A model for arc plasma's optical diagnosis by the measurement of the refractive index

A model, which introduces the ionization degree of plasma, is deduced to reconstruct the temperature and electron number density distributions for arc plasmas via the measurement of the refractive index. The rationality, applicability and superiority of the model are analyzed and discussed theoretically. To experimentally verify whether the model is rational and feasible, an argon arc plasma is chosen as a practical example for experiment, while the measurement of the refractive index is achieved by moiré deflection tomography with the probe wavelength 635 nm. The distribution and imprecision of the reconstructed temperature results indicate that the model is reasonable, feasible and dependable. Besides, the factors which may cause the imprecision of the reconstructed temperature are also analyzed and proposed.     

Temperature's optical tomography diagnosis of arc plasma jet flowing into air

An argon arc jet plasma flowing into air is chosen as a practical example to study the multiple species jet plasma's optical computerized tomography (OCT) diagnosis. The refractive index models of the pure argon and the multiple species arc plasmas are supplied. On the basis of which, the temperature reconstruction model of the multiple species arc plasma is further derived. By theoretical calculation, the effect of mixed air on the refractive index is given. For the sake of better proving the effect of directly omitting the mixed air on flow field's temperature reconstruction from the refractive index, a simulated experiment is supplied. Finally, the condition, which can be adopted to estimate that whether the pure argon arc plasma refractive index model still can be used as the temperature reconstruction model of the argon arc plasma jet flowing into air, is proposed.     

冲击压缩产生的氩等离子体辐射不透明度研究

采用平面冲击压缩方法产生密度和温度都均匀的氩等离子体,根据光谱辐射强度随时间的变化测量了氩等离子体在可见光区几个波长通道的辐射不透明度,等离子体温度在1.4—2.2eV范围,密度在0.0083—0.015gcm³之间.测量值和理论计算结果符合较好,说明平均原子模型可以较好地描述该热力学条件下氩等离子体的光子输运行为.基板表面的光反射率在确定辐射不透明度时是一个重要参数.采用简化的自洽方法求解基板表面的光反射率.结果表明,基板/氩气界面的光反射率R在0.4附近,与Erskine专门实验 关键词： 物态方程 不透明度 氩     

Numerical analysis of nitrogen-mixed argon plasma characteristicsand injected particle behavior in an ICP torch for ultrafine powdersynthesis

A numerical model is presented for the analysis of plasma characteristics of an ICP torch and gas mixing effects on the plasma when a nitrogen gas is added into the argon plasma as a carrier or sheath gas at the torch inlet, The fluid equations describing the plasma flow and temperature fields and the diffusions between two different gases are solved along with a magnetic vector potential equation for electromagnetic fields. The trajectory and the temperature change with time for a particle injected into the plasma are also investigated by a plasma-particle interaction model to find out optimum injection conditions for the synthesis of ultrafine nitride ceramic powders, It is found from the calculations that the nitrogen-mixed argon plasma with a nitrogen sheath gas is more favorable than the plasma with a nitrogen carrier gas for the reaction kinetics of nitride synthesis. It is also found that the radial injection through the holes of the tube wall Is preferable to the axial injection at the torch inlet for the complete evaporation of injected particle and the effective chemical reaction of reactant vapor with nitrogen. For the radial injection in an ICP torch of 20 cm in axial length, the optimum injection locations and initial velocities of 50 μm aluminum particles are found for synthesizing aluminum nitride are in the range of 6~12 cm apart from the torch inlet and over 15 m/s, respectively     

Femtosecond filament induced birefringence in argon and in air: Ultrafast refractive index change

The birefringence of a linearly polarized femtosecond laser filament in gases has been previously established. In this work, we report the time-dependent refractive index measurements of the filament based upon the spectral modulation of a weak probe pulse in air and in argon gas at 1 atmospheric pressure. The polarization dependence of the refractive index modulation induced by the delayed molecular alignment and by the electronic Kerr effect is highlighted. A numerical simulation of the refractive indices, which takes into account the molecular alignment, the electronic Kerr non-linearity and the plasma, is in good agreement with the measurements.     

真空中微波等离子体喷流电子数密度分布规律实验研究

为了准确诊断真空中微波等离子体喷流的电子数密度，利用统一的发射和单郎缪尔探针测量等离子体的空间电位，再测量等离子体的电流-电压特性曲线.根据空间电位测量结果，在等离子体的电流-电压特性曲线上能准确地获取饱和电流，从而处理出电子数密度.最后的诊断实验表明，当真空环境压强为2—6 Pa、等离子体发生器以60 W以下的微波功率击穿流量范围是42—106 mg/s的氩气时，所产生的微波等离子体喷流中电子数密度分布在1×10¹⁶—7.2×10¹⁶/m³范围内.     

Guiding of an electromagnetic pulse in a plasma immersed in combined wiggler and axial magnetic fields

We present a new plasma-based method of guiding an electromagnetic pulse. The scheme consists of an inhomogeneous magnetic field and a uniform density plasma, in contrast to existing schemes that rely on transverse plasma density gradients but need not be magnetized. The refractive index of a magnetized plasma depends on the strength and direction of the magnetic field as well as the plasma density. A guiding channel is formed by using field inhomogeneity to generate the desired transverse profile of the index of refraction. The concept is analyzed with an envelope equation and, for the specific example of a wiggler magnetic field, with a two-dimension particle-in-cell simulation. A simplified model of this scheme as producing a magnetic wall in analogy to metallic waveguides is presented, for which corresponding approximate relations for the guided mode axial wavelength and radius are derived as functions of the plasma and magnetic field parameter. These are seen to be in good agreement with particle-in-cell simulation results. Since the desired inhomogeneity of the refractive index can be made easily when the electromagnetic wave frequency is close to the cyclotron frequency, this guiding scheme is most readily applied in the microwave regime.     

Dependence of Arc Plasma Dispersion Capability on its Temperature

The relationship between the dispersion capability and the temperature of argon arc plasma at 1 atm is deduced in view of the plasma＇s refractive index equation. The results indicate that argon arc plasma has a normal dispersion and its dispersion capability is nonlinear to the plasma＇s temperature in a wide range of temperature and wavelength region. According to the results of numerical calculation, the preferred optical methods are believed to be suitable for the diagnosis of argon arc plasma in different temperature regions.     

Analysis on the feasibility of optical tomography in measuring gas jet flow velocity

Enlightened by the wide application of optical computerized tomography (OCT) in various flow fields’ visualization and parameter measurement, the potential feasibility of it on measuring gas jet flow velocity is discussed in this paper. The dependence of flow velocity on flow field's refractive index and dynamic pressure is deduced initially. An argon gas jet flow is chosen as an example for experiment, and the refractive index measurement is achieved by moiré tomography, while the dynamic pressure is obtained by a pressure sensor. In a word, both the theoretical and experimental results prove that OCT could be feasible to obtain the flow velocity of gas jet flows.     

非理想性参数在0.9～2.1区的氩等离子体物态方程研究

采用平面冲击压缩方法产生密度和温度都均匀的氩等离子体,根据辐射高温计记录和飞片速度的测定,通过阻抗匹配方法确定了氩等离子体的Hugoniot物态方程,等离子体温度在1.5 eV～2.6 eV范围,压力在0.2～0.8 GPa之间.计算表明,Saha-Debye-Hückel模型不适用于描述该密度区域的氩等离子体.本文采用Gryaznov模型的计算结果,测量值和理论计算结果符合较好.     

Polarization of light backscattered by small particles

We study scattering of light by wavelength-scale spherical, cubic, and spheroidal particles as well as clusters of spherical particles for equal-volume-sphere size parameters 4≤x≤10 and refractive indices 1.1≤m≤2.0. Such particles exhibit three specific features in the regime of backscattering: first, the intensity shows a backscattering peak; second, the degree of linear polarization for unpolarized incident light is negative; and, third, the depolarization ratio is double-lobed. We find that the overall characteristics of the scattering-matrix elements can be explained by an internal field composed of waves propagating in opposite directions near the particle perimeter and forming standing waves, as well as a wave propagating forward with the wavelength of the internal medium. When moving from the central axis of the particle toward its perimeter, the internal field changes from a forward-propagating wave with a wavelength dictated by the particle refractive index toward a standing wave with an apparent wavelength of the surrounding medium. The mapping of the internal field to the scattered far field is like an interference dial where rotation of the dial by a quarter of a wavelength on the particle perimeter results in a change from a destructive to constructive interference feature in the angular patterns (or vice versa). The dial is a manifestation of a well-known rule of thumb: the number of maxima or minima in the scattering-matrix elements is given by the size parameter. We explain the backscattering peak as deriving from the backward-propagating internal wave near the particle perimeter. Negative polarization follows from the spatial asymmetry of the internal fields: inside the particle, the fields are amplified near the central plane perpendicular to the polarization state of incident light, resulting in more pronounced interference effects for the perpendicular polarization than for the parallel polarization. The double-lobe feature in the depolarization results from the same internal-field structure with leading cross-polarized fields located slightly different from the copolarized fields. We discuss practical implications of these findings for the retrieval of particle sizes, shapes, and refractive indices from observations and laboratory experiments.     

Numerical study on the characteristics of nitrogen discharge at high pressure with induced plasma

Based on the fluid theory of plasma, a model is built to study the characteristics of nitrogen discharge at high pressure with induced argon plasma. In the model, species such as electrons, N2+, N4+, Ar+, and two metastable states (N 2(A3∑u+), N2 (a1 ∑u-)) are taken into account. The model includes the particle continuity equation, the electron energy balance equation, and Poisson抯equation. The model is solved with a finite difference method. The numerical results are obtained and used to investigate the effect of time taken to add nitrogen gas and initially-induced argon plasma pressure. It is found that lower speeds of adding the nitrogen gas and varying the gas pressure can induce higher plasma density, and inversely lower electron temperature. At high-pressure discharge, the electron density increases when the proportion of nitrogen component is below 40%, while the electron density will keep constant as the nitrogen component further increases. It is also shown that with the increase of initially-induced argon plasma pressure, the density of charged particles increases, and the electron temperature as well as the electric field decreases.     

介质中含孤立发光中心的纳米粒子的辐射寿命概率分布

含发光中心的纳米粒子在介质中随机分布,造成局域介质相对折射率的随机分布,导致了纳米粒子辐射寿命的涨落.分析纳米粒子数量在线度为发射光波长量级的体积内的概率密度,由此得出局域介质相对折射率的概率密度.通过纳米粒子辐射寿命对折射率的依赖关系,得到纳米粒子辐射寿命概率密度的解析表达.在此基础上,分析了Meltzer等人的实验中,含Eu³⁺离子的Y₂O₃粒子在甲醇溶液中辐射寿命的相对偏移量的涨落,并得出辐射寿命的不确定度(均方差)与纳米粒子体积、体积密度等物理量的关系.     

Study on 3-D arc plasma fields with holographic interferometry

In this paper,serveral temperature(refractive index)fields which are de-scribed by different kinds of functions are reconstructed by computer simulations based onholographic tomography theory.The obtained results are compared and analyzed.We de-signed a special multibeam holographic system in which the disturbance from the intense arclight can be filtered.With the system multidirectional holographic interferograms of arc fieldscan be taken simultaneously.We also calculate the quantitative distributions of temperature,the number density of particles and ionicity at a typical section of the argon arc field from theexperimeantal data.     

Mode transition in magnetic pole enhanced inductively coupled argon plasmas

The electrical probe (Langmuir probe) diagnostics of different plasma parameters and operation regimes (E/H modes) of magnetic pole enhanced, inductively coupled (MaPE-ICP) argon plasmas are investigated. It is shown that uniform, high density (n _e ∼ 10¹² cm^-3) and low electron temperature (T _e ∼ 1.5 eV) plasma can be produced in low pressure argon discharges at a low power (100 W). It is found that an MaPE-ICP reactor operates in two different modes; capacitive (E mode) and inductive (H mode). No density jump or hysteresis are reported between these modes. The effect of pressure on transition power, where the mode changes from E to H mode at 20 sccm gas flow rate are studied and it is found that for all pressures tested (∼7.5 mTorr to 75 mTorr) the transition power remains same. In the inductive mode, the above plasma parameters show a smooth variation with increasing filling gas pressure at fixed power. The intensity of the emission line at 750.4 nm due to 2p ₁ → 1s ₂ (Paschen’s notation) transition, closely follows the variation of n _e with RF power and filling gas pressure. Measured electron energy probability function (EEPF) shows that electron occupation mostly changes in the high-energy tail, which enlightens close similarity of the 750.4 nm argon line to electron number density (n _e ). The behaviour of the electron energy probability function (EEPF) with regard to pressure and RF power in two operational modes is presented.     

氦氩射频容性放电发射光谱分析

光抽运亚稳态稀有气体激光器利用放电等离子体作为激光的增益介质.为掌握容性射频放电的放电参数对等离子体各项参数的影响的基本规律,利用等离子体发射光谱法研究了氦氩混合气体在不同装置、不同Ar组分、不同气压和不同射频注入功率下的等离子体参数.利用残留水蒸气产生的OH自由基A~2Σ~+→X~2Π的转动光谱分析获得气体温度;利用电子态光谱的玻尔兹曼做图法获得电子激发温度,利用Ar原子696.5 nm谱线的斯塔克展宽获得电子密度.结果表明:气体温度随气压增加略微上升,在一个大气压下改变组分和放电功率,气体温度变化不大;电子激发温度随总气压的下降而上升,且随着Ar组分的增加而略微下降;目前放电条件下的电子密度均在10~(15)cm~(-3)量级;长时间放电监测表明,残留的水蒸气会导致电子温度的下降,从而降低Ar亚稳态的产率.     

Ar流速对多级弧放电装置中Ar等离子特性的影响

采用PLASIMO程序模拟了入口处Ar流速对多级弧放电产生的非热平衡Ar等离子体特性的影响。模拟结果发现:从入口处到出口处,沿中心轴线,压强逐渐降低,电子平均能量基本保持不变。当流速一定时,从器壁到中心轴线处,电子数密度呈增大趋势;从入口处到出口处,电子数密度呈先增大后减小的趋势;当流速分别为50,100,150和200 cm3/s时,电子数密度最大值分别为10.131021,16.311021,18.981021和26.331021 m-3;随着流速的增大,其电子数密度逐渐增大。当流速一定时,从器壁到中心轴线处,电子温度逐渐增大;从入口处到出口处,电子温度呈先增大后减小再增大的趋势,并在中心轴线处距入口55～60 mm有最大值,当流速分别为50,100,150和200 cm3/s时,其最大值分别为1.299,1.234,1.157和1.132 eV;由于入口处和器壁处的电子温度都为0.517 eV,所以随着Ar流速的增大,其电子温度逐渐减小。当Ar流速一定时,从器壁到中心轴线处,离子温度逐渐增大;从入口处到出口处,离子温度呈先增大后减小的趋势,并且在中心轴线距入口20～30 mm离子温度取得最大值,当流速分别为50,100,150和200 cm3/s时,离子温度最大值分别为0.815 6,0.907 02,0.975 2和1.014 eV。随入口处流速的增大,电弧腔体内的离子温度逐渐增大。     

Measurement of azimuthal magnetic fields in a Z-pinch gas discharge using the faraday rotation of a probe beam

The Faraday rotation of the plane of polarisation of a probe beam by azimuthal magnetic fields in the presence of beam deflection caused by refractive index gradients is discussed for a plasma carrying an axial current. A method for calculation of the magnetic field profile from experimental data is described. Bθ can be found by Abel inversion if the electron density is known and if deflected rays can be collected by an optical system and focussed onto a detector. Typical Faraday rotations calculated for the Bennett pinch assuming small beam deflection are found to be proportional to the plasma current and to the angle of deflection. If the probe beam wavelength is chosen to satisfy the approximate relation N₀λ² ≈ 3.5 × 10¹³ m^-1, where N₀ is the electron density on the axis, measurement of Bθ with beam deflections less than 2 × 10^-2 radians should be possible in cases where small rotations can be detected in the mid-to-far infra-red part of the spectrum.     

涂有半导体气敏薄膜的长周期光纤光栅气敏传感特性理论分析

首先利用耦合模理论研究了长周期光纤光栅LPFG折射率敏感特性,数值计算了长周期光纤光栅透射谱谐振波长与环境介质折射率的关系。其次分析了半导体氧化物气敏膜光学特性机理,当气体与薄膜接触时,气体会使敏感膜的消光系数、吸收系数和相应的折射率发生变化。基于上述两点,提出可将气敏膜涂于光栅表面,利用气敏膜的折射率随环境气体成分和浓度变化而变化的特性,从而影响LPFG透射谱谐振波长的变化,通过检测波长的变化达到探测气体成分和浓度的目的。由于长周期光纤光栅对环境介质折射率的灵敏度高于光纤,且其传感信号属于波长调制,测量信号不受光强波动及光纤损耗的影响,因此其灵敏度比强度型光纤气体传感器高。     

Numerical Study on Characteristics of Argon Radio-Frequency Glow Discharge with Varying gas Pressure

A one-dimensional fluid simulation on argon rf glow discharge with varying linearly gas pressure from 1 Torr to 100 Tort is performed. The model based on mass conservation equations for electron and ion under diffusion and mobility approximation, and the electron energy conservation equation is solved numerically by finite volume method. The numerical results show that a uniform plasma with high density can be obtained from rf glow discharge with varying gas pressure, and the density of plasma becomes higher as the gas pressure varies from 1 Tort to 100 Tort. It is also shown that in the range of the gas pressure from 1 Tort to 100 Tort with the slower rate of varying gas pressure, higher density of plasma can be obtained.