Lasing in random media

A random laser is a non-conventional laser whose feedback mechanism is based on disorder-induced light scattering. Depending on whether the feedback supplied by scattering is intensity feedback or amplitude feedback, random lasers are classified into two categories: random lasers with incoherent feedback and random lasers with coherent feedback. A brief survey of random lasers with incoherent feedback is presented. It is followed by a review of our recent experimental work on random lasers with coherent feedback, including measurement of the lasing threshold, lasing spectra, emission pattern, dynamical response, photon statistics, speckle pattern and the investigation of relevant length scales. Large disorder leads to spatial confinement of the lasing modes, that is the foundation for the micro random laser. Some theoretical models of random lasers with coherent feedback are briefly introduced. The study of random lasers improves our understanding of the interplay between light localization and coherent amplification.     

随机激光器的理论与研究现状

综述了随机激光器的最新理论与实验进展，对光散射理论、环形腔理论、环形波导理论等各种随机激光理论的内容、应用范围及其差异等进行了重点分析和评述，并介绍了一些随机激光器的重要实验。讨论了随机激光器未来的发展，并描述了随机激光器潜在的应用前景。     

Passive mode locking of thin-disk lasers: effects of spatial hole burning

We recently demonstrated that passive mode locking of a thin-disk Yb:YAG laser is possible and that this concept leads to sources of femtosecond pulses with very high average power. Here we discuss in detail the effect of spatial hole burning on the mode-locking behavior of such lasers. We have developed an efficient numerical model and arrive at quantitative stability criteria which agree well with experimental data. The main result is that stable soliton mode locking can in general be obtained only in a certain range of pulse durations. We use our model to investigate the influence of various cavity parameters and the situation for different gain media. We also consider several methods to reduce the effect of spatial hole burning in order to expand the range of possible pulse durations. Received: 4 September 2000 / Published online: 10 January 2001     

Multimode coupling and nonlinear-gain effects in distributed and helical feedback gas lasers

We present a detailed experimental and theoretical study on the waveguide modes of distributed feedback (DFB) and helical feedback (HFB) gas lasers including for the first time the experimental verification of multimode-coupling and nonlinear-gain phenomena. For this purpose we used oversized hollow metal waveguides with periodic or helical corrugations. The latter exhibit the symmetry of either the single helix or the double helix. For the interpretation of our observations we developed a coupled-wave theory extended to multi-mode coupling and adapted the nonlinear-gain approach for strong coupling by Haus. The experiments with DFB and HFB gas lasers give new relevant information on these phenomena.On leave from Academia Sinica, Beijing, People's Republic of China     

Theoretical investigation on temporal properties of random lasers pumped by femtosecond-lasing pulses

Pulsing random lasing property has been investigated in both one- and two-dimensional random medium by numerically solving Maxwell’s equations and rate equations in which the pumping rate is described by a time function with duration of 10s or 100s of femtoseconds. The peak intensity, width and delay time of a random lasing pulse are traced with the variation of the peak intensity, duration, shape and numbers of a pumping pulse. Results show that the behavior of random lasing depends strongly on the pumping process, some of which are in agreement with previously reported experiments pumped by femtosecond-lasing pulses. The present work enriches the knowledge about random lasers, especially in temporal regime, and could offer more guidance for relevant experiments.     

Polarization-resolved analysis of the characteristics of a Raman laser made with a polarization maintaining fiber

We derive a simple model describing steady characteristics of Raman fiber lasers made with polarization maintaining fibers. We show both theoretically and experimentally that this kind of laser simply consists of two independent Raman lasers linearly polarized along the fiber birefringence axes. The output power characteristics of the laser are shown not to be influenced by optical Kerr effect. Finally, we use our model to propose answers to questions recently raised about efficiency of Raman lasers made with polarization maintaining fibers.     

Effect of particle size and shape on nonresonant random laser action of dye-doped polymer random media

We present an experimental study of the light emission from dye-doped polymer random media dispersed with TiO₂ particles of various sizes, shapes, and structures. Random lasing with nonresonant feedback, similar to that for spherically shaped particles that are used for conventional random lasers, is observed for almost all types of particles and aggregates. The efficiency of random lasing for each medium is analyzed using the relationship between the emission spectrum and the transport mean free path (TMFP), which is measured by enhanced backscattering experiments. Results show that the peak emission intensity depends strongly on the particle shape and structure, whereas the spectral linewidth is governed by the TMFP.     

Lasing action due to the two-dimensional quasiperiodicity of photonic quasicrystals with a Penrose lattice

We have fabricated photonic quasicrystal lasers with a Penrose lattice that does not possess translational symmetry but has long-range order, and observed coherent lasing action due to the optical feedback from quasiperiodicity, exhibiting a variety of 10-fold-symmetric lasing spot patterns. The lattice constant dependence of lasing frequencies and spot patterns show complicated features very different from photonic crystal/random lasers, and we have quantitatively explained them by considering their reciprocal lattice. Unique diversity of their reciprocal lattice opens up new possibilities for the form of lasers.     

Active synchronization of two mode-locked lasers with optical cross correlation

Two mode-locked Ti:sapphire lasers of different wavelengths were precisely synchronized by a simple feedback system employing sum-frequency generation (cross correlation). When the timing error exceeded the pulse duration, the periodic bunch of the sum-frequency pulse was used for rough timing adjustment. Using cross correlation with a stretched pulse, we struck a balance between wide locking range and sensitive timing detection. When the two lasers were well-synchronized, we obtained a continuous cross-correlation pulse train for 3 min. The holding time of the laser synchronization was extended to over one hour by adding a motorized stage to the PZT-mounted cavity mirror. We estimated the rms timing jitter between the two lasers by a scanning cross-correlation measurement. We confirmed that the rms timing jitter of the two lasers during 1.8 s was 28 fs. Received: 30 January 2002 / Revised version: 14 June 2002 / Published online: 8 August 2002     

Spatial extent of random laser modes

We have experimentally studied the distribution of the spatial extent of modes and the crossover from essentially single-mode to distinctly multimode behavior inside a porous gallium phosphide random laser. This system serves as a paragon for random lasers due to its exemplary high index contrast. In the multimode regime, we observed mode competition. We have measured the distribution of spectral mode spacings in our emission spectra and found level repulsion that is well described by the Gaussian orthogonal ensemble of random-matrix theory.     

Spin-orbit coupling in Bose-Einstein condensate and degenerate Fermi gases

We review our recent experimental realization and investigation of a spin orbit （SO） coupled Bose Einstein condensate （BEC） and quantum degenerate Fermi gas. By using two counter-propagathlg Ranlan lasers and controlling the different frequency of two R,aman lasers to engineer the atom light interaction, we first study the SO coupling in BEC. Then we study SO coupling in Fermi gas. We, observe the spin dephasing in spin dynamics and momentum distribution asymmetry of the equilibrium state as halhnarks of SO coupling in a Fermi gas. To clearly reveal the, property of SO coupling Fermi gas, we also study the momentmn-resolved radio-frequency spectroscopy which characterizes the energy momentum dispersion and spin composition of the quantum states. We observe the change of errmion surfaces in different helieity branches with different atomic density, which indicates that a Lifshitz transition of the Fermi surface topology change can be found by further cooling the system. At last, we study the momentum-resolved Raman spectroscopy of an ultracoht Fermi gas.     

Experimental observation and simulation of fractal patterns of Au/Ge bilayer films

In this paper, we report on the simulation of fractal clusters and the comparison with experimental fractal patterns. We found that multiple fractal clusters can be formed in Au/Ge bilayer films for different annealing times. The fractal crystallization area increases with the increase in the annealing time. The random successive nucleation model can simulate the actual growth processes of multiple growth sites. The simulating fractal clusters are in good agreement with our experimental fractal patterns. Received: 21 June 2001 / Accepted: 15 December 2001 / Published online: 3 June 2002 RID="*" ID="*"Corresponding author. Fax: +86-551/3602-803, E-mail: chenzw@ustc.edu.cn     

Deconstructing the glass transition through critical experiments on colloids

The glass transition is the most enduring grand-challenge problem in contemporary condensed matter physics. Here, we review the contribution of colloid experiments to our understanding of this problem. First, we briefly outline the success of colloidal systems in yielding microscopic insights into a wide range of condensed matter phenomena. In the context of the glass transition, we demonstrate their utility in revealing the nature of spatial and temporal dynamical heterogeneity. We then discuss the evidence from colloid experiments in favor of various theories of glass formation that has accumulated over the last two decades. In the next section, we expound on the recent paradigm shift in colloid experiments from an exploratory approach to a critical one aimed at distinguishing between predictions of competing frameworks. We demonstrate how this critical approach is aided by the discovery of novel dynamical crossovers within the range accessible to colloid experiments. We also highlight the impact of alternate routes to glass formation such as random pinning, trajectory space phase transitions and replica coupling on current and future research on the glass transition. We conclude our review by listing some key open challenges in glass physics such as the comparison of growing static length scales and the preparation of ultrastable glasses that can be addressed using colloid experiments.     

Light transport and correlation length in a random laser

A random laser is a strongly disordered, laser‐active optical medium. The coherent laser feedback, which has been demonstrated experimentally to be present in these systems beyond doubt, requires the existence of spatially localized photonic quasimodes. However, the origin of these quasimodes has remained controversial. We develop an analytical theory for diffusive random lasers by coupling the transport theory of the disordered medium to the semiclassical laser rate equations, accounting for (coherent) stimulated and (incoherent) spontaneous emission. From the causality of wave propagation in an amplifying, diffusive medium we derive a novel length scale which we identify with the average mode radius of the lasing quasi‐modes. We show that truly localized modes do not exist in the system without photon number conservation. However, we find that causality in the amplifying medium implies the existence of a novel, finite intensity correlation length which we identify with the average mode volume of the lasing quasimodes. We show further that the surface of the laser‐active medium is crucial in order to stabilize a stationary lasing state. We solve the laser transport theory with appropriate surface boundary conditions to obtain the spatial distributions of the light intensity and of the occupation inversion. The dependence of the intensity correlation length on the pump rate agrees with experimental findings.     

Spectral-fluctuations test of the quark-model baryon spectrum

We study the low-lying baryon spectrum (up to 2.2 GeV) provided by experiments and different quark models using statistical tools which allow us to postulate the existence of missing levels in spectra. We confirm that the experimental spectrum is compatible with random matrix theory, the paradigmatic model of quantum chaos, and we find that the quark models are more similar to a Poisson distribution, which is not compatible with what should be expected in a correlated spectrum. From our analysis it stems that the spectral fluctuation properties of quark-model spectra are incompatible with experimental data. This result can be used to enlighten the problem of missing resonances.     

Influence of light polarization on dynamics of all-fiber Raman lasers: theoretical analysis

Using Stokes-vectors formalism, we present a simple model describing steady and dynamic characteristics of all-fiber Raman lasers. This model allows us to describe experimental behaviors that are not yet understood in Raman lasers. In lasers made with standard fibers we show theoretically that weak birefringence and the optical Kerr effect lead to the emergence of unstable regimes similar to those recently observed in experiments [Opt. Lett. 28, 2464 (2003)]. However, the model shows that lasers made with polarization-maintaining fibers are always stable, as evidenced in experiments.     

Frequency behavior of coherent random lasing in diffusive resonant media

We investigate diffusive propagation of light and consequent random lasing in an amplifying medium comprising resonant spherical scatterers. A Monte-Carlo calculation based on photon propagation via three-dimensional random walks is employed to obtain the dwell-times of light in the system. We compare the inter-scatterer and intra-scatterer dwell-times for representative resonant and non-resonant wavelengths. Our results show that more efficient random lasing, with intense coherent modes, is obtained for a system with intra-scatterer gain. This is also coupled with a larger reduction in frequency fluctuations. We find that such a system can yield almost thresholdless random lasing. Inspired by these results, we discuss a possible practical situation, based on a monodisperse aerosol, wherein frequency controlled coherent random lasing can be obtained. Since our analysis essentially investigates transport of intensity, the results are relevant to coherent random lasers under nonresonant feedback.     

Influence of spatial mode matching in end-pumped solid state lasers

We present investigations on the influence of mode matching on the efficiency of longitudinally pumped solid state lasers. In a theoretical part we enhance an existing model for four level lasers from idealized cylindrical modes to arbitary pump and laser modes in a random relative position thereby neglecting beam deformation due to thermal effects. The theoretical predictions were confirmed experimentally with an end-pumped Nd:YAG rod operated at 1064 nm. To investigate the effect of misalignment on the efficiency we used a Ti-Sapphire pump laser which was displaced relative to the laser beam. To establish the influence of arbitary pump modes on laser performance a diode laser equipped with coupling optics served as pump source for the same resonator. The resulting decrease in slope efficiency compared to the Ti-Sapphire pumped system could be explained in terms of limited mode overlap due to the characteristic pump field distribution produced by the diode coupling optics.     

Passive mode locking with slow saturable absorbers

We give a comprehensive overview on passive mode locking of solid-state lasers with slow saturable absorbers, based on analytical and numerical calculations. For picosecond lasers, we present a simple equation to estimate the obtained pulse duration and compare the results to those for mode locking with fast saturable absorbers. We also discuss how much shorter the pulse duration can be compared to the absorber recovery time and present a simple rule. The effect of self-phase modulation is found to be qualitatively different compared to the case of a fast saturable absorber, and the effect of phase changes in the absorber is also discussed. Finally, we discuss various issues concerning soliton mode-locked lasers. Received: 20 July 2001 / Revised version: 28 September 2001 / Published online: 7 November 2001     

Photon statistics of random lasers with resonant feedback

We have measured the photon statistics of random lasers with resonant feedback. With an increase of the pump intensity, the photon number distribution in a single mode changes continuously from Bose-Einstein distribution at the threshold to Poisson distribution well above the threshold. The second-order correlation coefficient drops gradually from 2 to 1. By comparing the photon statistics of a random laser with resonant feedback and that of a random laser with nonresonant feedback, we illustrate very different lasing mechanisms for the two types of random lasers.