Step dynamics in relaxation of sharp corners on crystal surfaces

The dynamic behavior of steps involved in the relaxation of sharp corners in microfabricated structures on crystalline surfaces have been studied. We find that during the early stages of relaxation of slightly tapered trenches on Si(0 0 1), wide (1 1 0) terraces perpendicular to the substrate are formed near the corners of the trench sidewalls. The evolution of a step profile around the corner region, where step density abruptly changes, is analyzed using one-dimensional step models. It is found that, in case that mass transport occurs through surface diffusion, the preexisting steps on the trench sidewall are accumulated in the corner region, and extensive terraces are formed near the corners.     

Vacuum polarization induced by a uniformly accelerated charge

We consider a point charge fixed in the Rindler coordinates which describe a uniformly accelerated frame. We determine an integral expression of the induced charge density due to the vacuum polarization at the first order in the fine structure constant. In the case where the acceleration is weak, we give explicitly the induced electrostatic potential.     

Experimental model of cracking induced by drying shrinkage

Drying induced shrinkage in materials may yield the formation of surface crack patterns. We report on various experimental observations of the geometry of the crack array and the kinetics of crack formation on a model system consisting of a layer of a paste made of clay, sand, and water deposited on a rigid substrate. We investigate in detail the influence of the layer geometry (size and thickness). Received 19 April 1999     

Strongly first order electroweak phase transition induced by primordial hypermagnetic fields

We consider the effect of the presence of a hypermagnetic field at the electroweak phase transition. Screening of the Z-component inside a bubble of the broken phase delays the phase transition and makes it stronger first order. We show that the sphaleron constraint can be evaded for m_H up to 100 GeV if a B_Y0.3T² exists at the time of the EW phase transition, thus resurrecting the possibility for baryogenesis within the minimal standard model (provided enough CP violation can be obtained). We estimate that for m_H100 GeV the Higgs condensate behaves like a type II superconductor with Z-vortices penetrating the bubble. Also, for such high Higgs masses the minimum B_Y field required for a strong first order phase transition is large enough to render the W-field unstable towards forming a condensate which changes the simple picture of the symmetry breaking.     

Analysis of characteristic X-ray generation induced by laser plasma electrons accelerated by an electric field

The results of experiments devoted to the study of spectral, spatial, and time characteristics of a spectrally bright point x-ray source based on a vacuum diode with a laser-plasma cathode and a titanium needle anode with a photon energy approximately equal to 4.5 keV are presented. The experimental results revealed a considerable difference between the electron emission from laser plasma in a strong electric field and the explosive electron emission and demonstrated the effectiveness of laser plasma as an electron source. The optimization of the laser radiation power density, the accelerating voltage, and the interelectrode spacing made it possible to create a point x-ray source whose spectral brightness exceeds available sources in the class of small-size pulse x-ray instruments (tubes with explosive cathodes). It has been proved experimentally that the maximum contrast of the characteristic lines of the anode material is attained in the case of an optimal choice of accelerating voltage. The x-ray source has the following parameters: (1) spectral brightness of the K-lines of titanium of the order of 10²¹ photons/cm² s sr keV; (2) emitting region size of 250 mm; and (3) laser pulse duration less than 20 ns.     

Adiabatic nano-focusing of plasmons by sharp metallic wedges

In this paper, we demonstrate the possibility of efficient adiabatic nano-focusing of plasmons by a sharp triangular metal wedge. The geometrical optics approach and the approximation of continuous electrodynamics are used for the analysis. In particular, it is demonstrated that both the phase and group velocities of an incident anti-symmetric (with respect to the magnetic field) plasmon tend to zero at the tip of the wedge, and the plasmon adiabatically slows down, eventually dissipating in the metal. Typically, the amplitude of the plasmon significantly increases near the wedge tip, but this increase is finite even in the absence of dissipation in the metal. The dependence of the local field enhancement near the tip on structural parameters, dissipation in the metal, angle of incidence, etc., is analyzed in this paper. It is also shown that an anti-symmetric film plasmon can effectively be guided by a triangular metal wedge, forming a wedge plasmon mode that is localized near the tip of the wedge and propagates along this tip. A new existence condition for these localized wedge plasmons is derived and discussed. PACS 78.67.-n; 68.37.Uv; 73.20.Mf     

Molecular dynamics simulation of composite nanochannels as nanopumps driven by symmetric temperature gradients

In this Letter, we propose a composite nanochannel system, where half of the channel is of low surface energy, while the other half has a relatively high surface energy. Molecular dynamics simulations show that fluids in such channels can be continuously driven by a symmetric temperature gradient. In the low surface energy part, the fluid moves from high to low temperature, while the fluid migrates from low to high temperature in the high surface energy part. The mechanisms that govern the flow are explained and the conditions required to guarantee the flow and the possible applications are discussed.     

Enhancement of water permeation across nanochannels by partial charges mimicked from biological channels

In biological water channel aquaporins （AQPs）, it is believed that the bipolar orientation of the single-file water molecules inside the channel blocks proton permeation but not water transport. In this paper, the water permeation and particularly the water-selective behaviour across a single-walled carbon nanotube （SWNT） with two partial charges adjacent to the wall of the SWNT are studied by molecular dynamics simulations, in which the distance between the two partial charges is varied from 0.14 nm to 0.5 nm and the charges each have a quantity of 0.5 e. The two partial charges are used to mimic the charge distribution of the conserved non-pseudoautosomal （NPA） （asparagine/proline/alanine） regions in AQPs. Compared with across the nanochannel in a system with one ＋1 ε charge, the water permeation across the nanochannel is greatly enhanced in a system with two ＋0.5 e charges when charges are close to the nanotube, i.e. the two partial charges permit more rapid water diffusion and maintain better bipolar order along the water file when the distance between the two charges and the wall of SWNT is smaller than about 0.05 nm. The bipolar orientation of the single-file water molecules is crucial for the exclusion of proton transfer. These findings may serve as guidelines for the future nanodevices by using charges to transport water and have biological implications because membrane water channels share a similar single-file water chain and positive charged region at centre and provide an insight into why two residues are necessitated in the central region of water channel protein.     

Concentration polarization in translocation of DNA through nanopores and nanochannels

In this Letter we provide a theory to show that high-field electrokinetic translocation of DNA through nanopores or nanochannels causes large transient variations of the ionic concentrations in front and at the back of the DNA due to concentration polarization (CP). The CP causes strong local conductivity variations, which can successfully explain the nontrivial current transients and ionic distributions observed in molecular dynamics simulations of nanopore DNA translocations as well as the transient current dips and spikes measured for translocating hairpin DNA. Most importantly, as the future of sequencing of DNA by nanopore translocation will be based on time-varying electrical conductance, CP, must be considered in experimental design and interpretation--currently these studies are mostly based on the incomplete pore conductance models that ignore CP and transients in the electrical conductance.     

Statics and dynamics of single DNA molecules confined in nanochannels

The successful design of nanofluidic devices for the manipulation of biopolymers requires an understanding of how the predictions of soft condensed matter physics scale with device dimensions. Here we present measurements of DNA extended in nanochannels and show that below a critical width roughly twice the persistence length there is a crossover in the polymer physics.     

Compression and free expansion of single DNA molecules in nanochannels

We investigated compression and ensuing expansion of long DNA molecules confined in nanochannels. Transverse confinement of DNA molecules in the nanofluidic channels leads to elongation of their unconstrained equilibrium configuration. The extended molecules were compressed by electrophoretically driving them into porelike constrictions inside the nanochannels. When the electric field was turned off, the DNA strands expanded. This expansion, the dynamics of which has not previously been observable in artificial systems, is explained by a model that is a variation of de Gennes's polymer model.     

Wide-angle diffraction of the laser beam by a sharp edge

Using a rigorous theory of diffraction, we explain the origin and analyze the structure of a wide-angle illuminated area observed when a limited beam is diffracted by the sharp edge of an opaque screen. It is shown that the formed plume has the structure of a cylindrical wave traveling from the screen edge and its amplitude is proportional to the beam amplitude at this edge. The observed structure is Young’s boundary wave produced by diffraction of the limited beam.     

Diffraction of a Gaussian Beam by a Strongly Elongated Spheroid

Acoustical Physics - A high-frequency diffraction problem is considered for a Gaussian beam incident parallel to the axis of a strongly elongated spheroid. The parabolic equation method in...     

Decay of plasma cluster accelerated by coaxial gun

In this paper the decay of air cluster accelerated into the vacual tube is studied. The time dependence of electron density and electron temperature is introduced and the influence of various recombination processes is discussed. The observed plasma decay shows an exponential law, and is for various gun regimes independent and may be explained by ambipolar diffusion to the tube walls.     

Hierarchical modeling of diffusive transport through nanochannels by coupling molecular dynamics with finite element method

We present a successful hierarchical modeling approach which accounts for interface effects on diffusivity, ignored in classical continuum theories. A molecular dynamics derived diffusivity scaling scheme is incorporated into a finite element method to model transport through a nanochannel. In a 5 nm nanochannel, the approach predicts 2.2 times slower mass release than predicted by Fick’s law by comparing time spent to release 90% of mass. The scheme was validated by predicting experimental glucose diffusion through a nanofluidic membrane with a correlation coefficient of 0.999. Comparison with experiments through a nanofluidic membrane showed interface effects to be crucial. We show robustness of our discrete continuum model in addressing complex diffusion phenomena in biomedical and engineering applications by providing flexible hierarchical coupling of molecular scale effects and preserving computational finite element method speed.     

Self-organization of triblock copolymer patterns obtained by drying and dewetting

Self-organized block copolymer structures derived from dewetting of thin films are becoming important in nanotechnology because of the various spontaneous and regular sub-micrometric surface patterns that may be obtained. Here, we report on the self-organization of a poly(styrene)-b-poly(ethene-co-butene-1)-b-poly(styrene) triblock copolymer during drying of its solution over a mica substrate. Regular submicrometric arrangements with long-range order were formed at critical polymer concentrations, consisting of parallel ribbons and hexagonal arrays of dots (droplets). This variety of highly ordered structures is explained by the interplay between forming mechanisms, mainly due to “fingering instabilities” at the three-phase line of the copolymer solution during drying. The thickness of the structures was “quantized” due to the microphase separation of the block copolymer. The formation of hexagonal patterns may be attributed to Marangoni instability at the liquid film surface prior to dewetting.