separated from the large-scale mixing process.     

Structures and stabilization of low calorific value gas turbulent partially premixed flames in a conical burner

Experiments are carried out on partially premixed turbulent flames stabilized in a conical burner. The investigated gaseous fuels are methane, methane diluted with nitrogen, and mixtures of CH₄, CO, CO₂, H₂ and N₂, simulating typical products from gasification of biomass, and co-firing of gasification gas with methane. The fuel and air are partially premixed in concentric tubes. Flame stabilization behavior is investigated and significantly different stabilization characteristics are observed in flames with and without the cone. Planar laser induced fluorescence (LIF) imaging of a fuel-tracer species, acetone, and OH radicals is carried out to characterize the flame structures. Large eddy simulations of the conical flames are carried out to gain further understanding of the flame/flow interaction in the cone. The data show that the flames with the cone are more stable than those without the cone. Without the cone (i.e. jet burner) the critical jet velocities for blowoff and liftoff of biomass derived gases are higher than that for methane/nitrogen mixture with the same heating values, indicating the enhanced flame stabilization by hydrogen in the mixture. With the cone the stability of flames is not sensitive to the compositions of the fuels, owing to the different flame stabilization mechanism in the conical flames than that in the jet flames. From the PLIF images it is shown that in the conical burner, the flame is stabilized by the cone at nearly the same position for different fuels. From large eddy simulations, the flames are shown to be controlled by the recirculation flows inside cone, which depends on the cone angle, but less sensitive to the fuel compositions and flow speed. The flames tend to be hold in the recirculation zones even at very high flow speed. Flame blowoff occurs when significant local extinction in the main body of the flame appears at high turbulence intensities.     

Combined Influence of Strain and Heat Loss on Turbulent Premixed Flame Stabilization

The present paper argues that the prediction of turbulent premixed flames under non-adiabatic conditions can be improved by considering the combined effects of strain and heat loss on reaction rates. The effect of strain in the presence of heat loss on the consumption speed of laminar premixed flames was quantified by calculations of asymmetric counterflow configurations (“fresh-to-burnt”) with detailed chemistry. Heat losses were introduced by setting the temperature of the incoming stream of products on the “burnt” side to values below those corresponding to adiabatic conditions. The consumption speed decreased in a roughly exponential manner with increasing strain rate, and this tendency became more pronounced in the presence of heat losses. An empirical relation in terms of Markstein number, Karlovitz Number and a non-dimensional heat loss parameter was proposed for the combined influence of strain and heat losses on the consumption speed. Combining this empirical relation with a presumed probability density function for strain in turbulent flows, an attenuation factor that accounts for the effect of strain and heat loss on the reaction rate in turbulent flows was deduced and implemented into a turbulent combustion model. URANS simulations of a premixed swirl burner were carried out and validated against flow field and OH chemiluminescence measurements. Introducing the effects of strain and heat loss into the combustion model, the flame topology observed experimentally was correctly reproduced, with good agreement between experiment and simulation for flow field and flame length.     

The effect of oxidant flow rate on a coaxial oxy-fuel flame

The effect of oxidant flow rate on temperature, heat transfer, and NO_x formation of an oxy-fuel flame is investigated using numerical simulation. The finite volume approach is used to solve the governing equations. The realizable k-ε turbulence model and β-PDF model are adopted to simulate the turbulence-combustion interaction. There is a good agreement between the present numerical results and the reference experimental data. The exhaust temperature is decreased with decreasing the oxidant inlet flow rate. As an important result, the adiabatic flame temperature can be considered a key parameter in the oxy-fuel flame applications. Also, it is observed that increasing oxygen inlet angle causes a decrease in NO formation.     

Natural convection with surface radiation from a planar heat generating element mounted freely in a vertical channel

Experiments and numerical simulations have been conducted to study the conjugate heat transfer by natural convection and surface radiation from a planar heat generating element placed centrally between two adiabatic vertical plates. The relevant problem dependent parameters considered in this study are modified Rayleigh number, channel aspect ratio, stream-wise location of the heat generating element, and surface emissivities of the heat generating element and the adiabatic side plates. Experiments are conducted for different values of modified Rayleigh number ranging from 3.2 × 10⁵ to 1.6 × 10⁷ and surface emissivities 0.05, 0.55, 0.75 and 0.85. The interdependence between the heat transfer mechanism and the flow field under the influence of surface radiation on natural convection is explored and discussed. Experimental correlations for total and convective Nusselt number, and dimensionless temperature in terms of relevant parameters have been developed. The mathematical model governing the problem has been numerically solved using a commercial computational fluid dynamics package FLUENT 6.3 and the numerical predictions substantiate the experimental observations.     

Heat flux measurements in stagnation point methane/air flames with thermographic phosphors

Light-induced phosphorescence from thermographic phosphors was used to study the wall temperatures and heat fluxes from nearly one-dimensional flat premixed flames. The investigated flames were stoichiometric, lean and rich laminar methane/air flames with equivalence ratios of φ = 1, φ = 0.75 and φ = 1.25 at ambient pressure. The flames were burning in a stagnation point arrangement against a water-cooled plate. The central part of this plate was an alumina ceramic plate coated from both sides with chromium-doped alumina (ruby) and excited with a Nd:YAG laser or a green light-emitting diode (LED) array to measure the wall temperature from both sides and thus the heat flux rate from the flame. The outlet velocity of the gases was varied from 0.1 to 1.2 m/s. The burner to plate distance (H) ranged from 0.5 to 2 times the burner exit diameter (d = 30 mm). The measured heat flux rates indicate the change of the flame stabilization mechanism from a burner stabilized to a stagnation plate stabilized flame. The results were compared to modeling results of a one-dimensional stagnation point flow, with a detailed reaction mechanism. In order to prove the model, gas phase temperatures were measured by OH-LIF for a stoichiometric stagnation point flame. It turns out that the flame stabilization mechanism and with it the heat fluxes change from low to high mass fluxes. This geometry may be well suited for further studies of the elementary flame wall interaction.     

Influence of Co-flow on Flickering Diffusion Flame

The influence of air co-flow on flickering methane diffusion flame was studied experimentally using the image processing technique and the proper orthogonal decomposition (POD) analysis. The flickering of the flame is characterized by the mean height, the oscillation amplitude and the Strouhal number, which are measured by the digital image analysis of the diffusion flame. The experiments are carried out for various combinations of burner diameters, fuel velocities and co-flow velocities. With increasing the velocity ratio of the co-flow to the fuel flow, the oscillation amplitude is decreased and the Strouhal number is increased slightly in proportional to the inverse Froude number, while the frequency jump occurs in the low co-flow velocity ratio. These results are commonly observed in all the burners of different diameters, while the critical co-flow velocity ratio to suppress the flickering is found to be increased with increasing the burner diameters due to the influence of Froude number. The POD analysis of the flickering flame shows that the flickering energy is dominant in the first two POD modes and they are axisymmetric except for the zero co-flow velocity case and fully suppressed case. The correlation of POD coefficients in the first two fluctuating POD modes suggests the suppression of large-scale structure of flickering due to the influence of co-flow.     

Ultra-low-emission steam boiler constituted of reciprocal flow porous burner

This experimental study examined a low-emission steam boiler in which the filtration combustion technology was employed. This new boiler concept is consisted of a reciprocal flow porous burner, in which a combustion wave propagates along the reactor length. The boiler’s burner is filled up by an inert porous material, which leads to a stable burning of ultra-lean fuel/air mixtures, operating below flammability limits of conventional burners. In reciprocal filtration combustion, the reaction zone travels back and forth along the length of the burner, maintaining a typical trapezoidal temperature distribution favorable to the energy extraction. Embedding heat exchangers into the ends of the porous bed results in an alternative low-emission high-efficiency boiler. The heat re-circulation inside the porous matrix and the low degree of thermal non-equilibrium between the gas and the solid phases result in ultra-low levels of CO and NO_x. Over an equivalence ratio range from 0.20 to 1.0 and a gas flow velocity range from 0.2 to 0.6 m/s, burning the technical methane, the developed prototype has reached efficiencies superior to 90% and NO_x and CO emission levels lower than 1.0 and 0.5 ppm, respectively.     

Heat Release Imaging in Turbulent Premixed Ethylene-Air Flames Near Blow-off

The focus of this work is to visualise the regions of CH₂O and heat release (HR) of an unconfined turbulent premixed bluff body stabilised ethylene-air flame at conditions approaching lean blow-off using simultaneous imaging of OH- and CH₂O-PLIF. The HR regions are estimated from the product of the OH and CH₂O profiles. At conditions near blow-off, wide regions of CH₂O are observed inside the recirculation zone (RZ). The presence of CH₂O and HR inside the RZ is observed to follow fragmentation of the downstream flame parts near the top of the RZ. The presence of wide regions void of both OH and CH₂O inside the RZ at conditions very close to blow-off indicates the possible entrainment of un-reacted gases into the RZ. The behaviour of the lean ethylene-air flame with Lewis number (Le) greater than 1 is compared to that of a lean methane-air flame with Le of approximately 1. For both fuels, qualitatively similar observations of flame fragmentation downstream followed by build-up of CH₂O and HR inside the RZ are observed at conditions near lean blow-off. Also, a similar trend of flame front curvature conditioned on HR was observed for both the ethylene-air and methane-air flames, where the magnitude of HR was observed to increase with the absolute value of curvature.     

Combined radiation and natural convection in a rectangular cavity with a transparent wall and containing a non-participating fluid

This paper describes a numerical method for the study of combined natural convection and radiation in a rectangular, two-dimensional cavity containing a non-participating (i.e. transparent) fluid. One wall of the cavity is isothermal, being heated either by solar radiation or independently. The opposite wall is partially transparent, permitting radiation exchanges between the cavity and its surroundings and/or the Sun; that wall also exchanges heat by convection from its external surface to the surroundings. The other two walls are adiabatic: convection and radiation there are balanced, so that there is no heat transfer through those walls. The equations of motion and energy are solved by finite difference methods. Coupled to these equations are the radiative flux boundary conditions which are used to determine the temperature distribution along the non-isothermal walls. A two-band radiation model has been employed. Results are presented for a square cavity with a vertical hot wall at 150 °C, the ambient at 20 °C and 10⁴ ? Ra ? 3 × 10⁵, in the absence of direct insolation. The effects on the flow and heat transfer in the cavity of radiation and external convection have been examined. More extensive results will be presented in subsequent papers.     

Slip effects on unsteady mixed convection of hybrid nanofluid flow near the stagnation point

The unsteady mixed convection of the Al2O3-Cu/H2O hybrid nanofluid flow near the stagnation point past a vertical plate is analyzed. The bvp4c technique is used to solve the resulting ordinary differential equations. The combined effects of the velocity and thermal slip are addressed. The effects of different relevant physical parameters are studied numerically. The results show that the heat transfer rate is reduced when the volume fraction of the nanoparticles increases, while the unsteadiness...