低能Ar3+ + Ar碰撞反应过程实验研究

测量了入射离子能量为27 keV、45 keV和66 keV时Ar3 Ar碰撞反应各子过程的分截面,通过将其归一化到Bliman,Dousson等人所测量的截面值,获得了绝对截面.结果表明,该能区电子俘获过程仍占主导地位,但转移电离过程已不能忽略.结果还表明,各子过程反应截面基本不随能量变化.与考虑自电离的MCBM(Molecular Coulombic overBarrier Model)模型比较发现,模型所给截面普遍高于实验测量值,这在一定程度上是由于归一化时带来的系统误差.在误差允许的范围内,单电子和双电子俘获截面符合的比较好,但三电子俘获截面却相差一个数量级.对于实验观测到的转移电离过程,模型却预言并没有此过程发生.     

Electron scattering with LiH molecule including a realistic dipole potential

Various electron scattering processes are examined theoretically for the strongly polar lithium hydride molecule. We have introduced a realistic dipole potential to calculate rotational cross sections of LiH upon electron impact. From the ionization threshold onwards total cross sections for elastic and inelastic scattering are evaluated in the complex molecular potential, and total ionization cross sections are extracted by CSP-ic method developed in recent years. While most of the results are new some indirect comparisons are made to draw conclusions.     

Ionization of heavy ions in collisions with neutral atoms at relativistic energies

Ionization processes of heavy ions colliding with atoms and ions at relativistic energies are considered. Formulaes for calculating ionization cross sections in the Born approximation using momentum-transfer representation without regard to magnetic interactions are given as well as those in dipole and impulse approximations. Using the LOSS-R [25] and HERION codes, calculations of relativistic cross sections are performed for H-like multiply changed ions with the nuclear charge Z ≈ 80?90, colliding with neutral atoms and for multiply changed uranium ions colliding with protons and carbon atoms. The results of calculations are compared with available experimental data and calculations performed by other authors.     

应用ECPSSR理论研究重离子引起原子的内壳层电离

ECPSSR理论是解释离子-原子碰撞内壳层电离最成功的理论之一.我们用VISUAL FORTRAN编写了ECPSSR理论计算程序,修正了ISICS程序中的错误,本程序可以对各种入射离子与靶原子的组合进行计算,给出K,L,M的壳层及次壳层电离截面以及相应的X射线产生截面,并根据需要选择是否对入射离子运动进行相对论修正.采用所编写的程序计算了一些碰撞体系的电离截面和X射线产生截面,并与其他程序的计算结果和实验数据分别进行了比较.     

Al^q＋（q=0～12）的电子碰撞电离截面和速率系数

使用扭曲波玻恩交换(DWBE)近似计算Al^q (q=0～12)的电子碰撞电离截面和速率系数,其中电离截面的高能行为由Bethe系数决定。分析了计算数据随电离度的变化规律,并且与可得到的实验的和其他计算的数据进行了比较,表明结果可靠。     

H<Superscript>+</Superscript> and He<Superscript>2+</Superscript> impact charge transfer cross sections of magnesium

H⁺ impact single and He²⁺ impact single and double electron capture cross sections of magnesium atoms have been calculated in the modified binary encounter approximation (BEA). The accurate expressions of ion impact s_DE\sigma _{\Delta {E}} (cross section for energy transfer DE\Delta E) and Hartree-Fock momentum distributions of the target electrons have been used throughout the calculations. On the basis of the present work it is concluded that inner shell captures by H⁺ and He²⁺ ions incident on magnesium atoms contribute partly to single electron capture and partly to transfer ionization cross sections. The calculated He²⁺ impact double electron capture cross sections of magnesium are in reasonably good agreement with the experimental observations. This indicates the success of the present theoretical approach in study of charge transfer cross sections of atoms as indirect mechanisms do not interfere with double electron capture processes in this case.     

Cq+ 和Oq+与原子碰撞的电子俘获过程的理论研究

在ECPSSR理论的基础上， 利用OBKN近似描述电子俘获过程， 得到了包括电子俘获过程贡献的ECPSSR理论， 编写了相应的计算程序。 采用该程序计算了不同电荷态离子与多种靶原子碰撞的电子俘获截面和相应的X 射线产生截面， 将计算得到的包含电子俘获过程贡献的X 射线产生截面与实验结果进行了比较。 对于具有满K壳层的入射离子碰撞， X 射线产生截面与入射离子电荷态基本无关； 对于以直接电离为主导的碰撞过程， 计算得到的X 射线产生截面与实验数据符合得很好； 对于全裸和单K空穴入射离子的碰撞， 计算高估了X 射线产生截面。 Based on the ECPSSR theory, the contribution of the electron capture is described by the OBKN theory. The cross sections of electron capture and X ray production for the collision of different charge state projectiles with various targets are calculated, and compared with the available experimental data. It is found that the obtained X ray production cross sections are almost independent of the projectile charge states for projectiles without a K vacancy. For the collision processes of direct ionization, the present calculated results agree well with the experimental data. The calculations overestimate the X ray production cross sections for the projectiles with full and a K vacancy.     

Electron impact ionization of SiCl<Subscript>2</Subscript> and SiCl

We measured absolute partial cross sections for the formation of all singly charged positive ions produced by electron impact on SiCl₂ and SiCl from threshold to 200 eV using the fast-neutral-beam technique. Some of the cross section curves exhibit an unusual energy dependence with a pronounced low-energy maximum at an energy around 30 eV, which may be indicative of the presence of indirect ionization channels. Dissociative ionization channels are dominant for both species. The experimentally determined total single ionization cross sections for both species agree very well with calculated cross sections using the Deutsch-M?rk (DM) formalism. A brief summary of the ionization cross sections determined for all four SiCl_x (x=1–4) species is given highlighting similarities and differences.     

Multiple ionization processes involving fast charged particles

This review is devoted to certain aspects of the theory of multiple ionization of a quantum target by a fast charged particle. Atoms and molecules, and their ions as well, are considered as targets, while electrons and protons are considered as projectiles. Special attention is paid to the effective charge approximation while constructing continuum wave functions for several charged fragments in the exit channel of the reaction. Theoretical calculations of differential and total cross sections of various multiple ionization processes are presented and, where possible, comparison of the results of these calculations with experimental data is carried out.     

H<Superscript>+</Superscript><Emphasis Type="Bold">and He</Emphasis><Superscript>2+</Superscript> impact single and double ionization of lead

H⁺ and He²⁺ impact single and double ionization cross sections of ground state lead atoms have been calculated in the binary encounter approximation. Calculations of direct double ionization cross sections have been performed in the modified double binary encounter model. The accurate expressions of σ_ΔE (cross-section for energy transfer ΔE) and Hartree-Fock velocity distributions for the target electrons have been used throughout the calculations. Contributions to double ionization from Auger effect following ionization of inner shells have been considered in the present work. Our H⁺ impact single and double ionization cross sections are in good agreement with the experimental observations. In calculations of He²⁺ impact cross sections, the present theoretical approach shows limited success in the experimentally investigated region (50–350 keV amu^-1).     

Electron-impact ionization cross sections and rates for ions of argon

A distorted-wave Born exchange (DWBE) approximation including relativistic correction is used to calculate the electron-impact ionization cross sections and rate coefficients for the highly charged ions Ar⁷⁺,…,Ar¹⁷⁺. The comparison of the calculated results with the experimental data and other theoretical calculations shows that the DWBE method is valid for these ions of argon. The calculated results for direct ionization cross sections and excitation autoionization were fitted by empirical formulas to meet the requirements of applications. A set of improved empirical formulas are used for the fast and accurate calculations of rate coefficients from the fit parameters of cross sections.     

N‐shell ionization cross sections by proton impact in the BEA

The N‐subshell ionizations cross sections of heavy elements by proton impact have been calculated in the binary‐encounter approximation. The momentum distribution of target electrons is taken into account by the use of the nonrelativistic and relativistic hydrogenic models and the Hartree–Fock–Roothaan and the relativistic Hartree–Fock–Roothaan methods. The obtained subshell ionization cross sections are compared with the experimental data and other theoretical calculations. The electronic relativistic effect and the wave‐function effect on N‐shell ionization cross sections are discussed.     

Positron scattering and ionization of neon atoms—theoretical investigations

Although positron scattering with inert gas atoms has been studied in theory as well as in experiment, there are discrepancies. The present work reports all the major total cross sections of e+-neon scattering at incident energies above ionization threshold, originating from a complex potential formalism. Elastic and cumulative inelastic scatterings are treated in the complex spherical e+-atom potential. Our total inelastic cross section includes positronium formation together with ionization and excitation channels in Ne. Because of the Ps formation channel it is difficult to separate out ionization cross sections from the total inelastic cross sections. An approximate method similar to electron-atom scattering has been applied to bifurcate ionization and cumulative excitation cross sections at energies from threshold to 2000 eV. Comparisons of present results with available data are made. An important outcome of this work is the relative contribution of different scattering processes, which we have shown by a bar-chart at the ionization peak.     

Atomic magneto-dipole photoionization

The special features of magneto-dipole photoionization of atomic s states are analyzed and the possibilities of experimental observation of this effect are discussed. It has been shown that despite the smallness of total cross sections for magnetic processes as compared with electric-dipole ones, the experimental observation of magnetic effects is possible, in principle, if photoelectrons are detected in the directions perpendicular to both the polarization vector of photon and its momentum; i.e. in the directions where the differential cross section for electric-dipole ionization of atomic s states is close to zero. The capabilities of the derived general formulas for the magneto-dipole cross sections are illustrated by numerical calculations for s subshells of He and Be atoms.     

Cross sections of inelastic processes in collisions between relativistic structured heavy ions and atoms

A nonperturbative method is developed for the calculation of cross sections of inelastic processes in collisions between structured high-charge heavy ions moving at relativistic velocities and atoms. By structure ions are meant partly stripped ions consisting of an ion nucleus and a number of bound electrons which partly compensate the core charge and form the electron “coat” of the ion. The single ionization cross section of hydrogen atom and single and double ionization cross sections of helium atom are calculated. It is demonstrated that the inclusion of the extent of ion charge may bring about a marked variation of the respective cross sections compared to ionization by point ions of the same charge and energy.     

电子与多电荷离子的碰撞电离(英文)

主要揭示了不同电离机制对高电荷态离子单电离和多重电离的贡献 ,包括直接电离 (一步过程 )、激发 自电离 (两步过程 )以及内壳Auger过程 ,研究了高电荷态镨离子的电子碰撞电离. Electron-impact ionization of ions is one of the most fundamental processes in every kind of plasma. Especially in high-temperature plasmas-whether in laboratory (nuclear fusion) or in astrophysics (atmosphere of stars)-atoms become ionized into multiply-charged ions by electron impact. The main purpose of our investigations is to unravel the contributions from different ionization mechanisms-like direct ionization (one-step process), excitation-autoionization (two-step process) and...     

电子碰撞电离截面的全相对论扭曲波计算

在相对论框架下 ,给出了电子与高电荷态离子碰撞直接电离截面的扭曲波玻恩交换近似计算方法 .作为示例 ,计算了几个离子 (类氢、类锂和类氖离子 )的电离截面 ,计算结果与实验值和其它理论计算值有比较好的符合. A fully relativistic distorted-wave exchange approximation method is presented. It can be used to obtain electron impact ionization cross section of highly charged ions. The ionization cross sections of several H-, Li, and Ne-like ions have been calculated. Good agreement is obtained while the calculated values are compared with the experiments or other relativistic calculations.     

Core-excited resonance enhancement in the two-photon complete fragmentation of helium

A time-dependent close-coupling method is used to calculate, for the first time, fully differential cross sections for the complete fragmentation of helium by two photons. Surprising differences in the magnitude of the total-integral cross sections are found in comparisons with other calculations. These differences are found to be due to a core-excited resonance enhancement of the two-photon process for both single and double ionization. These calculations provide theoretical support for ground-breaking measurements expected to be obtained from free-electron laser experiments in the near future.     

Electron impact ionization cross sections of beryllium and beryllium hydrides

We report calculated electron impact ionization cross sections (EICSs) for beryllium (Be) and some of its hydrides from the ionization threshold to 1 keV using the Deutsch-Märk (DM) and the Binary-Encounter-Bethe (BEB) formalisms. The positions of the maxima of the DM and BEB cross sections are very close in each case while the DM cross section values at the maxima are consistently higher. Our calculations for Be are in qualitative agreement with results from earlier calculations (convergent close-coupling, R matrix, distorted-wave and plane-wave Born approximation) in the low energy region. For the various beryllium hydrides, we know of no other available data. The maximum cross section values for the various compounds range from 4.0 × 10^?16 to 9.4 × 10^?16 cm² at energies of 44 to 56 eV for the DM cross sections and 3.0 × 10^?16 to 5.4 × 10^?16 cm² at energies of 40.5 to 60 eV for the BEB cross sections.